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Light-induced softening of azobenzene dye-doped polymer films probed with quartz crystal resonators
(2000)
Krasneralgebren
(2000)
Surface light emitting diodes SLEDs , in which previously microfabricated electrodes were coated with a conjugated polymer, were made with greatly different electrode spacings 250 nm and 10 or 20 mm and with different electrode material combinations. The fabrication process allowed us to compare several electrode materials. The SLED structures also enabled imaging of the light emission zone with fluorescence video microscopy. Conventional sandwich structures were also made for comparison electrode separation 50 nm. In this study, the emitting layer was poly[3- (2',5'-bis(1'',4'',7''trioxaoctyl)phenyl)-2,2'-bithiophene] (EO-PT), a conjugated polymer based on polythiophene with oligo ethyleneoxide side chains. The current-voltage (I(V)) and light-voltage (L(V)) characteristics of the SLEDs were largely insensitive to electrode separation except at high voltages, at which the current in the devices with the largest separations was limited. Sandwich structures had the same light output at a given current. Light could be obtained in forward and reverse bias from indium tin oxide ITO -aluminum, gold silicide-aluminum, and gold silicide-gold SLEDs, but the turn-on voltages were lowest with the ITO-aluminum devices, and these were also the brightest and most reliable. Adding salt to the EO-PT increased the current and brightness, decreased the turn-on voltages, and made the I(V) characteristics symmetric; thus, a device with an electrode separation of 10 mm had the extraordinarily low turn-on voltage of 6 V. The location of the light emission was at the electron-injecting contact.
Dielectric loss spectroscopy (DLS) was performed at compact samples and lamellary organized Langmuir-Blodgett (LB) films from various fatty acid salts. Previous thermoanalytical measurements at compact samples revealed the appearance of two different phase transition temperatures; the lower one is related to the acid the second one to the acid salt molecules. In spite of ill defined electrical contacts with the film the characteristic DLS frequencies obtained from about 100nm thick multilayer films are similar to those recorded from bulk samples. No significant variations of frequencies were found changing the counter ions. Besides conductivity influence at low frequncies we found two relaxations related to the mobility of the dipolar carboxylat-metal group at about 100 and 10000Hz. One of these frequencies is related to the rotation around the chain axis. The strength of this relaxation increases significantly with increasing the sample temperature above 105°C. This temperature is connected with a structural phase transition observed by X-ray reflectometry. In case of Pb-stearate the results of the dielectric measurements help to interprete this structural change as a transition from an orthorhombic into a free-rotator phase. The uncorrelated rotation of molecules around their molecular axes initiates a much increased relaxation strength at the carboxylat-metal sites.
Microlensing results from APO monitoring of the double quasar Q0957+561A,B between 1995 and 1998
(2000)
If the halo of the lensing galaxy 0957+561 is made of massive compact objects (MACHOs), they must affect the lightcurves of the quasar images Q0957+561 A and B differently. We search for this microlensing effect in the double quasar by comparing monitoring data for the two images A and B - obtained with the 3.5m Apache Point Observatory from 1995 to 1998 - with intensive numerical simulations. This way we test whether the halo of the lensing galaxy can be made of MACHOs of various masses. We can exclude a halo entirely made out of MACHOs with masses between 10-6 Msun and 10-2 Msun for quasar sizes of less than 3x 1014 h60-1/2 cm, hereby extending previous limits upwards by one order of magnitude.
Elektronische Struktur niedrigdimensionaler Systeme auf Oberflächen mit zweizähliger Symmetrie
(2000)
New substituted 2,5-diphenyl-1,3,4-oxadiazoles are reported as luminescent materials in light emitting diodes LEDs . The investigated new oxadiazoles show efficient blue and green emission in single layer devices. The combination with a hole transporting and red emitting polythiophene led to a white emission with higher quantum efficiency (QE).
Planeten um andere Sterne
(2000)
Conceptual models of blocking structures are constructed by reducing the twodimensional atmospheric vorticity field to a few point vortices. The flow is assumed to be barotropic and divergence-free, and a blocking event is represented by a point vortex dipole. The focus is here on the motion of the blocking dipole under the influence of the zonal mean flow. This is modelled in three different ways: A dipole embedded in a latitude-dependent zonal mean flow exhibits neutrally stable oscillations; their period is estimated analytically. A cyclonic point vortex approaching from upstream can either pass the dipole or break it up, so that an $Omega$-shaped pattern of three vortices emerges. The stationarity of a blocking between two troughs is modelled by four point vortices. These low-order point vortex models are compared with the dynamics of real blockings in case studies. Despite their high degree of simplification, those models reproduce the kinematics of blocking events properly. This results from the discretization of the flow to its actual physical states, the vortices, in contrast to the common, purely mathematical discretization to grid points. Thus, point vortex dynamics are proposed to be a powerful completion of continuous fluid dynamics in explaining blocking events.
Standard time and frequency parameters of heart rate variability (HRV) describe only linear and periodic behaviour, whereas more complex relationships cannot be recognised. A method that may be capable of assessing more complex properties is the non-linear measure of 'renormalised entropy.' A new concept of the method, RE(AR), has been developed, based on a non-linear renormalisation of autoregressive spectral distributions. To test the hypothesis that renormalised entropy may improve the result of high-risk stratification after myocardial infarction, it is applied to a clinical pilot study (41 subjects) and to prospective data of the St George's Hospital post- infarction database (572 patients). The study shows that the new RE(AR) method is more reproducible and more stable in time than a previously introduced method (p<0.001). Moreover, the results of the study confirm the hypothesis that on average, the survivors have negative values of RE(AR) (-0.11+/-0.18), whereas the non-survivors have positive values (0.03+/-0.22, p<0.01). Further, the study shows that the combination of an HRV triangular index and RE(AR) leads to a better prediction of sudden arrhythmic death than standard measurements of HRV. In summary, the new RE(AR) method is an independent measure in HRV analysis that may be suitable for risk stratification in patients after myocardial infarction.
Doubly stochastic resonance
(2000)
We report the effect of doubly stochastic resonance which appears in nonlinear extended systems if the influence of noise is twofold: A multiplicative noise induces bimodality of the mean field of the coupled network and an independent additive noise governs the dynamic behavior in response to small periodic driving. For optimally selected values of the additive noise intensity stochastic resonance is observed, which is manifested by a maximal coherence between the dynamics of the mean field and the periodic input. Numerical simulations of the signal-to-noise ratio and theoretical results from an effective two state model are in good quantitative agreement.
Ventricular tachycardia or fibrillation (VT-VF) as fatal cardiac arrhythmias are the main factors triggering sudden cardiac death. The objective of this study is to find early signs of sustained VT-VF in patients with an implanted cardioverter-defibrillator (ICD). These devices are able to safeguard patients by returning their hearts to a normal rhythm via strong defibrillatory shocks; additionally, they store the 1000 beat-to-beat intervals immediately before the onset of a life-threatening arrhythmia. We study these 1000 beat-to-beat intervals of 17 chronic heart failure ICD patients before the onset of a life-threatening arrhythmia and at a control time, i.e., without a VT-VF event. To characterize these rather short data sets, we calculate heart rate variability parameters from the time and frequency domain, from symbolic dynamics as well as the finite-time growth rates. We find that neither the time nor the frequency domain parameters show significant differences between the VT-VF and the control time series. However, two parameters from symbolic dynamics as well as the finite-time growth rates discriminate significantly both groups. These findings could be of importance in algorithms for next generation ICD's to improve the diagnostics and therapy of VT-VF.
The effect of additive noise on transitions in nonlinear systems far from equilibrium is studied. It is shown that additive noise in itself can induce a hidden phase transition, which is similar to the transition induced by multiplicative noise in a nonlinear oscillator [P. Landa and A. Zaikin, Phys. Rev. E 54, 3535 (1996)]. Investigation of different nonlinear models that demonstrate phase transitions induced by multiplicative noise shows that the influence of additive noise upon such phase transitions can be crucial: additive noise can either blur such a transition or stabilize noise-induced oscillations.
In-plane strain and shape analysis of Si/SiGe nanostructures by grazing incidence diffraction
(2000)
Dust cloud near the sun
(2000)
A dust cloud around Ganymede Maintained by hypervelocity impacts of interplanetary micrometeoroids
(2000)
The spectra of 18 WN stars in the Large Magellanic Cloud (LMC) are quantitatively analyzed by means of "standard" Wolf-Rayet model atmospheres, using the helium and nitrogen lines as well as the spectral energy distribution. The hydrogen abundance is also determined. Carbon is included for a subset of 4 stars. The studied sample covers all spectral subtypes (WN2 ... WN9) and also includes one WN/WC transition object. The luminosities of the program stars span a wide range ( L/Lsun = 5.0 ... 6.5). Due to the given LMC membership, these results are free from uncertainties inferred from the distance. 50 % of the studied stars (both, late and early WN subtypes) have rather low luminosity (L/Lsun < 5.5). This puts tough constraints on their evolutionary formation. If coming from single stars, it provides evidence for strong internal mixing processes. The empirical mass-loss rates are scaled down by a factor of about two due to the impact of clumping, compared to previous studies adopting homogeneous winds. There is no obvious strong correlation between the mass-loss rates and other parameters like luminosity, temperature and composition. The stellar parameters for the present LMC sample are not systematically different from those of the Galactic WN stars studied previously with the same techniques, in contrast to the expected metallicity effects.
The main intention of this contribution is to discuss different nonlinear approaches to heart rate and blood pressure variability analysis for a better understanding of the cardiovascular regulation. We investigate measures of complexity which are based on symbolic dynamics, renormalised entropy and the finite time growth rates. The dual sequence method to estimate the baroreflex sensitivity and the maximal correlation method to estimate the nonlinear coupling between time series are employed for analysing bivariate data. The latter appears to be a suitable method to estimate the strength of the nonlinear coupling and the coupling direction. Heart rate and blood pressure data from clinical pilot studies and from very large clinical studies are analysed. We demonstrate that parameters from nonlinear dynamics are useful for risk stratification after myocardial infarction, for the prediction of life-threatening cardiac events even in short time series, and for modelling the relationship between heart rate and blood pressure regulation. These findings could be of importance for clinical diagnostics, in algorithms for risk stratification, and for therapeutic and preventive tools of next generation implantable cardioverter defibrillators.