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A soft X-ray approach to electron-phonon interactions beyond the Born-Oppenheimer approximation

  • With modern soft X-ray methods, the whole field of electron-phonon interactions becomes accessible directly in the ultrafast time domain with ultrashort pulsed X-ray sources, as well as in the energy domain through modern highly resolving spectrometers. The well-known core-hole clock approach plays an intermediate role, resolving energetic and temporal features at the same time. In this perspective paper, we review several experiments to illustrate the modern advances in the selective study of electron-phonon interactions as fundamentally determining ingredients for materials properties. We present the different complementary approaches that can be taken with soft X-ray methods to conquer this field beyond the Born-Oppenheimer approximation.

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Metadaten
Author:M. Beye, Alexander FöhlischORCiDGND
DOI:https://doi.org/10.1016/j.elspec.2010.12.032
ISSN:0368-2048 (print)
Parent Title (English):Journal of electron spectroscopy and related phenomena : the international journal on theoretical and experimental aspects of electron spectroscopy
Publisher:Elsevier
Place of publication:Amsterdam
Document Type:Article
Language:English
Year of first Publication:2011
Year of Completion:2011
Release Date:2017/03/26
Tag:Electron-phonon coupling; Near edge X-ray absorption fine structure; Resonant inelastic X-ray scattering; X-ray emission spectroscopy
Volume:184
Issue:3-6
Pagenumber:5
First Page:313
Last Page:317
Organizational units:Mathematisch-Naturwissenschaftliche Fakultät / Institut für Physik und Astronomie
Peer Review:Referiert