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Analysis of the halo background in femtosecond slicing experiments

  • The slicing facility FemtoSpeX at BESSY II offers unique opportunities to study photo-induced dynamics on femtosecond time scales by means of X-ray magnetic circular dichroism, resonant and non-resonant X-ray diffraction, and X-ray absorption spectroscopy experiments in the soft X-ray regime. Besides femtosecond X-ray pulses, slicing sources inherently also produce a so-called `halo' background with a different time structure, polarization and pointing. Here a detailed experimental characterization of the halo radiation is presented, and a method is demonstrated for its correct and unambiguous removal from femtosecond time-resolved data using a special laser triggering scheme as well as analytical models. Examples are given for time-resolved measurements with corresponding halo correction, and errors of the relevant physical quantities caused by either neglecting or by applying a simplified model to describe this background are estimated.

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Author details:Daniel Schick, Loic Le Guyader, Niko Pontius, Ilie Radu, Torsten KachelORCiD, Rolf MitznerORCiDGND, Thomas Zeschke, Christian Schuessler-LangeheineORCiD, Alexander FöhlischORCiDGND, Karsten Holldack
DOI:https://doi.org/10.1107/S160057751600401X
ISSN:1600-5775
Pubmed ID:https://pubmed.ncbi.nlm.nih.gov/27140149
Title of parent work (English):Journal of synchrotron radiation
Publisher:International Union of Crystallography
Place of publishing:Chester
Publication type:Article
Language:English
Year of first publication:2016
Publication year:2016
Release date:2020/03/22
Tag:X-ray scattering; XMCD; femtosecond slicing; halo; pump-probe
Volume:23
Number of pages:12
First page:700
Last Page:711
Funding institution:Helmholtz Association [PD-142]; European Union through FEMTOSPIN program; Peter-Paul-Ewald Fellowship of the Volkswagen Stiftung
Organizational units:Mathematisch-Naturwissenschaftliche Fakultät / Institut für Physik und Astronomie
Peer review:Referiert
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