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Year of publication
Document Type
- Article (967) (remove)
Keywords
- diffusion (25)
- anomalous diffusion (22)
- gamma rays: general (20)
- ISM: supernova remnants (12)
- cosmic rays (12)
- stars: massive (11)
- organic solar cells (9)
- stars: atmospheres (9)
- astroparticle physics (8)
- perovskite solar cells (8)
Institute
- Institut für Physik und Astronomie (890)
- Institut für Chemie (37)
- Institut für Mathematik (15)
- Extern (8)
- Institut für Geowissenschaften (6)
- Institut für Umweltwissenschaften und Geographie (6)
- Mathematisch-Naturwissenschaftliche Fakultät (5)
- Institut für Biochemie und Biologie (4)
- Fachgruppe Politik- & Verwaltungswissenschaft (3)
- Hasso-Plattner-Institut für Digital Engineering gGmbH (3)
Archambault, S. ; Archer, A. ; Benbow, Wystan ; Bird, Ralph ; Bourbeau, E. ; Buchovecky, M. ; Buckley, J. H. ; Bugaev, V. ; Cerruti, M. ; Connolly, M. P. ; Cui, W. ; Dwarkadas, Vikram V. ; Errando, M. ; Falcone, A. ; Feng, Q. ; Finley, J. P. ; Fleischhack, H. ; Fortson, L. ; Furniss, A. ; Griffin, S. ; Huetten, M. ; Hanna, D. ; Holder, J. ; Johnson, C. A. ; Kaaret, P. ; Kar, P. ; Kelley-Hoskins, N. ; Kertzman, M. ; Kieda, D. ; Krause, M. ; Kumar, S. ; Lang, M. J. ; Maier, G. ; McArthur, S. ; McCann, A. ; Moriarty, P. ; Mukherjee, R. ; Nieto, D. ; Ong, R. A. ; Otte, A. N. ; Park, Nahee ; Pohl, Martin ; Popkow, A. ; Pueschel, Elisa ; Quinn, J. ; Ragan, K. ; Reynolds, P. T. ; Richards, G. T. ; Roache, E. ; Sadeh, I. ; Santander, M. ; Sembroski, G. H. ; Shahinyan, K. ; Slane, P. ; Staszak, D. ; Telezhinsky, Igor O. ; Trepanier, S. ; Tyler, J. ; Wakely, S. P. ; Weinstein, A. ; Weisgarber, T. ; Wilcox, P. ; Wilhelm, Alina ; Williams, D. A. ; Zitzer, B.
Archambault, S. ; Archer, A. ; Benbow, W. ; Bird, Ralph ; Bourbeau, E. ; Bouvier, A. ; Buchovecky, M. ; Bugaev, V. ; Cardenzana, J. V. ; Cerruti, M. ; Ciupik, L. ; Connolly, M. P. ; Cui, W. ; Daniel, M. K. ; Errando, M. ; Falcone, A. ; Feng, Q. ; Finley, J. P. ; Fleischhack, H. ; Fortson, L. ; Furniss, A. ; Gillanders, G. H. ; Griffin, S. ; Hanna, D. ; Hervet, O. ; Holder, J. ; Hughes, G. ; Humensky, T. B. ; Hutten, M. ; Johnson, C. A. ; Kaaret, P. ; Kar, P. ; Kertzman, M. ; Kieda, D. ; Krause, M. ; Lang, M. J. ; Lin, T. T. Y. ; Maier, G. ; McArthur, S. ; Moriarty, P. ; Mukherjee, R. ; Nieto, D. ; Ong, R. A. ; Otte, A. N. ; Park, N. ; Pohl, Martin ; Popkow, A. ; Pueschel, Elisa ; Quinn, J. ; Ragan, K. ; Reynolds, P. T. ; Richards, G. T. ; Roache, E. ; Rulten, C. ; Sadeh, I. ; Sembroski, G. H. ; Shahinyan, K. ; Staszak, D. ; Telezhinsky, Igor O. ; Trepanier, S. ; Wakely, S. P. ; Weinstein, A. ; Wilcox, P. ; Williams, D. A. ; Zitzer, B.
Imaging atmospheric Cherenkov telescopes (IACTs) are equipped with sensitive photomultiplier tube (PMT) cameras. Exposure to high levels of background illumination degrades the efficiency of and potentially destroys these photo-detectors over time, so IACTs cannot be operated in the same configuration in the presence of bright moonlight as under dark skies. Since September 2012, observations have been carried out with the VERITAS IACTs under bright moonlight (defined as about three times the night-sky-background (NSB) of a dark extragalactic field, typically occurring when Moon illumination > 35%) in two observing modes, firstly by reducing the voltage applied to the PMTs and, secondly, with the addition of ultra-violet (UV) bandpass filters to the cameras. This has allowed observations at up to about 30 times previous NSB levels (around 80% Moon illumination), resulting in 30% more observing time between the two modes over the course of a year. These additional observations have already allowed for the detection of a flare from the 1ES 1727 + 502 and for an observing program targeting a measurement of the cosmic-ray positron fraction. We provide details of these new observing modes and their performance relative to the standard VERITAS observations. (C) 2017 Elsevier B.V. All rights reserved.
Ortiz-Amezcua, Pablo ; Guerrero-Rascado, Juan Luis ; Jose Granados-Munoz, Maria ; Benavent-Oltra, Jose Antonio ; Böckmann, Christine ; Samaras, Stefanos ; Stachlewska, Iwona Sylwia ; Janicka, Lucja ; Baars, Holger ; Bohlmann, Stephanie ; Alados-Arboledas, Lucas
Strong events of long-range transported biomass burning aerosol were detected during July 2013 at three EARLINET (European Aerosol Research Lidar Network) stations, namely Granada (Spain), Leipzig (Germany) and Warsaw (Poland). Satellite observations from MODIS (Moderate Resolution Imaging Spectroradiometer) and CALIOP (Cloud-Aerosol Lidar with Orthogonal Polarization) instruments, as well as modeling tools such as HYSPLIT (Hybrid Single-Particle Lagrangian Integrated Trajectory) and NAAPS (Navy Aerosol Analysis and Prediction System), have been used to estimate the sources and transport paths of those North American forest fire smoke particles. A multiwavelength Raman lidar technique was applied to obtain vertically resolved particle optical properties, and further inversion of those properties with a regularization algorithm allowed for retrieving microphysical information on the studied particles. The results highlight the presence of smoke layers of 1-2 km thickness, located at about 5 km a.s.l. altitude over Granada and Leipzig and around 2.5 km a.s.l. at Warsaw. These layers were intense, as they accounted for more than 30% of the total AOD (aerosol optical depth) in all cases, and presented optical and microphysical features typical for different aging degrees: color ratio of lidar ratios (LR532/LR355) around 2, alpha-related angstrom exponents of less than 1, effective radii of 0.3 mu m and large values of single scattering albedos (SSA), nearly spectrally independent. The intensive microphysical properties were compared with columnar retrievals form co-located AERONET (Aerosol Robotic Network) stations. The intensity of the layers was also characterized in terms of particle volume concentration, and then an experimental relationship between this magnitude and the particle extinction coefficient was established.
In order to analyse the sensitivity of the equatorial ionospheric current system, i.e. the solar quiet current system and the equatorial electrojet, to solar cycle variations and to the secular variation of the geomagnetic main field, we have analysed 51 years (1935-1985) of geomagnetic observatory data from Huancayo, Peru. This period is ideal to analyse the influence of the main field strength on the amplitude of the quiet daily variation, since the main field decreases significantly from 1935 to 1985, while the distance of the magnetic equator to the observatory remains stable. To this end, we digitised some 19 years of hourly mean values of the horizontal component (H), which have not been available digitally at the World Data Centres. Then, the sensitivity of the amplitude Ali of the quiet daily variation to both solar cycle variations (in terms of sunspot numbers and solar flux F10.7) and changes of the geomagnetic main field strength (due to secular variation) was determined. We confirm an increase of Delta H for the decreasing main field in this period, as expected from physics based models (Cnossen, 2016), but with a somewhat smaller rate of 4.4% (5.8% considering one standard error) compared with 6.9% predicted by the physics based model.
Jošt, Marko ; Albrecht, Steve ; Kegelmann, Lukas ; Wolff, Christian Michael ; Lang, Felix ; Lipovšek, Benjamin ; Krč, Janez ; Korte, Lars ; Neher, Dieter ; Rech, Bernd ; Topič, Marko
Inorganic-organic perovskites like methylammonium-lead-iodide have proven to be an effective class of 17 materials for fabricating efficient solar cells. To improve their performance, light management techniques using textured surfaces, similar to those used in established solar cell technologies, should be considered. Here, we apply a light management foil created by UV nanoimprint lithography on the glass side of an inverted (p-i-n) perovskite solar cell with 16.3% efficiency. The obtained 1 mA cm(-2) increase in the short-circuit current density translates to a relative improvement in cell performance of 5%, which results in a power conversion efficiency of 17.1%. Optical 3D simulations based on experimentally obtained parameters were used to support the experimental findings. A good match between the simulated and experimental data was obtained, validating the model. Optical simulations reveal that the main improvement in device performance is due to a reduction in total reflection and that relative improvement in the short-circuit current density of up to 10% is possible for large-area devices. Therefore, our results present the potential of light management foils for improving the device performance of perovskite solar cells and pave the way for further use of optical simulations in the field of perovskite solar cells.
Absorption Tails of Donor
(2017)
Vandewal, Koen ; Benduhn, Johannes ; Schellhammer, Karl Sebastian ; Vangerven, Tim ; Rückert, Janna E. ; Piersimoni, Fortunato ; Scholz, Reinhard ; Zeika, Olaf ; Fan, Yeli ; Barlow, Stephen ; Neher, Dieter ; Marder, Seth R. ; Manca, Jean ; Spoltore, Donato ; Cuniberti, Gianaurelio ; Ortmann, Frank
In disordered organic semiconductors, the transfer of a rather localized charge carrier from one site to another triggers a deformation of the molecular structure quantified by the intramolecular relaxation energy. A similar structural relaxation occurs upon population of intermolecular charge-transfer (CT) states formed at organic electron donor (D)-acceptor (A) interfaces. Weak CT absorption bands for D A complexes occur at photon energies below the optical gaps of both the donors and the C-60 acceptor as a result of optical transitions from the neutral ground state to the ionic CT state. In this work, we show that temperature-activated intramolecular vibrations of the ground state play a major role in determining the line shape of such CT absorption bands. This allows us to extract values for the relaxation energy related to the geometry change from neutral to ionic CT complexes. Experimental values for the relaxation energies of 20 D:C-60 CT complexes correlate with values calculated within density functional theory. These results provide an experimental method for determining the polaron relaxation energy in solid-state organic D-A blends and show the importance of a reduced relaxation energy, which we introduce to characterize thermally activated CT processes.
Schubert, Marcel ; Frisch, Johannes ; Allard, Sybille ; Preis, Eduard ; Scherf, Ullrich ; Koch, Norbert ; Neher, Dieter
The recent development of donor–acceptor copolymers has led to an enormous improvement in the performance of organic solar cells and organic field-effect transistors. Here we describe the synthesis, detailed characterisation, and application of a series of structurally modified copolymers to investigate fundamental structure–property relationships in this class of conjugated polymers. The interplay between chemical structure and optoelectronic properties is investigated. These are further correlated to the charge transport and solar cell performance, which allows us to link their chemical structure to the observed physical properties.
Abeysekara, A. U. ; Archambault, S. ; Archer, A. ; Benbow, Wystan ; Bird, Ralph ; Buchovecky, M. ; Buckley, J. H. ; Bugaev, V. ; Byrum, K. ; Cerruti, M. ; Chen, X. ; Ciupik, L. ; Cui, W. ; Dickinson, H. J. ; Eisch, J. D. ; Errando, M. ; Falcone, A. ; Feng, Q. ; Finley, J. P. ; Fleischhack, H. ; Fortson, L. ; Furniss, A. ; Gillanders, G. H. ; Griffin, S. ; Grube, J. ; Hutten, M. ; Hakansson, N. ; Hanna, D. ; Holder, J. ; Humensky, T. B. ; Johnson, C. A. ; Kaaret, P. ; Kar, P. ; Kertzman, M. ; Kieda, D. ; Krause, M. ; Krennrich, F. ; Kumar, S. ; Lang, M. J. ; Maier, G. ; McArthur, S. ; McCann, A. ; Meagher, K. ; Moriarty, P. ; Mukherjee, R. ; Nguyen, T. ; Nieto, D. ; Ong, R. A. ; Otte, A. N. ; Park, N. ; Pelassa, V. ; Pohl, Martin ; Popkow, A. ; Pueschel, Elisa ; Quinn, J. ; Ragan, K. ; Reynolds, P. T. ; Richards, G. T. ; Roache, E. ; Rulten, C. ; Santander, M. ; Sembroski, G. H. ; Shahinyan, K. ; Staszak, D. ; Telezhinsky, Igor O. ; Tucci, J. V. ; Tyler, J. ; Wakely, S. P. ; Weiner, O. M. ; Weinstein, A. ; Wilhelm, Alina ; Williams, D. A. ; Fegan, S. ; Giebels, B. ; Horan, D. ; Berdyugin, A. ; Kuan, J. ; Lindfors, E. ; Nilsson, K. ; Oksanen, A. ; Prokoph, H. ; Reinthal, R. ; Takalo, L. ; Zefi, F.
B2 1215+30 is a BL-Lac-type blazar that was first detected at TeV energies by the MAGIC atmospheric Cherenkov telescopes and subsequently confirmed by the Very Energetic Radiation Imaging Telescope Array System (VERITAS) observatory with data collected between 2009 and 2012. In 2014 February 08, VERITAS detected a large-amplitude flare from B2. 1215+30 during routine monitoring observations of the blazar 1ES. 1218+304, located in the same field of view. The TeV flux reached 2.4 times the Crab Nebula flux with a variability timescale of <3.6 hr. Multiwavelength observations with Fermi-LAT, Swift, and the Tuorla Observatory revealed a correlated high GeV flux state and no significant optical counterpart to the flare, with a spectral energy distribution where the gamma-ray luminosity exceeds the synchrotron luminosity. When interpreted in the framework of a onezone leptonic model, the observed emission implies a high degree of beaming, with Doppler factor delta > 10, and an electron population with spectral index p < 2.3.
Significant progress has been made in recent years in understanding acceleration mechanisms in the Earth's radiation belts. In particular, a number of studies demonstrated the importance of the local acceleration by analyzing the radial profiles of phase space density (PSD) and observing building up peaks in PSD. In this study, we focus on understanding of the local loss using very similar tools. The profiles of PSD for various values of the first adiabatic invariants during the previously studied 17 January 2013 storm are presented and discussed. The profiles of PSD show clear deepening minimums consistent with the scattering by electromagnetic ion cyclotron waves. Long-term evolution shows that local minimums in PSD can persist for relatively long times. During considered interval of time the deepening minimums were observed around L* = 4 during 17 January 2013 storm and around L* = 3.5 during 1 March 2013 storm. This study shows a new method that can help identify the location, magnitude, and time of the local loss and will help quantify local loss in the future. This study also provides additional clear and definitive evidence that local loss plays a major role for the dynamics of the multi-MeV electrons.
gamma Cassiopeia (gamma Cas), is known to be a binary system consisting of a Be-type star and a low-mass (M similar to 1M(circle dot)) companion of unknown nature orbiting in the Be-disc plane. Here, we apply the quasi-spherical accretion theory on to a compact magnetized star and show that if the low-mass companion of gamma Cas is a fast spinning neutron star, the key observational signatures of. Cas are remarkably well reproduced. Direct accretion on to this fast rotating neutron star is impeded by the propeller mechanism. In this case, around the neutron star magnetosphere a hot shell is formed which emits thermal X-rays in qualitative and quantitative agreement with observed properties of the X-ray emission from gamma Cas. We suggest that gamma Cas and its analogues constitute a new subclass of Be-type X-ray binaries hosting rapidly rotating neutron stars formed in supernova explosions with small kicks. The subsequent evolutionary stage of gamma Cas and its analogues should be the X Per-type binaries comprising low-luminosity slowly rotating X-ray pulsars. The model explains the enigmatic X-ray emission from gamma Cas, and also establishes evolutionary connections between various types of rotating magnetized neutron stars in Be-binaries.