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Free-electron laser based resonant inelastic X-ray scattering on molecules and liquids

  • The unprecedented beam properties of free-electron laser based X-ray sources enable novel resonant inelastic X-ray scattering (RIXS) experiments. Femtosecond time-resolved RIXS can be used to follow charge, spin and structural dynamics of dilute solute molecules in solution. Ultrashort X-ray pulses allow probing of highly radiation sensitive states of matter such as the metastable phase of supercooled liquid water. Nonlinear X-ray probes like amplified spontaneous emission and stimulated resonant X-ray scattering provide an enhanced selectivity and sensitivity as well as a path to control radiation damage and increase the photon yields in RIXS experiments. (C) 2015 Elsevier B.V. All rights reserved.

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Author:Kristjan Kunnus, Simon Schreck, Alexander FöhlischORCiDGND
ISSN:0368-2048 (print)
ISSN:1873-2526 (online)
Parent Title (English):Journal of electron spectroscopy and related phenomena : the international journal on theoretical and experimental aspects of electron spectroscopy
Place of publication:Amsterdam
Document Type:Article
Year of first Publication:2015
Year of Completion:2015
Release Date:2017/03/27
Tag:Free-electron laser; Liquids; Molecules; Nonlinear X-ray spectroscopy; Pump-probe; RIXS
First Page:345
Last Page:355
Organizational units:Mathematisch-Naturwissenschaftliche Fakultät / Institut für Physik und Astronomie
Peer Review:Referiert