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Auger- and photoelectron coincidences of molecular O2 adsorbed on Ag(111)

  • The oxygen on Ag(111) system has been investigated with Auger electron-photoelectron coincidence spectroscopy (APECS). The coincidence spectra between O 1s core level photoelectrons and O KLL Auger electrons have been studied together with Ag(3)d/AgM4,5NN coincidences. We also describe the electron-electron coincidence spectrometer setup, CoESCA, consisting of two angle resolved time-of-flight spectrometers at a synchrotron light source. Contributions from molecular oxygen and chemisorbed oxygen are assigned using the coincidence data, conclusions are drawn primarily from the O 1s/O KLL data. The data acquisition and treatment procedure are also outlined. The chemisorbed oxygen species observed are relevant for the catalytic ethylene oxidation.

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Author details:Fredrik O. L. JohanssonORCiD, Torsten LeitnerGND, Ieva BidermaneORCiD, Artur BornGND, Alexander FöhlischORCiDGND, Svante Svensson, Nils MårtenssonORCiD, Andreas LindbladORCiD
DOI:https://doi.org/10.1016/j.elspec.2022.147174
ISSN:0368-2048
ISSN:1873-2526
Title of parent work (English):Journal of electron spectroscopy and related phenomena : the international journal on theoretical and experimental aspects of electron spectroscopy
Publisher:Elsevier
Place of publishing:New York, NY [u.a.]
Publication type:Article
Language:English
Date of first publication:2022/04/01
Publication year:2022
Release date:2024/05/02
Tag:APECS; Auger electron; coincidence; oxygen/Ag(111); photoelectron; spectroscopy
Volume:256
Article number:147174
Number of pages:6
Funding institution:European Union [730872]; Swedish Research Council [2014-6463,; 2018-05336]; Marie Sklodowska Curie Actions [INCA 600398]; K G Westman; foundation
Organizational units:Mathematisch-Naturwissenschaftliche Fakultät / Institut für Physik und Astronomie
Peer review:Referiert
Publishing method:Open Access / Hybrid Open-Access
License (German):License LogoCC-BY - Namensnennung 4.0 International
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