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Mapping a plasmonic hologram with photosensitive polymer films: standing versus propagating waves

  • We use a photosensitive layer containing azobenzene moieties to map near-field intensity patterns in the vicinity of nanogrids fabricated within a thin silver layer. It is known that azobenzene containing films deform permanently during irradiation, following the pattern of the field intensity. The photosensitive material reacts only to stationary waves whose intensity patterns do not change in time. In this study, we have found a periodic deformation above the silver film outside the nanostructure, even if the latter consists of just one groove. This is in contradiction to the widely accepted viewpoint that propagating surface plasmon modes dominate outside nanogrids. We explain our observation based on an electromagnetic hologram formed by the constructive interference between a propagating surface plasmon wave and the incident light. This hologram contains a stationary intensity and polarization grating that even appears in the absence of the polymer layer.

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Metadaten
Author details:Thomas Papke, Nataraja Sekhar Yadavalli, Carsten HenkelORCiDGND, Svetlana SanterORCiDGND
DOI:https://doi.org/10.1021/am503501y
ISSN:1944-8244
Pubmed ID:https://pubmed.ncbi.nlm.nih.gov/25046798
Title of parent work (English):ACS applied materials & interfaces
Publisher:American Chemical Society
Place of publishing:Washington
Publication type:Article
Language:English
Year of first publication:2014
Publication year:2014
Release date:2017/03/27
Tag:azobenzene containing photosensitive material; nanostructured metal surface; propagating surface plasmons; surface relief grating
Volume:6
Issue:16
Number of pages:7
First page:14174
Last Page:14180
Organizational units:Mathematisch-Naturwissenschaftliche Fakultät / Institut für Physik und Astronomie
Peer review:Referiert
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