T. Katayama, Toyli Anniyev, Martin Beye, Ryan Coffee, M. Dell'Angela, Alexander Föhlisch, J. Gladh, S. Kaya, O. Krupin, A. Nilsson, D. Nordlund, W. F. Schlotter, J. A. Sellberg, Florian Sorgenfrei, J. J. Turner, W. Wurth, H. Öström, H. Ogasawara
- We report on an experimental system designed to probe chemical reactions on solid surfaces on a sub-picosecond timescale using soft X-ray emission spectroscopy at the Linac Coherent Light Source (LCLS) free electron laser (FEL) at the SLAC National Accelerator Laboratory. We analyzed the O 1s X-ray emission spectra recorded from atomic oxygen adsorbed on a Ru(0001) surface at a synchrotron beamline (SSRL, BL13-2) and an FEL beamline (LCLS, SXR). We have demonstrated conditions that provide negligible amount of FEL induced damage of the sample. In addition we show that the setup is capable of tracking the temporal evolution of electronic structure during a surface reaction of submonolayer quantities of CO molecules desorbing from the surface.
Metadaten| Author details: | T. Katayama, Toyli Anniyev, Martin BeyeORCiDGND, Ryan Coffee, M. Dell'Angela, Alexander FöhlischORCiDGND, J. Gladh, S. Kaya, O. Krupin, A. Nilsson, D. Nordlund, W. F. Schlotter, J. A. Sellberg, Florian SorgenfreiORCiDGND, J. J. Turner, W. Wurth, H. Öström, H. Ogasawara |
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| DOI: | https://doi.org/10.1016/j.elspec.2013.03.006 |
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| ISSN: | 0368-2048 |
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| Title of parent work (English): | Journal of electron spectroscopy and related phenomena : the international journal on theoretical and experimental aspects of electron spectroscopy |
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| Publisher: | Elsevier |
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| Place of publishing: | Amsterdam |
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| Publication type: | Article |
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| Language: | English |
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| Year of first publication: | 2013 |
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| Publication year: | 2013 |
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| Release date: | 2017/03/26 |
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| Tag: | Free electron laser; Surface science; Ultrafast; X-ray emission spectroscopy |
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| Volume: | 187 |
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| Issue: | 1 |
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| Number of pages: | 6 |
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| First page: | 9 |
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| Last Page: | 14 |
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| Funding institution: | LCLS, Stanford University through the Stanford Institute for Materials
Energy Sciences (SIMES); Lawrence Berkeley National Laboratory (LBNL);
University of Hamburg through the BMBF priority program FSP 301; Center
for Free Electron Laser Science (CFEL); US Department of Energy's Office
of Basic Energy Sciences; Japan Science and Technology Agency; Swedish
research council (VR); Alexander von Humboldt foundation;
VolkswagenStiftung |
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| Organizational units: | Mathematisch-Naturwissenschaftliche Fakultät / Institut für Physik und Astronomie |
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| Peer review: | Referiert |
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