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To evaluate the spatiotemporal variations of ground motions in northern Chile, we built a high-quality rock seismic acceleration database and an interface earthquakes catalog. Two ground-motion prediction equation (GMPE) models for subduction zones have been tested and validated for the area. They were then used as backbone models to describe the time-space variations of earthquake frequency content (Fourier and response spectra). Consistent with previous studies of large subduction earthquakes, moderate interface earthquakes in northern Chile show an increase of the high-frequency energy released with depth. A regional variability of earthquake frequency content is also observed, which may be related to a lateral segmentation of the mechanical properties of the subduction interface. Finally, interface earthquakes show a temporal evolution of their frequency content in the earthquake sequence associated with the 2014 Iquique M-w 8.1 megathrust earthquake. Surprisingly, the change does not occur with the mainshock but is associated with an 8 month slow slip preceding the megathrust. Electronic Supplement: Strong-motion database.