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Shortening x-ray pulses for pump-probe experiments at synchrotrons

  • We implemented an experimental scheme for ultrafast x-ray diffraction at storage rings based on a laser-driven Bragg-switch that shortens the x-ray pulses emitted from an undulator. The increased time-resolution is demonstrated by observing changes of intensity, position and width of the diffraction peaks of a La(0.7)Sr(0.3)MnO(3)/SrTiO(3) superlattice sample after optical excitation, i.e., by quantitatively measuring the propagation of an expansion wave through the sample. These experimental transients with timescales of 35 to 60 ps evidence a reduction of the x-ray pulse duration by a factor of two.

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Author details:Hengameh A. Navirian, Marc HerzogORCiDGND, J. Goldshteyn, Wolfram LeitenbergerGND, Ionella Vrejoiu, D. Khakhulin, M. Wulff, Roman Shayduk, P. Gaal, Matias BargheerORCiDGND
DOI:https://doi.org/10.1063/1.3601057
ISSN:0021-8979
Title of parent work (English):Journal of applied physics
Publisher:American Institute of Physics
Place of publishing:Melville
Publication type:Article
Language:English
Year of first publication:2011
Publication year:2011
Release date:2017/03/26
Volume:109
Issue:12
Number of pages:3
Funding institution:BMBF [05K10IP1]; DFG [SFB 762]
Organizational units:Mathematisch-Naturwissenschaftliche Fakultät / Institut für Physik und Astronomie
Peer review:Referiert
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