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- Metzler, Ralf (9)
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Erscheinungsjahr
- 2014 (102) (entfernen)
Dokumenttyp
- Postprint (102) (entfernen)
Gehört zur Bibliographie
- ja (102) (entfernen)
Schlagworte
- anomalous diffusion (5)
- living cells (4)
- Cardiac rehabilitation (2)
- RPA (2)
- acquisition (2)
- ancient DNA (2)
- arsenolipids present (2)
- behavior (2)
- cod-liver (2)
- damage (2)
Institut
- Institut für Chemie (32)
- Mathematisch-Naturwissenschaftliche Fakultät (17)
- Humanwissenschaftliche Fakultät (14)
- Institut für Biochemie und Biologie (9)
- Institut für Physik und Astronomie (6)
- Institut für Anglistik und Amerikanistik (5)
- Department Sport- und Gesundheitswissenschaften (4)
- Institut für Germanistik (3)
- Philosophische Fakultät (3)
- Wirtschafts- und Sozialwissenschaftliche Fakultät (2)
Mondal, Suvendu Sekhar ; Behrens, Karsten ; Matthes, Philipp R. ; Schönfeld, Fabian ; Nitsch, Jörn ; Steffen, Andreas ; Primus, Philipp-Alexander ; Kumke, Michael Uwe ; Müller-Buschbaum, Klaus ; Holdt, Hans-Jürgen
Co-doping of the MOF 3∞[Zn(2-methylimidazolate-4-amide-5-imidate)] (IFP-1 = Imidazolate Framework Potsdam-1) with luminescent Eu3+ and Tb3+ ions presents an approach to utilize the porosity of the MOF for the intercalation of luminescence centers and for tuning of the chromaticity to the emission of white light of the quality of a three color emitter. Organic based fluorescence processes of the MOF backbone as well as metal based luminescence of the dopants are combined to one homogenous single source emitter while retaining the MOF's porosity. The lanthanide ions Eu3+ and Tb3+ were doped in situ into IFP-1 upon formation of the MOF by intercalation into the micropores of the growing framework without a structure directing effect. Furthermore, the color point is temperature sensitive, so that a cold white light with a higher blue content is observed at 77 K and a warmer white light at room temperature (RT) due to the reduction of the organic emission at higher temperatures. The study further illustrates the dependence of the amount of luminescent ions on porosity and sorption properties of the MOF and proves the intercalation of luminescence centers into the pore system by low-temperature site selective photoluminescence spectroscopy, SEM and EDX. It also covers an investigation of the border of homogenous uptake within the MOF pores and the formation of secondary phases of lanthanide formates on the surface of the MOF. Crossing the border from a homogenous co-doping to a two-phase composite system can be beneficially used to adjust the character and warmth of the white light. This study also describes two-color emitters of the formula Ln@IFP-1a–d (Ln: Eu, Tb) by doping with just one lanthanide Eu3+ or Tb3+.
The system of German capitalisation seems to be based on dissimilar levels of linguistic description, i. e. semantics, morphology, and syntax. This leads to several competing scientific models as well as a large range of different rules which appear to be widely autonomous and incompatible with each other. This paper opens an integrative view on the topic by focussing on a pragmatic perspective, which is capable not only on integrating all major application areas of German capitalisation but also of motivating them. Based on theDiscourse Representation Theory (DRT) the text pragmatic model can add a functional perspective to established theories by making similar predictions on capitalisation but additionally specifying communicative reasons for them. Therefore it claims explanatory adequacy from the functional perspective.