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Rivers transfer particulate organic carbon (POC) from eroding mountains into geological sinks. Organic carbon source composition and selective mobilization have been shown to affect the type and quantity of POC export, but their combined effects across complex mountain ranges remain underexplored. Here, we examine the variation in organic carbon sourcing and transport in the trans-Himalayan Kali Gandaki River catchment, along strong gradients in precipitation, rock type and vegetation. Combining bulk stable nitrogen, and stable and radioactive organic carbon isotopic composition of bedrock, litter, soil and river sediment samples with a Bayesian end-member mixing approach, we differentiate POC sources along the river and quantify their export. Our analysis shows that POC export from the Tibetan segment of the catchment, where carbon bearing shales are partially covered by aged and modern soils, is dominated by petrogenic POC. Based on our data we re-assess the presence of aged biospheric OC in this part of the catchment, and its contribution to the river load. In the High Himalayan segment, we observed low inputs of petrogenic and biospheric POC, likely due to very low organic carbon concentrations in the metamorphic bedrock, combined with erosion dominated by deep-seated landslides. Our findings show that along the Kali Gandaki River, the sourcing of sediment and organic carbon are decoupled, due to differences in rock organic carbon content, soil and above ground carbon stocks, and geomorphic process activity. While the fast eroding High Himalayas are the principal source of river sediment, the Tibetan headwaters, where erosion rates are lower, are the principal source of organic carbon. To robustly estimate organic carbon export from the Himalayas, the mountain range should be divided into tectono-physiographic zones with distinct organic carbon yields due to differences in substrate and erosion processes and rates.
Thermal erosion is a major mechanism of permafrost degradation, resulting in characteristic landforms. We inventory thermo-erosional valleys in ice-rich coastal lowlands adjacent to the Siberian Laptev Sea based on remote sensing, Geographic Information System (GIS), and field investigations for a first regional assessment of their spatial distribution and characteristics. Three study areas with similar geological (Yedoma Ice Complex) but diverse geomorphological conditions vary in valley areal extent, incision depth, and branching geometry. The most extensive valley networks are incised deeply (up to 35 m) into the broad inclined lowland around Mamontov Klyk. The flat, low-lying plain forming the Buor Khaya Peninsula is more degraded by thermokarst and characterized by long valleys of lower depth with short tributaries. Small, isolated Yedoma Ice Complex remnants in the Lena River Delta predominantly exhibit shorter but deep valleys. Based on these hydrographical network and topography assessments, we discuss geomorphological and hydrological connections to erosion processes. Relative catchment size along with regional slope interact with other Holocene relief-forming processes such as thermokarst and neotectonics. Our findings suggest that thermo-erosional valleys are prominent, hitherto overlooked permafrost degradation landforms that add to impacts on biogeochemical cycling, sediment transport, and hydrology in the degrading Siberian Yedoma Ice Complex.
The overarching goal of this dissertation is to provide a better understanding of the role of wind and water in shaping Earth’s Cenozoic orogenic plateaus - prominent high-elevation, low relief sectors in the interior of Cenozoic mountain belts. In particular, the feedbacks between surface uplift, the build-up of topography and ensuing changes in precipitation, erosion, and vegetation patterns are addressed in light of past and future climate change. Regionally, the study focuses on the two world’s largest plateaus, the Altiplano-Puna Plateau of the Andes and Tibetan Plateau, both characterized by average elevations of >4 km. Both plateaus feature high, deeply incised flanks with pronounced gradients in rainfall, vegetation, hydrology, and surface processes. These characteristics are rooted in the role of plateaus to act as efficient orographic barriers to rainfall and to force changes in atmospheric flow.
The thesis examines the complex topics of tectonic and climatic forcing of the surface-process regime on three different spatial and temporal scales: (1) bedrock wind-erosion rates are quantified in the arid Qaidam Basin of NW Tibet over millennial timescales using cosmogenic radionuclide dating; (2) present-day stable isotope composition in rainfall is examined across the south-central Andes in three transects between 22° S and 28° S; these data are modeled and assessed with remotely sensed rainfall data of the Tropical Rainfall Measuring Mission and the Moderate Resolution Imaging Spectroradiometer; (3) finally, a 2.5-km-long Mio-Pliocene sedimentary record of the intermontane Angastaco Basin (25°45’ S, 66°00’ W) is presented in the context of hydrogen and carbon compositions of molecular lipid biomarker, and oxygen and carbon isotopes obtained from pedogenic carbonates; these records are compared to other environmental proxies, including hydrated volcanic glass shards from volcanic ashes intercalated in the sedimentary strata.
There are few quantitative estimates of eolian bedrock-removal rates from arid, low relief landscapes. Wind-erosion rates from the western Qaidam Basin based on cosmogenic 10Be measurements document erosion rates between 0.05 to 0.4 mm/yr. This finding indicates that in arid environments with strong winds, hyperaridity, exposure of friable strata, and ongoing rock deformation and uplift, wind erosion can outpace fluvial erosion. Large eroded sediment volumes within the Qaidam Basin and coeval dust deposition on the Chinese Loess plateau, exemplify the importance of dust production within arid plateau environments for marine and terrestrial depositional processes, but also health issues and fertilization of soils.
In the south-central Andes, the analysis of 234 stream-water samples for oxygen and hydrogen reveals that areas experiencing deep convective storms do not show the commonly observed patterns of isotopic fractionation and the expected co-varying relationships between oxygen and hydrogen with increasing elevation. These convective storms are formed over semi-arid intermontane basins in the transition between the broken foreland of the Sierras Pampeanas, the Eastern Cordillera, and the Puna Plateau in the interior of the orogen. Here, convective rainfall dominates the precipitation budget and no systematic stable isotope-elevation relationship exists. Regions to the north, in the transition between the broken foreland and the Subandean foreland fold-and-thrust belt, the impact of convection is subdued, with lower degrees of storminess and a stronger expected isotope-elevation relationship. This finding of present-day fractionation trends of meteoric water is of great importance for paleoenvironmental studies in attempts to use stable isotope relationships in the reconstruction of paleoelevations.
The third part of the thesis focuses on the paleohydrological characteristics of the Mio-Pliocene (10-2 Ma) Angastaco Basin sedimentary record, which reveals far-reaching environmental changes during Andean uplift and orographic barrier formation. A precipitation- evapotranspiration record identifies the onset of a precipitation regime related to the South American Low Level Jet at this latitude after 9 Ma. Humid foreland conditions existed until 7 Ma, followed by orographic barrier uplift to the east of the present-day Angastaco Basin. This was superseded by rapid (~0.5 Myr) aridification in an intermontane basin, highlighting the effects of eastward-directed deformation. A transition in vegetation cover from a humid C3 forest ecosystem to semi-arid C4-dominated vegetation was coeval with continued basin uplift to modern elevations.
The idea that climatically modulated erosion may impact orogenic processes has challenged geoscientists for decades. Although modeling studies and physical calculations have provided a solid theoretical basis supporting this interaction, to date, field-based work has produced inconclusive results. The central-western Alborz Mountains in the northern sectors of the Arabia-Eurasia collision zone constitute a promising area to explore these potential feedbacks. This region is characterized by asymmetric precipitation superimposed on an orogen with a history of spatiotemporal changes in exhumation rates, deformation patterns, and prolonged, km-scale base-level changes. Our analysis suggests that despite the existence of a strong climatic gradient at least since 17.5 Ma, the early orogenic evolution (from similar to 36 to 9-6 Ma) was characterized by decoupled orographic precipitation and tectonics. In particular, faster exhumation and sedimentation along the more arid southern orogenic flank point to a north-directed accretionary flux and underthrusting of Central Iran. Conversely, from 6 to 3 Ma, erosion rates along the northern orogenic flank became higher than those in the south, where they dropped to minimum values. This change occurred during a similar to 3-Myr-long, km-scale base-level lowering event in the Caspian Sea. We speculate that mass redistribution processes along the northern flank of the Alborz and presumably across all mountain belts adjacent to the South Caspian Basin and more stable areas of the Eurasian plate increased the sediment load in the basin and ultimately led to the underthrusting of the Caspian Basin beneath the Alborz Mountains. This underthrusting in turn triggered a new phase of northward orogenic expansion, transformed the wetter northern flank into a new pro-wedge, and led to the establishment of apparent steady-state conditions along the northern orogenic flank (i.e., rock uplift equal to erosion rates). Conversely, the southern mountain front became the retro-wedge and experienced limited tectonic activity. These observations overall raise the possibility that mass-distribution processes during a pronounced erosion phase driven by base-level changes may have contributed to the inferred regional plate-tectonic reorganization of the northern Arabia-Eurasia collision during the last similar to 5 Ma. (C) 2015 Elsevier B.V. All rights reserved.
Erosion in the Himalaya is responsible for one of the greatest mass redistributions on Earth and has fueled models of feedback loops between climate and tectonics. Although the general trends of erosion across the Himalaya are reasonably well known, the relative importance of factors controlling erosion is less well constrained. Here we present 25 Be-10-derived catchment-averaged erosion rates from the Yamuna catchment in the Garhwal Himalaya, northern India. Tributary erosion rates range between similar to 0.1 and 0.5mmyr(-1) in the Lesser Himalaya and similar to 1 and 2mmyr(-1) in the High Himalaya, despite uniform hillslope angles. The erosion-rate data correlate with catchment-averaged values of 5 km radius relief, channel steepness indices, and specific stream power but to varying degrees of nonlinearity. Similar nonlinear relationships and coefficients of determination suggest that topographic steepness is the major control on the spatial variability of erosion and that twofold to threefold differences in annual runoff are of minor importance in this area. Instead, the spatial distribution of erosion in the study area is consistent with a tectonic model in which the rock uplift pattern is largely controlled by the shortening rate and the geometry of the Main Himalayan Thrust fault (MHT). Our data support a shallow dip of the MHT underneath the Lesser Himalaya, followed by a midcrustal ramp underneath the High Himalaya, as indicated by geophysical data. Finally, analysis of sample results from larger main stem rivers indicates significant variability of Be-10-derived erosion rates, possibly related to nonproportional sediment supply from different tributaries and incomplete mixing in main stem channels.
The role of feedback between erosional unloading and tectonics controlling the development of the Himalaya is a matter of current debate. The distribution of precipitation is thought to control surface erosion, which in turn results in tectonic exhumation as an isostatic compensation process. Alternatively, subsurface structures can have significant influence in the evolution of this actively growing orogen. Along the southern Himalayan front new 40Ar/39Ar white mica and apatite fission track (AFT) thermochronologic data provide the opportunity to determine the history of rock-uplift and exhumation paths along an approximately 120-km-wide NE-SW transect spanning the greater Sutlej region of the northwest Himalaya, India. 40Ar/39Ar data indicate, consistent with earlier studies that first the High Himalayan Crystalline, and subsequently the Lesser Himalayan Crystalline nappes were exhumed rapidly during Miocene time, while the deformation front propagated to the south. In contrast, new AFT data delineate synchronous exhumation of an elliptically shaped, NE-SW-oriented ~80 x 40 km region spanning both crystalline nappes during Pliocene-Quaternary time. The AFT ages correlate with elevation, but show within the resolution of the method no spatial relationship to preexisting major tectonic structures, such as the Main Central Thrust or the Southern Tibetan Fault System. Assuming constant exhumation rates and geothermal gradient, the rocks of two age vs. elevation transects were exhumed at ~1.4 ±0.2 and ~1.1 ±0.4 mm/a with an average cooling rate of ~50-60 °C/Ma during Pliocene-Quaternary time. The locus of pronounced exhumation defined by the AFT data coincides with a region of enhanced precipitation, high discharge, and sediment flux rates under present conditions. We therefore hypothesize that the distribution of AFT cooling ages might reflect the efficiency of surface processes and fluvial erosion, and thus demonstrate the influence of erosion in localizing rock-uplift and exhumation along southern Himalayan front, rather than encompassing the entire orogen.Despite a possible feedback between erosion and exhumation along the southern Himalayan front, we observe tectonically driven, crustal exhumation within the arid region behind the orographic barrier of the High Himalaya, which might be related to and driven by internal plateau forces. Several metamorphic-igneous gneiss dome complexes have been exhumed between the High Himalaya to the south and Indus-Tsangpo suture zone to the north since the onset of Indian-Eurasian collision ~50 Ma ago. Although the overall tectonic setting is characterized by convergence the exhumation of these domes is accommodated by extensional fault systems.Along the Indian-Tibetan border the poorly described Leo Pargil metamorphic-igneous gneiss dome (31-34°N/77-78°E) is located within the Tethyan Himalaya. New field mapping, structural, and geochronologic data document that the western flank of the Leo Pargil dome was formed by extension along temporally linked normal fault systems. Motion on a major detachment system, referred to as the Leo Pargil detachment zone (LPDZ) has led to the juxtaposition of low-grade metamorphic, sedimentary rocks in the hanging wall and high-grade metamorphic gneisses in the footwall. However, the distribution of new 40Ar/39Ar white mica data indicate a regional cooling event during middle Miocene time. New apatite fission track (AFT) data demonstrate that subsequently more of the footwall was extruded along the LPDZ in a brittle stage between 10 and 2 Ma with a minimum displacement of ~9 km. Additionally, AFT-data indicate a regional accelerated cooling and exhumation episode starting at ~4 Ma. Thus, tectonic processes can affect the entire orogenic system, while potential feedbacks between erosion and tectonics appear to be limited to the windward sides of an orogenic systems.
Graphite forms the endpoint for organic carbon metamorphism; it is extremely resilient to physical, biological and chemical degradation. Carbonaceous materials (CM) contained within sediments, collected across Taiwan and from the Gaoping submarine canyon, were analyzed using Raman spectroscopy to determine the crystallinity. This allowed the erosional and orogenic movements of petrogenic organic carbon (OCpetro) during the Taiwanese orogeny to be deduced. After automatically fitting and classifying spectra, the distribution of four groups of CM within the sediments provides evidence that many forms of OCpetro have survived at least one previous cycle of erosion, transport and burial before forming rocks in the Western Foothills of the island. There is extensive detrital graphite present in rocks that have not experienced high-grade metamorphism, and graphite flakes are also found in recently deposited marine sediments off Taiwan. The tectonic and geological history of the island shows that these graphite flakes must have survived at least three episodes of recycling. Therefore, transformation to graphite during burial and orogeny is a mechanism for stabilizing organic carbon over geological time, removing biospheric carbon from the active carbon cycle and protecting it from oxidation during future erosion events.
The article describes a systematic investigation of the effects of an aqueous NaOH treatment of 3D printed poly(lactic acid) (PLA) scaffolds for surface activation. The PLA surface undergoes several morphology changes and after an initial surface roughening, the surface becomes smoother again before the material dissolves. Erosion rates and surface morphologies can be controlled by the treatment. At the same time, the bulk mechanical properties of the treated materials remain unaltered. This indicates that NaOH treatment of 3D printed PLA scaffolds is a simple, yet viable strategy for surface activation without compromising the mechanical stability of PLA scaffolds.
The article describes a systematic investigation of the effects of an aqueous NaOH treatment of 3D printed poly(lactic acid) (PLA) scaffolds for surface activation. The PLA surface undergoes several morphology changes and after an initial surface roughening, the surface becomes smoother again before the material dissolves. Erosion rates and surface morphologies can be controlled by the treatment. At the same time, the bulk mechanical properties of the treated materials remain unaltered. This indicates that NaOH treatment of 3D printed PLA scaffolds is a simple, yet viable strategy for surface activation without compromising the mechanical stability of PLA scaffolds.
The article describes a systematic investigation of the effects of an aqueous NaOH treatment of 3D printed poly(lactic acid) (PLA) scaffolds for surface activation. The PLA surface undergoes several morphology changes and after an initial surface roughening, the surface becomes smoother again before the material dissolves. Erosion rates and surface morphologies can be controlled by the treatment. At the same time, the bulk mechanical properties of the treated materials remain unaltered. This indicates that NaOH treatment of 3D printed PLA scaffolds is a simple, yet viable strategy for surface activation without compromising the mechanical stability of PLA scaffolds.