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Interference between Resonant and Nonresonant Inelastic X-Ray Scattering

  • A detailed study of inelastic x-ray scattering from the ground state to the (3)Sigma(g)(3 sigma(-1)(g)3s(g)(1)) state of the O-2 molecule is presented. The observed angular anisotropy shows that the vibrational excitations within this final state are strongly dependent on the polarization of the incident radiation. The analysis demonstrates that this is a manifestation of interference between resonant and direct nonresonant inelastic x-ray scattering. This interference provides a new tool to monitor nuclear dynamics by relative rotation of the polarization vectors of the incident and scattered photons.

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Metadaten
Author:Y. -P. Sun, Q. Miao, A. Pietzsch, F. Hennies, T. Schmitt, V. N. Strocov, Joakim Andersson, B. Kennedy, J. Schlappa, A. Foehlisch, Gel&rsquo, F. mukhanov, J. -E. Rubensson
DOI:https://doi.org/10.1103/PhysRevLett.110.223001
ISSN:0031-9007 (print)
Parent Title (English):PHYSICAL REVIEW LETTERS
Publisher:AMER PHYSICAL SOC
Place of publication:COLLEGE PK
Document Type:Article
Language:English
Year of first Publication:2013
Year of Completion:2013
Release Date:2017/03/26
Volume:110
Issue:22
Pagenumber:4
Funder:European Community [226716]; Helmholtz Virtual Institute "Dynamic Pathways in Multidimensional Landscapes’’; Swedish Research Council (VR); Carl Tryggers Stiftelse (CTS); National Natural Science Foundation of China [11204163, 10974121]; National Basic Research Program of China [2011CB808100]