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Rydberg-Resolved Resonant Inelastic Soft X-Ray Scattering: Dynamics at Core Ionization Thresholds

  • Resonant inelastic x-ray scattering spectra excited in the immediate vicinity of the core-level ionization thresholds of N-2 have been recorded. Final states of well-resolved symmetry-selected Rydberg series converging to valence-level ionization thresholds with vibrational excitations are observed. The results are well described by a quasi-two-step model which assumes that the excited electron is unaffected by the radiative decay. This threshold dynamics simplifies the interpretation of resonant inelastic x-ray scattering spectra considerably and facilitates characterization of low-energy excited final states in molecular systems.

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Author:Jan-Erik Rubensson, Johan Soderstrom, Christian Binggeli, Joakim Grasjo, Johan Andersson, Conny Sathe, Franz Hennies, Valentina Bisogni, Yaobo Huang, Paul Olalde, Thorsten Schmitt, Vladimir N. Strocov, Alexander FöhlischORCiDGND, Brian Kennedy, Annette Pietzsch
DOI:https://doi.org/10.1103/PhysRevLett.114.133001
ISSN:0031-9007 (print)
ISSN:1079-7114 (online)
Pubmed Id:http://www.ncbi.nlm.nih.gov/pubmed?term=25884123
Parent Title (English):Physical review letters
Publisher:American Physical Society
Place of publication:College Park
Document Type:Article
Language:English
Year of first Publication:2015
Year of Completion:2015
Release Date:2017/03/27
Volume:114
Issue:13
Pagenumber:5
Funder:Swedish Research Council (VR)
Organizational units:Mathematisch-Naturwissenschaftliche Fakultät / Institut für Physik und Astronomie
Peer Review:Referiert