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We have used x-ray waveguides as highly confining optical elements for nanoscale imaging of unstained biological cells using the simple geometry of in-line holography. The well-known twin-image problem is effectively circumvented by a simple and fast iterative reconstruction. The algorithm which combines elements of the classical Gerchberg-Saxton scheme and the hybrid-input-output algorithm is optimized for phase-contrast samples, well-justified for imaging of cells at multi-keV photon energies. The experimental scheme allows for a quantitative phase reconstruction from a single holographic image without detailed knowledge of the complex illumination function incident on the sample, as demonstrated for freeze-dried cells of the eukaryotic amoeba Dictyostelium discoideum. The accessible resolution range is explored by simulations, indicating that resolutions on the order of 20 nm are within reach applying illumination times on the order of minutes at present synchrotron sources.
Oskinova, Lidia M. ; Hamann, Wolf-Rainer ; Cassinelli, Joseph P. ; Brown, John C. ; Todt, Helge Tobias
We investigate the connections between the magnetic fields and the X-ray emission from massive stars. Our study shows that the X-ray properties of known strongly magnetic stars are diverse: while some comply to the predictions of the magnetically confined wind model, others do not. We conclude that strong, hard, and variable X-ray emission may be a sufficient attribute of magnetic massive stars, but it is not a necessary one. We address the general properties of X-ray emission from "normal" massive stars, especially the long standing mystery about the correlations between the parameters of X-ray emission and fundamental stellar properties. The recent development in stellar structure modeling shows that small-scale surface magnetic fields may be common. We suggest a "hybrid" scenario which could explain the X-ray emission from massive stars by a combination of magnetic mechanisms on the surface and shocks in the stellar wind. The magnetic mechanisms and the wind shocks are triggered by convective motions in sub-photospheric layers. This scenario opens the door for a natural explanation of the well established correlation between bolometric and X-ray luminosities.
Working memory maintenance of grasp-target information in the human posterior parietal cortex
(2011)
Fiehler, Katja ; Bannert, Michael M. ; Bischoff, Matthias ; Blecker, Carlo ; Stark, Rudolf ; Vaitl, Dieter ; Franz, Volker H. ; Roesler, Frank
Event-related functional magnetic resonance imaging was applied to identify cortical areas involved in maintaining target information in working memory used for an upcoming grasping action. Participants had to grasp with their thumb and index finger of the dominant right hand three-dimensional objects of different size and orientation. Reaching-to-grasp movements were performed without visual feedback either immediately after object presentation or after a variable delay of 2-12 s. The right inferior parietal cortex demonstrated sustained neural activity throughout the delay, which overlapped with activity observed during encoding of the grasp target. Immediate and delayed grasping activated similar motor-related brain areas and showed no differential activity. The results suggest that the right inferior parietal cortex plays an important functional role in working memory maintenance of grasp-related information. Moreover, our findings confirm the assumption that brain areas engaged in maintaining information are also involved in encoding the same information, and thus extend previous findings on working memory function of the posterior parietal cortex in saccadic behavior to reach-to-grasp movements.
Aliu, E. ; Arlen, T. ; Aune, T. ; Beilicke, M. ; Benbow, W. ; Boettcher, Markus ; Bouvier, A. ; Bradbury, S. M. ; Buckley, J. H. ; Bugaev, V. ; Cannon, A. ; Cesarini, A. ; Ciupik, L. ; Collins-Hughes, E. ; Connolly, M. P. ; Cui, W. ; Dickherber, R. ; Errando, M. ; Falcone, A. ; Finley, J. P. ; Fortson, L. ; Furniss, A. ; Galante, N. ; Gall, D. ; Gillanders, G. H. ; Godambe, S. ; Griffin, S. ; Grube, J. ; Gyuk, G. ; Hanna, D. ; Holder, J. ; Huan, H. ; Hughes, G. ; Hui, C. M. ; Humensky, T. B. ; Kaaret, P. ; Karlsson, N. ; Kertzman, M. ; Kieda, D. ; Krawczynski, H. ; Krennrich, F. ; Madhavan, A. S. ; Maier, G. ; Majumdar, P. ; McArthur, S. ; McCann, A. ; Moriarty, P. ; Mukherjee, R. ; Ong, R. A. ; Orr, M. ; Otte, A. N. ; Park, N. ; Perkins, J. S. ; Pichel, A. ; Pohl, Martin ; Prokoph, H. ; Quinn, J. ; Ragan, K. ; Reyes, L. C. ; Reynolds, P. T. ; Roache, E. ; Rose, H. J. ; Ruppel, J. ; Saxon, D. B. ; Schroedter, M. ; Sembroski, G. H. ; Skole, C. ; Smith, A. W. ; Staszak, D. ; Tesic, G. ; Theiling, M. ; Thibadeau, S. ; Tsurusaki, K. ; Tyler, J. ; Varlotta, A. ; Vincent, S. ; Vivier, M. ; Wakely, S. P. ; Ward, J. E. ; Weinstein, A. ; Weisgarber, T. ; Williams, D. A.
We report on very high energy (>100 GeV) gamma-ray observations of Swift J164449.3+573451, an unusual transient object first detected by the Swift Observatory and later detected by multiple radio, optical, and X-ray observatories. A total exposure of 28 hr was obtained on Swift J164449.3+573451 with the Very Energetic Radiation Imaging Telescope Array System ( VERITAS) during 2011 March 28-April 15. We do not detect the source and place a differential upper limit on the emission at 500 GeV during these observations of 1.4 x 10(-12) erg cm(-2) s(-1) (99% confidence level). We also present time-resolved upper limits and use a flux limit averaged over the X-ray flaring period to constrain various emission scenarios that can accommodate both the radio-through-X-ray emission detected from the source and the lack of detection by VERITAS.
Acciari, V. A. ; Aliu, E. ; Arlen, T. ; Aune, T. ; Beilicke, M. ; Benbow, W. ; Bradbury, S. M. ; Buckley, J. H. ; Bugaev, V. ; Byrum, K. ; Cannon, A. ; Cesarini, A. ; Ciupik, L. ; Collins-Hughes, E. ; Connolly, M. P. ; Cui, W. ; Dickherber, R. ; Duke, C. ; Errando, M. ; Falcone, A. ; Finley, J. P. ; Finnegan, G. ; Fortson, L. ; Furniss, A. ; Galante, N. ; Gall, D. ; Gillanders, G. H. ; Godambe, S. ; Griffin, S. ; Grube, J. ; Guenette, R. ; Gyuk, G. ; Hanna, D. ; Holder, J. ; Hughes, G. ; Hui, C. M. ; Humensky, T. B. ; Kaaret, P. ; Karlsson, N. ; Kertzman, M. ; Kieda, D. ; Krawczynski, H. ; Krennrich, F. ; Lang, M. J. ; LeBohec, S. ; Maier, G. ; Majumdar, P. ; McArthur, S. ; McCann, A. ; Moriarty, P. ; Mukherjee, R. ; Ong, R. A. ; Orr, M. ; Otte, A. N. ; Park, N. ; Perkins, J. S. ; Pohl, Martin ; Prokoph, H. ; Quinn, J. ; Ragan, K. ; Reyes, L. C. ; Reynolds, P. T. ; Roache, E. ; Rose, H. J. ; Ruppel, J. ; Saxon, D. B. ; Schroedter, M. ; Sembroski, G. H. ; Senturk, G. D. ; Smith, A. W. ; Staszak, D. ; Tesic, G. ; Theiling, M. ; Thibadeau, S. ; Tsurusaki, K. ; Varlotta, A. ; Vassiliev, V. V. ; Vincent, S. ; Vivier, M. ; Wakely, S. P. ; Ward, J. E. ; Weekes, T. C. ; Weinstein, A. ; Weisgarber, T. ; Williams, D. A. ; Zitzer, B.
We present the results of observations of the TeV binary LS I + 61 degrees 303 with the VERITAS telescope array between 2008 and 2010, at energies above 300 GeV. In the past, both ground-based gamma-ray telescopes VERITAS and MAGIC have reported detections of TeV emission near the apastron phases of the binary orbit. The observations presented here show no strong evidence for TeV emission during these orbital phases; however, during observations taken in late 2010, significant emission was detected from the source close to the phase of superior conjunction (much closer to periastron passage) at a 5.6 standard deviation (5.6 sigma) post-trials significance. In total, between 2008 October and 2010 December a total exposure of 64.5 hr was accumulated with VERITAS on LS I + 61 degrees 303, resulting in an excess at the 3.3 sigma significance level for constant emission over the entire integrated data set. The flux upper limits derived for emission during the previously reliably active TeV phases (i.e., close to apastron) are less than 5% of the Crab Nebula flux in the same energy range. This result stands in apparent contrast to previous observations by both MAGIC and VERITAS which detected the source during these phases at 10% of the Crab Nebula flux. During the two year span of observations, a large amount of X-ray data were also accrued on LS I + 61 degrees 303 by the Swift X-ray Telescope and the Rossi X-ray Timing Explorer Proportional Counter Array. We find no evidence for a correlation between emission in the X-ray and TeV regimes during 20 directly overlapping observations. We also comment on data obtained contemporaneously by the Fermi Large Area Telescope.
Acciari, V. A. ; Aliu, E. ; Arlen, T. ; Aune, T. ; Beilicke, M. ; Benbow, W. ; Bradbury, S. M. ; Buckley, J. H. ; Bugaev, V. ; Byrum, K. ; Cannon, A. ; Cesarini, A. ; Christiansen, J. L. ; Ciupik, L. ; Collins-Hughes, E. ; Connolly, M. P. ; Cui, W. ; Duke, C. ; Errando, M. ; Falcone, A. ; Finley, J. P. ; Finnegan, G. ; Fortson, L. ; Furniss, A. ; Galante, N. ; Gall, D. ; Godambe, S. ; Griffin, S. ; Grube, J. ; Guenette, R. ; Gyuk, G. ; Hanna, D. ; Holder, J. ; Hughes, G. ; Hui, C. M. ; Humensky, T. B. ; Jackson, D. J. ; Kaaret, P. ; Karlsson, N. ; Kertzman, M. ; Kieda, D. ; Krawczynski, H. ; Krennrich, F. ; Lang, M. J. ; Madhavan, A. S. ; Maier, G. ; McArthur, S. ; McCann, A. ; Moriarty, P. ; Newbold, M. D. ; Ong, R. A. ; Orr, M. ; Otte, A. N. ; Park, N. ; Perkins, J. S. ; Pohl, Martin ; Prokoph, H. ; Quinn, J. ; Ragan, K. ; Reyes, L. C. ; Reynolds, P. T. ; Roache, E. ; Rose, H. J. ; Ruppel, J. ; Saxon, D. B. ; Schroedter, M. ; Sembroski, G. H. ; Sentuerk, G. D. ; Smith, A. W. ; Staszak, D. ; Swordy, S. P. ; Tesic, G. ; Theiling, M. ; Thibadeau, S. ; Tsurusaki, K. ; Varlotta, A. ; Vassiliev, V. V. ; Vincent, S. ; Vivier, M. ; Wakely, S. P. ; Ward, J. E. ; Weekes, T. C. ; Weinstein, A. ; Weisgarber, T. ; Williams, D. A. ; Wood, M.
We present the results of 16 Swift-triggered Gamma-ray burst (GRB) follow-up observations taken with the Very Energetic Radiation Imaging Telescope Array System (VERITAS) telescope array from 2007 January to 2009 June. The median energy threshold and response time of these observations were 260 GeV and 320 s, respectively. Observations had an average duration of 90 minutes. Each burst is analyzed independently in two modes: over the whole duration of the observations and again over a shorter timescale determined by the maximum VERITAS sensitivity to a burst with a t(-1.5) time profile. This temporal model is characteristic of GRB afterglows with high-energy, long-lived emission that have been detected by the Large Area Telescope on board the Fermi satellite. No significant very high energy (VHE) gamma-ray emission was detected and upper limits above the VERITAS threshold energy are calculated. The VERITAS upper limits are corrected for gamma-ray extinction by the extragalactic background light and interpreted in the context of the keV emission detected by Swift. For some bursts the VHE emission must have less power than the keV emission, placing constraints on inverse Compton models of VHE emission.
Arhammar, C. ; Pietzsch, Annette ; Bock, Nicolas ; Holmstroem, Erik ; Araujo, C. Moyses ; Grasjo, Johan ; Zhao, Shuxi ; Green, Sara ; Peery, T. ; Hennies, Franz ; Amerioun, Shahrad ; Föhlisch, Alexander ; Schlappa, Justine ; Schmitt, Thorsten ; Strocov, Vladimir N. ; Niklasson, Gunnar A. ; Wallace, Duane C. ; Rubensson, Jan-Erik ; Johansson, Borje ; Ahuja, Rajeev C.
Amorphous materials represent a large and important emerging area of material's science. Amorphous oxides are key technological oxides in applications such as a gate dielectric in Complementary metal-oxide semiconductor devices and in Silicon-Oxide-Nitride-Oxide-Silicon and TANOS (TaN-Al2O3-Si3N4-SiO2-Silicon) flash memories. These technologies are required for the high packing density of today's integrated circuits. Therefore the investigation of defect states in these structures is crucial. In this work we present X-ray synchrotron measurements, with an energy resolution which is about 5-10 times higher than is attainable with standard spectrometers, of amorphous alumina. We demonstrate that our experimental results are in agreement with calculated spectra of amorphous alumina which we have generated by stochastic quenching. This first principles method, which we have recently developed, is found to be superior to molecular dynamics in simulating the rapid gas to solid transition that takes place as this material is deposited for thin film applications. We detect and analyze in detail states in the band gap that originate from oxygen pairs. Similar states were previously found in amorphous alumina by other spectroscopic methods and were assigned to oxygen vacancies claimed to act mutually as electron and hole traps. The oxygen pairs which we probe in this work act as hole traps only and will influence the information retention in electronic devices. In amorphous silica oxygen pairs have already been found, thus they may be a feature which is characteristic also of other amorphous metal oxides.
Polymer foams and void-containing polymer-film systems with internally charged voids combine large piezoelectricity with mechanical flexibility and elastic compliance. This new class of soft materials (often called ferro-or piezoelectrets) has attracted considerable attention from science and industry. It has been found that the voids can be internally charged by means of dielectric barrier discharges (DBDs) under high electric fields. The charged voids can be considered as man-made macroscopic dipoles. Depending on the ferroelectret structure and the pressure of the internal gas, the voids may be highly compressible. Consequently, very large dipole-moment changes can be induced by mechanical or electrical stresses, leading to large piezoelectricity. DBD charging of the voids is a critical process for rendering polymer foams piezoelectric. Thus a comprehensive exploration of DBD charging is essential for the understanding and the optimization of piezoelectricity in ferroelectrets. Recent studies show that DBDs in the voids are triggered when the internal electric field reaches a threshold value according to Townsend's model of Paschen breakdown. During the DBDs, charges of opposite polarity are generated and trapped at the top and bottom internal surfaces of the gas-filled voids, respectively. The deposited charges induce an electric field opposite to the externally applied one and thus extinguish the DBDs. Back discharges may eventually be triggered when the external voltage is reduced or turned off. In order to optimize the efficiency of DBD charging, the geometry (in particular the height) of the voids, the type of gas and its pressure inside the voids are essential factors to be considered and to be optimized. In addition, the influence of the plasma treatment on the internal void surfaces during the DBDs should be taken into consideration.
Pontius, N. ; Kachel, T. ; Schüssler-Langeheine, C. ; Schlotter, W. F. ; Beye, Martin ; Sorgenfrei, Nomi ; Chang, C. F. ; Föhlisch, Alexander ; Wurth, W. ; Metcalf, P. ; Leonov, I. ; Yaresko, A. ; Stojanovic, N. ; Berglund, Martin ; Guerassimova, N. ; Duesterer, S. ; Redlin, H. ; Duerr, H. A.
Resonant soft x-ray diffraction (RSXD) with femtosecond (fs) time resolution is a powerful tool for disentangling the interplay between different degrees of freedom in strongly correlated electron materials. It allows addressing the coupling of particular degrees of freedom upon an external selective perturbation, e. g., by an optical or infrared laser pulse. Here, we report a time-resolved RSXD experiment from the prototypical correlated electron material magnetite using soft x-ray pulses from the free-electron laser FLASH in Hamburg. We observe ultrafast melting of the charge-orbital order leading to the formation of a transient phase, which has not been observed in equilibrium.
Blakesley, James C. ; Schubert, Marcel ; Steyrleuthner, Robert ; Chen, Zhihua ; Facchetti, Antonio ; Neher, Dieter
We investigate charge transport in a high-electron mobility polymer, poly(N, N-bis 2-octyldodecyl-naphthalene-1,4,5,8-bis dicarboximide-2,6-diyl-alt-5,5-2,2-bithiophene) [P(NDI2OD-T2), Polyera ActivInk (TM) N2200]. Time-of-flight measurements reveal electron mobilities approaching those measured in field-effect transistors, the highest ever recorded in a conjugated polymer using this technique. The modest temperature dependence and weak dispersion of the transients indicate low energetic disorder in this material. Steady-state electron-only current measurements reveal a barrier to injection of about 300 meV. We propose that this barrier is located within the P(NDI2OD-T2) film and arises from molecular orientation effects.