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Quantum dynamics of laser-induced desorption from metal and semiconductor surfaces, and related phenomena

  • Recent progress towards a quantum theory of laser-induced desorption and related phenomena is reviewed, for specific examples. These comprise the photodesorption of NO from Pt(111), the scanning tunnelling microscope and laser- induced desorption and switching of H at Si(100), and the electron stimulated desorption and dissociation of CO at Ru(0001). The theoretical methods used for nuclear dynamics range from open-system density matrix theory over nonadiabatically coupled multi-state models to electron-nuclear wavepackets. Also, aspects of time-dependent spectroscopy to probe ultrafast nonadiabatic processes at surfaces will be considered for the example of two-photon photoemission of solvated electrons in ice layers on Cu(111)

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Metadaten
Author details:Peter SaalfrankORCiDGND, Mathias NestGND, Igor V. Andrianov, Tillmann KlamrothORCiDGND, Dominic Kroner, Stephanie BeyversGND
URL:http://iopscience.iop.org/0953-8984/18/30/S05/pdf/0953-8984_18_30_S05.pdf
DOI:https://doi.org/10.1088/0953-8984/18/30/S05
ISSN:1361-648X
ISSN:0953-8984
Publisher:IOP Publ.
Place of publishing:Bristol
Publication type:Article
Language:English
Date of first publication:2006/07/14
Publication year:2006
Release date:2017/03/24
Volume:18
Issue:30
First page:S1425
Last Page:S1459
Source:Journal of physics-condensed matter. - 18 (2006), 30, S. S1425 - S1459
Organizational units:Mathematisch-Naturwissenschaftliche Fakultät / Institut für Physik und Astronomie
DDC classification:5 Naturwissenschaften und Mathematik / 53 Physik / 530 Physik
Peer review:Referiert
Institution name at the time of the publication:Mathematisch-Naturwissenschaftliche Fakultät / Institut für Physik
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