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Microphysical characterization of long-range transported biomass burning particles from North America at three EARLINET stations

  • Strong events of long-range transported biomass burning aerosol were detected during July 2013 at three EARLINET (European Aerosol Research Lidar Network) stations, namely Granada (Spain), Leipzig (Germany) and Warsaw (Poland). Satellite observations from MODIS (Moderate Resolution Imaging Spectroradiometer) and CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) instruments, as well as modeling tools such as HYSPLIT (Hybrid Single-Particle Lagrangian Integrated Trajectory) and NAAPS (Navy Aerosol Analysis and Prediction System), have been used to estimate the sources and transport paths of those North American forest fire smoke particles. A multiwavelength Raman lidar technique was applied to obtain vertically resolved particle optical properties, and further inversion of those properties with a regularization algorithm allowed for retrieving microphysical information on the studied particles. The results highlight the presence of smoke layers of 1-2 km thickness, located at about 5 km a.s.l. altitude over Granada and LeipzigStrong events of long-range transported biomass burning aerosol were detected during July 2013 at three EARLINET (European Aerosol Research Lidar Network) stations, namely Granada (Spain), Leipzig (Germany) and Warsaw (Poland). Satellite observations from MODIS (Moderate Resolution Imaging Spectroradiometer) and CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) instruments, as well as modeling tools such as HYSPLIT (Hybrid Single-Particle Lagrangian Integrated Trajectory) and NAAPS (Navy Aerosol Analysis and Prediction System), have been used to estimate the sources and transport paths of those North American forest fire smoke particles. A multiwavelength Raman lidar technique was applied to obtain vertically resolved particle optical properties, and further inversion of those properties with a regularization algorithm allowed for retrieving microphysical information on the studied particles. The results highlight the presence of smoke layers of 1-2 km thickness, located at about 5 km a.s.l. altitude over Granada and Leipzig and around 2.5 km a.s.l. at Warsaw. These layers were intense, as they accounted for more than 30% of the total AOD (aerosol optical depth) in all cases, and presented optical and microphysical features typical for different aging degrees: color ratio of lidar ratios (LR532/LR355) around 2, alpha-related angstrom exponents of less than 1, effective radii of 0.3 mu m and large values of single scattering albedos (SSA), nearly spectrally independent. The intensive microphysical properties were compared with columnar retrievals form co-located AERONET (Aerosol Robotic Network) stations. The intensity of the layers was also characterized in terms of particle volume concentration, and then an experimental relationship between this magnitude and the particle extinction coefficient was established.zeige mehrzeige weniger

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Verfasserangaben:Pablo Ortiz-AmezcuaORCiD, Juan Luis Guerrero-RascadoORCiD, Maria Jose Granados-Munoz, Jose Antonio Benavent-OltraORCiD, Christine BöckmannORCiDGND, Stefanos SamarasORCiDGND, Iwona Sylwia StachlewskaORCiD, Lucja Janicka, Holger BaarsORCiD, Stephanie Bohlmann, Lucas Alados-ArboledasORCiD
DOI:https://doi.org/10.5194/acp-17-5931-2017
ISSN:1680-7316
ISSN:1680-7324
Titel des übergeordneten Werks (Englisch):Atmospheric Chemistry and Physics
Verlag:Copernicus
Verlagsort:Göttingen
Publikationstyp:Wissenschaftlicher Artikel
Sprache:Englisch
Datum der Erstveröffentlichung:15.05.2017
Erscheinungsjahr:2017
Datum der Freischaltung:10.06.2022
Band:17
Seitenanzahl:16
Erste Seite:5931
Letzte Seite:5946
Fördernde Institution:Andalusia Regional Government [P12-RNM-2409]; Spanish Ministry of Economy and Competitiveness [CGL2013-45410-R]; Spanish Ministry of Education, Culture and Sports [FPU14/03684]; European Union [654169, 262254]; University of Granada; FNITP, Poland [519/FNITP/115/2010]; SONATA-BIS project - NCN, Poland [2012/05/E/ST10/01578]
Organisationseinheiten:Mathematisch-Naturwissenschaftliche Fakultät / Institut für Physik und Astronomie
DDC-Klassifikation:5 Naturwissenschaften und Mathematik / 53 Physik / 530 Physik
Peer Review:Referiert
Publikationsweg:Open Access / Gold Open-Access
DOAJ gelistet
Lizenz (Englisch):License LogoCreative Commons - Namensnennung-Weitergabe zu gleichen Bedingungen 3.0 Unported
Externe Anmerkung:Zweitveröffentlichung in der Schriftenreihe Postprints der Universität Potsdam : Postprints der Universität Potsdam : Mathematisch-Naturwissenschaftliche Reihe ; 614
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