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Spatial quantum beats in vibrational resonant inelastic soft X-ray scattering at dissociating states in oxygen

  • Resonant inelastic soft x-ray scattering (RIXS) spectra excited at the 1 sigma(g) -> 3 sigma(u) resonance in gas-phase O-2 show excitations due to the nuclear degrees of freedom with up to 35 well-resolved discrete vibronic states and a continuum due to the kinetic energy distribution of the separated atoms. The RIXS profile demonstrates spatial quantum beats caused by two interfering wave packets with different momenta as the atoms separate. Thomson scattering strongly affects both the spectral profile and the scattering anisotropy.

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Author:Annette Pietzsch, Y. -P. Sun, Franz Hennies, Z. Rinkevicius, Hans O. Karlsson, Thorsten Schmitt, Vladimir N. Strocov, Joakim Andersson, B. Kennedy, J. Schlappa, Alexander Foehlisch, Jan-Erik Rubensson, F. Gel'mukhanov
DOI:https://doi.org/10.1103/PhysRevLett.106.153004
ISSN:0031-9007 (print)
Parent Title (English):Physical review letters
Publisher:American Physical Society
Place of publication:College Park
Document Type:Article
Language:English
Year of first Publication:2011
Year of Completion:2011
Release Date:2017/03/26
Volume:106
Issue:15
Pagenumber:4
Funder:Swedish Research Council (VR); Carl Tryggers Stiftelse (CTS)
Organizational units:Mathematisch-Naturwissenschaftliche Fakultät / Institut für Physik und Astronomie
Peer Review:Referiert