Catalytic bio–chemo and bio–bio tandem oxidation reactions for amide and carboxylic acid synthesis
- A catalytic toolbox for three different water-based one-pot cascades to convert aryl alcohols to amides and acids and cyclic amines to lactams, involving combination of oxidative enzymes (monoamine oxidase, xanthine dehydrogenase, galactose oxidase and laccase) and chemical oxidants (TBHP or CuI(cat)/H2O2) at mild temperatures, is presented. Mutually compatible conditions were found to afford products in good to excellent yields.
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| Author details: | Beatrice Bechi, Susanne Herter, Shane McKenna, Christopher Riley, Silke LeimkühlerORCiDGND, Nicholas J. Turner, Andrew J. Carnell |
|---|---|
| URN: | urn:nbn:de:kobv:517-opus4-99414 |
| Publication series (Volume number): | Zweitveröffentlichungen der Universität Potsdam : Mathematisch-Naturwissenschaftliche Reihe (282) |
| Publication type: | Postprint |
| Language: | English |
| Date of first publication: | 2014/08/18 |
| Publication year: | 2014 |
| Publishing institution: | Universität Potsdam |
| Release date: | 2016/11/17 |
| Source: | Green Chem. (2014) Nr. 16, S. 4524-4529. - DOI: 10.1039/c4gc01321b |
| Organizational units: | Mathematisch-Naturwissenschaftliche Fakultät / Institut für Biochemie und Biologie |
| DDC classification: | 5 Naturwissenschaften und Mathematik / 54 Chemie / 540 Chemie und zugeordnete Wissenschaften |
| Peer review: | Referiert |
| Publishing method: | Open Access |
| License (German): |  Keine öffentliche Lizenz: Unter Urheberrechtsschutz |
