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A molecular precursor approach to tunable porous tin-rich indium tin oxide with durable high electrical conductivity for bioelectronic devices

  • The preparation of porous, i.e., high surface area electrodes from transparent conducting oxides, is a valuable goal in materials chemistry as such electrodes can enable further development of optoelectronic, electrocatalytic, or bioelectronic devices. In this work the first tin-rich mesoporous indium tin oxide is prepared using the molecular heterobimetallic single-source precursor, indium tin tris-tert-butoxide, together with an appropriate structure-directing template, yielding materials with high surface areas and tailorable pore size. The resulting mesoporous tin-rich ITO films show a high and durable electrical conductivity and transparency, making them interesting materials for hosting electroactive biomolecules such as proteins. In fact, its unique performance in bioelectronic applications has been demonstrated by immobilization of high amounts of cytochrome c into the mesoporous film which undergo redox processes directly with the conductive electrode material.

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Metadaten
Author:Yilmaz Aksu, Stefano Frasca, Ursula WollenbergerORCiDGND, Matthias Driess, Arne Thomas
DOI:https://doi.org/10.1021/cm103087p
ISSN:0897-4756 (print)
Parent Title (English):Chemistry of materials : a publication of the American Chemical Society
Publisher:American Chemical Society
Place of publication:Washington
Document Type:Article
Language:English
Year of first Publication:2011
Year of Completion:2011
Release Date:2017/03/26
Tag:bioelectrochemistry; cytochrome c; device; electrode; indium tin oxide ITO
Volume:23
Issue:7
Pagenumber:7
First Page:1798
Last Page:1804
Funder:Deutsche Forschungsgemeinschaft; TU Berlin
Organizational units:Mathematisch-Naturwissenschaftliche Fakultät / Institut für Biochemie und Biologie
Peer Review:Referiert