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Condensation and crystallization are omnipresent phenomena in nature. The formation of droplets or crystals on a solid surface are familiar processes which, beyond their scientific interest, are required in many technological applications. In recent years, experimental techniques have been developed which allow patterning a substrate with surface domains of molecular thickness, surface area in the mesoscopic scale, and different wettabilities (i.e., different degrees of preference for a substance that is in contact with the substrate). The existence of new patterned surfaces has led to increased theoretical efforts to understand wetting phenomena in such systems.
In this thesis, we deal with some problems related to the equilibrium of phases (e.g., liquid-vapor coexistence) and the kinetics of phase separation in the presence of chemically patterned surfaces. Two different cases are considered: (i) patterned surfaces in contact with liquid and vapor, and (ii) patterned surfaces in contact with a crystalline phase. One of the problems that we have studied is the following: It is widely believed that if air containing water vapor is cooled to its dew point, droplets of water are immediately formed. Although common experience seems to support this view, it is not correct. It is only when air is cooled well below its dew point that the phase transition occurs immediately. A vapor cooled slightly below its dew point is in a metastable state, meaning that the liquid phase is more stable than the vapor, but the formation of droplets requires some time to occur, which can be very long.
It was first pointed out by J. W. Gibbs that the metastability of a vapor depends on the energy necessary to form a nucleus (a droplet of a critical size). Droplets smaller than the critical size will tend to disappear, while droplets larger than the critical size will tend to grow. This is consistent with an energy barrier that has its maximum at the critical size, as is the case for droplets formed directly in the vapor or in contact with a chemically uniform planar wall. Classical nucleation theory describes the time evolution of the condensation in terms of the random process of droplet growth through this energy barrier. This process is activated by thermal fluctuations, which eventually will form a droplet of the critical size.
We consider nucleation of droplets from a vapor on a substrate patterned with easily wettable (lyophilic) circular domains. Under certain conditions of pressure and temperature, the condensation of a droplet on a lyophilic circular domain proceeds through a barrier with two maxima (a double barrier). We have extended classical nucleation theory to account for the kinetics of nucleation through a double barrier, and applied this extension to nucleation on lyophilic circular domains.
Inhalt:
- Eberhard Knobloch und Ingo Schwarz: Alexander von Humboldt und Hector Berlioz
- Oliver Lubrich: „[M]on extrême répugnance à écrire la relation de mon voyage“ – Alejandro de Humboldt deconstruye la relación de viaje
- Eva-Maria Siegel: Repräsentation und Augenschein. Organisation des Wissens und Wahrnehmung des Fremden um 1800 am Beispiel der Reiseberichte und -tagebücher Alexander von Humboldts
- Engelhard Weigl: Acclimatization: The Schomburgk brothers in South Australia
Inhalt:
- Ursula Thiemer-Sachse: El “Museo histórico indiano” de Lorenzo Boturini Benaduci y los esfuerzos del erudito alemán Alejandro de Humboldt para preservar sus restos para una interpretación científica
- Ursula Thiemer-Sachse: Petroglifos en rocas de la Cordillera de la Costa así como en los raudales de los ríos de la selva virgen venezolana. La interpretación por Alejandro de Humboldt y observaciones actuales
- Ingo Schwarz: „Ein beschränkter Verstandesmensch ohne Einbildungskraft“ – Anmerkungen zu Friedrich Schillers Urteil über Alexander von Humboldt
- Michael Zeuske: Humboldteanización del mundo occidental? La importancia del viaje de Humboldt para Europa y América Latina
De processibus matrimonialibus : Fachzeitschrift zu Fragen des kanonischen Ehe- und Prozeßrechtes
(2003)
The Parody of "Parody as Cultural Memory" in Richard Powers" Galatea 2.2 : a response to Anca Rosu
(2003)