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Alkyne-X modification of polypeptoids

  • Poly(N-propargyl glycine) (PNPG) can be readily prepared by ring-opening polymerization of N-propargyl glycine N-carboxyanhydride (NCA) and modified using various addition reactions such as copper catalyzed [3+2] cycloaddition of azide, radical (photo-)addition of thiol, nucleophilic addition of ethylene oxide, and thermal induced cross-linking. It is demonstrated that PNPG can serve as a modular platform to produce a bibliography of novel functional polypeptoid or pseudopeptide materials, including polypeptoid ionic liquids and graft copolymers.

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Metadaten
Author:Christian Secker, Joshua W. Robinson, Helmut SchlaadORCiDGND
DOI:https://doi.org/10.1016/j.eurpolymj.2014.08.028
ISSN:0014-3057 (print)
ISSN:1873-1945 (online)
Parent Title (English):European polymer journal
Publisher:Elsevier
Place of publication:Oxford
Document Type:Article
Language:English
Year of first Publication:2015
Year of Completion:2015
Release Date:2017/03/27
Tag:Click chemistry; NCA; Polypeptoid; Post-polymerization modification
Volume:62
Pagenumber:6
First Page:394
Last Page:399
Funder:Max Planck Society
Organizational units:Mathematisch-Naturwissenschaftliche Fakultät / Institut für Chemie
Peer Review:Referiert