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Discrete Polymetallic Arrangements of Ag-I and Cu-I Ions Based on Multiple Bridging Phosphane Ligands and pi-pi Interactions

  • A simple and straightforward approach to new polymetallic Ag-I and Cu-I supramolecules is presented. The reaction of N,P,N,P,N ligand 2 with Ag-I ions affords a trimetallic complex bearing a triangular Ag-3 core; metallophilic interactions are stabilized by ligands that display a multiple bridging coordination mode as 10-electron donors. Heteroleptic polymetallic Ag-I and Cu-I complexes based on ligand 2 and the 1,12-diazaperylene (dape) ligand are obtained by an alternative molecular organization of the polymetallic arrays compared to that in homoleptic complexes of ligand 2.

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Author details:Bianca Attenberger, Mehdi El Sayed Moussa, Thomas Martin BrietzkeGND, Volodimir Vreshch, Hans-Jürgen HoldtORCiD, Christophe Lescop, Manfred Scheer
DOI:https://doi.org/10.1002/ejic.201500445
ISSN:1434-1948
ISSN:1099-0682
Title of parent work (English):European journal of inorganic chemistry : a journal of ChemPubSoc Europe
Publisher:Wiley-VCH
Place of publishing:Weinheim
Publication type:Article
Language:English
Year of first publication:2015
Publication year:2015
Release date:2017/03/27
Tag:Heterocycles; N; P ligands; Pi interactions; Polyaromatic fragments; Supramolecular chemistry
Issue:18
Number of pages:5
First page:2934
Last Page:2938
Funding institution:National de la Recherche Scientifique (CNRS); Ministere des Affaires Etrangeres et Europeennes; Agence Nationale de la Recherche (ANR) [ANR-12-BS07-0004-METALHEL-01]; Campus France; Deutsche Forschungsgemeinschaft (DFG); COST action PhoSciNet for short-term scientific mission (STSM) grants; Alexander von Humboldt Foundation
Organizational units:Mathematisch-Naturwissenschaftliche Fakultät / Institut für Chemie
Peer review:Referiert
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