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forum:logopädie 31.2017, 1
(2017)
forum:logopädie 31.2017, 2
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forum:logopädie 31.2017, 3
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forum:logopädie 31.2017, 4
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forum:logopädie 31.2017, 5
(2017)
forum:logopädie 31.2017, 6
(2017)
In many regions of the world, snow accumulation and melt constitute important components of the hydrologic cycle. With the objective to improve model performance of the hydrological model WASA-SED (Water Availability in Semi-Arid environments - SEDiments) in catchments affected by snow and ice, a physically-based snow routine has been implemented into the model. The snow routine bases on the energy-balance method of the ECHSE (Eco-hydrological Simulation Environment) software. A first test application has been conducted in two sub-basins of the Isábena river catchment (Central Spanish Pre-Pyrenees). Results were validated using satellite-derived snow cover data. Furthermore, a rainfall gauge correction algorithm to restore the liquid precipitation signal of measurements affected by solid precipitation was applied. The snow module proved to be able to capture the dynamics of the snow cover forming during the cold months of the year. The temporary storage of water in the snow cover is able to improve simulations of river discharge. General patterns of the temporal evolution of observed and simulated snow cover fractions coincide. The work conducted only represents a first step in the process of implementation and evaluation of a physically-based snow routine into WASA-SED. Future work is necessary to further improve and test the snow routine and to resolve difficulties that occurred during model applications in the catchment.
Stable isotopes in precipitation: Modelling intra-event variations using meteorological parameters
(2017)
The short-term variability of the isotopic composition of precipitation in Golm, Germany was assessed and modelled. Isotopic data (D/H and 18O/16O) on intra-event timescales as well as meteorological data from a weather station and a micro rain radar was used. After data preparation and the combination of all three data sets, a multivariate linear regression analysis was conducted. This was done for four different isotopic response variables and for the entire data set as well as for the two subsets Summer and Winter. The used response variables are the δ18O values as the difference to the corresponding event-based mean and as the difference to the median, and the deuterium excess values as the difference to both the mean and the median. The models were evaluated by comparing the modelled values with the observed ones. This showed that the observations could not be reproduced in a satisfactory way. Therefore, several suggestions on how to possibly improve the methods and thus the modelling results are given in the end.
The dynamics of fragmentation and vibration of molecular systems with a large number of coupled degrees of freedom are key aspects for understanding chemical reactivity and properties. Here we present a resonant inelastic X-ray scattering (RIXS) study to show how it is possible to break down such a complex multidimensional problem into elementary components. Local multimode nuclear wave packets created by X-ray excitation to different core-excited potential energy surfaces (PESs) will act as spatial gates to selectively probe the particular ground-state vibrational modes and, hence, the PES along these modes. We demonstrate this principle by combining ultra-high resolution RIXS measurements for gas-phase water with state-of-the-art simulations.
Die Femtosekundendynamik nach resonanten Photoanregungen mit optischen und Röntgenpulsen ermöglicht eine selektive Verformung von chemischen N‐H‐ und N‐C‐Bindungen in 2‐Thiopyridon in wässriger Lösung. Die Untersuchung der orbitalspezifischen elektronischen Struktur und ihrer Dynamik auf ultrakurzen Zeitskalen mit resonanter inelastischer Röntgenstreuung an der N1s‐Resonanz am Synchrotron und dem Freie‐Elektronen‐Laser LCLS in Kombination mit quantenchemischen Multikonfigurationsberechnungen erbringen den direkten Nachweis dieser kontrollierten photoinduzierten Molekülverformungen und ihrer ultrakurzen Zeitskala.