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A setup for resonant inelastic soft x-ray scattering on liquids at free electron laser light sources

  • We present a flexible and compact experimental setup that combines an in vacuum liquid jet with an x-ray emission spectrometer to enable static and femtosecond time-resolved resonant inelastic soft x-ray scattering (RIXS) measurements from liquids at free electron laser (FEL) light sources. We demonstrate the feasibility of this type of experiments with the measurements performed at the Linac Coherent Light Source FEL facility. At the FEL we observed changes in the RIXS spectra at high peak fluences which currently sets a limit to maximum attainable count rate at FELs. The setup presented here opens up new possibilities to study the structure and dynamics in liquids.

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Author:Kristjan Kunnus, Ivan Rajkovic, Simon Schreck, Wilson Quevedo, Sebastian Eckert, Martin Beye, Edlira Suljoti, Christian Weniger, Christian Kalus, Sebastian Gruebel, Mirko Scholz, Dennis Nordlund, Wenkai Zhang, Robert W. Hartsock, Kelly J. Gaffney, William F. Schlotter, Joshua J. Turner, Brian Kennedy, Franz Hennies, Simone Techert, Philippe Wernet, Alexander FöhlischORCiDGND
DOI:https://doi.org/10.1063/1.4772685
ISSN:0034-6748 (print)
Parent Title (English):Review of scientific instruments : a monthly journal devoted to scientific instruments, apparatus, and techniques
Publisher:American Institute of Physics
Place of publication:Melville
Document Type:Article
Language:English
Year of first Publication:2012
Year of Completion:2012
Release Date:2017/03/26
Volume:83
Issue:12
Pagenumber:8
Funder:Advanced Study Group; DFG [SFB 602, SFB 755]; Nanoscale Photonic Imaging [SFB 755]; VolkswagenStiftung; Chemical Sciences, Geosciences, and Biosciences Division of the Office of Basic Energy Sciences, Office of Science, U.S. Department of Energy; LCLS, Stanford University through the Stanford Institute for Materials Energy Sciences (SIMES); Lawrence Berkeley National Laboratory (LBNL), University of Hamburg through the BMBF [FSP 301]; Center for Free Electron Laser Science (CFEL)
Organizational units:Mathematisch-Naturwissenschaftliche Fakultät / Institut für Physik und Astronomie
Peer Review:Referiert