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We present the first detection of HCO+ absorption in the Magellanic System. Using the ATCA, we observed nine extragalactic radio continuum sources behind the Magellanic System and detected HCO+ absorption toward one source located behind the leading edge of the Magellanic Bridge. The detection is located at an LSR velocity of v = 214.0 +/- 0.4 km s(-1), with an FWHM of Delta v = 4.5 +/- 1.0 km s(-1), and an optical depth of tau (HCO+) = 0.10 +/- 0.02. Although there is abundant neutral hydrogen (H I) surrounding the sight line in position-velocity space, at the exact location of the absorber the H I column density is low, <10(20) cm(-2), and there is little evidence for dust or CO emission from Planck observations. While the origin and survival of molecules in such a diffuse environment remain unclear, dynamical events such as H I flows and cloud collisions in this interacting system likely play an important role.