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Pride is linked to conviviality, to the practice of life-with-an-other, and to an awareness of the limitations of the life forms and life norms which guide and regulate the life of culturally, socially, and historically defined communities. Assuming this link, pride in living-together and conviviality appear as concepts creating a framework for future perspectives. But these concepts need a space in which they can unfold critically and confidently with a view to the future. For millennia, the literatures of the world have created this space of simulation and experimentation in which knowledge of how-to-live-with-an-other has been put down on paper through the open-ended tradition of writing. It is the space of the life forms and life norms of conviviality: it offers us prospective knowledge for the future by translating the imaginable into the thinkable, and the readable into the livable.
Electrochemical fluorination in anhydrous HF, also known as the Simons process, is a widely used industrial method for fluorination of organic compounds. Its mechanism, being not so well understood, has long been debated and is believed to involve higher valent nickel fluorides formed on the nickel-plated anode during the process. One of these is speculated to be Ni2F5, which was previously reported in the literature and assigned via infrared spectroscopy, but its crystal structure is not yet known. We have identified known crystal structures of compounds with similar stoichiometries as Ni2F5 and utilized them as a starting point for our periodic DFT investigations, applying the PBE+U method. Ni2F5 as the most stable polymorph was found to be of the same crystal structure as another mixed valent fluoride, Cr2F5. The calculated lattice parameters are a = 7.24 angstrom, b = 7.40 angstrom, c = 7.08 angstrom and beta = 118.9 degrees with an antiferromagnetic ordering of the nickel magnetic moments.
Most South Asian countries have challenges in ensuring water, energy, and food (WEF) security, which are often interacting positively or negatively. To address these challenges, the nexus approach provides a framework to identify the interactions of the WEF sectors as an integrated system. However, most nexus studies only qualitatively discuss the interactions between these sectors. This study conducts a systematic analysis of the WEF security nexus in South Asia by using open data sources at the country scale. We analyze interactions between the WEF sectors statistically, defining positive and negative correlations between the WEF security indicators as synergies and trade-offs, respectively. By creating networks of the synergies and trade-offs, we further identify most positively and negatively influencing indicators in the WEF security nexus. We observe a larger share of trade-offs than synergies within the water and energy sectors and a larger share of synergies than trade-offs among the WEF sectors for South Asia. However, these observations vary across the South Asian countries. Our analysis highlights that strategies on promoting sustainable energy and discouraging fossil fuel use could have overall positive effects on the WEF security nexus in the countries. This study provides evidence for considering the WEF security nexus as an integrated system rather than just a combination of three different sectors or securities.
Introduction:
mobile phone technology is increasingly used to overcome traditional barriers to limiting access to diabetes care. This study evaluated mobile phone ownership and willingness to receive and pay for mobile phone-based diabetic services among people with diabetes in South-West, Nigeria.
Methods:
two hundred and fifty nine patients with diabetes were consecutively recruited from three tertiary health institutions in South-West, Nigeria. Questionnaire was used to evaluate mobile phone ownership, willingness to receive and pay for mobile phone-based diabetic health care services via voice call and text messaging.
Results:
97.3% owned a mobile phone, with 38.9% and 61.1% owning smartphone and basic phone respectively. Males were significantly more willing to receive mobile-phone-based health services than females (81.1% vs 68.1%, p=0.025), likewise married compared to unmarried [77.4% vs 57.1%, p=0.0361. Voice calls (41.3%) and text messages (32.4%), were the most preferred modes of receiving diabetes-related health education with social media (3.1%) and email (1.5%) least. Almost three-quarter of participants (72.6%) who owned mobile phone, were willing to receive mobile phone-based diabetes health services. The educational status of patients (adjusted OR [AORJ: 1.7(95% CI: 1.6 to 2.11), glucometers possession (ACM: 2.0 [95% CI: 1.9 to 2.1) and type of mobile phone owned (AOR: 2.9 [95% CI: 2.8 to 5.0]) were significantly associated with the willingness to receive mobile phone-based diabetic services.
Conclusion:
the majority of study participants owned mobile phones and would be willing to receive and pay for diabetes-related healthcare delivery services provided the cost is minimal and affordable.
India is facing a double burden of malnourishment with co-existences of under- and over-nourishment. Various socioeconomic factors play an essential role in determining dietary choices. Agriculture is one of the major emitters of greenhouse gases (GHGs) in India, contributing 18% of total emissions. It also consumes freshwater and uses land significantly. We identify eleven Indian diets by applying k-means cluster analysis on latest data from the Indian household consumer expenditure survey. The diets vary in calorie intake [2289-3218 kcal/Consumer Unit (CU)/day] and dietary composition. Estimated embodied GHG emissions in the diets range from 1.36 to 3.62 kg CO2eq./CU/day, land footprint from 4 to 5.45 m(2)/CU/day, whereas water footprint varies from 2.13 to 2.97m(3)/CU/day. Indian diets deviate from a healthy reference diet either with too much or too little consumption of certain food groups. Overall, cereals, sugar, and dairy products intake are higher. In contrast, the consumption of fruits and vegetables, pulses, and nuts is lower than recommended. Our study contributes to deriving required polices for the sustainable transformation of food systems in India to eliminate malnourishment and to reduce the environmental implications of the food systems. (c) 2020 Elsevier B.V. All rights reserved.
Four topics were investigated in this longitudinal person-centered study: (a) profiles of subjective task values and ability self-concepts of adolescents in the domain of mathematics, (b) the stability of and changes to the profiles of motivational beliefs from Grade 7 to 12, (c) the relation of changes to student-perceived classroom characteristics, and (d) the extent to which profile membership in early adolescence predicted mathematics achievement and career plans in late adolescence and the choice of math-related college majors and occupations in adulthood. Data were drawn from the Michigan Study of Adolescent and Adult Life Transitions Study. We focused on students who participated in the following 4 waves of data collection (N = 867): at the beginning of Grade 7 (Wave 3), at the end of Grade 7, in Grade 10 (Wave 5), and in Grade 12 (Wave 6). Four profiles that were stable across Grades 7 to 12 were identified using Latent Profile Analysis. Student-reported fairness and friendliness and competition in class predicted changes in profile membership. Profile membership in Grade 7 predicted math-related career plans in Grade 12. Profile membership in Grade 12 predicted the choice of math-related college major after finishing school and of math-related occupations in adulthood.
Porphyry copper deposits are formed by fluids released from felsic magmatic intrusions of batholithic dimensions, which are inferred to have been incrementally built up by a series of sill injections. The growth of the magma chamber is primarily controlled by the volumetric injection rate from deeper-seated magma reservoirs, but can further be influenced by hydrothermal convection and fluid release. To quantify the interplay between magma chamber growth, volatile expulsion and hydrothermal fluid flow during ore formation, we used numerical simulations that can model episodic sill injections in concert with multi-phase fluid flow. To build up a magma chamber that constantly maintains a small region of melt within a period of about 50 kyrs, an injection rate of at least 1.3 x 10(-3) km(3)/y is required. Higher magma influxes of 1.9 to 7.6 x 10(-3) km(3)/y are able to form magma chambers with a thickness of 2 to 3 km. Such an intrusion continuously produces magmatic volatiles which can precipitate a copper ore shell in the host rock about 2 km above the fluid injection location. The steady fluid flux from such an incrementally growing magma chamber maintains a stable magmatic fluid plume, precipitating a copper ore shell in a more confined region and resulting in higher ore grades than the ones generated by an instantaneous emplacement of a voluminous magma chamber. Our simulation results suggest that magma chambers related to porphyry copper deposits form by rapid and episodic injection of magma. Slower magma chamber growth rates more likely result in barren plutonic rocks, although they are geochemically similar to porphyry-hosting plutons. However, these low-frequency sill injection events without a significant magma chamber growth can generate magmatic fluid pulses that can reach the shallow subsurface and are typical for high-sulfidation epithermal deposits.
Accelerograms are the primary source for characterizing strong ground motion. It is therefore of paramount interest to have high-quality recordings free from any nonphysical contamination. Frequently, accelerograms are affected by baseline jumps and drifts, either related to the instrument and/or a major earthquake. In this work, I propose a correction method for these undesired baseline drifts based on segmented linear least squares. The algorithm operates on the integrated waveforms and combines all three instrument components to estimate a model that modifies the baseline to be at zero continuously. The procedure consists of two steps: first a suite of models with variable numbers of discontinuities is derived for all three instrument components. During this process, the number of discontinuities is reduced in a parsimonious way, for example, two very close discontinuities are merged into a single one. In the second step, the optimal model is selected on the basis of the Bayesian information criterion. I exemplify the application on synthetic waveforms with known discontinuities and on observed waveforms from a unified strong-motion database of the Japan Meteorological Agency (JMA) and the National Research Institute for Earth Science and Disaster Prevention (NIED, Japan) networks for the major events of the 2016 Kumamoto earthquakes. After the baseline jump correction, the waveforms are furthermore corrected for displacement according to Wang et al.(2011). The resulting displacements are comparable to the Interferometric Synthetic Aperture Radar-derived displacement estimates for the Kumamoto earthquake sequence.
Impact of multivalence and self-assembly in the design of polymeric antimicrobial peptide mimics
(2020)
Antimicrobial resistance is an increasingly serious challenge for public health and could result in dramatic negative consequences for the health care sector during the next decades. To solve this problem, antibacterial materials that are unsusceptible toward the development of bacterial resistance are a promising branch of research. In this work, a new type of polymeric antimicrobial peptide mimic featuring a bottlebrush architecture is developed, using a combination of reversible addition-fragmentation chain transfer (RAFT) polymerization and ring-opening metathesis polymerization (ROMP). This approach enables multivalent presentation of antimicrobial subunits resulting in improved bioactivity and an increased hemocompatibility, boosting the selectivity of these materials for bacterial cells. Direct probing of membrane integrity of treated bacteria revealed highly potent membrane disruption caused by bottlebrush copolymers. Multivalent bottlebrush copolymers clearly outperformed their linear equivalents regarding bioactivity and selectivity. The effect of segmentation of cationic and hydrophobic subunits within bottle brushes was probed using heterograft copolymers. These materials were found to self-assemble under physiological conditions, which reduced their antibacterial activity, highlighting the importance of precise structural control for such applications. To the best of our knowledge, this is the first example to demonstrate the positive impact of multivalence, generated by a bottlebrush topology in polymeric antimicrobial peptide mimics, making these polymers a highly promising material platform for the design of new bactericidal systems.
This paper continues the line of research aimed at investigating the relationship between logic programs and first-order theories. We extend the definition of program completion to programs with input and output in a subset of the input language of the ASP grounder gringo, study the relationship between stable models and completion in this context, and describe preliminary experiments with the use of two software tools, anthem and vampire, for verifying the correctness of programs with input and output. Proofs of theorems are based on a lemma that relates the semantics of programs studied in this paper to stable models of first-order formulas.
Recent theoretical investigations claim that tailored laser pulses may selectively steer benzene's aromatic ground state to localized non-aromatic excited states. For instance, it has been shown that electronic wavepackets, involving the two lowest electronic eigenstates, exhibit subfemtosecond charge oscillation between equivalent Kekule resonance structures. In this contribution, we show that such dynamical electron-localization in the molecule-fixed frame contravenes the principle of the indistinguishability of identical particles. This breach stems from a total omission of the nuclear degrees of freedom, giving rise to nonsymmetric electronic wavepackets under nuclear permutations. Enforcement of the latter leads to entanglement between the electronic and nuclear states. To obey quantum statistics, the entangled molecular states should involve compensating nuclear-permutation symmetries. This in turn engenders complete quenching of dynamical electron-localization in the molecule-fixed frame. Indeed, for the (six-fold) equilibrium geometry of benzene, group-theoretic analysis reveals that any electronic wavepacket exhibits a (D-6h) totally symmetric electronic density, at all times. Thus, our results clearly show that the six carbon atoms, and the six C-C bonds, always have equal Mulliken charges, and equal bond orders, respectively. However, electronic wavepackets may display dynamical localization of the electronic density in the space-fixed frame, whenever they involve both even and odd space-inversion (parity) or permutation-inversion symmetry. Dynamical spatial-localization can be probed experimentally in the laboratory frame, but it should not be deemed equivalent to charge oscillation between benzene's identical electronic substructures, such as Kekule resonance structures.
Earthquake source arrays
(2020)
A collection of earthquake sources recorded at a single station, under specific conditions, are considered as a source array (SA), that is interpreted as if earthquake sources originate at the station location and are recorded at the source location. Then, array processing methods, that is array beamforming, are applicable to analyse the recorded signals. A possible application is to use source array multiple event techniques to locate and characterize near-source scatterers and structural interfaces. In this work the aim is to facilitate the use of earthquake source arrays by presenting an automatic search algorithm to configure the source array elements. We developed a procedure to search for an optimal source array element distribution given an earthquake catalogue including accurate origin time and hypocentre locations. The objective function of the optimization process can be flexibly defined for each application to ensure the prerequisites (criteria) of making a source array. We formulated four quantitative criteria as subfunctions and used the weighted sum technique to combine them in one single scalar function. The criteria are: (1) to control the accuracy of the slowness vector estimation using the time domain beamforming method, (2) to measure the waveform coherency of the array elements, (3) to select events with lower location error and (4) to select traces with high energy of specific phases, that is, sp- or ps-phases. The proposed procedure is verified using synthetic data as well as real examples for the Vogtland region in Northwest Bohemia. We discussed the possible application of the optimized source arrays to identify the location of scatterers in the velocity model by presenting a synthetic test and an example using real waveforms.
The GRACE-FO satellites launched in May 2018 are able to quantify the water mass deficit in Central Europe during the two consecutive summer droughts of 2018 and 2019. Relative to the long-term climatology, the water mass deficits were-112 +/- 10.5 Gt in 2018 and-145 +/- 12 Gt in 2019. These deficits are 73% and 94% of the mean amplitude of seasonal water storage variations, which is so severe that a recovery cannot be expected within 1 year. The water deficits in 2018 and 2019 are the largest in the whole GRACE and GRACE-FO time span. Globally, the data do not show an offset between the two missions, which proves the successful continuation of GRACE by GRACE-FO and thus the reliability of the observed extreme events in Central Europe. This allows for a joint assessment of the four Central European droughts in 2003, 2015, 2018, and 2019 in terms of total water storage deficits.
Diese Masterarbeit zielt darauf ab, exemplarisch an zoologischen Gärten für das politische Spannungsverhältnis zwischen Mensch und Tier zu sensibilisieren sowie die damit einhergehenden Aushandlungsprozesse auf individueller bzw. gesamtgesellschaftlicher Ebene didaktisch anschlussfähig zu machen. Nach einer kurzen begrifflichen Einführung der titelgebenden Termini werden in diesem Sinne vier verschiedene Ausdrucksformen ambivalenter Mensch-Tier-Beziehungen erörtert: die Entwicklungsgeschichte und Architektur sowie die Artenschutz- bzw. Bildungsleistungen der Zoos. Dabei wird der historisch vorbelastete Balanceakt zoologischer Gärten deutlich, in Gegenwart und Zukunft menschliche und tierliche Interessen glaubhaft in Einklang bringen zu müssen. Als Grundübel dieses Dilemmas wird wiederum der menschliche Anspruch identifiziert, Naturzustände vor dem Hintergrund eines fragwürdigen Legitimationsnarratives kulturell nachstellen zu wollen.
Außerdem entfaltet der Autor die These, dass der Zoo gerade durch die ihn prägenden Ambivalenzen gegenüber anderen Problembereichen der Mensch-Tier-Beziehungen an Kontroversität gewinnt und somit prädestiniert ist, um als politikdidaktische Reibungsfläche zeitgemäßer Mensch-Tier-Beziehungen zu fungieren. Dementsprechend werden abschließend Zugänge vorgeschlagen, um den Zoo als außerschulischen politischen Lernort vor dem Hintergrund vielfältiger Streitfragen erkunden und produktiv erörtern zu können.
Indem Schülerinnen und Schüler demnach die Wert- und Zweckrationalität der Zoos auf den Prüfstand stellen, werden sie dazu angeregt, sich selbst- und gesellschaftskritisch mit dem politischen Verhältnis zwischen Tieren und Menschen auseinanderzusetzen. Die dabei exemplarisch am Zoo gewonnenen Erkenntnisse und Überzeugungen lassen sich in Bezug auf die ebenso drängende wie polarisierende Tierfrage abstrahieren. Durch den somit geschaffenen Orientierungsrahmen werden die Lernenden nicht zuletzt in die Lage versetzt, ihre gereiften Vorstellungen von einem angemessenen Umgang mit (nichtmenschlichen) Tieren öffentlich zu vertreten.
Discrete element modeling of boulder and cliff morphologies on comet 67P/Churyumov-Gerasimenko
(2020)
Context:
Even after the Rosetta mission, some of the mechanical parameters of comet 67P/Churyumov-Gerasimenko's surface material are not yet well constrained. These parameters are needed to improve our understanding of cometary activity or for planning sample return missions.
Aims:
We study some of the physical processes involved in the formation of selected surface features and investigate the mechanical and geometrical parameters involved.
Methods:
Applying the discrete element method (DEM) in a low-gravity environment, we numerically simulated the surface layer particle dynamics involved in the formation of selected morphological features. The material considered is a mixture of polydisperse ice and dust spheres with inter-particle forces given by the Hertz contact model, translational friction, rolling friction, cohesion from unsintered contacts, and optionally due to bonds from ice sintering. We determined a working set of parameters that enables the simulations to be reasonably realistic and investigated morphological changes due to modifications thereof.
Results:
The selected morphological features are reasonably well reproduced using model materials with a tensile strength on the order of 1-10 Pa. Increasing the diameters of the spherical particles decreases the material strength, and increasing the friction leads to a more brittle but somewhat stronger material. High friction is required to make the material sufficiently brittle to match observations, which points to the presence of very rough, even angular particles. Reasonable seismic activity does not suffice to trigger the collapses of cliffs without material heterogeneities or structural defects.
Conclusions:
DEM modeling can be a powerful tool to investigate mechanical parameters of cometary surface material. However, many uncertainties arise from our limited understanding of particle shapes, spatial configurations, and size distributions, all on multiple length scales. Further numerical work, in situ measurements, and sample return missions are needed to better understand the mechanics of cometary material and cometary activity.
LiCSBAS
(2020)
For the past five years, the 2-satellite Sentinel-1 constellation has provided abundant and useful Synthetic Aperture Radar (SAR) data, which have the potential to reveal global ground surface deformation at high spatial and temporal resolutions. However, for most users, fully exploiting the large amount of associated data is challenging, especially over wide areas. To help address this challenge, we have developed LiCSBAS, an open-source SAR interferometry (InSAR) time series analysis package that integrates with the automated Sentinel-1 InSAR processor (LiCSAR). LiCSBAS utilizes freely available LiCSAR products, and users can save processing time and disk space while obtaining the results of InSAR time series analysis. In the LiCSBAS processing scheme, interferograms with many unwrapping errors are automatically identified by loop closure and removed. Reliable time series and velocities are derived with the aid of masking using several noise indices. The easy implementation of atmospheric corrections to reduce noise is achieved with the Generic Atmospheric Correction Online Service for InSAR (GACOS). Using case studies in southern Tohoku and the Echigo Plain, Japan, we demonstrate that LiCSBAS applied to LiCSAR products can detect both large-scale (>100 km) and localized (similar to km) relative displacements with an accuracy of <1 cm/epoch and similar to 2 mm/yr. We detect displacements with different temporal characteristics, including linear, periodic, and episodic, in Niigata, Ojiya, and Sanjo City, respectively. LiCSBAS and LiCSAR products facilitate greater exploitation of globally available and abundant SAR datasets and enhance their applications for scientific research and societal benefit.
No correlation between short term weight gain and lower leg length gain in healthy German children
(2020)
Background:
Length-for-age is considered the indicator of choice in monitoring the long-term impact of chronic nutritional deficiency. Aim: We hypothesized that short term increments of body weight cross-correlate with increments of the lower leg length.
Sample and methods:
We re-analyzed the association between weekly measurements of weight and of lower leg length in 34 healthy German children, aged 2.9-15.9 years. The data are a subset of measurements originally published in 1988 (Hermanussen et al. 1988a). As the growth measurements were often not equally spaced in time due to interposed holidays and illness, the incremental rates for weight and lower leg length were smoothed using spline functions. Autocorrelation and cross-correlation functions were calculated for weight increments and lower leg length increments.
Results:
Height and weight increments are pulsatile. Autocorrelations indicated that mini growth spurts occur at irregular intervals. Lack of cross-correlations between weight and lower leg length indicated that mini spurts in weight gain do not coincide with mini spurts in length gain even when considering lag times of up to 10 weeks. Short term changes of weight gain and lower leg length gain in healthy children show no temporal association.
Understanding the complexity of metabolic networks has implications for manipulation of their functions. The complexity of metabolic networks can be characterized by identifying multireaction dependencies that are challenging to determine due to the sheer number of combinations to consider. Here, we propose the concept of concordant complexes that captures multireaction dependencies and can be efficiently determined from the algebraic structure and operational constraints of metabolic networks. The concordant complexes imply the existence of concordance modules based on which the apparent complexity of 12 metabolic networks of organisms from all kingdoms of life can be reduced by at least 78%. A comparative analysis against an ensemble of randomized metabolic networks shows that the metabolic network of Escherichia coli contains fewer concordance modules and is, therefore, more tightly coordinated than expected by chance. Together, our findings demonstrate that metabolic networks are considerably simpler than what can be perceived from their structure alone.
Die Sekundärprävention der koronaren Herzkrankheit umfasst einerseits eine pharmakologische, andererseits eine lebensstilbasierte Säule, die idealerweise interagieren und sich potenzieren. Neben der medikamentösen Blutdruck- und Lipideinstellung auf leitlinienorientierte Zielwerte ermöglichen moderne Antidiabetika eine Optimierung des glukometabolischen Kontinuums und eine Prognosebesserung. Die Lebensstiloptimierung setzt sich aus koronarprotektiver Ernährung, einer individualisierten Trainingstherapie, einer konsequenten Nikotinkarenz und stressreduzierenden Maßnahmen zusammen. Die kardiologische Rehabilitation (Phase II) schließt sich idealerweise unmittelbar einem stationären Aufenthalt wegen eines akuten Koronarereignisses an, kann aber auch im Rahmen einer stabilen Koronarsituation im Rahmen eines allgemeinen Antragsverfahrens durchgeführt werden. Randomisierte und prospektiv angelegte Interventionsstudien belegen die prognostische Wertigkeit der kardiologischen Rehabilitation auch im Zeitalter akuter Revaskularisationstherapie mit 24-h-PCI und moderner Pharmakotherapie.
Natural ponds are perceived as spatially and temporally highly variable ecosystems. This perception is in contrast to the often-applied sampling design with high spatial but low temporal replication. Based on a data set covering a period of six years and 20 permanently to periodically inundated ponds, we investigated whether this widely applied sampling design is sufficient to identify differences between single ponds or single years with regard to water quality and macrophyte community composition as measures of ecosystem integrity.
In our study, the factor "pond", which describes differences between individual ponds, explained 56 % and 63 %, respectively, of the variance in water quality and macrophyte composition. In contrast, the factor "year" that refers to changes between individual years, contributed less to understand the observed variability in water quality and macrophyte composition (10 % and 7 % respectively, of the variance explained). The low explanation of variance for "year" and the low year-to-year correlation for the single water quality parameter or macrophyte coverage values, respectively, indicated high but non-consistent temporal variability affecting individual pond patterns.
In general, the results largely supported the ability of the widely applied sampling strategy with about one sampling date per year to capture differences in water quality and macrophyte community composition between ponds. Hence, future research can be rest upon sampling designs that give more weight to the number of ponds than the number of years in dependence on the research question and the available resources. Nonetheless, pond research would miss a substantial amount of information (7 to 10 % of the variance explained), when the sampling would generally be restricted to one year. Moreover, we expect that the importance of multiple-year sampling will likely increase in periods and regions of higher hydrological variability compared to the average hydrological conditions encountered in the studied period.