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Direct time-domain sampling of subterahertz coherent acoustic phonon spectra in SrTiO3 using ultrafast x-ray diffraction

  • We synthesize sub-THz longitudinal quasimonochromatic acoustic phonons in a SrTiO3 single crystal using a SrRuO3/SrTiO3 superlattice as an optical-acoustic transducer. The generated acoustic phonon spectrum is determined using ultrafast x-ray diffraction. The analysis of the generated phonon spectrum in the time domain reveals a k-vector dependent phonon lifetime. It is observed that even at sub-THz frequencies the phonon lifetime agrees with the 1/omega(2) power law known from Akhiezer's model for hyper sound attenuation. The observed shift of the synthesized spectrum to the higher q is discussed in the framework of nonlinear effects appearing due to the high amplitude of the synthesized phonons.

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Metadaten
Author details:Roman Shayduk, Marc HerzogORCiDGND, Andre BojahrGND, Daniel Schick, Peter Gaal, Wolfram LeitenbergerGND, Hengameh Navirian, Mathias Sander, Jevgenij Goldshteyn, Ionela Vrejoiu, Matias BargheerORCiDGND
DOI:https://doi.org/10.1103/PhysRevB.87.184301
ISSN:1098-0121
Title of parent work (English):Physical review : B, Condensed matter and materials physics
Publisher:American Physical Society
Place of publishing:College Park
Publication type:Article
Language:English
Year of first publication:2013
Publication year:2013
Release date:2017/03/26
Volume:87
Issue:18
Number of pages:7
Funding institution:BMBF [05K 2012-OXIDE]
Organizational units:Mathematisch-Naturwissenschaftliche Fakultät / Institut für Physik und Astronomie
Peer review:Referiert
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