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Synchrotron-based ultrafast x-ray diffraction at high repetition rates

  • We present a setup for ultrafast x-ray diffraction (UXRD) based at the storage ring BESSY II, in particular, a pump laser that excites the sample using 250 fs laser-pulses at repetition rates ranging from 208 kHz to 1.25 MHz. We discuss issues connected to the high heat-load and spatio-temporal alignment strategies in the context of a UXRD experiment at high repetition rates. The spatial overlap between laser pump and x-ray probe pulse is obtained with 10 mu m precision and transient lattice changes can be recorded with an accuracy of delta a/a(0) = 10(-6). We also compare time-resolved x-ray diffraction signals from a laser excited LSMO/STO superlattice with phonon dynamics simulations. From the analysis we determine the x-ray pulse duration to 120 ps in standard operation mode and below 10 ps in low-alpha mode.

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Author details:H. Navirian, R. Shayduk, Wolfram LeitenbergerGND, J. Goldshteyn, P. Gaal, Matias BargheerORCiDGND
DOI:https://doi.org/10.1063/1.4727872
ISSN:0034-6748
Title of parent work (English):Review of scientific instruments : a monthly journal devoted to scientific instruments, apparatus, and techniques
Publisher:American Institute of Physics
Place of publishing:Melville
Publication type:Article
Language:English
Year of first publication:2012
Publication year:2012
Release date:2017/03/26
Volume:83
Issue:6
Number of pages:7
Funding institution:BMBF [05K10IP1]; Deutsche Forschungsgemeinschaft (DFG) [SFB 762]
Organizational units:Mathematisch-Naturwissenschaftliche Fakultät / Institut für Physik und Astronomie
Peer review:Referiert
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