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Synthesis of Magnaldehydes B and E and Dictyobiphenyl B by Microwave-Promoted Cross-Coupling of Boronophenols
- Magnaldehydes B and E along with their 4'-methylated derivatives are naturally occurring 2,4'-biphenols that have been isolated from the Magnoliaceae. Herein, these natural products have been synthesized from a common intermediate, which was obtained by a microwave-promoted, hetero-geneously catalyzed, and protecting-group-free Suzuki-Miyaura coupling reaction in an aqueous medium. These reaction conditions were also successfully applied to a one-step synthesis of the slime mold metabolite dictyobiphenyl B.
| Verfasserangaben: | Bernd SchmidtORCiDGND, Martin Riemer |
|---|---|
| DOI: | https://doi.org/10.1002/ejoc.201500350 |
| ISSN: | 1434-193X |
| ISSN: | 1099-0690 |
| Titel des übergeordneten Werks (Englisch): | European journal of organic chemistry |
| Verlag: | Wiley-VCH |
| Verlagsort: | Weinheim |
| Publikationstyp: | Wissenschaftlicher Artikel |
| Sprache: | Englisch |
| Jahr der Erstveröffentlichung: | 2015 |
| Erscheinungsjahr: | 2015 |
| Datum der Freischaltung: | 27.03.2017 |
| Freies Schlagwort / Tag: | Biaryls; Cross-coupling; Natural products; Palladium; Phenols; Total synthesis |
| Ausgabe: | 17 |
| Seitenanzahl: | 7 |
| Erste Seite: | 3760 |
| Letzte Seite: | 3766 |
| Organisationseinheiten: | Mathematisch-Naturwissenschaftliche Fakultät / Institut für Chemie |
| Peer Review: | Referiert |
