TY  - JOUR
A1  - Stange, Maike
A1  - Hintsche, Marius
A1  - Sachse, Kirsten
A1  - Gerhardt, Matthias
A1  - Valleriani, Angelo
A1  - Beta, Carsten
T1  - Analyzing the spatial positioning of nuclei in polynuclear giant cells
JF  - Journal of Physics D: Applied Physics
N2  - How cells establish and maintain a well-defined size is a fundamental question of cell biology. Here we investigated to what extent the microtubule cytoskeleton can set a predefined cell size, independent of an enclosing cell membrane. We used electropulse-induced cell fusion to form giant multinuclear cells of the social amoeba Dictyostelium discoideum. Based on dual-color confocal imaging of cells that expressed fluorescent markers for the cell nucleus and the microtubules, we determined the subcellular distributions of nuclei and centrosomes in the giant cells. Our two- and three-dimensional imaging results showed that the positions of nuclei in giant cells do not fall onto a regular lattice. However, a comparison with model predictions for random positioning showed that the subcellular arrangement of nuclei maintains a low but still detectable degree of ordering. This can be explained by the steric requirements of the microtubule cytoskeleton, as confirmed by the effect of a microtubule degrading drug.
KW  - Dictyostelium
KW  - cell nucleus
KW  - positioning
KW  - imaging
KW  - spatial poisson distribution
Y1  - 2017
U6  - https://doi.org/10.1088/1361-6463/aa8da0
SN  - 0022-3727
SN  - 1361-6463
VL  - 50
IS  - 46
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Kurzke, Henning
A1  - Kiethe, Jan
A1  - Heuer, Axel
A1  - Jechow, Andreas
T1  - Frequency doubling of incoherent light from a superluminescent diode in a periodically poled lithium niobate waveguide crystal
JF  - Laser physics letters
N2  - The amplified spontaneous emission from a superluminescent diode was frequency doubled in a periodically poled lithium niobate waveguide crystal. The temporally incoherent radiation of such a superluminescent diode is characterized by a relatively broad spectral bandwidth and thermal-like photon statistics, as the measured degree of second order coherence, g((2))(0)= 1.9 +/- 0.1, indicates. Despite the non-optimized scenario in the spectral domain, we achieve six orders of magnitude higher conversion efficiency than previously reported with truly incoherent light. This is possible by using single spatial mode radiation and quasi phase matched material with a waveguide architecture. This work is a principle step towards efficient frequency conversion of temporally incoherent radiation in one spatial mode to access wavelengths where no radiation from superluminescent diodes is available, especially with tailored quasi phase matched crystals. The frequency doubled light might find application in imaging, metrology and quantum optics experiments.
KW  - nonlinear frequency conversion
KW  - periodically poled material
KW  - waveguides
KW  - incoherent radiation
Y1  - 2017
U6  - https://doi.org/10.1088/1612-202X/aa6889
SN  - 1612-2011
SN  - 1612-202X
VL  - 14
PB  - IOP Publ.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Kamann, Sebastian
A1  - Husser, T. -O.
A1  - Dreizler, S.
A1  - Emsellem, E.
A1  - Weilbacher, Peter Michael
A1  - Martens, S.
A1  - Bacon, R.
A1  - den Brok, M.
A1  - Giesers, B.
A1  - Krajnovic, Davor
A1  - Roth, Martin M.
A1  - Wendt, Martin
A1  - Wisotzki, Lutz
T1  - A stellar census in globular clusters with MUSE
BT  - the contribution of rotation to cluster dynamics studied with 200 000 stars
JF  - Monthly notices of the Royal Astronomical Society
N2  - This is the first of a series of papers presenting the results from our survey of 25 Galactic globular clusters with the MUSE integral-field spectrograph. In combination with our dedicated algorithm for source deblending, MUSE provides unique multiplex capabilities in crowded stellar fields and allows us to acquire samples of up to 20 000 stars within the half-light radius of each cluster. The present paper focuses on the analysis of the internal dynamics of 22 out of the 25 clusters, using about 500 000 spectra of 200 000 individual stars. Thanks to the large stellar samples per cluster, we are able to perform a detailed analysis of the central rotation and dispersion fields using both radial profiles and two-dimensional maps. The velocity dispersion profiles we derive show a good general agreement with existing radial velocity studies but typically reach closer to the cluster centres. By comparison with proper motion data, we derive or update the dynamical distance estimates to 14 clusters. Compared to previous dynamical distance estimates for 47 Tuc, our value is in much better agreement with other methods. We further find significant (>3 sigma) rotation in the majority (13/22) of our clusters. Our analysis seems to confirm earlier findings of a link between rotation and the ellipticities of globular clusters. In addition, we find a correlation between the strengths of internal rotation and the relaxation times of the clusters, suggesting that the central rotation fields are relics of the cluster formation that are gradually dissipated via two-body relaxation.
KW  - techniques: imaging spectroscopy
KW  - stars: kinematics and dynamics
KW  - globular clusters: general
Y1  - 2017
U6  - https://doi.org/10.1093/mnras/stx2719
SN  - 0035-8711
SN  - 1365-2966
VL  - 473
IS  - 4
SP  - 5591
EP  - 5616
PB  - Oxford Univ. Press
CY  - Oxford
ER  - 
TY  - JOUR
A1  - Hani, Maan H.
A1  - Sparre, Martin
A1  - Ellison, Sara L.
A1  - Torrey, Paul
A1  - Vogelsberger, Mark
T1  - Galaxy mergers moulding the circum-galactic medium
BT  - I. The impact of a major merger
JF  - Monthly notices of the Royal Astronomical Society
N2  - Galaxies are surrounded by sizeable gas reservoirs which host a significant amount of metals: the circum-galactic medium (CGM). The CGM acts as a mediator between the galaxy and the extragalactic medium. However, our understanding of how galaxy mergers, a major evolutionary transformation, impact the CGM remains deficient. We present a theoretical study of the effect of galaxy mergers on the CGM. We use hydrodynamical cosmological zoom-in simulations of a major merger selected from the Illustris project such that the z = 0 descendant has a halo mass and stellar mass comparable to the Milky Way. To study the CGM we then re-simulated this system at a 40 times better mass resolution, and included detailed post-processing ionization modelling. Our work demonstrates the effect the merger has on the characteristic size of the CGM, its metallicity, and the predicted covering fraction of various commonly observed gas-phase species, such as H I, C IV, and O VI. We show that merger-induced outflows can increase the CGM metallicity by 0.2-0.3 dex within 0.5 Gyr post-merger. These effects last up to 6 Gyr post-merger. While the merger increases the total metal covering fractions by factors of 2-3, the covering fractions of commonly observed UV ions decrease due to the hard ionizing radiation from the active galactic nucleus, which we model explicitly. Our study of the single simulated major merger presented in this work demonstrates the significant impact that a galaxy interaction can have on the size, metallicity, and observed column densities of the CGM.
KW  - methods: numerical
KW  - galaxies: evolution
KW  - galaxies: haloes
KW  - galaxies: interactions
Y1  - 2017
U6  - https://doi.org/10.1093/mnras/stx3252
SN  - 0035-8711
SN  - 1365-2966
VL  - 475
IS  - 1
SP  - 1160
EP  - 1176
PB  - Oxford Univ. Press
CY  - Oxford
ER  - 
TY  - JOUR
A1  - Beta, Carsten
A1  - Kruse, Karsten
T1  - Intracellular oscillations and waves
JF  - Annual review of condensed matter physics
N2  - Dynamic processes in living cells are highly organized in space and time. Unraveling the underlying molecular mechanisms of spatiotemporal pattern formation remains one of the outstanding challenges at the interface between physics and biology. A fundamental recurrent pattern found in many different cell types is that of self-sustained oscillations. They are involved in a wide range of cellular functions, including second messenger signaling, gene expression, and cytoskeletal dynamics. Here, we review recent developments in the field of cellular oscillations and focus on cases where concepts from physics have been instrumental for understanding the underlying mechanisms. We consider biochemical and genetic oscillators as well as oscillations that arise from chemo-mechanical coupling. Finally, we highlight recent studies of intracellular waves that have increasingly moved into the focus of this research field.
KW  - self-sustained oscillations
KW  - biochemical oscillators
KW  - genetic networks
KW  - chemomechanical coupling
KW  - actin waves
Y1  - 2017
SN  - 978-0-8243-5008-6
U6  - https://doi.org/10.1146/annurev-conmatphys-031016-025210
SN  - 1947-5454
VL  - 8
SP  - 239
EP  - 264
PB  - Annual Reviews
CY  - Palo Alto
ER  - 
TY  - JOUR
A1  - Mardoukhi, Ahmad
A1  - Mardoukhi, Yousof
A1  - Hokka, Mikko
A1  - Kuokkala, Veli-Tapani
T1  - Effects of strain rate and surface cracks on the mechanical behaviour of Balmoral Red granite
JF  - Philosophical Transactions of the Royal Society of London, Series A : Mathematical, Physical and Engineering Sciences
N2  - This work presents a systematic study on the effects of strain rate and surface cracks on the mechanical properties and behaviour of Balmoral Red granite. The tensile behaviour of the rock was studied at low and high strain rates using Brazilian disc samples. Heat shocks were used to produce samples with different amounts of surface cracks. The surface crack patterns were analysed using optical microscopy, and the complexity of the patterns was quantified by calculating the fractal dimensions of the patterns. The strength of the rock clearly drops as a function of increasing fractal dimensions in the studied strain rate range. However, the dynamic strength of the rock drops significantly faster than the quasi-static strength, and, because of this, also the strain rate sensitivity of the rock decreases with increasing fractal dimensions. This can be explained by the fracture behaviour and fragmentation during the dynamic loading, which is more strongly affected by the heat shock than the fragmentation at low strain rates.
KW  - split Hopkinson pressure bar
KW  - rock
KW  - granite
KW  - dynamic loading
KW  - fractal dimension
KW  - surface cracks
Y1  - 2017
U6  - https://doi.org/10.1098/rsta.2016.0179
SN  - 1364-503X
SN  - 1471-2962
VL  - 375
IS  - 2085
PB  - Royal Society
CY  - London
ER  - 
TY  - JOUR
A1  - Roland, Steffen
A1  - Yan, Liang
A1  - Zhang, Qianqian
A1  - Jiao, Xuechen
A1  - Hunt, Adrian
A1  - Ghasemi, Masoud
A1  - Ade, Harald
A1  - You, Wei
A1  - Neher, Dieter
T1  - Charge Generation and Mobility-Limited Performance of Bulk Heterojunction Solar Cells with a Higher Adduct Fullerene
JF  - The journal of physical chemistry : C, Nanomaterials and interfaces
N2  - Alternative electron acceptors are being actively explored in order to advance the development of bulk-heterojunction (BHJ) organic solar cells (OSCs). The indene-C-60 bisadduct (ICBA) has been regarded as a promising candidate, as it provides high open-circuit voltage in BHJ solar cells; however, the photovoltaic performance of such ICBA-based devices is often inferior when compared to cells with the omnipresent PCBM electron acceptor. Here, by pairing the high performance polymer (FTAZ) as the donor with either PCBM or ICBA as the acceptor, we explore the physical mechanism behind the reduced performance of the ICBA-based device. Time delayed collection field (TDCF) experiments reveal reduced, yet field-independent free charge generation in the FTAZ:ICBA system, explaining the overall lower photocurrent in its cells. Through the analysis of the photoluminescence, photogeneration, and electroluminescence, we find that the lower generation efficiency is neither caused by inefficient exciton splitting, nor do we find evidence for significant energy back-transfer from the CT state to singlet excitons. In fact, the increase in open circuit voltage when replacing PCBM by ICBA is entirely caused by the increase in the CT energy, related to the shift in the LUMO energy, while changes in the radiative and nonradiative recombination losses are nearly absent. On the other hand, space charge limited current (SCLC) and bias-assisted charge extraction (BACE) measurements consistently reveal a severely lower electron mobilitiy in the FTAZ:ICBA blend. Studies of the blends with resonant soft X-ray scattering (R-SoXS), grazing incident wide-angle X-ray scattering (GIWAXS), and scanning transmission X-ray microscopy (STXM) reveal very little differences in the mesoscopic morphology but significantly less nanoscale molecular ordering of the fullerene domains in the ICBA based blends, which we propose as the main cause for the lower generation efficiency and smaller electron mobility. Calculations of the JV curves with an analytical model, using measured values, show good agreement with the experimentally determined JV characteristics, proving that these devices suffer from slow carrier extraction, resulting in significant bimolecular recombination losses. Therefore, this study highlights the importance of high charge carrier mobility for newly synthesized acceptor materials, in addition to having suitable energy levels.
Y1  - 2017
U6  - https://doi.org/10.1021/acs.jpcc.7b02288
SN  - 1932-7447
VL  - 121
SP  - 10305
EP  - 10316
PB  - American Chemical Society
CY  - Washington
ER  - 
TY  - JOUR
A1  - Ahnen, M. L.
A1  - Ansoldi, S.
A1  - Antonelli, L. A.
A1  - Antoranz, P.
A1  - Babic, A.
A1  - Banerjee, B.
A1  - Bangale, P.
A1  - de Almeida, U. Barres
A1  - Barrio, J. A.
A1  - Gonzalez, J. Becerra
A1  - Bednarek, W.
A1  - Bernardini, E.
A1  - Berti, A.
A1  - Biasuzzi, B.
A1  - Biland, A.
A1  - Blanch, O.
A1  - Bonnefoy, S.
A1  - Bonnoli, G.
A1  - Borracci, F.
A1  - Bretz, T.
A1  - Buson, S.
A1  - Carosi, A.
A1  - Chatterjee, A.
A1  - Clavero, R.
A1  - Colin, P.
A1  - Colombo, E.
A1  - Contreras, J. L.
A1  - Cortina, J.
A1  - Covino, S.
A1  - Da Vela, P.
A1  - Dazzi, F.
A1  - De Angelis, A.
A1  - De Lotto, B.
A1  - Wilhelmi, E. de Ona
A1  - Di Pierro, F.
A1  - Doert, M.
A1  - Dominguez, A.
A1  - Prester, D. Dominis
A1  - Dorner, D.
A1  - Doro, M.
A1  - Einecke, S.
A1  - Glawion, D. Eisenacher
A1  - Elsaesser, D.
A1  - Engelkemeier, M.
A1  - Ramazani, V. Fallah
A1  - Fernandez-Barral, A.
A1  - Fidalgo, D.
A1  - Fonseca, M. V.
A1  - Font, L.
A1  - Frantzen, K.
A1  - Fruck, C.
A1  - Galindo, D.
A1  - Lopez, R. J. Garcia
A1  - Garczarczyk, M.
A1  - Terrats, D. Garrido
A1  - Gaug, M.
A1  - Giammaria, P.
A1  - Godinovic, N.
A1  - Gonzalez Munoz, A.
A1  - Gora, D.
A1  - Guberman, D.
A1  - Hadasch, D.
A1  - Hahn, A.
A1  - Hanabata, Y.
A1  - Hayashida, M.
A1  - Herrera, J.
A1  - Hose, J.
A1  - Hrupec, D.
A1  - Hughes, G.
A1  - Idec, W.
A1  - Kodani, K.
A1  - Konno, Y.
A1  - Kubo, H.
A1  - Kushida, J.
A1  - La Barbera, A.
A1  - Lelas, D.
A1  - Lindfors, E.
A1  - Lombardi, S.
A1  - Longo, F.
A1  - Lopez, M.
A1  - Lopez-Coto, R.
A1  - Majumdar, P.
A1  - Makariev, M.
A1  - Mallot, K.
A1  - Maneva, G.
A1  - Manganaro, M.
A1  - Mannheim, K.
A1  - Maraschi, L.
A1  - Marcote, B.
A1  - Mariotti, M.
A1  - Martinez, M.
A1  - Mazin, D.
A1  - Menzel, U.
A1  - Miranda, J. M.
A1  - Mirzoyan, R.
A1  - Moralejo, A.
A1  - Moretti, E.
A1  - Nakajima, D.
A1  - Neustroev, V.
A1  - Niedzwiecki, A.
A1  - Rosillo, M. Nievas
A1  - Nilsson, K.
A1  - Nishijima, K.
A1  - Noda, K.
A1  - Nogues, L.
A1  - Overkemping, A.
A1  - Paiano, S.
A1  - Palacio, J.
A1  - Palatiello, M.
A1  - Paneque, D.
A1  - Paoletti, R.
A1  - Paredes, J. M.
A1  - Paredes-Fortuny, X.
A1  - Pedaletti, G.
A1  - Peresano, M.
A1  - Perri, L.
A1  - Persic, M.
A1  - Poutanen, J.
A1  - Moroni, P. G. Prada
A1  - Prandini, E.
A1  - Puljak, I.
A1  - Reichardt, I.
A1  - Rhode, W.
A1  - Ribo, M.
A1  - Rico, J.
A1  - Rodriguez Garcia, J.
A1  - Saito, T.
A1  - Satalecka, K.
A1  - Schroder, S.
A1  - Schultz, C.
A1  - Schweizer, T.
A1  - Shore, S. N.
A1  - Sillanpaa, A.
A1  - Sitarek, J.
A1  - Snidaric, I.
A1  - Sobczynska, D.
A1  - Stamerra, A.
A1  - Steinbring, T.
A1  - Strzys, M.
A1  - Suric, T.
A1  - Takalo, L.
A1  - Tavecchio, F.
A1  - Temnikov, P.
A1  - Terzic, T.
A1  - Tescaro, D.
A1  - Teshima, M.
A1  - Thaele, J.
A1  - Torres, D. F.
A1  - Toyama, T.
A1  - Treves, A.
A1  - Vanzo, G.
A1  - Verguilov, V.
A1  - Vovk, I.
A1  - Ward, J. E.
A1  - Will, M.
A1  - Wu, M. H.
A1  - Zanin, R.
A1  - Abeysekara, A. U.
A1  - Archambault, S.
A1  - Archer, A.
A1  - Benbow, W.
A1  - Bird, R.
A1  - Buchovecky, M.
A1  - Buckley, J. H.
A1  - Bugaev, V.
A1  - Connolly, M. P.
A1  - Cui, W.
A1  - Dickinson, H. J.
A1  - Falcone, A.
A1  - Feng, Q.
A1  - Finley, J. P.
A1  - Fleischhack, H.
A1  - Flinders, A.
A1  - Fortson, L.
A1  - Gillanders, G. H.
A1  - Griffin, S.
A1  - Grube, J.
A1  - Huetten, M.
A1  - Hanna, D.
A1  - Holder, J.
A1  - Humensky, T. B.
A1  - Kaaret, P.
A1  - Kar, P.
A1  - Kelley-Hoskins, N.
A1  - Kertzman, M.
A1  - Kieda, D.
A1  - Krause, M.
A1  - Krennrich, F.
A1  - Lang, M. J.
A1  - Maier, G.
A1  - McCann, A.
A1  - Moriarty, P.
A1  - Mukherjee, R.
A1  - Nieto, D.
A1  - Ong, R. A.
A1  - Otte, N.
A1  - Park, N.
A1  - Perkins, J.
A1  - Pichel, A.
A1  - Pohl, M.
A1  - Popkow, A.
A1  - Pueschel, Elisa
A1  - Quinn, J.
A1  - Ragan, K.
A1  - Reynolds, P. T.
A1  - Richards, G. T.
A1  - Roache, E.
A1  - Rovero, A. C.
A1  - Rulten, C.
A1  - Sadeh, I.
A1  - Santander, M.
A1  - Sembroski, G. H.
A1  - Shahinyan, K.
A1  - Telezhinsky, Igor O.
A1  - Tucci, J. V.
A1  - Tyler, J.
A1  - Wakely, S. P.
A1  - Weinstein, A.
A1  - Wilcox, P.
A1  - Wilhelm, Alina
A1  - Williams, D. A.
A1  - Zitzer, B.
A1  - Razzaque, S.
A1  - Villata, M.
A1  - Raiteri, C. M.
A1  - Aller, H. D.
A1  - Aller, M. F.
A1  - Larionov, V. M.
A1  - Arkharov, A. A.
A1  - Blinov, D. A.
A1  - Efimova, N. V.
A1  - Grishina, T. S.
A1  - Hagen-Thorn, V. A.
A1  - Kopatskaya, E. N.
A1  - Larionova, L. V.
A1  - Larionova, E. G.
A1  - Morozova, D. A.
A1  - Troitsky, I. S.
A1  - Ligustri, R.
A1  - Calcidese, P.
A1  - Berdyugin, A.
A1  - Kurtanidze, O. M.
A1  - Nikolashvili, M. G.
A1  - Kimeridze, G. N.
A1  - Sigua, L. A.
A1  - Kurtanidze, S. O.
A1  - Chigladze, R. A.
A1  - Chen, W. P.
A1  - Koptelova, E.
A1  - Sakamoto, T.
A1  - Sadun, A. C.
A1  - Moody, J. W.
A1  - Pace, C.
A1  - Pearson, R.
A1  - Yatsu, Y.
A1  - Mori, Y.
A1  - Carraminyana, A.
A1  - Carrasco, L.
A1  - de la Fuente, E.
A1  - Norris, J. P.
A1  - Smith, P. S.
A1  - Wehrle, A.
A1  - Gurwell, M. A.
A1  - Zook, A.
A1  - Pagani, C.
A1  - Perri, M.
A1  - Capalbi, M.
A1  - Cesarini, A.
A1  - Krimm, H. A.
A1  - Kovalev, Y. Y.
A1  - Kovalev, Yu. A.
A1  - Ros, E.
A1  - Pushkarev, A. B.
A1  - Lister, M. L.
A1  - Sokolovsky, K. V.
A1  - Kadler, M.
A1  - Piner, G.
A1  - Lahteenmaki, A.
A1  - Tornikoski, M.
A1  - Angelakis, E.
A1  - Krichbaum, T. P.
A1  - Nestoras, I.
A1  - Fuhrmann, L.
A1  - Zensus, J. A.
A1  - Cassaro, P.
A1  - Orlati, A.
A1  - Maccaferri, G.
A1  - Leto, P.
A1  - Giroletti, M.
A1  - Richards, J. L.
A1  - Max-Moerbeck, W.
A1  - Readhead, A. C. S.
T1  - Multiband variability studies and novel broadband SED modeling of Mrk 501 in 2009
JF  - Astronomy and astrophysics : an international weekly journal
N2  - Aims. We present an extensive study of the BL Lac object Mrk 501 based on a data set collected during the multi-instrument campaign spanning from 2009 March 15 to 2009 August 1, which includes, among other instruments, MAGIC, VERITAS, Whipple 10 m, and Fermi-LAT to cover the gamma-ray range from 0.1 GeV to 20 TeV; RXTE and Swift to cover wavelengths from UV to hard X-rays; and GASP-WEBT, which provides coverage of radio and optical wavelengths. Optical polarization measurements were provided for a fraction of the campaign by the Steward and St. Petersburg observatories. We evaluate the variability of the source and interband correlations, the gamma-ray flaring activity occurring in May 2009, and interpret the results within two synchrotron self-Compton (SSC) scenarios. Methods. The multiband variability observed during the full campaign is addressed in terms of the fractional variability, and the possible correlations are studied by calculating the discrete correlation function for each pair of energy bands where the significance was evaluated with dedicated Monte Carlo simulations. The space of SSC model parameters is probed following a dedicated grid-scan strategy, allowing for a wide range of models to be tested and offering a study of the degeneracy of model-to-data agreement in the individual model parameters, hence providing a less biased interpretation than the "single-curve SSC model adjustment" typically reported in the literature. Results. We find an increase in the fractional variability with energy, while no significant interband correlations of flux changes are found on the basis of the acquired data set. The SSC model grid-scan shows that the flaring activity around May 22 cannot be modeled adequately with a one-zone SSC scenario (using an electron energy distribution with two breaks), while it can be suitably described within a two (independent) zone SSC scenario. Here, one zone is responsible for the quiescent emission from the averaged 4.5-month observing period, while the other one, which is spatially separated from the first, dominates the flaring emission occurring at X-rays and very-high-energy (> 100 GeV, VHE) gamma-rays. The flaring activity from May 1, which coincides with a rotation of the electric vector polarization angle (EVPA), cannot be satisfactorily reproduced by either a one-zone or a two-independent-zone SSC model, yet this is partially affected by the lack of strictly simultaneous observations and the presence of large flux changes on sub-hour timescales (detected at VHE gamma rays). Conclusions. The higher variability in the VHE emission and lack of correlation with the X-ray emission indicate that, at least during the 4.5-month observing campaign in 2009, the highest energy (and most variable) electrons that are responsible for the VHE gamma rays do not make a dominant contribution to the similar to 1 keV emission. Alternatively, there could be a very variable component contributing to the VHE gamma-ray emission in addition to that coming from the SSC scenario. The studies with our dedicated SSC grid-scan show that there is some degeneracy in both the one-zone and the two-zone SSC scenarios probed, with several combinations of model parameters yielding a similar model-to-data agreement, and some parameters better constrained than others. The observed gamma-ray flaring activity, with the EVPA rotation coincident with the first gamma-ray flare, resembles those reported previously for low frequency peaked blazars, hence suggesting that there are many similarities in the flaring mechanisms of blazars with different jet properties.
KW  - BL Lacertae objects: individual: Markarian 501
KW  - methods: data analysis
Y1  - 2017
U6  - https://doi.org/10.1051/0004-6361/201629540
SN  - 1432-0746
VL  - 603
PB  - EDP Sciences
CY  - Les Ulis
ER  - 
TY  - JOUR
A1  - Stete, Felix
A1  - Koopman, Wouter-Willem Adriaan
A1  - Bargheer, Matias
T1  - Signatures of strong coupling on nanoparticles
BT  - revealing absorption anticrossing by tuning the dielectric environment
JF  - ACS Photonics
N2  - In the strong coupling regime, exciton and plasmon excitations are hybridized into combined system excitations. The correct identification of the coupling regime in these systems is currently debated, from both experimental and theoretical perspectives. In this article we show that the extinction spectra may show a large peak splitting, although the energy loss encoded in the absorption spectra clearly rules out the strong coupling regime. We investigate the coupling of J-aggregate excitons to the localized surface plasmon polaritons on gold nanospheres and nanorods by fine-tuning the plasmon resonance via layer-by-layer deposition of polyelectrolytes. While both structures show a characteristic anticrossing in extinction and scattering experiments, the careful assessment of the systems’ light absorption reveals that strong coupling of the plasmon to the exciton is not present in the nanosphere system. In a phenomenological model of two classical coupled oscillators, a Fano-like regime causes only the resonance of the light-driven oscillator to split up, while the other one still dissipates energy at its original frequency. Only in the strong-coupling limit do both oscillators split up the frequencies at which they dissipate energy, qualitatively explaining our experimental finding.
KW  - hybrid nanoparticles
KW  - exciton plasmon coupling
KW  - layer-by-layer deposition
KW  - strong coupling
KW  - absorption measurements
Y1  - 2017
U6  - https://doi.org/10.1021/acsphotonics.7b00113
SN  - 2330-4022
VL  - 4
SP  - 1669
EP  - 1676
PB  - American Chemical Society
CY  - Washington
ER  - 
TY  - JOUR
A1  - Benduhn, Johannes
A1  - Tvingstedt, Kristofer
A1  - Piersimoni, Fortunato
A1  - Ullbrich, Sascha
A1  - Fan, Yeli
A1  - Tropiano, Manuel
A1  - McGarry, Kathryn A.
A1  - Zeika, Olaf
A1  - Riede, Moritz K.
A1  - Douglas, Christopher J.
A1  - Barlow, Stephen
A1  - Marder, Seth R.
A1  - Neher, Dieter
A1  - Spoltore, Donato
A1  - Vandewal, Koen
T1  - Intrinsic non-radiative voltage losses in fullerene-based organic solar cells
JF  - Nature Energy
N2  - Organic solar cells demonstrate external quantum efficiencies and fill factors approaching those of conventional photovoltaic technologies. However, as compared with the optical gap of the absorber materials, their open-circuit voltage is much lower, largely due to the presence of significant non-radiative recombination. Here, we study a large data set of published and new material combinations and find that non-radiative voltage losses decrease with increasing charge-transfer-state energies. This observation is explained by considering non-radiative charge-transfer-state decay as electron transfer in the Marcus inverted regime, being facilitated by a common skeletal molecular vibrational mode. Our results suggest an intrinsic link between non-radiative voltage losses and electron-vibration coupling, indicating that these losses are unavoidable. Accordingly, the theoretical upper limit for the power conversion efficiency of single-junction organic solar cells would be reduced to about 25.5% and the optimal optical gap increases to (1.45-1.65) eV, that is, (0.2-0.3) eV higher than for technologies with minimized non-radiative voltage losses.
Y1  - 2017
U6  - https://doi.org/10.1038/nenergy.2017.53
SN  - 2058-7546
VL  - 2
PB  - Nature Publ. Group
CY  - London
ER  -