Free-electron laser based resonant inelastic X-ray scattering on molecules and liquids
- The unprecedented beam properties of free-electron laser based X-ray sources enable novel resonant inelastic X-ray scattering (RIXS) experiments. Femtosecond time-resolved RIXS can be used to follow charge, spin and structural dynamics of dilute solute molecules in solution. Ultrashort X-ray pulses allow probing of highly radiation sensitive states of matter such as the metastable phase of supercooled liquid water. Nonlinear X-ray probes like amplified spontaneous emission and stimulated resonant X-ray scattering provide an enhanced selectivity and sensitivity as well as a path to control radiation damage and increase the photon yields in RIXS experiments. (C) 2015 Elsevier B.V. All rights reserved.
Author details: | Kristjan KunnusORCiD, Simon Schreck, Alexander FöhlischORCiDGND |
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DOI: | https://doi.org/10.1016/j.elspec.2015.08.012 |
ISSN: | 0368-2048 |
ISSN: | 1873-2526 |
Title of parent work (English): | Journal of electron spectroscopy and related phenomena : the international journal on theoretical and experimental aspects of electron spectroscopy |
Publisher: | Elsevier |
Place of publishing: | Amsterdam |
Publication type: | Article |
Language: | English |
Year of first publication: | 2015 |
Publication year: | 2015 |
Release date: | 2017/03/27 |
Tag: | Free-electron laser; Liquids; Molecules; Nonlinear X-ray spectroscopy; Pump-probe; RIXS |
Volume: | 204 |
Number of pages: | 11 |
First page: | 345 |
Last Page: | 355 |
Organizational units: | Mathematisch-Naturwissenschaftliche Fakultät / Institut für Physik und Astronomie |
Peer review: | Referiert |