@article{NishikawaHardeeDutanetal.2014, author = {Nishikawa, Ken-Ichi and Hardee, P. E. and Dutan, I. and Niemiec, J. and Medvedev, M. and Mizuno, Y. and Meli, A. and Sol, H. and Zhang, B. and Pohl, Martin and Hartmann, D. H.}, title = {Magnetic agnetic field generation in core-sheath jets via the kinetic Kelvin-Helmholtz instability}, series = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, volume = {793}, journal = {The astrophysical journal : an international review of spectroscopy and astronomical physics}, number = {1}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0004-637X}, doi = {10.1088/0004-637X/793/1/60}, pages = {16}, year = {2014}, abstract = {We have investigated magnetic field generation in velocity shears via the kinetic Kelvin-Helmholtz instability (kKHI) using a relativistic plasma jet core and stationary plasma sheath. Our three-dimensional particle-in-cell simulations consider plasma jet cores with Lorentz factors of 1.5, 5, and 15 for both electron-proton and electron-positron plasmas. For electron-proton plasmas, we find generation of strong large-scale DC currents and magnetic fields that extend over the entire shear surface and reach thicknesses of a few tens of electron skin depths. For electron-positron plasmas, we find generation of alternating currents and magnetic fields. Jet and sheath plasmas are accelerated across the shear surface in the strong magnetic fields generated by the kKHI. The mixing of jet and sheath plasmas generates a transverse structure similar to that produced by the Weibel instability.}, language = {en} } @article{GodecBauerMetzler2014, author = {Godec, Aljaz and Bauer, Maximilian and Metzler, Ralf}, title = {Collective dynamics effect transient subdiffusion of inert tracers in flexible gel networks}, series = {New journal of physics : the open-access journal for physics}, volume = {16}, journal = {New journal of physics : the open-access journal for physics}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {1367-2630}, doi = {10.1088/1367-2630/16/9/092002}, pages = {13}, year = {2014}, abstract = {Based on extensive Brownian dynamics simulations we study the thermal motion of a tracer bead in a cross-linked, flexible gel in the limit when the tracer particle size is comparable to or even larger than the equilibrium mesh size of the gel. The analysis of long individual trajectories of the tracer demonstrates the existence of pronounced transient anomalous diffusion. From the time averaged mean squared displacement and the time averaged van Hove correlation functions we elucidate the many-body origin of the non-Brownian tracer bead dynamics. Our results shed new light onto the ongoing debate over the physical origin of steric tracer interactions with structured environments.}, language = {en} } @article{MiedemaBeyeKoenneckeetal.2014, author = {Miedema, P. S. and Beye, Martin and Koennecke, R. and Schiwietz, G. and F{\"o}hlisch, Alexander}, title = {The angular- and crystal-momentum transfer through electron-phonon coupling in silicon and silicon-carbide: similarities and differences}, series = {New journal of physics : the open-access journal for physics}, volume = {16}, journal = {New journal of physics : the open-access journal for physics}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {1367-2630}, doi = {10.1088/1367-2630/16/9/093056}, pages = {17}, year = {2014}, abstract = {Electron-phonon scattering has been studied for silicon carbide (6H-SiC) with resonant inelastic x-ray scattering at the silicon 2p edge. The observed electron-phonon scattering yields a crystal momentum transfer rate per average phonon in 6H-SiC of 1.8 fs(-1) while it is 0.2 fs(-1) in crystalline silicon. The angular momentum transfer rate per average phonon for 6H-SiC is 0.1 fs(-1), which is much higher than 0.0035 fs(-1) obtained for crystalline silicon in a previous study. The higher electron-phonon scattering rates in 6H-SiC are a result of the larger electron localization at the silicon atoms in 6H-SiC as compared to crystalline silicon. While delocalized valence electrons can screen effectively (part of) the electron-phonon interaction, this effect is suppressed for 6H-SiC in comparison to crystalline silicon. Smaller contributions to the difference in electron-phonon scattering rates between 6H-SiC and silicon arise from the lower atomic mass of carbon versus silicon and the difference in local symmetry.}, language = {en} } @article{XuBrennerChabanneetal.2014, author = {Xu, Jingsan and Brenner, Thomas J. K. and Chabanne, Laurent and Neher, Dieter and Antonietti, Markus and Shalom, Menny}, title = {Liquid-Based growth of polymeric carbon nitride layers and their use in a mesostructured polymer solar cell with V-oc exceeding 1 V}, series = {Journal of the American Chemical Society}, volume = {136}, journal = {Journal of the American Chemical Society}, number = {39}, publisher = {American Chemical Society}, address = {Washington}, issn = {0002-7863}, doi = {10.1021/ja508329c}, pages = {13486 -- 13489}, year = {2014}, abstract = {Herein we report a general liquid-mediated pathway for the growth of continuous polymeric carbon nitride (C3N4) thin films. The deposition method consists of the use of supramolecular complexes that transform to the liquid state before direct thermal condensation into C3N4 solid films. The resulting films exhibit continuous porous C3N4 networks on various substrates. Moreover, the optical absorption can be easily tuned to cover the solar spectrum by the insertion of an additional molecule into the starting complex. The strength of the deposition method is demonstrated by the use of the C3N4 layer as the electron acceptor in a polymer solar cell that exhibits a remarkable open-circuit voltage exceeding 1 V. The easy, safe, and direct synthesis of carbon nitride in a continuous layered architecture on different functional substrates opens new possibilities for the fabrication of many energy-related devices.}, language = {en} } @article{DiFlorioBruendermannYadavallietal.2014, author = {Di Florio, G. and Bruendermann, E. and Yadavalli, Nataraja Sekhar and Santer, Svetlana and Havenith, Martina}, title = {Graphene multilayer as nanosized optical strain gauge for polymer surface relief gratings}, series = {Nano letters : a journal dedicated to nanoscience and nanotechnology}, volume = {14}, journal = {Nano letters : a journal dedicated to nanoscience and nanotechnology}, number = {10}, publisher = {American Chemical Society}, address = {Washington}, issn = {1530-6984}, doi = {10.1021/nl502631s}, pages = {5754 -- 5760}, year = {2014}, abstract = {In this paper, we show how graphene can be utilized as a nanoscopic probe in order to characterize local opto-mechanical forces generated within photosensitive azobenzene containing polymer films. Upon irradiation with light interference patterns, photosensitive films deform according to the spatial intensity variation, leading to the formation of periodic topographies such as surface relief gratings (SRG). The mechanical driving forces inscribing a pattern into the films are supposedly fairly large, because the deformation takes place without photofluidization; the polymer is in a glassy state throughout. However, until now there has been no attempt to characterize these forces by any means. The challenge here is that the forces vary locally on a nanometer scale. Here, we propose to use Raman analysis of the stretching of the graphene layer adsorbed on top of polymer film under deformation in order to probe the strength of the material transport spatially resolved. With the well-known mechanical properties of graphene, we can obtain lower bounds on the forces acting within the film. Upon the basis of our experimental results, we can deduce that the internal pressure in the film due to grating formation can exceed 1 GPa. The graphene-based nanoscopic gauge opens new possibilities to characterize opto-mechanical forces generated within photosensitive polymer films.}, language = {en} } @article{SteffenHubrigTodtetal.2014, author = {Steffen, M. and Hubrig, Swetlana and Todt, Helge Tobias and Schoeller, M. and Hamann, Wolf-Rainer and Sandin, Christer and Sch{\"o}nberner, Detlef}, title = {Weak magnetic fields in central stars of planetary nebulae?}, series = {Astronomy and astrophysics : an international weekly journal}, volume = {570}, journal = {Astronomy and astrophysics : an international weekly journal}, publisher = {EDP Sciences}, address = {Les Ulis}, issn = {0004-6361}, doi = {10.1051/0004-6361/201423842}, pages = {15}, year = {2014}, abstract = {Context. It is not yet clear whether magnetic fields play an essential role in shaping planetary nebulae (PNe), or whether stellar rotation alone and/or a close binary companion, stellar or substellar, can account for the variety of the observed nebular morphologies. Aims. In a quest for empirical evidence verifying or disproving the role of magnetic fields in shaping planetary nebulae, we follow up on previous attempts to measure the magnetic field in a representative sample of PN central stars. Methods. We obtained low-resolution polarimetric spectra with FORS2 installed on the Antu telescope of the VLT for a sample of 12 bright central stars of PNe with different morphologies, including two round nebulae, seven elliptical nebulae, and three bipolar nebulae. Two targets are Wolf-Rayet type central stars. Results. For the majority of the observed central stars, we do not find any significant evidence for the existence of surface magnetic fields. However, our measurements may indicate the presence of weak mean longitudinal magnetic fields of the order of 100 Gauss in the central star of the young elliptical planetary nebula IC 418 as well as in the Wolf-Rayet type central star of the bipolar nebula Hen 2-113 and the weak emission line central star of the elliptical nebula Hen 2-131. A clear detection of a 250 G mean longitudinal field is achieved for the A-type companion of the central star of NGC 1514. Some of the central stars show a moderate night-to-night spectrum variability, which may be the signature of a variable stellar wind and/or rotational modulation due to magnetic features. Conclusions. Since our analysis indicates only weak fields, if any, in a few targets of our sample, we conclude that strong magnetic fields of the order of kG are not widespread among PNe central stars. Nevertheless, simple estimates based on a theoretical model of magnetized wind bubbles suggest that even weak magnetic fields below the current detection limit of the order of 100 G may well be sufficient to contribute to the shaping of the surrounding nebulae throughout their evolution. Our current sample is too small to draw conclusions about a correlation between nebular morphology and the presence of stellar magnetic fields.}, language = {en} } @article{MeibohmSchreckWernet2014, author = {Meibohm, Jan and Schreck, Simon and Wernet, Philippe}, title = {Temperature dependent soft x-ray absorption spectroscopy of liquids}, series = {Review of scientific instruments : a monthly journal devoted to scientific instruments, apparatus, and techniques}, volume = {85}, journal = {Review of scientific instruments : a monthly journal devoted to scientific instruments, apparatus, and techniques}, number = {10}, publisher = {American Institute of Physics}, address = {Melville}, issn = {0034-6748}, doi = {10.1063/1.4896977}, pages = {7}, year = {2014}, abstract = {A novel sample holder is introduced which allows for temperature dependent soft x-ray absorption spectroscopy of liquids in transmission mode. The setup is based on sample cells with x-ray transmissive silicon nitride windows. A cooling circuit allows for temperature regulation of the sample liquid between -10 degrees C and +50 degrees C. The setup enables to record soft x-ray absorption spectra of liquids in transmission mode with a temperature resolution of 0.5K and better. Reliability and reproducibility of the spectra are demonstrated by investigating the characteristic temperature-induced changes in the oxygen K-edge x-ray absorption spectrum of liquid water. These are compared to the corresponding changes in the oxygen K-edge spectra from x-ray Raman scattering. (C) 2014 AIP Publishing LLC.}, language = {en} } @article{Goychuk2014, author = {Goychuk, Igor}, title = {Life and death of stationary linear response in anomalous continuous time random walk dynamics}, series = {Communications in theoretical physics : a series journal of the Chinese Physical Society (A)}, volume = {62}, journal = {Communications in theoretical physics : a series journal of the Chinese Physical Society (A)}, number = {4}, publisher = {IOP Publ. Ltd.}, address = {Bristol}, issn = {0253-6102}, pages = {497 -- 504}, year = {2014}, abstract = {Linear theory of stationary response in systems at thermal equilibrium requires to find equilibrium correlation function of unperturbed responding system. Studies of the response of the systems exhibiting anomalously slow dynamics are often based on the continuous time random walk description (CTRW) with divergent mean waiting times. The bulk of the literature on anomalous response contains linear response functions like one by Cole-Cole calculated from such a CTRW theory and applied to systems at thermal equilibrium. Here we show within a fairly simple and general model that for the systems with divergent mean waiting times the stationary response at thermal equilibrium is absent, in accordance with some recent studies. The absence of such stationary response (or dying to zero non-stationary response in aging experiments) would confirm CTRW with divergent mean waiting times as underlying physical relaxation mechanism, but reject it otherwise. We show that the absence of stationary response is closely related to the breaking of ergodicity of the corresponding dynamical variable. As an important new result, we derive a generalized Cole-Cole response within ergodic CTRW dynamics with finite waiting time. Moreover, we provide a physically reasonable explanation of the origin and wide presence of 1/f noise in condensed matter for ergodic dynamics close to normal, rather than strongly deviating.}, language = {en} } @article{KralemannPikovskijRosenblum2014, author = {Kralemann, Bjoern and Pikovskij, Arkadij and Rosenblum, Michael}, title = {Reconstructing connectivity of oscillator networks from multimodal observations}, series = {Biomedizinische Technik = Biomedical engineering}, volume = {59}, journal = {Biomedizinische Technik = Biomedical engineering}, publisher = {De Gruyter}, address = {Berlin}, issn = {0013-5585}, doi = {10.1515/bmt-2014-4089}, pages = {S220 -- S220}, year = {2014}, language = {en} } @article{SchreckBeyeSellbergetal.2014, author = {Schreck, Simon and Beye, Martin and Sellberg, Jonas A. and McQueen, Trevor and Laksmono, Hartawan and Kennedy, Brian and Eckert, Sebastian and Schlesinger, Daniel and Nordlund, Dennis and Ogasawara, Hirohito and Sierra, Raymond G. and Segtnan, Vegard H. and Kubicek, Katharina and Schlotter, William F. and Dakovski, Georgi L. and Moeller, Stefan P. and Bergmann, Uwe and Techert, Simone and Pettersson, Lars G. M. and Wernet, Philippe and Bogan, Michael J. and Harada, Yoshihisa and Nilsson, Anders and F{\"o}hlisch, Alexander}, title = {Reabsorption of soft x-ray emission at high x-ray free-electron laserfluences}, series = {Physical review letters}, volume = {113}, journal = {Physical review letters}, number = {15}, publisher = {American Physical Society}, address = {College Park}, issn = {0031-9007}, doi = {10.1103/PhysRevLett.113.153002}, pages = {6}, year = {2014}, abstract = {We report on oxygen K-edge soft x-ray emission spectroscopy from a liquid water jet at the Linac Coherent Light Source. We observe significant changes in the spectral content when tuning over a wide range of incident x-ray fluences. In addition the total emission yield decreases at high fluences. These modifications result from reabsorption of x-ray emission by valence-excited molecules generated by the Auger cascade. Our observations have major implications for future x-ray emission studies at intense x-ray sources. We highlight the importance of the x-ray pulse length with respect to the core-hole lifetime.}, language = {en} }