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Aliu, E. ; Archambault, S. ; Arlen, T. ; Aune, T. ; Beilicke, M. ; Benbow, W. ; Bouvier, A. ; Bradbury, S. M. ; Buckley, J. H. ; Bugaev, V. ; Byrum, K. ; Cannon, A. ; Cesarini, A. ; Ciupik, L. ; Collins-Hughes, E. ; Connolly, M. P. ; Cui, W. ; Decerprit, G. ; Dickherber, R. ; Duke, C. ; Dumm, J. ; Dwarkadas, Vikram V. ; Errando, M. ; Falcone, A. ; Feng, Q. ; Finley, J. P. ; Finnegan, G. ; Fortson, L. ; Furniss, A. ; Galante, N. ; Gall, D. ; Godambe, S. ; Griffin, S. ; Grube, J. ; Gyuk, G. ; Hanna, D. ; Holder, J. ; Huan, H. ; Hughes, G. ; Humensky, T. B. ; Kaaret, P. ; Karlsson, N. ; Kertzman, M. ; Khassen, Y. ; Kieda, D. ; Krawczynski, H. ; Krennrich, F. ; Lang, M. J. ; Lee, K. ; Maier, G. ; Majumdar, P. ; McArthur, S. ; McCann, A. ; Millis, J. ; Moriarty, P. ; Mukherjee, R. ; Nunez, P. D. ; Ong, R. A. ; Orr, M. ; Otte, A. N. ; Pandel, D. ; Park, N. ; Perkins, J. S. ; Pohl, M. ; Prokoph, H. ; Quinn, J. ; Ragan, K. ; Reyes, L. C. ; Reynolds, P. T. ; Roache, E. ; Rose, H. J. ; Ruppel, J. ; Saxon, D. B. ; Schroedter, M. ; Sembroski, G. H. ; Skole, C. ; Smith, A. W. ; Staszak, D. ; Telezhinsky, Igor O. ; Tesic, G. ; Theiling, M. ; Thibadeau, S. ; Tsurusaki, K. ; Tyler, J. ; Varlotta, A. ; Vincent, S. ; Vivier, M. ; Wakely, S. P. ; Ward, J. E. ; Weekes, T. C. ; Weinstein, A. ; Weisgarber, T. ; Welsing, R. ; Williams, D. A. ; Zitzer, B.
We report on very high energy (E > 100 GeV) gamma-ray observations of V407 Cygni, a symbiotic binary that underwent a nova outburst producing 0.1-10 GeV gamma rays during 2010 March 10-26. Observations were made with the Very Energetic Radiation Imaging Telescope Array System during 2010 March 19-26 at relatively large zenith angles due to the position of V407 Cyg. An improved reconstruction technique for large zenith angle observations is presented and used to analyze the data. We do not detect V407 Cygni and place a differential upper limit on the flux at 1.6 TeV of 2.3 x 10(-12) erg cm(-2) s(-1) (at the 95% confidence level). When considered jointly with data from Fermi-LAT, this result places limits on the acceleration of very high energy particles in the nova.
Acciari, V. A. ; Aliu, E. ; Arlen, T. ; Aune, T. ; Beilicke, M. ; Benbow, W. ; Bradbury, S. M. ; Buckley, J. H. ; Bugaev, V. ; Byrum, K. ; Cannon, A. ; Cesarini, A. ; Ciupik, L. ; Collins-Hughes, E. ; Connolly, M. P. ; Cui, W. ; Dickherber, R. ; Duke, C. ; Errando, M. ; Falcone, A. ; Finley, J. P. ; Finnegan, G. ; Fortson, L. ; Furniss, A. ; Galante, N. ; Gall, D. ; Gillanders, G. H. ; Godambe, S. ; Griffin, S. ; Grube, J. ; Guenette, R. ; Gyuk, G. ; Hanna, D. ; Holder, J. ; Hughes, G. ; Hui, C. M. ; Humensky, T. B. ; Kaaret, P. ; Karlsson, N. ; Kertzman, M. ; Kieda, D. ; Krawczynski, H. ; Krennrich, F. ; Lang, M. J. ; LeBohec, S. ; Maier, G. ; Majumdar, P. ; McArthur, S. ; McCann, A. ; Moriarty, P. ; Mukherjee, R. ; Ong, R. A. ; Orr, M. ; Otte, A. N. ; Park, N. ; Perkins, J. S. ; Pohl, Martin ; Prokoph, H. ; Quinn, J. ; Ragan, K. ; Reyes, L. C. ; Reynolds, P. T. ; Roache, E. ; Rose, H. J. ; Ruppel, J. ; Saxon, D. B. ; Schroedter, M. ; Sembroski, G. H. ; Senturk, G. D. ; Smith, A. W. ; Staszak, D. ; Tesic, G. ; Theiling, M. ; Thibadeau, S. ; Tsurusaki, K. ; Varlotta, A. ; Vassiliev, V. V. ; Vincent, S. ; Vivier, M. ; Wakely, S. P. ; Ward, J. E. ; Weekes, T. C. ; Weinstein, A. ; Weisgarber, T. ; Williams, D. A. ; Zitzer, B.
We present the results of observations of the TeV binary LS I + 61 degrees 303 with the VERITAS telescope array between 2008 and 2010, at energies above 300 GeV. In the past, both ground-based gamma-ray telescopes VERITAS and MAGIC have reported detections of TeV emission near the apastron phases of the binary orbit. The observations presented here show no strong evidence for TeV emission during these orbital phases; however, during observations taken in late 2010, significant emission was detected from the source close to the phase of superior conjunction (much closer to periastron passage) at a 5.6 standard deviation (5.6 sigma) post-trials significance. In total, between 2008 October and 2010 December a total exposure of 64.5 hr was accumulated with VERITAS on LS I + 61 degrees 303, resulting in an excess at the 3.3 sigma significance level for constant emission over the entire integrated data set. The flux upper limits derived for emission during the previously reliably active TeV phases (i.e., close to apastron) are less than 5% of the Crab Nebula flux in the same energy range. This result stands in apparent contrast to previous observations by both MAGIC and VERITAS which detected the source during these phases at 10% of the Crab Nebula flux. During the two year span of observations, a large amount of X-ray data were also accrued on LS I + 61 degrees 303 by the Swift X-ray Telescope and the Rossi X-ray Timing Explorer Proportional Counter Array. We find no evidence for a correlation between emission in the X-ray and TeV regimes during 20 directly overlapping observations. We also comment on data obtained contemporaneously by the Fermi Large Area Telescope.
Aliu, E. ; Arlen, T. ; Aune, T. ; Beilicke, M. ; Benbow, W. ; Boettcher, Markus ; Bouvier, A. ; Bradbury, S. M. ; Buckley, J. H. ; Bugaev, V. ; Cannon, A. ; Cesarini, A. ; Ciupik, L. ; Collins-Hughes, E. ; Connolly, M. P. ; Cui, W. ; Dickherber, R. ; Errando, M. ; Falcone, A. ; Finley, J. P. ; Fortson, L. ; Furniss, A. ; Galante, N. ; Gall, D. ; Gillanders, G. H. ; Godambe, S. ; Griffin, S. ; Grube, J. ; Gyuk, G. ; Hanna, D. ; Holder, J. ; Huan, H. ; Hughes, G. ; Hui, C. M. ; Humensky, T. B. ; Kaaret, P. ; Karlsson, N. ; Kertzman, M. ; Kieda, D. ; Krawczynski, H. ; Krennrich, F. ; Madhavan, A. S. ; Maier, G. ; Majumdar, P. ; McArthur, S. ; McCann, A. ; Moriarty, P. ; Mukherjee, R. ; Ong, R. A. ; Orr, M. ; Otte, A. N. ; Park, N. ; Perkins, J. S. ; Pichel, A. ; Pohl, Martin ; Prokoph, H. ; Quinn, J. ; Ragan, K. ; Reyes, L. C. ; Reynolds, P. T. ; Roache, E. ; Rose, H. J. ; Ruppel, J. ; Saxon, D. B. ; Schroedter, M. ; Sembroski, G. H. ; Skole, C. ; Smith, A. W. ; Staszak, D. ; Tesic, G. ; Theiling, M. ; Thibadeau, S. ; Tsurusaki, K. ; Tyler, J. ; Varlotta, A. ; Vincent, S. ; Vivier, M. ; Wakely, S. P. ; Ward, J. E. ; Weinstein, A. ; Weisgarber, T. ; Williams, D. A.
We report on very high energy (>100 GeV) gamma-ray observations of Swift J164449.3+573451, an unusual transient object first detected by the Swift Observatory and later detected by multiple radio, optical, and X-ray observatories. A total exposure of 28 hr was obtained on Swift J164449.3+573451 with the Very Energetic Radiation Imaging Telescope Array System ( VERITAS) during 2011 March 28-April 15. We do not detect the source and place a differential upper limit on the emission at 500 GeV during these observations of 1.4 x 10(-12) erg cm(-2) s(-1) (99% confidence level). We also present time-resolved upper limits and use a flux limit averaged over the X-ray flaring period to constrain various emission scenarios that can accommodate both the radio-through-X-ray emission detected from the source and the lack of detection by VERITAS.
Archambault, S. ; Beilicke, M. ; Benbow, W. ; Berger, K. ; Bird, R. ; Bouvier, A. ; Buckley, J. H. ; Bugaev, V. ; Byrum, K. ; Cerruti, M. ; Chen, Xuhui ; Ciupik, L. ; Connolly, M. P. ; Cui, W. ; Duke, C. ; Dumm, J. ; Errando, M. ; Falcone, A. ; Federici, Simone ; Feng, Q. ; Finley, J. P. ; Fortson, L. ; Furniss, A. ; Galante, N. ; Gillanders, G. H. ; Griffin, S. ; Griffiths, S. T. ; Grube, J. ; Gyuk, G. ; Hanna, D. ; Holder, J. ; Hughes, G. ; Humensky, T. B. ; Kaaret, P. ; Kertzman, M. ; Khassen, Y. ; Kieda, D. ; Krawczynski, H. ; Lang, M. J. ; Madhavan, A. S. ; Maier, G. ; Majumdar, P. ; McArthur, S. ; McCann, A. ; Moriarty, P. ; Mukherjee, R. ; Nieto, D. ; de Bhroithe, A. O'Faolain ; Ong, R. A. ; Otte, A. N. ; Pandel, D. ; Park, N. ; Perkins, J. S. ; Pohl, Martin ; Popkow, A. ; Prokoph, H. ; Quinn, J. ; Ragan, K. ; Rajotte, J. ; Reyes, L. C. ; Reynolds, P. T. ; Richards, G. T. ; Roache, E. ; Sembroski, G. H. ; Sheidaei, F. ; Smith, A. W. ; Staszak, D. ; Telezhinsky, Igor O. ; Theiling, M. ; Tucci, J. V. ; Tyler, J. ; Varlotta, A. ; Vincent, S. ; Wakely, S. P. ; Weekes, T. C. ; Weinstein, A. ; Williams, D. A. ; Zitzer, B. ; McCollough, M. L.
We report results from TeV gamma-ray observations of the microquasar Cygnus X-3. The observations were made with the Very Energetic Radiation Imaging Telescope Array System (VERITAS) over a time period from 2007 June 11 to 2011 November 28. VERITAS is most sensitive to gamma rays at energies between 85 GeV and 30 TeV. The effective exposure time amounts to a total of about 44 hr, with the observations covering six distinct radio/X-ray states of the object. No significant TeV gamma-ray emission was detected in any of the states, nor with all observations combined. The lack of a positive signal, especially in the states where GeV gamma rays were detected, places constraints on TeV gamma-ray production in Cygnus X-3. We discuss the implications of the results.
Schick, Daniel ; Eckert, Sebastian ; Pontius, Niko ; Mitzner, Rolf ; Föhlisch, Alexander ; Holldack, Karsten ; Sorgenfrei, Nomi
We present an X-ray-optical cross-correlator for the soft (> 150 eV) up to the hard X-ray regime based on a molybdenum-silicon superlattice. The cross-correlation is done by probing intensity and position changes of superlattice Bragg peaks caused by photoexcitation of coherent phonons. This approach is applicable for a wide range of X-ray photon energies as well as for a broad range of excitation wavelengths and requires no external fields or changes of temperature. Moreover, the cross-correlator can be employed on a 10 ps or 100 fs time scale featuring up to 50% total X-ray reflectivity and transient signal changes of more than 20%. (C) 2016 Author(s).
Schick, Daniel ; Eckert, Sebastian ; Pontius, Niko ; Mitzner, Rolf ; Föhlisch, Alexander ; Holldack, Karsten ; Sorgenfrei, Nomi
We present an X-ray-optical cross-correlator for the soft (> 150 eV) up to the hard X-ray regime based on a molybdenum-silicon superlattice. The cross-correlation is done by probing intensity and position changes of superlattice Bragg peaks caused by photoexcitation of coherent phonons. This approach is applicable for a wide range of X-ray photon energies as well as for a broad range of excitation wavelengths and requires no external fields or changes of temperature. Moreover, the cross-correlator can be employed on a 10 ps or 100 fs time scale featuring up to 50% total X-ray reflectivity and transient signal changes of more than 20%. (C) 2016 Author(s).
Two images, taken by the Cassini spacecraft near Saturn's equinox in 2009 August, show the Earhart propeller casting a 350 km long shadow, offering the opportunity to watch how the ring height, excited by the propeller moonlet, relaxes to an equilibrium state. From the shape of the shadow cast and a model of the azimuthal propeller height relaxation, we determine the exponential cooling constant of this process to be lambda = 0.07 +/- 0.02 km(-1), and thereby determine the collision frequency of the ring particles in the vertically excited region of the propeller to be omega(c)/Omega = 0.9 +/- 0.2.
We study the vertical extent of propeller structures in Saturn's rings (i) by extending the model of Spahn and Sremcevic (Spahn, F., Sremcevic, M. [2000]. Astron. Astrophys., 358, 368-372) to include the vertical direction and (ii) by performing N-body box simulations of a perturbing moonlet embedded into the rings. We find that the gravitational interaction of ring particles with a non-inclined moonlet does not induce considerable vertical excursions of ring particles, but causes a considerable thermal motion in the ring plane. We expect ring particle collisions to partly convert the lateral induced thermal motion into vertical excursions of ring particles in the course of a quasi-thermalization. The N-body box simulations lead to maximal propeller heights of about 0.6-0.8 Hill radii of the embedded perturbing moonlet. Moonlet sizes estimated by this relation are in good agreement with size estimates from radial propeller scalings for the propellers Bleriot and Earhart. For large propellers, the extended hydrodynamical propeller model predicts an exponential propeller height relaxation, confirmed by N-body box simulations of non-self gravitating ring particles. Exponential cooling constants, calculated from the hydrodynamical propeller model agree fairly well with values from fits to the tail of the azimuthal height decay of the N-body box simulations. From exponential cooling constants, determined from shadows cast by the propeller Earhart and imaged by the Cassini spacecraft, we estimate collision frequencies of about 6 collisions per particle per orbit in the propeller gap region and about 11 collisions per particle per orbit in the propeller wake region. (C) 2015 Elsevier Inc. All rights reserved.
Kayser, Markus ; Maturilli, Marion ; Graham, Robert M. ; Hudson, Stephen R. ; Rinke, Annette ; Cohen, Lana ; Kim, Joo-Hong ; Park, Sang-Jong ; Moon, Woosok ; Granskog, Mats A.
The Norwegian young sea ICE (N-ICE2015) expedition was designed to investigate the atmosphere-snow-ice-ocean interactions in the young and thin sea ice regime north of Svalbard. Radiosondes were launched twice daily during the expedition from January to June 2015. Here we use these upper air measurements to study the multiple cyclonic events observed during N-ICE2015 with respect to changes in the vertical thermodynamic structure, moisture content, and boundary layer characteristics. We provide statistics of temperature inversion characteristics, static stability, and boundary layer extent. During winter, when radiative cooling is most effective, we find the strongest impact of synoptic cyclones. Changes to thermodynamic characteristics of the boundary layer are associated with transitions between the radiatively "clear" and "opaque" atmospheric states. In spring, radiative fluxes warm the surface leading to lifted temperature inversions and a statically unstable boundary layer. Further, we compare the N-ICE2015 static stability distributions to corresponding profiles from ERA-Interim reanalysis, from the closest land station in the Arctic North Atlantic sector, Ny-Alesund, and to soundings from the SHEBA expedition (1997/1998). We find similar stability characteristics for N-ICE2015 and SHEBA throughout the troposphere, despite differences in location, sea ice thickness, and snow cover. For Ny-Alesund, we observe similar characteristics above 1000 m, while the topography and ice-free fjord surrounding Ny-Alesund generate great differences below. The long-term radiosonde record (1993-2014) from Ny-Alesund indicates that during the N-ICE2015 spring period, temperatures were close to the climatological mean, while the lowest 3000 m were 1-3 degrees C warmer than the climatology during winter. Plain Language Summary The Norwegian young sea ICE (N-ICE2015) expedition was designed to investigate the atmosphere-snow-ice-ocean interactions in the young and thin sea ice regime north of Svalbard. Radiosondes were launched twice daily during the expedition from January to June 2015. Here we use these upper air measurements to study the multiple cyclonic events observed during N-ICE2015 with respect to changes in the vertical thermodynamic structure, moisture content, and the atmospheric boundary layer characteristics. During winter, we find the strongest impact of synoptic cyclones, which transport warm and moist air into the cold and dry Arctic atmosphere. In spring, incoming solar radiation warms the surface. This leads to very different thermodynamic conditions and higher moisture content, which reduces the contrast between stormy and calm periods. Further, we compare the N-ICE2015 measurements to corresponding profiles from ERA-Interim reanalysis, from the closest land station in the Arctic North Atlantic sector, Ny-Alesund, and to soundings from the SHEBA expedition (1997/1998). We find similar stability characteristics for N-ICE2015 and SHEBA throughout the troposphere, despite differences in location, sea ice thickness, and snow cover. The comparisons highlight the value of the N-ICE2015 observation and show the importance of winter time observations in the Arctic North Atlantic sector.
Aliu, E. ; Archambault, S. ; Archer, A. ; Arlen, T. ; Aune, T. ; Barnacka, Anna ; Behera, B. ; Beilicke, M. ; Benbow, W. ; Berger, K. ; Bird, R. ; Böttcher, Markus ; Bouvier, A. ; Buchovecky, M. ; Buckley, J. H. ; Bugaev, V. ; Cardenzana, J. V. ; Cerruti, M. ; Cesarini, A. ; Chen, Xuhui ; Ciupik, L. ; Collins-Hughes, E. ; Connolly, M. P. ; Cui, W. ; Dumm, J. ; Eisch, J. D. ; Falcone, A. ; Federici, Simone ; Feng, Q. ; Finley, J. P. ; Fleischhack, H. ; Fortin, P. ; Fortson, L. ; Furniss, A. ; Galante, N. ; Gall, D. ; Gillanders, G. H. ; Griffin, S. ; Griffiths, S. T. ; Grube, J. ; Gyuk, G. ; Hütten, M. ; Hakansson, Nils ; Holder, J. ; Hughes, G. ; Humensky, T. B. ; Johnson, C. A. ; Kaaret, P. ; Kar, P. ; Kelley-Hoskins, N. ; Kertzman, M. ; Khassen, Y. ; Kieda, D. ; Krause, M. ; Krawczynski, H. ; Krennrich, F. ; Lang, M. J. ; Madhavan, A. S. ; Maier, G. ; McArthur, S. ; McCann, A. ; Meagher, K. ; Millis, J. ; Moriarty, P. ; Mukherjee, R. ; Nieto, D. ; Ong, R. A. ; Orr, M. ; Otte, A. N. ; Pandel, D. ; Park, N. ; Pelassa, V. ; Perkins, J. S. ; Pichel, A. ; Pohl, Martin ; Popkow, A. ; Quinn, J. ; Ragan, K. ; Reyes, L. C. ; Reynolds, P. T. ; Roache, E. ; Rousselle, J. ; Rovero, A. C. ; Saxon, D. B. ; Sembroski, G. H. ; Shahinyan, K. ; Sheidaei, F. ; Skole, C. ; Smith, A. W. ; Staszak, D. ; Telezhinsky, Igor O. ; Theiling, M. ; Todd, N. W. ; Tucci, J. V. ; Tyler, J. ; Varlotta, A. ; Vassiliev, V. V. ; Vincent, S. ; Wakely, S. P. ; Weiner, O. M. ; Weinstein, A. ; Welsing, R. ; Wilhelm, Alina ; Williams, D. A. ; Zitzer, B. ; Baring, M. G. ; Gonzalez, J. Becerra ; Cillis, A. N. ; Horan, D. ; Paneque, D.
The very high energy (VHE; E > 100 GeV) blazar Markarian 501 was observed between April 17 and May 5 (MJD 54 938-54 956), 2009, as part of an extensive multiwavelength campaign from radio to VHE. Strong VHE yray activity was detected on May 1st with Whipple and VERITAS, when the flux (E > 400 GeV) increased to 10 times the preflare baseline flux (3.9 x 10(-11) ph cm(-2) s(-1)), reaching five times the flux of the Crab Nebula. This coincided with a decrease in the optical polarization and a rotation of the polarization angle by 15. This VHE flare showed a fast flux variation with an increase of a factor similar to 4 in 25 min, and a falling time of similar to 50 min. We present the observations of the quiescent state previous to the flare and of the high state after the flare, focusing on the flux and spectral variability from Whipple, VERITAS, Fermi-LAT, RXTE, and Swift combined with optical and radio data.
Abdalla, Hassan E. ; Adam, Remi ; Aharonian, Felix A. ; Benkhali, Faical Ait ; Angüner, Ekrem Oǧuzhan ; Arakawa, Masanori ; Arcaro, C ; Armand, Catherine ; Armstrong, T. ; Egberts, Kathrin
We report on the detection of very high energy (VHE; E > 100 GeV) gamma-ray emission from the BL Lac objects KUV 00311-1938 and PKS 1440-389 with the High Energy Stereoscopic System (H.E.S.S.). H.E.S.S. observations were accompanied or preceded by multiwavelength observations with Fermi/LAT, XRT and UVOT onboard the Swift satellite, and ATOM. Based on an extrapolation of the Fermi/LAT spectrum towards the VHE gamma-ray regime, we deduce a 95 per cent confidence level upper limit on the unknown redshift of KUV 00311-1938 of z < 0.98 and of PKS 1440-389 of z < 0.53. When combined with previous spectroscopy results, the redshift of KUV 00311-1938 is constrained to 0.51 <= z < 0.98 and of PKS 1440-389 to 0.14 (sic) z < 0.53.
Abdalla, Hassan E. ; Adam, Remi ; Aharonian, Felix A. ; Benkhali, Faical Ait ; Angüner, Ekrem Oǧuzhan ; Arakawa, Masanori ; Arcaro, C ; Armand, Catherine ; Armstrong, T. ; Egberts, Kathrin
We report on the detection of very high energy (VHE; E > 100 GeV) gamma-ray emission from the BL Lac objects KUV 00311-1938 and PKS 1440-389 with the High Energy Stereoscopic System (H.E.S.S.). H.E.S.S. observations were accompanied or preceded by multiwavelength observations with Fermi/LAT, XRT and UVOT onboard the Swift satellite, and ATOM. Based on an extrapolation of the Fermi/LAT spectrum towards the VHE gamma-ray regime, we deduce a 95 per cent confidence level upper limit on the unknown redshift of KUV 00311-1938 of z < 0.98 and of PKS 1440-389 of z < 0.53. When combined with previous spectroscopy results, the redshift of KUV 00311-1938 is constrained to 0.51 <= z < 0.98 and of PKS 1440-389 to 0.14 (sic) z < 0.53.
Archer, A. ; Barnacka, Anna ; Beilicke, M. ; Benbow, W. ; Berger, K. ; Bird, R. ; Biteau, Jonathan ; Buckley, J. H. ; Bugaev, V. ; Byrum, K. ; Cardenzana, J. V. ; Cerruti, M. ; Chen, W. ; Chen, Xiaoming ; Ciupik, L. ; Connolly, M. P. ; Cui, W. ; Dickinson, H. J. ; Dumm, J. ; Eisch, J. D. ; Falcone, A. ; Federici, Simone ; Feng, Q. ; Finley, J. P. ; Fleischhack, H. ; Fortson, L. ; Furniss, A. ; Galante, N. ; Griffin, S. ; Griffiths, S. T. ; Grube, J. ; Gyuk, G. ; Hakansson, Nils ; Hanna, D. ; Holder, J. ; Hughes, G. ; Johnson, C. A. ; Kaaret, P. ; Kar, P. ; Kertzman, M. ; Khassen, Y. ; Kieda, D. ; Krawczynski, H. ; Kumar, S. ; Lang, M. J. ; Maier, G. ; McArthur, S. ; McCann, A. ; Meagher, K. ; Moriarty, P. ; Mukherjee, R. ; Nieto, D. ; Ong, R. A. ; Otte, A. N. ; Park, N. ; Perkins, J. S. ; Pohl, Manuela ; Popkow, A. ; Prokoph, H. ; Pueschel, Elisa ; Quinn, J. ; Ragan, K. ; Rajotte, J. ; Reyes, L. C. ; Reynolds, P. T. ; Richards, G. T. ; Roache, E. ; Sembroski, G. H. ; Shahinyan, K. ; Smith, A. W. ; Staszak, D. ; Telezhinsky, Igor O. ; Tucci, J. V. ; Tyler, J. ; Varlotta, A. ; Vincent, S. ; Wakely, S. P. ; Weinstein, A. ; Welsing, R. ; Wilhelm, Alina ; Williams, D. A. ; Zajczyk, A. ; Zitzer, B.
The Galactic center is an interesting region for high-energy (0.1-100 GeV) and very-high-energy (E > 100 GeV) gamma-ray observations. Potential sources of GeV/TeV gamma-ray emission have been suggested, e.g., the accretion of matter onto the supermassive black hole, cosmic rays from a nearby supernova remnant (e.g., Sgr A East), particle acceleration in a plerion, or the annihilation of dark matter particles. The Galactic center has been detected by EGRET and by Fermi/LAT in the MeV/GeV energy band. At TeV energies, the Galactic center was detected with moderate significance by the CANGAROO and Whipple 10 m telescopes and with high significance by H.E.S.S., MAGIC, and VERITAS. We present the results from three years of VERITAS observations conducted at large zenith angles resulting in a detection of the Galactic center on the level of 18 standard deviations at energies above similar to 2.5 TeV. The energy spectrum is derived and is found to be compatible with hadronic, leptonic, and hybrid emission models discussed in the literature. Future, more detailed measurements of the high-energy cutoff and better constraints on the high-energy flux variability will help to refine and/or disentangle the individual models.
Allen, C. ; Archambault, S. ; Archer, A. ; Benbow, W. ; Bird, R. ; Bourbeau, E. ; Brose, Robert ; Buchovecky, M. ; Buckley, J. H. ; Bugaev, V. ; Cardenzana, J. V. ; Cerruti, M. ; Chen, Xuhui ; Christiansen, J. L. ; Connolly, M. P. ; Cui, W. ; Daniel, M. K. ; Eisch, J. D. ; Falcone, Abe ; Feng, Q. ; Fernandez-Alonso, M. ; Finley, J. P. ; Fleischhack, H. ; Flinders, A. ; Fortson, L. ; Furniss, A. ; Gillanders, G. H. ; Griffin, S. ; Grube, J. ; Huetten, M. ; Hakansson, N. ; Hanna, D. ; Hervet, O. ; Holder, J. ; Hughes, G. ; Humensky, T. B. ; Johnson, C. A. ; Kaaret, P. ; Kar, P. ; Kelley-Hoskins, N. ; Kertzman, M. ; Kieda, D. ; Krause, M. ; Krennrich, F. ; Kumar, S. ; Lang, M. J. ; Maier, G. ; McArthur, S. ; McCann, A. ; Meagher, K. ; Moriarty, P. ; Mukherjee, R. ; Nguyen, T. ; Nieto, D. ; Ong, R. A. ; Otte, A. N. ; Park, N. ; Petrashyk, A. ; Pichel, A. ; Pohl, Martin ; Popkow, A. ; Pueschel, Elisa ; Quinn, J. ; Ragan, K. ; Reynolds, P. T. ; Richards, G. T. ; Roache, E. ; Rovero, A. C. ; Rulten, C. ; Sadeh, I. ; Santander, Marcos ; Sembroski, G. H. ; Shahinyan, K. ; Telezhinsky, Igor O. ; Tucci, J. V. ; Tyler, J. ; Wakely, S. P. ; Weinstein, A. ; Wilhelm, Alina ; Williams, D. A.
We present very-high-energy gamma-ray observations of the BL Lac object 1ES 2344+514 taken by the Very Energetic Radiation Imaging Telescope Array System between 2007 and 2015. 1ES 2344+514 is detected with a statistical significance above the background of 20.8 sigma in 47.2 h (livetime) of observations, making this the most comprehensive very-high-energy study of 1ES 2344+514 to date. Using these observations, the temporal properties of 1ES 2344+514 are studied on short and long times-scales. We fit a constant-flux model to nightly and seasonally binned light curves and apply a fractional variability test to determine the stability of the source on different time-scales. We reject the constant-flux model for the 2007-2008 and 2014-2015 nightly binned light curves and for the long-term seasonally binned light curve at the > 3 sigma level. The spectra of the time-averaged emission before and after correction for attenuation by the extragalactic background light are obtained. The observed time-averaged spectrum above 200 GeV is satisfactorily fitted (x(2)/NDF = 7.89/6) by a power-law function with an index Gamma = 2.46 +/- 0.06(stat) +/- 0.20(sys) and extends to at least 8 TeV. The extragalactic-backgroundlight-deabsorbed spectrum is adequately fit (x(2)/NDF = 6.73/6) by a power-law function with an index Gamma = 2.15 +/- 0.06(stat) +/- 0.20(sys) while an F-test indicates that the power law with an exponential cut-off function provides a marginally better fit (x(2)/NDF = 2.56/5) at the 2.1 sigma level. The source location is found to be consistent with the published radio location and its spatial extent is consistent with a point source.
Abdalla, Hassan E. ; Aharonian, Felix A. ; Benkhali, F. Ait ; Angüner, Ekrem Oǧuzhan ; Arakawa, M. ; Arcaro, C. ; Armand, C. ; Arrieta, M. ; Backes, M. ; Barnard, M. ; Becherini, Y. ; Tjus, J. Becker ; Berge, D. ; Bernhard, S. ; Bernloehr, K. ; Blackwell, R. ; Bottcher, M. ; Boisson, C. ; Bolmont, J. ; Bonnefoy, S. ; Bordas, Pol ; Bregeon, J. ; Brun, F. ; Brun, P. ; Bryan, M. ; Buechele, M. ; Bulik, T. ; Bylund, T. ; Capasso, M. ; Caroff, S. ; Carosi, A. ; Casanova, Sabrina ; Cerruti, M. ; Chakraborty, N. ; Chandra, S. ; Chaves, R. C. G. ; Chen, A. ; Colafrancesco, S. ; Condon, B. ; Davids, I. D. ; Dei, C. ; Devin, J. ; deWilt, P. ; Dirson, L. ; Djannati-Atai, A. ; Dmytriiev, A. ; Donath, A. ; Dyks, J. ; Egberts, Kathrin ; Emery, G. ; Ernenwein, J. -P. ; Eschbach, S. ; Fegan, S. ; Fiasson, A. ; Fontaine, G. ; Funk, S. ; Füssling, Matthias ; Gabici, S. ; Gallant, Y. A. ; Garrigoux, T. ; Gate, F. ; Giavitto, G. ; Glawion, D. ; Glicenstein, J. F. ; Gottschall, D. ; Grondin, M. -H. ; Hahn, J. ; Haupt, M. ; Heinzelmann, G. ; Henri, G. ; Hermann, G. ; Hinton, J. A. ; Hofmann, W. ; Hoischen, Clemens ; Holch, T. L. ; Holler, M. ; Horns, D. ; Huber, D. ; Iwasaki, H. ; Jacholkowska, A. ; Jamrozy, M. ; Jankowsky, D. ; Jankowsky, F. ; Jouvin, L. ; Jung-Richardt, I. ; Kastendieck, M. A. ; Katarzynski, K. ; Katsuragawa, M. ; Katz, U. ; Kerszberg, D. ; Khangulyan, D. ; Khelifi, B. ; King, J. ; Klepser, S. ; Kluzniak, W. ; Komin, Nu. ; Kosack, K. ; Krakau, S. ; Kraus, M. ; Kruger, R. R. ; Lamanna, G. ; Lau, J. ; Lefaucheur, J. ; Lemiere, A. ; Lemoine-Goumard, M. ; Lenain, J. -P. ; Leser, Eva ; Lohse, T. ; Lorentz, M. ; Lopez-Coto, R. ; Lypova, I. ; Malyshev, D. ; Marandon, V. ; Marcowith, Alexandre ; Mariaud, C. ; Marti-Devesa, G. ; Marx, R. ; Maurin, G. ; Meintjes, P. J. ; Mitche, A. M. W. ; Moderski, R. ; Mohamed, M. ; Mohrmann, L. ; Moulin, Emmanuel ; Murach, T. ; Nakashima, S. ; de Naurois, M. ; Ndiyavala, H. ; Niederwanger, F. ; Niemiec, J. ; Oakes, L. ; Odaka, H. ; Ohm, S. ; Ostrowski, M. ; Oya, I. ; Padovani, M. ; Panter, M. ; Parsons, R. D. ; Perennes, C. ; Petrucci, P. -O. ; Peyaud, B. ; Piel, Q. ; Pita, S. ; Poireau, V. ; Noel, A. Priyana ; Prokhorov, D. A. ; Prokoph, H. ; Puehlhofer, G. ; Punch, M. ; Quirrenbach, A. ; Raab, S. ; Rauth, R. ; Reimer, A. ; Reimer, O. ; Renaud, M. ; Rieger, F. ; Rinchiuso, L. ; Romoli, C. ; Rowell, G. ; Rudak, B. ; Ruiz-Velasco, E. ; Sahakian, V. ; Saito, S. ; Sanchez, David M. ; Santangelo, Andrea ; Sasaki, M. ; Schlickeiser, R. ; Schussler, F. ; Schulz, A. ; Schwanke, U. ; Schwemmer, S. ; Seglar-Arroyo, M. ; Senniappan, M. ; Seyffert, A. S. ; Shafi, N. ; Shilon, I. ; Shiningayamwe, K. ; Simoni, R. ; Sinha, A. ; Sol, H. ; Spanier, F. ; Specovius, A. ; Spir-Jacob, M. ; Stawarz, L. ; Steenkamp, R. ; Stegmann, Christian ; Steppa, Constantin Beverly ; Sushch, Iurii ; Takahashi, T. ; Tavernet, J. -P. ; Tavernier, T. ; Taylor, A. M. ; Terrier, R. ; Tibaldo, L. ; Tiziani, D. ; Tluczykont, M. ; Trichard, C. ; Tsirou, M. ; Tsuji, N. ; Tuffs, R. ; Uchiyama, Y. ; van der Walt, D. J. ; van Eldik, C. ; van Rensburg, C. ; van Soelen, B. ; Vasileiadis, G. ; Veh, J. ; Venter, C. ; Viana, A. ; Vincent, P. ; Vink, J. ; Voisin, F. ; Voelk, H. J. ; Vuillaume, T. ; Wadiasingh, Z. ; Wagner, S. J. ; Wagner, P. ; Wagner, R. M. ; White, R. ; Wierzcholska, A. ; Woernlein, A. ; Yang, R. ; Zaborov, D. ; Zacharias, M. ; Zanin, R. ; Zdziarski, A. A. ; Zech, Alraune ; Zefi, F. ; Ziegler, A. ; Zorn, J. ; Zywucka, N.
A hotspot at a position compatible with the BL. Lac object 1ES 2322-409 was serendipitously detected with H.E.S.S. during observations performed in 2004 and 2006 on the blazar PKS 2316-423. Additional data on 1ES 2322-409 were taken in 2011 and 2012, leading to a total live-time of 22.3 h. Point-like very-high-energy (VHE; E > 100 GeV) gamma-ray emission is detected from a source centred on the IFS 2322-409 position, with an excess of 116.7 events at a significance of 6.0 sigma. The average VHE gamma-ray spectrum is well described with a power law with a photon index Gamma = 3.40 +/- 0.66(stat) +/- 0.20(sys) and an integral flux Phi(E > 200 GeV) = (3.11 +/- 0.71(stat) 0.62(sys)) x 10(-2)cm(-2)s(-1), which corresponds to 1.1 per cent of the Crab nebula flux above 200 GeV. Multiwavelength data obtained with Fermi LAT, Swift XRT and UVOT, RXTE PCA, ATOM, and additional data from WISE, GROND, and Catalina are also used to characterize the broad-band non-thermal emission of lES 2322-409. The multiwavelength behaviour indicates day-scale variability. Swift UVOT and XRT data show strong variability at longer scales. A spectral energy distribution (SED) is built from contemporaneous observations obtained around a high state identified in Swift data. A modelling of the SED is performed with a stationary homogeneous one-zone synchrotronself-Compton leptonic model. The redshift of the source being unknown, two plausible values were tested for the modelling. A systematic scan of the model parameters space is performed, resulting in a well-constrained combination of values providing a good description of the broad-band behaviour of 1ES 2322-409.
We study the overdamped version of two coupled anharmonic oscillators under the influence of both low- and high-frequency forces respectively and a Gaussian noise term added to one of the two state variables of the system. The dynamics of the system is first studied in the presence of both forces separately without noise. In the presence of only one of the forces, no resonance behaviour is observed, however, hysteresis happens there. Then the influence of the high-frequency force in the presence of a low-frequency, i.e. biharmonic forcing, is studied. Vibrational resonance is found to occur when the amplitude of the high-frequency force is varied. The resonance curve resembles a stochastic resonance-like curve. It is maximum at the value of g at which the orbit lies in one well during one half of the drive cycle of the low-frequency force and in the other for the remaining half cycle. Vibrational resonance is characterized using the response amplitude and mean residence time. We show the occurrence of stochastic resonance behaviour in the overdamped system by replacing the high-frequency force by Gaussian noise. Similarities and differences between both types of resonance are presented. (c) 2006 Elsevier B.V. All rights reserved.
We report on the effect of vibrational resonance in a spatially extended system of coupled noisy oscillators under the action of two periodic forces, a low-frequency one (signal) and a high-frequency one (carrier). Vibrational resonance manifests itself in the fact that for optimally selected values of high-frequency force amplitude, the response of the system to a low-frequency signal is optimal. This phenomenon is a synthesis of two effects, a noise- induced phase transition leading to bistability, and a conventional vibrational resonance, resulting in the optimization of signal processing. Numerical simulations, which demonstrate this effect for an extended system, can be understood by means of a zero-dimensional "effective" model. The behavior of this "effective" model is also confirmed by an experimental realization of an electronic circuit.
In der Nanotechnologie und der molekularen Biologie werden immer kleinere Strukturelemente, wie beispielsweise einzelne Atomlagen oder Molekülgruppen, manipuliert, um bestimmte Funktionen zu erzielen. Veränderungen in solchen Systemen laufen auf atomarer Längen- und Zeitskala ab. Für das physikalische Verständnis dieser ultraschnellen Prozesse ist ein anschauliches Bild wichtig. Dank ihrer hohen Struktur- und Zeitauflösung liefert die Femtosekunden-Röntgenbeugung Bildsequenzen atomarer Bewegung von Molekülen und Festkörpern und ermöglicht somit Rückschlüsse über die komplexe Wechselwirkung zwischen Elektronen- und Kernbewegungen. Die aktuellen und zukünftigen Möglichkeiten, Atomen bei ihren Bewegungen zuzusehen, diskutiert der Referent an aktuellen Beispielen.
Kunnus, Kristjan ; Zhang, Wenkai ; Delcey, Mickael G. ; Pinjari, Rahul V. ; Miedema, Piter S. ; Schreck, Simon ; Quevedo, Wilson ; Schröder, Henning ; Föhlisch, Alexander ; Gaffney, Kelly J. ; Lundberg, Marcus ; Odelius, Michael ; Wernet, Philippe
The valence-excited states of ferric and ferrous hexacyanide ions in aqueous solution were mapped by resonant inelastic X-ray scattering (RIXS) at the Fe L-2,L-3 and N K edges. Probing of both the central Fe and the ligand N atoms enabled identification of the metal-and ligand-centered excited states, as well as ligand-to-metal and metal-to-ligand charge-transfer excited states. Ab initio calculations utilizing the RASPT2 method were used to simulate the Fe L-2,L-3-edge RIXS spectra and enabled quantification of the covalencies of both occupied and empty orbitals of pi and sigma symmetry. We found that pi back-donation in the ferric complex is smaller than that in the ferrous complex. This is evidenced by the relative amounts of Fe 3d character in the nominally 2 pi CN- molecular orbital of 7% and 9% in ferric and ferrous hexacyanide, respectively. Utilizing the direct sensitivity of Fe L-3-edge RIXS to the Fe 3d character in the occupied molecular orbitals, we also found that the donation interactions are dominated by sigma bonding. The latter was found to be stronger in the ferric complex, with an Fe 3d contribution to the nominally 5 sigma CN- molecular orbitals of 29% compared to 20% in the ferrous complex. These results are consistent with the notion that a higher charge at the central metal atom increases donation and decreases back-donation.
Rauch, Thomas ; Quinet, P. ; Hoyer, D. ; Werner, K. ; Richter, Philipp ; Kruk, J. W. ; Demleitner, M.
Context. For the spectral analysis of high-resolution and high signal-to-noise (S/N) spectra of hot stars, state-of-the-art non-local thermodynamic equilibrium (NLTE) model atmospheres are mandatory. These are strongly dependent on the reliability of the atomic data that is used for their calculation. Aims. New Kr IV-VII oscillator strengths for a large number of lines enable us to construct more detailed model atoms for our NLTE model-atmosphere calculations. This enables us to search for additional Kr lines in observed spectra and to improve Kr abundance determinations. Methods. We calculated Kr IV-VII oscillator strengths to consider radiative and collisional bound-bound transitions in detail in our NLTE stellar-atmosphere models for the analysis of Kr lines that are exhibited in high-resolution and high S/N ultraviolet (UV) observations of the hot white dwarf RE 0503-289. Results. We reanalyzed the effective temperature and surface gravity and determined T-eff = 70 000 +/- 2000 K and log (g/cm s(-2)) = 7.5 +/- 0.1. We newly identified ten Kr V lines and one Kr vi line in the spectrum of RE 0503-289. We measured a Kr abundance of 3.3 +/- 0.3 (logarithmic mass fraction). We discovered that the interstellar absorption toward RE 0503-289 has a multi-velocity structure within a radial-velocity interval of -40 km s(-1) < upsilon(rad) < +18 km s(-1). Conclusions. Reliable measurements and calculations of atomic data are a prerequisite for state-of-the-art NLTE stellar-atmosphere modeling. Observed Kr V-VII line profiles in the UV spectrum of the white dwarf RE 0503-289 were simultaneously well reproduced with our newly calculated oscillator strengths.
Violation of the Core Mass - Luminosity relation for AGB models wich experience the thord dredge-up
(1999)
Viscoelastic subdiffusion governed by a fractional Langevin equation is studied numerically in a random Gaussian environment modeled by stationary Gaussian potentials with decaying spatial correlations. This anomalous diffusion is archetypal for living cells, where cytoplasm is known to be viscoelastic and a spatial disorder also naturally emerges. We obtain some first important insights into it within a model one-dimensional study. Two basic types of potential correlations are studied: short-range exponentially decaying and algebraically slow decaying with an infinite correlation length, both for a moderate (several kBT, in the units of thermal energy), and strong (5–10kBT) disorder. For a moderate disorder, it is shown that on the ensemble level viscoelastic subdiffusion can easily overcome the medium's disorder. Asymptotically, it is not distinguishable from the disorder-free subdiffusion. However, a strong scatter in single-trajectory averages is nevertheless seen even for a moderate disorder. It features a weak ergodicity breaking, which occurs on a very long yet transient time scale. Furthermore, for a strong disorder, a very long transient regime of logarithmic, Sinai-type diffusion emerges. It can last longer and be faster in the absolute terms for weakly decaying correlations as compared with the short-range correlations. Residence time distributions in a finite spatial domain are of a generalized log-normal type and are reminiscent also of a stretched exponential distribution. They can be easily confused for power-law distributions in view of the observed weak ergodicity breaking. This suggests a revision of some experimental data and their interpretation.
Viscous overstability in Saturn's B ring : II. Hydrodynamic theory and comparison to simulations
(2001)
Stolterfoht, Martin ; Wolff, Christian Michael ; Marquez, Jose A. ; Zhang, Shanshan ; Hages, Charles J. ; Rothhardt, Daniel ; Albrecht, Steve ; Burn, Paul L. ; Meredith, Paul ; Unold, Thomas ; Neher, Dieter
The performance of perovskite solar cells is predominantly limited by non-radiative recombination, either through trap-assisted recombination in the absorber layer or via minority carrier recombination at the perovskite/transport layer interfaces. Here, we use transient and absolute photoluminescence imaging to visualize all non-radiative recombination pathways in planar pintype perovskite solar cells with undoped organic charge transport layers. We find significant quasi-Fermi-level splitting losses (135 meV) in the perovskite bulk, whereas interfacial recombination results in an additional free energy loss of 80 meV at each individual interface, which limits the open-circuit voltage (V-oc) of the complete cell to similar to 1.12 V. Inserting ultrathin interlayers between the perovskite and transport layers leads to a substantial reduction of these interfacial losses at both the p and n contacts. Using this knowledge and approach, we demonstrate reproducible dopant-free 1 cm(2) perovskite solar cells surpassing 20% efficiency (19.83% certified) with stabilized power output, a high V-oc (1.17 V) and record fill factor (>81%).
We report on sub-wavelength structuring of photosensitive azo-containing polymer films induced by a surface plasmon interference intensity pattern. The two surface plasmon waves generated at neighboring nano-slits in the metal layer during irradiation interfere constructively, resulting in an intensity pattern with a periodicity three times smaller than the wavelength of the incoming light. The near field pattern interacts with the photosensitive polymer film placed above it, leading to a topography change which follows the intensity pattern exactly, resulting in the formation of surface relief gratings of a size below the diffraction limit. We analyze numerically and experimentally how the depth of the nano-slit alters the interference pattern of surface plasmons and find that the sub-wavelength patterning of the polymer surface could be optimized by modifying the geometry and the size of the nano-slit.
We present the results of phase-referenced VLBA+Effelsberg observations at five frequencies of the double-image gravitational lens WAS B0218+357, made to establish the precise registration of the A and B lensed image positions. The motivation behind these observations is to investigate the anomalous variation of the image flux-density ratio (A[B) with frequency - this ratio changes by almost a factor of two over a frequency range from 1.65 GHz to 15.35 GHz. We investigate whether frequency dependent image positions, combined with a magnification gradient across the image field, could give rise to the anomaly. Our observations confirm the variation of image flux-density ratio with frequency. The results from Our phase-reference astrometry, taken together with the lens mass model of Wucknitz et al. (2004, MNRAS, 349, 14), show that shifts of the image peaks and centroids are too small to account for the observed frequency- dependent ratio
Vlijanie solneécnoj aktivnosti na prozraécnost§ atmosfery i optiéceskie svojstva açerozolja
(2005)
Voided space-charge electrets : piezoelectric transducer materials for electro-acoustic applications
(2004)
Stolterfoht, Martin ; Le Corre, Vincent M. ; Feuerstein, Markus ; Caprioglio, Pietro ; Koster, Lambert Jan Anton ; Neher, Dieter
Optimizing the photoluminescence (PL) yield of a solar cell has long been recognized as a key principle to maximize the power conversion efficiency. While PL measurements are routinely applied to perovskite films and solar cells under open circuit conditions (V-OC), it remains unclear how the emission depends on the applied voltage. Here, we performed PL(V) measurements on perovskite cells with different hole transport layer thicknesses and doping concentrations, resulting in remarkably different fill factors (FFs). The results reveal that PL(V) mirrors the current-voltage (JV) characteristics in the power-generating regime, which highlights an interesting correlation between radiative and nonradiative recombination losses. In particular, high FF devices show a rapid quenching of PL(V) from open-circuit to the maximum power point. We conclude that, while the PL has to be maximized at V-OC at lower biases < V-OC the PL must be rapidly quenched as charges need to be extracted prior to recombination.
Entanglement entropy obeys area law scaling for typical physical quantum systems. This may naively be argued to follow from the locality of interactions. We show that this is not the case by constructing an explicit simple spin chain Hamiltonian with nearest-neighbor interactions that presents an entanglement volume scaling law. This non- translational model is contrived to have couplings that force the accumulation of singlet bonds across the half-chain. This configuration of the couplings is suggested by real-space renormalization group arguments. Computation of the entanglement entropy is performed by mapping the system to free fermions and diagonalizing numerically its correlation matrix. An analytical relationship between the entanglement entropy and the Frobenius norm of the correlation matrix is also established. Our result is complementary to the known relationship between non-translational invariant, nearest- neighbor interacting Hamiltonians and quantum Merlin-Arthur (QMA)complete problems.
In the light of recent intensity-voltage low energy electron diffraction (LEED-IV) experiments [Surf. Sci. 316, 92 (1994); Surf. Rev. Lett. 10, 487 (2003)], the electronic and geometric structure of a water bilayer adsorbed at the Ru(0001) surface are investigated through first-principles total energy calculations, using periodic slab geometries and gradient-corrected density functional theory (DFT). We consider five possible bilayer structures, all roughly consistent with the LEED-IV analysis (three intact structures and two half-dissociated), and a water single layer at Ru(0001). Adsorption energies and substrate-adsorbate geometry parameters are given and discussed in the light of the experiments. We also give a comparative analysis of the electron density redistribution (Delta rho) and of the dipole moment change (Delta mu) induced by water adsorption on the Ru(0001) surface. In agreement with Feibelman [Science 295, 99 (2002)], the half-dissociated structures are found to be more stable than the intact ones, and their adsorption geometries in better agreement with the LEED-IV data. However, the Delta rho analysis shows that a half-dissociated structure induces a Delta mu>0, which would be incompatible with the experimentally measured decrease of the work function following bilayer adsorption; the latter would be consistent, instead, with the Delta mu < 0 induced by the intact structures. It is the aim of this paper to compare various possible adsorption structures, most of them already considered previously, with one and the same method. For this purpose, thick slabs and restrictive computational parameters are chosen to generally address the accuracy and the limits of DFT in reproducing adsorption energies and bond lengths of water-metal interacting systems
Crovetto, Andrea ; Hempel, Hannes ; Rusu, Marin ; Choubrac, Leo ; Kojda, Sandrino Danny ; Habicht, Klaus ; Unold, Thomas
CuI has been recently rediscovered as a p-type transparent conductor with a high figure of merit. Even though many metal iodides are hygroscopic, the effect of moisture on the electrical properties of CuI has not been clarified. In this work, we observe a 2-fold increase in the conductivity of CuI after exposure to ambient humidity for 5 h, followed by slight long-term degradation. Simultaneously, the work function of CuI decreases by almost 1 eV, which can explain the large spread in the previously reported work function values. The conductivity increase is partially reversible and is maximized at intermediate humidity levels. On the basis of the large intragrain mobility measured by THz spectroscopy, we suggest that hydration of grain boundaries may be beneficial for the overall hole mobility.
Steigert, Alexander ; Kojda, Sandrino Danny ; Ibaceta-Jaña, Josefa Fernanda ; Abou-Ras, Daniel ; Gunder, René ; Alktash, Nivin ; Habicht, Klaus ; Wagner, Markus Raphael ; Klenk, Reiner ; Raoux, Simone ; Szyszka, Bernd ; Lauermann, Iver ; Muydinov, Ruslan
Transparent conductive materials based on indium oxide remain yet irreplaceable in various optoelectronic applications. Amorphous oxides appear especially attractive for technology as they are isotropic, demonstrate relatively high electron mobility and can be processed at low temperatures. Among them is indium zinc oxide (IZO) with a large zinc content that is crucial for keeping the amorphous state but redundant for the doping. In this work we investigated water-free and water containing IZO films obtained by radio frequency sputtering. The correlation between temperature driven changes of the chemical state, the optical and electrical properties as well as the progression of crystallization was in focus. Such characterization methods as: scanning electron microscopy, X-ray diffraction, X-ray photoelectron spectroscopy, Raman spectroscopy, temperature dependent Hall-effect measurements and others were applied. Temperature dependent electrical properties of amorphous IZO and IZO:H2O films were found to evolve similarly. Based on our experience in In2O3:H2O (In2O3:H or IOH) we proposed an explanation for the changes observed. Water admixture was found to decrease crystallization temperature of IZO significantly from similar to 550 degrees C to similar to 280 degrees C. Herewith, the presence and concentration of water and/or hydroxyls was found to determine Zn distribution in the film. In particular, Zn enrichment was detected at the film's surface respective to the high water and/or hydroxyl amount. Raman spectra revealed a two-dimensional crystallization of w-ZnO which precedes regardless water presence an extensive In2O3 crystallization. An abrupt loss of electron mobility as a result of crystallization was attributed to the formation of ZnO interlayer on grain boundaries.
Differential absorption spectroscopy techniques serve as powerful techniques to study the excited species in organic solar cells. However, it has always been challenging to employ these techniques for characterizing thick-junction organic solar cells, especially when a reflective top contact is involved. In this work, we present a detailed and systematic study on how a combination of the presence of the interference effect and a nonuniform charge-distribution profile, severely manipulates experimental spectra and the decay dynamics. Furthermore, we provide a practical methodology to correct these optical artifacts in differential absorption spectroscopies. The results and the proposed correction method generally apply to all kinds of differential absorption spectroscopy techniques and various thin-film systems, such as organics, perovskites, kesterites, and two-dimensional materials. Notably, it is found that the shape of differential absorption spectra can be strongly distorted, starting from 150-nm active-layer thickness; this matches the thickness range of thick-junction organic solar cells and most perovskite solar cells and needs to be carefully considered in experiments. In addition, the decay dynamics of differential absorption spectra is found to be disturbed by optical artifacts under certain conditions. With the help of the proposed correction formalism, differential spectra and the decay dynamics can be characterized on the full device of thin-film solar cells in transmission mode and yield accurate and reliable results to provide design rules for further progress.
Shprits, Yuri ; Drozdov, Alexander ; Spasojevic, Maria ; Kellerman, Adam C. ; Usanova, Maria E. ; Engebretson, Mark J. ; Agapitov, Oleksiy V. ; Zhelavskaya, Irina ; Raita, Tero J. ; Spence, Harlan E. ; Baker, Daniel N. ; Zhu, Hui ; Aseev, Nikita
Middelanis, Robin ; Willner, Sven N. ; Otto, Christian ; Kuhla, Kilian ; Quante, Lennart ; Levermann, Anders
Tropical cyclones range among the costliest disasters on Earth. Their economic repercussions along the supply and trade network also affect remote economies that are not directly affected. We here simulate possible global repercussions on consumption for the example case of Hurricane Sandy in the US (2012) using the shock-propagation model Acclimate. The modeled shock yields a global three-phase ripple: an initial production demand reduction and associated consumption price decrease, followed by a supply shortage with increasing prices, and finally a recovery phase. Regions with strong trade relations to the US experience strong magnitudes of the ripple. A dominating demand reduction or supply shortage leads to overall consumption gains or losses of a region, respectively. While finding these repercussions in historic data is challenging due to strong volatility of economic interactions, numerical models like ours can help to identify them by approaching the problem from an exploratory angle, isolating the effect of interest. For this, our model simulates the economic interactions of over 7000 regional economic sectors, interlinked through about 1.8 million trade relations. Under global warming, the wave-like structures of the economic response to major hurricanes like the one simulated here are likely to intensify and potentially overlap with other weather extremes.
The precise knowledge of one of two complementary experimental outcomes prevents us from obtaining complete information about the other one. This formulation of Niels Bohr's principle of complementarity when applied to the paradigm of wave-particle dualism-that is, to Young's double-slit experiment-implies that the information about the slit through which a quantum particle has passed erases interference. In the present paper we report a double-slit experiment using two photons created by spontaneous parametric down-conversion where we observe interference in the signal photon despite the fact that we have located it in one of the slits due to its entanglement with the idler photon. This surprising aspect of complementarity comes to light by our special choice of the TEM01 pump mode. According to quantum field theory the signal photon is then in a coherent superposition of two distinct wave vectors giving rise to interference fringes analogous to two mechanical slits.
In this work we investigated ultrafast demagnetization in a Heusler-alloy. This material belongs to the halfmetal and exists in a ferromagnetic phase. A special feature of investigated alloy is a structure of electronic bands. The last leads to the specific density of the states. Majority electrons form a metallic like structure while minority electrons form a gap near the Fermi-level, like in semiconductor. This particularity offers a good possibility to use this material as model-like structure and to make some proof of principles concerning demagnetization. Using pump-probe experiments we carried out time-resolved measurements to figure out the times of demagnetization. For the pumping we used ultrashort laser pulses with duration around 100 fs. Simultaneously we used two excitation regimes with two different wavelengths namely 400 nm and 1240 nm. Decreasing the energy of photons to the gap size of the minority electrons we explored the effect of the gap on the demagnetization dynamics. During this work we used for the first time OPA (Optical Parametrical Amplifier) for the generation of the laser irradiation in a long-wave regime. We tested it on the FETOSPEX-beamline in BASSYII electron storage ring. With this new technique we measured wavelength dependent demagnetization dynamics. We estimated that the demagnetization time is in a correlation with photon energy of the excitation pulse. Higher photon energy leads to the faster demagnetization in our material. We associate this result with the existence of the energy-gap for minority electrons and explained it with Elliot-Yaffet-scattering events. Additionally we applied new probe-method for magnetization state in this work and verified their effectivity. It is about the well-known XMCD (X-ray magnetic circular dichroism) which we adopted for the measurements in reflection geometry. Static experiments confirmed that the pure electronic dynamics can be separated from the magnetic one. We used photon energy fixed on the L3 of the corresponding elements with circular polarization. Appropriate incidence angel was estimated from static measurements. Using this probe method in dynamic measurements we explored electronic and magnetic dynamics in this alloy.