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Year of publication
Language
- English (248)
Is part of the Bibliography
- yes (248)
Keywords
- organic solar cells (13)
- perovskite solar cells (12)
- morphology (5)
- solar cells (5)
- voltage losses (5)
- Organic solar cells (4)
- charge transport (4)
- conjugated polymers (4)
- non-fullerene acceptors (4)
- photoluminescence (4)
Institute
- Institut für Physik und Astronomie (248) (remove)
Oda, Masao ; Nothofer, Heinz-Georg ; Lieser, G. ; Scherf, Ullrich ; Meskers, S. C. J. ; Neher, Dieter
Pralle, Martin U. ; Urayama, Kenji ; Tew, Gregory N. ; Neher, Dieter ; Wegner, Gerhard ; Stupp, Samuel I.
Enhanced charge selectivity via anodic-C60 layer reduces nonradiative losses in organic solar cells
(2021)
Pranav, Manasi ; Benduhn, Johannes ; Nyman, Mathias ; Hosseini, Seyed Mehrdad ; Kublitski, Jonas ; Shoaee, Safa ; Neher, Dieter ; Leo, Karl ; Spoltore, Donato
Interfacial layers in conjunction with suitable charge-transport layers can significantly improve the performance of optoelectronic devices by facilitating efficient charge carrier injection and extraction.
This work uses a neat C-60 interlayer on the anode to experimentally reveal that surface recombination is a significant contributor to nonradiative recombination losses in organic solar cells.
These losses are shown to proportionally increase with the extent of contact between donor molecules in the photoactive layer and a molybdenum oxide (MoO3) hole extraction layer, proven by calculating voltage losses in low- and high-donor-content bulk heterojunction device architectures.
Using a novel in-device determination of the built-in voltage, the suppression of surface recombination, due to the insertion of a thin anodic-C-60 interlayer on MoO3, is attributed to an enhanced built-in potential.
The increased built-in voltage reduces the presence of minority charge carriers at the electrodes-a new perspective on the principle of selective charge extraction layers.
The benefit to device efficiency is limited by a critical interlayer thickness, which depends on the donor material in bilayer devices.
Given the high popularity of MoO3 as an efficient hole extraction and injection layer and the increasingly popular discussion on interfacial phenomena in organic optoelectronic devices, these findings are relevant to and address different branches of organic electronics, providing insights for future device design.
Li, Tian-yi ; Benduhn, Johannes ; Qiao, Zhi ; Liu, Yuan ; Li, Yue ; Shivhare, Rishi ; Jaiser, Frank ; Wang, Pei ; Ma, Jie ; Zeika, Olaf ; Neher, Dieter ; Mannsfeld, Stefan C. B. ; Ma, Zaifei ; Vandewal, Koen ; Leo, Karl
An understanding of the factors limiting the open-circuit voltage (V-oc) and related photon energy loss mechanisms is critical to increase the power conversion efficiency (PCE) of small-molecule organic solar cells (OSCs), especially those with near-infrared (NIR) absorbers. In this work, two NIR boron dipyrromethene (BODIPY) molecules are characterized for application in planar (PHJ) and bulk (BHJ) heterojunction OSCs. When two H atoms are substituted by F atoms on the peripheral phenyl rings of the molecules, the molecular aggregation type in the thin film changes from the H-type to J-type. For PHJ devices, the nonradiative voltage loss of 0.35 V in the J-aggregated BODIPY is lower than that of 0.49 V in the H-aggregated device. In BHJ devices with a nonradiative voltage loss of 0.35 V, a PCE of 5.5% is achieved with an external quantum efficiency (EQE) maximum of 68% at 700 nm.
Yang, Xiao Hui ; Jaiser, Frank ; Stiller, Burkhard ; Neher, Dieter ; Galbrecht, Frank ; Scherf, Ullrich
It is shown that several polymers can form insoluble interfacial layers on a poly (ethylenedioxythiophene):poly(styrene sulfonate) (PEDOT:PSS) layer after annealing of the double-layer structure. The thickness of the interlayer is dependent on the characteristics of the underlying PEDOT.PSS and the molecular weight of the polymers. It is further shown that the electronic structures of the interlayer polymers have a significant effect on the properties of red-light-emitting polymer-based electrophosphorescent devices. Upon increasing the highest occupied molecular orbital and lowest unoccupied molecular orbital positions, a significant increase in current density and device efficiency is observed. This is attributed to efficient blocking of electrons in combination with direct injection of holes from the interlayer to the phosphorescent dye. Upon proper choice of the interlayer polymer, efficient red, polymer-based electrophosphorescent devices with a peak luminance efficiency of 5.5 cd A(-1) (external quantum efficiency = 6 %) and a maximum power-conversion efficiency of 5 Im W-1 can be realized.
Kurpiers, Jona ; Ferron, Thomas ; Roland, Steffen ; Jakoby, Marius ; Thiede, Tobias ; Jaiser, Frank ; Albrecht, Steve ; Janietz, Silvia ; Collins, Brian A. ; Howard, Ian A. ; Neher, Dieter
The fact that organic solar cells perform efficiently despite the low dielectric constant of most photoactive blends initiated a long-standing debate regarding the dominant pathways of free charge formation. Here, we address this issue through the accurate measurement of the activation energy for free charge photogeneration over a wide range of photon energy, using the method of time-delayed collection field. For our prototypical low bandgap polymer:fullerene blends, we find that neither the temperature nor the field dependence of free charge generation depend on the excitation energy, ruling out an appreciable contribution to free charge generation though hot carrier pathways. On the other hand, activation energies are on the order of the room temperature thermal energy for all studied blends. We conclude that charge generation in such devices proceeds through thermalized charge transfer states, and that thermal energy is sufficient to separate most of these states into free charges.