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Institute
- Institut für Biochemie und Biologie (224)
- Institut für Physik und Astronomie (196)
- Institut für Chemie (164)
- Institut für Geowissenschaften (159)
- Department Psychologie (73)
- Institut für Ernährungswissenschaft (55)
- Institut für Informatik und Computational Science (33)
- Institut für Mathematik (30)
- Department Linguistik (28)
- Department Sport- und Gesundheitswissenschaften (28)
We present a momentum transfer mechanism mediated by electromagnetic fields that originates in a system of two nearby molecules: one excited (donor D*) and the other in ground state (acceptor A). An intermolecular force related to fluorescence resonant energy or Forster transfer (FRET) arises in the unstable D* A molecular system, which differs from the equilibrium van der Waals interaction. Due to the its finite lifetime, a mechanical impulse is imparted to the relative motion in the system. We analyze the FRET impulse when the molecules are embedded in free space and find that its magnitude can be much greater than the single recoil photon momentum, getting comparable with the thermal momentum (Maxwell-Boltzmann distribution) at room temperature. In addition, we propose that this FRET impulse can be exploited in the generation of acoustic waves inside a film containing layers of donor and acceptor molecules, when a picosecond laser pulse excites the donors. This acoustic transient is distinguishable from that produced by thermal stress due to laser absorption, and may therefore play a role in photoacoustic spectroscopy. The effect can be seen as exciting a vibrating system like a string or organ pipe with light; it may be used as an opto-mechanical transducer.
Empirical species distribution models (SDMs) constitute often the tool of choice for the assessment of rapid climate change effects on species vulnerability. Conclusions regarding extinction risks might be misleading, however, because SDMs do not explicitly incorporate dispersal or other demographic processes. Here, we supplement SDMs with a dynamic population model 1) to predict climate-induced range dynamics for black grouse in Switzerland, 2) to compare direct and indirect measures of extinction risks, and 3) to quantify uncertainty in predictions as well as the sources of that uncertainty. To this end, we linked models of habitat suitability to a spatially explicit, individual-based model. In an extensive sensitivity analysis, we quantified uncertainty in various model outputs introduced by different SDM algorithms, by different climate scenarios and by demographic model parameters. Potentially suitable habitats were predicted to shift uphill and eastwards. By the end of the 21st century, abrupt habitat losses were predicted in the western Prealps for some climate scenarios. In contrast, population size and occupied area were primarily controlled by currently negative population growth and gradually declined from the beginning of the century across all climate scenarios and SDM algorithms. However, predictions of population dynamic features were highly variable across simulations. Results indicate that inferring extinction probabilities simply from the quantity of suitable habitat may underestimate extinction risks because this may ignore important interactions between life history traits and available habitat. Also, in dynamic range predictions uncertainty in SDM algorithms and climate scenarios can become secondary to uncertainty in dynamic model components. Our study emphasises the need for principal evaluation tools like sensitivity analysis in order to assess uncertainty and robustness in dynamic range predictions. A more direct benefit of such robustness analysis is an improved mechanistic understanding of dynamic species responses to climate change.
Data limitations can lead to unrealistic fits of predictive species distribution models (SDMs) and spurious extrapolation to novel environments. Here, we want to draw attention to novel combinations of environmental predictors that are within the sampled range of individual predictors but are nevertheless outside the sample space. These tend to be overlooked when visualizing model behaviour. They may be a cause of differing model transferability and environmental change predictions between methods, a problem described in some studies but generally not well understood. We here use a simple simulated data example to illustrate the problem and provide new and complementary visualization techniques to explore model behaviour and predictions to novel environments. We then apply these in a more complex real-world example. Our results underscore the necessity of scrutinizing model fits, ecological theory and environmental novelty.
The c-Fosc-Jun complex forms the activator protein 1 transcription factor, a therapeutic target in the treatment of cancer. Various synthetic peptides have been designed to try to selectively disrupt the interaction between c-Fos and c-Jun at its leucine zipper domain. To evaluate the binding affinity between these synthetic peptides and c-Fos, polarizable and nonpolarizable molecular dynamics (MD) simulations were conducted, and the resulting conformations were analyzed using the molecular mechanics generalized Born surface area (MM/GBSA) method to compute free energies of binding. In contrast to empirical and semiempirical approaches, the estimation of free energies of binding using a combination of MD simulations and the MM/GBSA approach takes into account dynamical properties such as conformational changes, as well as solvation effects and hydrophobic and hydrophilic interactions. The predicted binding affinities of the series of c-Jun-based peptides targeting the c-Fos peptide show good correlation with experimental melting temperatures. This provides the basis for the rational design of peptides based on internal, van der Waals, and electrostatic interactions.
Determination of the source rocks for the diatexites from the Edough Massif, Annaba, NE Algeria
(2012)
The crystalline Edough Massif is located in the oriental part of the Algerian coastline. It consists of two tectonically superposed units of gneisses, augen-gneisses and migmatitic gneisses in the lower unit and micaschists in the upper unit. The crystalline rocks underwent a low to moderate degree of metamorphism; the gneisses suffered partial melting. They display migmatitic features such as nebulitic structures with contorted leucosome layers and K-feldspar porphyroblasts and thus can be classified as diatexites. The mineralogical composition of these rocks is very homogenous and consists of K-feldspar, micas and quartz. The feldspar-rich, arkosic nature of the outcrop implies a granitic source rock. High K2O/Na2O ratios and high A/CNK > 1.1 indicate an S-type granite source and a peraluminous composition of the protolith respectively. Chondrite normalized REE distribution patterns of the Edough diatexites show gently inclined patterns with a minor negative Eu anomaly (Eu/Eu* = 0.36-0.49), which points to a very slightly differentiated granitic source. The REE pattern and trace element data of the diatexites are similar to those of average Proterozoic upper continental crust, which suggests that they are derived mainly from upper continental crust and were deposited in continental margins.
Magnetic ionogels (MagIGs) were prepared from organosilane-coated iron oxide nanoparticles, N-isopropylacrylamide, and the ionic liquid trihexyl(tetradecyl)phosphonium dicyanamide. The ionogels prepared with the silane-modified nanoparticles are more homogeneous than ionogels prepared with unmodified magnetite particles. The silane-modified particles are immobilized in the ionogel and are resistant tonanoparticle leaching. The modified particles also render the ionogels mechanically more stable than the ionogels synthesized with unmodified nanoparticles. The ionogels respond to external permanent magnets and are therefore prototypes of a new soft magnetic actuator.
The adoption, in Kampala in June 2010, of amendments to the Rome Statute on the crime of aggression was hailed as a historic milestone in the development of the international Criminal Court (ICC). However, the manner in which these amendments are supposed to enter into force runs the risk of undermining the rules of the international law of treaties, as well as the legality and acceptability of the Kampala compromise itself The author examines the relevant amendment procedures provided for in the ICC Statute and the compatibility with them of the amendment procedure chosen in Kampala and ultimately warns of the legal consequences which may follow from the Review Conference's somewhat-Alexandrian solution.
State sucession in treaties
(2012)
Continuity of states
(2012)
Forests seem to represent low-erosion systems, according to most, but not all, studies of suspended-sediment yield. We surmised that this impression reflects an accidental bias in the selection of monitoring sites towards those with prevailing vertical hydrological flowpaths, rather than a tight causal link between vegetation cover and erosion alone. To evaluate this conjecture, we monitored, over a 2-year period, a 3.3 ha old-growth rainforest catchment prone to frequent and widespread overland flow. We sampled stream flow at two and overland flow at three sites in a nested arrangement on a within-event basis, and monitored the spatial and temporal frequency of overland flow. Suspended-sediment concentrations were modeled with Random Forest and Quantile Regression Forest to be able to estimate the annual yields for the 2 years, which amounted to 1 t ha(-1) and 2 t ha(-1) in a year with below-average and with average precipitation, respectively. These estimates place our monitoring site near the high end of reported suspended-sediment yields and lend credence to the notion that low yields reflect primarily the dominance of vertical flowpaths and not necessarily and exclusively the kind of vegetative cover. Undisturbed forest and surface erosion are certainly no contradiction in terms even in the absence of mass movements.
Multidirectional communicative interactions in social networks can have a profound effect on mate choice behavior. Male Atlantic molly Poecilia mexicana exhibit weaker mating preferences when an audience male is presented. This could be a male strategy to reduce sperm competition risk: interacting more equally with different females may be advantageous because rivals might copy mate choice decisions. In line with this hypothesis, a previous study found males to show a strong audience effect when being observed while exercising mate choice, but not when the rival was presented only before the choice tests. Audience effects on mate choice decisions have been quantified in poeciliid fishes using association preference designs, but it remains unknown if patterns found from measuring association times translate into actual mating behavior. Thus, we created five audience treatments simulating different forms of perceived sperm competition risk and determined focal males' mating preferences by scoring pre-mating (nipping) and mating behavior (gonopodial thrusting). Nipping did not reflect the pattern that was found when association preferences were measured, while a very similar pattern was uncovered in thrusting behavior. The strongest response was observed when the audience could eavesdrop on the focal male's behavior. A reduction in the strength of focal males' preferences was also seen after the rival male had an opportunity to mate with the focal male's preferred mate. In comparison, the reduction of mating preferences in response to an audience was greater when measuring association times than actual mating behavior. While measuring direct sexual interactions between the focal male and both stimulus females not only the male's motivational state is reflected but also females' behavior such as avoidance of male sexual harassment.
A membrane of a dielectric elastomer coated with compliant electrodes may form wrinkles as the applied voltage is ramped up. We present a combination of experiment and theory to investigate the transition to wrinkles using a clamped membrane subject to a constant force and a voltage ramp. Two types of transitions are identified. In type-I transition, the voltage-stretch curve is N-shaped, and flat and wrinkled regions coexist in separate areas of the membrane. The type-I transition progresses by nucleation of small wrinkled regions, followed by the growth of the wrinkled regions at the expense of the flat regions, until the entire membrane is wrinkled. By contrast, in type-II transition, the voltage-stretch curve is monotonic, and the entire flat membrane becomes wrinkled with no nucleation barrier. The two types of transitions are analogous to the first and the second order phase transitions. While the type-I transition is accompanied by a jump in the vertical displacement, type-II transition is accompanied by a continuous change in the vertical displacement. Such transitions may enable applications in muscle-like actuation and energy harvesting, where large deformation and large energy of conversion are desired.
The switching kinetics of thin thermo-responsive hydrogel films of poly(monomethoxy-diethyleneglycol-acrylate) (PMDEGA) are investigated. Homogeneous and smooth PMDEGA films with a thickness of 35.9 nm are prepared on silicon substrates by spin coating. As probed with white light interferometry, PMDEGA films with a thickness of 35.9 nm exhibit a phase transition temperature of the lower critical solution temperature (LCST) type of 40 degrees C. In situ neutron reflectivity is performed to investigate the thermo-responsive behavior of these PMDEGA hydrogel films in response to a sudden thermal stimulus in deuterated water vapor atmosphere. The collapse transition proceeds in a complex way which can be seen as three steps. The first step is the shrinkage of the initially swollen film by a release of water. In the second step the thickness remains constant with water molecules embedded in the film. In the third step, perhaps due to a conformational rearrangement of the collapsed PMDEGA chains, water is reabsorbed from the vapor atmosphere, thereby giving rise to a relaxation process. Both the shrinkage and relaxation processes can be described by a simple model of hydrogel deswelling.
In order to identify the areas in the Xilingele grassland which are sensitive to wind erosion, a computational fluid dynamics model (CFD-WEM) was used to simulate the wind fields over a region of 37 km(2) which contains different topography and land use types. Previous studies revealed the important influences of topography and land use on wind erosion in the Xilingele grassland. Topography influences wind fields at large scale, and land use influences wind fields near the ground. Two steps were designed to implement the CFD wind simulation, and they were respectively to simulate the influence of topography and surface roughness on the wind. Digital elevation model (DEM) and surface roughness length were the key inputs for the CFD simulation. The wind simulation by CFD-WEM was validated by a wind data set which was measured simultaneously at six positions in the field. Three scenarios with different wind velocities were designed based on observed dust storm events, and wind fields were simulated according to these scenarios to predict the sensitive areas to wind erosion. General assumptions that cropland is the most sensitive area to wind erosion and heavily and moderately grazed grasslands are both sensitive etc. can be refined by the modelling of CFD-WEM. Aided by the results of this study, the land use planning and protection measures against wind erosion can be more efficient. Based on the case study in the Xilingele grassland, a method of regional wind erosion assessment aided by CFD wind simulation is summarized. The essence of this method is a combination of CFD wind simulation and determination of threshold wind velocity for wind erosion. Because of the physically-based simulation and the flexibility of the method, it can be generalised to other regions.