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Optimized spatial overlap in optical pump-X-ray probe experiments with high repetition rate using laser-induced surface distortions

  • Ultrafast X-ray diffraction experiments require careful adjustment of the spatial overlap between the optical excitation and the X-ray probe pulse. This is especially challenging at high laser repetition rates. Sample distortions caused by the large heat load on the sample and the relatively low optical energy per pulse lead to only tiny signal changes. In consequence, this results in small footprints of the optical excitation on the sample, which turns the adjustment of the overlap difficult. Here a method for reliable overlap adjustment based on reciprocal space mapping of a laser excited thin film is presented.

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Metadaten
Author details:Matthias Reinhardt, Azize Koc, Wolfram LeitenbergerGND, Peter Gaal, Matias BargheerORCiDGND
DOI:https://doi.org/10.1107/S1600577515024443
ISSN:1600-5775
Pubmed ID:https://pubmed.ncbi.nlm.nih.gov/26917135
Title of parent work (English):Journal of synchrotron radiation
Publisher:International Union of Crystallography
Place of publishing:Chester
Publication type:Article
Language:English
Year of first publication:2016
Publication year:2016
Release date:2020/03/22
Tag:heat diffusion; nanostructures; optical pump; surface deformation; ultrafast X-ray diffraction
Volume:23
Number of pages:6
First page:474
Last Page:479
Organizational units:Mathematisch-Naturwissenschaftliche Fakultät / Institut für Physik und Astronomie
Peer review:Referiert
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