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Year of publication
Document Type
- Article (233) (remove)
Language
- English (233)
Is part of the Bibliography
- yes (233)
Keywords
- organic solar cells (11)
- perovskite solar cells (10)
- morphology (5)
- solar cells (5)
- charge transport (4)
- conjugated polymers (4)
- non-fullerene acceptors (4)
- voltage losses (4)
- Solar cells (3)
- open-circuit voltage (3)
Institute
- Institut für Physik und Astronomie (233) (remove)
Perdigón-Toro, Lorena ; Le Quang Phuong ; Zeiske, Stefan ; Vandewal, Koen ; Armin, Ardalan ; Shoaee, Safa ; Neher, Dieter
Non-fullerene acceptors (NFAs) are far more emissive than their fullerene-based counterparts. Here, we study the spectral properties of photocurrent generation and recombination of the blend of the donor polymer PM6 with the NFA Y6. We find that the radiative recombination of free charges is almost entirely due to the re-occupation and decay of Y6 singlet excitons, but that this pathway contributes less than 1% to the total recombination. As such, the open-circuit voltage of the PM6:Y6 blend is determined by the energetics and kinetics of the charge-transfer (CT) state. Moreover, we find that no information on the energetics of the CT state manifold can be gained from the low-energy tail of the photovoltaic external quantum efficiency spectrum, which is dominated by the excitation spectrum of the Y6 exciton. We, finally, estimate the charge-separated state to lie only 120 meV below the Y6 singlet exciton energy, meaning that this blend indeed represents a high-efficiency system with a low energetic offset.
Warby, Jonathan ; Zu, Fengshuo ; Zeiske, Stefan ; Gutierrez-Partida, Emilio ; Frohloff, Lennart ; Kahmann, Simon ; Frohna, Kyle ; Mosconi, Edoardo ; Radicchi, Eros ; Lang, Felix ; Shah, Sahil ; Pena-Camargo, Francisco ; Hempel, Hannes ; Unold, Thomas ; Koch, Norbert ; Armin, Ardalan ; De Angelis, Filippo ; Stranks, Samuel D. ; Neher, Dieter ; Stolterfoht, Martin
Perovskite semiconductors are an attractive option to overcome the limitations of established silicon based photovoltaic (PV) technologies due to their exceptional opto-electronic properties and their successful integration into multijunction cells. However, the performance of single- and multijunction cells is largely limited by significant nonradiative recombination at the perovskite/organic electron transport layer junctions. In this work, the cause of interfacial recombination at the perovskite/C-60 interface is revealed via a combination of photoluminescence, photoelectron spectroscopy, and first-principle numerical simulations. It is found that the most significant contribution to the total C-60-induced recombination loss occurs within the first monolayer of C-60, rather than in the bulk of C-60 or at the perovskite surface. The experiments show that the C-60 molecules act as deep trap states when in direct contact with the perovskite. It is further demonstrated that by reducing the surface coverage of C-60, the radiative efficiency of the bare perovskite layer can be retained. The findings of this work pave the way toward overcoming one of the most critical remaining performance losses in perovskite solar cells.
Ye, Fangyuan ; Zhang, Shuo ; Warby, Jonathan ; Wu, Jiawei ; Gutierrez-Partida, Emilio ; Lang, Felix ; Shah, Sahil ; Saglamkaya, Elifnaz ; Sun, Bowen ; Zu, Fengshuo ; Shoai, Safa ; Wang, Haifeng ; Stiller, Burkhard ; Neher, Dieter ; Zhu, Wei-Hong ; Stolterfoht, Martin ; Wu, Yongzhen
Inverted perovskite solar cells still suffer from significant non-radiative recombination losses at the perovskite surface and across the perovskite/C₆₀ interface, limiting the future development of perovskite-based single- and multi-junction photovoltaics. Therefore, more effective inter- or transport layers are urgently required. To tackle these recombination losses, we introduce ortho-carborane as an interlayer material that has a spherical molecular structure and a three-dimensional aromaticity. Based on a variety of experimental techniques, we show that ortho-carborane decorated with phenylamino groups effectively passivates the perovskite surface and essentially eliminates the non-radiative recombination loss across the perovskite/C₆₀ interface with high thermal stability. We further demonstrate the potential of carborane as an electron transport material, facilitating electron extraction while blocking holes from the interface. The resulting inverted perovskite solar cells deliver a power conversion efficiency of over 23% with a low non-radiative voltage loss of 110 mV, and retain >97% of the initial efficiency after 400 h of maximum power point tracking. Overall, the designed carborane based interlayer simultaneously enables passivation, electron-transport and hole-blocking and paves the way toward more efficient and stable perovskite solar cells.