Free-electron laser based resonant inelastic X-ray scattering on molecules and liquids
- The unprecedented beam properties of free-electron laser based X-ray sources enable novel resonant inelastic X-ray scattering (RIXS) experiments. Femtosecond time-resolved RIXS can be used to follow charge, spin and structural dynamics of dilute solute molecules in solution. Ultrashort X-ray pulses allow probing of highly radiation sensitive states of matter such as the metastable phase of supercooled liquid water. Nonlinear X-ray probes like amplified spontaneous emission and stimulated resonant X-ray scattering provide an enhanced selectivity and sensitivity as well as a path to control radiation damage and increase the photon yields in RIXS experiments. (C) 2015 Elsevier B.V. All rights reserved.
| Verfasserangaben: | Kristjan KunnusORCiD, Simon Schreck, Alexander FöhlischORCiDGND |
|---|---|
| DOI: | https://doi.org/10.1016/j.elspec.2015.08.012 |
| ISSN: | 0368-2048 |
| ISSN: | 1873-2526 |
| Titel des übergeordneten Werks (Englisch): | Journal of electron spectroscopy and related phenomena : the international journal on theoretical and experimental aspects of electron spectroscopy |
| Verlag: | Elsevier |
| Verlagsort: | Amsterdam |
| Publikationstyp: | Wissenschaftlicher Artikel |
| Sprache: | Englisch |
| Jahr der Erstveröffentlichung: | 2015 |
| Erscheinungsjahr: | 2015 |
| Datum der Freischaltung: | 27.03.2017 |
| Freies Schlagwort / Tag: | Free-electron laser; Liquids; Molecules; Nonlinear X-ray spectroscopy; Pump-probe; RIXS |
| Band: | 204 |
| Seitenanzahl: | 11 |
| Erste Seite: | 345 |
| Letzte Seite: | 355 |
| Organisationseinheiten: | Mathematisch-Naturwissenschaftliche Fakultät / Institut für Physik und Astronomie |
| Peer Review: | Referiert |
