Quantum dynamics of laser-induced desorption from metal and semiconductor surfaces, and related phenomena
- Recent progress towards a quantum theory of laser-induced desorption and related phenomena is reviewed, for specific examples. These comprise the photodesorption of NO from Pt(111), the scanning tunnelling microscope and laser- induced desorption and switching of H at Si(100), and the electron stimulated desorption and dissociation of CO at Ru(0001). The theoretical methods used for nuclear dynamics range from open-system density matrix theory over nonadiabatically coupled multi-state models to electron-nuclear wavepackets. Also, aspects of time-dependent spectroscopy to probe ultrafast nonadiabatic processes at surfaces will be considered for the example of two-photon photoemission of solvated electrons in ice layers on Cu(111)
Author details: | Peter SaalfrankORCiDGND, Mathias NestGND, Igor V. Andrianov, Tillmann KlamrothORCiDGND, Dominic Kroner, Stephanie BeyversGND |
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URL: | http://iopscience.iop.org/0953-8984/18/30/S05/pdf/0953-8984_18_30_S05.pdf |
DOI: | https://doi.org/10.1088/0953-8984/18/30/S05 |
ISSN: | 1361-648X |
ISSN: | 0953-8984 |
Publisher: | IOP Publ. |
Place of publishing: | Bristol |
Publication type: | Article |
Language: | English |
Date of first publication: | 2006/07/14 |
Publication year: | 2006 |
Release date: | 2017/03/24 |
Volume: | 18 |
Issue: | 30 |
First page: | S1425 |
Last Page: | S1459 |
Source: | Journal of physics-condensed matter. - 18 (2006), 30, S. S1425 - S1459 |
Organizational units: | Mathematisch-Naturwissenschaftliche Fakultät / Institut für Physik und Astronomie |
DDC classification: | 5 Naturwissenschaften und Mathematik / 53 Physik / 530 Physik |
Peer review: | Referiert |
Institution name at the time of the publication: | Mathematisch-Naturwissenschaftliche Fakultät / Institut für Physik |