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Time resolved resonant inelastic X-ray scattering: a supreme tool to understand dynamics in solids and molecules

  • Dynamics in materials typically involve different degrees of freedom, like charge, lattice, orbital and spin in a complex interplay. Time-resolved resonant inelastic X-ray scattering (RIXS) as a highly selective tool can provide unique insight and follow the details of dynamical processes while resolving symmetries, chemical and charge states, momenta, spin configurations, etc. In this paper, we review examples where the intrinsic scattering duration time is used to study femtosecond phenomena. Free-electron lasers access timescales starting in the sub-ps range through pump-probe methods and synchrotrons study the time scales longer than tens of ps. In these examples, time-resolved resonant inelastic X-ray scattering is applied to solids as well as molecular systems.

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Metadaten
Author:M. Beye, Ph. Wernet, Christian Schüßler-Langeheine, Alexander FöhlischORCiDGND
DOI:https://doi.org/10.1016/j.elspec.2013.04.013
ISSN:0368-2048 (print)
Parent Title (English):Journal of electron spectroscopy and related phenomena : the international journal on theoretical and experimental aspects of electron spectroscopy
Publisher:Elsevier
Place of publication:Amsterdam
Document Type:Article
Language:English
Year of first Publication:2013
Year of Completion:2013
Release Date:2017/03/26
Tag:Molecular dynamics; Phase transitions; Resonant inelastic X-ray scattering; Ultrafast spectroscopy
Volume:188
Issue:3
Pagenumber:11
First Page:172
Last Page:182
Funder:VolkswagenStiftung
Organizational units:Mathematisch-Naturwissenschaftliche Fakultät / Institut für Physik und Astronomie
Peer Review:Referiert