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In this contribution, we provide a detailed dynamical analysis of the interfacial hydrogen migration mediated by scanning tunneling microscopy (STM). Contributions from the STM-current and from the non-adiabatic couplings are taken into account using only first principle models. The slight asymmetry of the tunnelling rates with respect to the potential bias sign inferred from experimental observations is reproduced by weighting the contributions of the metal acceptor–donor states for the propagation of the impinging electrons. The quasi-thermal inelastic collision mechanism is treated perturbatively. The influence of hydrogen pre-coverage is also investigated using new potential energy surfaces obtained from periodic density functional theory calculations. Fully quantum dynamical simulations of the system evolution are performed by solving the Pauli master equation, providing insight into the reaction mechanism of STM manipulation of subsurface hydrogens. It is observed that the hydrogen impurity favors resurfacing over occupation of the bulk and subsurface sites whenever possible. The present simulations give strong indication that the experimentally observed protuberances after STM-excitation are due to hydrogen accumulating in the vicinity of the surface.
In June 2013, widespread flooding and consequent damage and losses occurred in Central Europe, especially in Germany. This paper explores what data are available to investigate the adverse impacts of the event, what kind of information can be retrieved from these data and how well data and information fulfil requirements that were recently proposed for disaster reporting on the European and international levels. In accordance with the European Floods Directive (2007/60/EC), impacts on human health, economic activities (and assets), cultural heritage and the environment are described on the national and sub-national scale. Information from governmental reports is complemented by communications on traffic disruptions and surveys of flood-affected residents and companies.
Overall, the impacts of the flood event in 2013 were manifold. The study reveals that flood-affected residents suffered from a large range of impacts, among which mental health and supply problems were perceived more seriously than financial losses. The most frequent damage type among affected companies was business interruption. This demonstrates that the current scientific focus on direct (financial) damage is insufficient to describe the overall impacts and severity of flood events.
The case further demonstrates that procedures and standards for impact data collection in Germany are widely missing. Present impact data in Germany are fragmentary, heterogeneous, incomplete and difficult to access. In order to fulfil, for example, the monitoring and reporting requirements of the Sendai Framework for Disaster Risk Reduction 2015–2030 that was adopted in March 2015 in Sendai, Japan, more efforts on impact data collection are needed.
Beyond the Crystal-Image
(2016)
A Conjunction of Mysteries
(2016)
Singular quantified terms
(2016)
In this paper, I discuss the behavior of singular partitives, focusing on Hebrew. I show that group noun-headed singular quantified terms behave essentially different from other singular quantified terms. Specifically, the domain of quantification in the former is a discrete set (the members of the group), while in the latter the domain of quantification is a set of mass entities. I propose a preliminary analysis of singular quantified terms in Hebrew, respecting the properties peculiar to this language as well as the observations about group vs. non-group singular quantified terms. This analysis is based on a novel class of quantifiers I name ’Measure Quantifiers’, which instantiate relations between algebraic sums. Using shifts between algebraic sums, we can represent the different readings of singular and plural individual or group terms.
This paper investigates an unnoticed difference in Mandarin between the Q-adjectives and the gradable adjectives of quality and shows that this observation follows straightforwardly from a theory that differentiates gradable predication of quantity and that of quality (e.g., Rett 2008; Lin 2014; Solt 2015; a.o.).