TY - JOUR A1 - Jeon, Jae-Hyung A1 - Chechkin, Aleksei V. A1 - Metzler, Ralf T1 - Scaled Brownian motion: a paradoxical process with a time dependent diffusivity for the description of anomalous diffusion JF - Physical chemistry, chemical physics : PCCP N2 - Anomalous diffusion is frequently described by scaled Brownian motion (SBM){,} a Gaussian process with a power-law time dependent diffusion coefficient. Its mean squared displacement is ?x2(t)? [similar{,} equals] 2K(t)t with K(t) [similar{,} equals] t[small alpha]-1 for 0 < [small alpha] < 2. SBM may provide a seemingly adequate description in the case of unbounded diffusion{,} for which its probability density function coincides with that of fractional Brownian motion. Here we show that free SBM is weakly non-ergodic but does not exhibit a significant amplitude scatter of the time averaged mean squared displacement. More severely{,} we demonstrate that under confinement{,} the dynamics encoded by SBM is fundamentally different from both fractional Brownian motion and continuous time random walks. SBM is highly non-stationary and cannot provide a physical description for particles in a thermalised stationary system. Our findings have direct impact on the modelling of single particle tracking experiments{,} in particular{,} under confinement inside cellular compartments or when optical tweezers tracking methods are used. KW - single-particle tracking KW - living cells KW - random-walks KW - subdiffusion KW - dynamics KW - nonergodicity KW - coefficients KW - transport KW - membrane KW - behavior Y1 - 2014 U6 - https://doi.org/10.1039/C4CP02019G VL - 30 IS - 16 SP - 15811 EP - 15817 PB - The Royal Society of Chemistry CY - Cambridge ER - TY - JOUR A1 - Metzler, Ralf A1 - Bauer, Maximilian A1 - Rasmussen, Emil S. A1 - Lomholt, Michael A. T1 - Real sequence effects on the search dynamics of transcription factors on DNA JF - Scientific Reports N2 - Recent experiments show that transcription factors (TFs) indeed use the facilitated diffusion mechanism to locate their target sequences on DNA in living bacteria cells: TFs alternate between sliding motion along DNA and relocation events through the cytoplasm. From simulations and theoretical analysis we study the TF-sliding motion for a large section of the DNA-sequence of a common E. coli strain, based on the two-state TF-model with a fast-sliding search state and a recognition state enabling target detection. For the probability to detect the target before dissociating from DNA the TF-search times self-consistently depend heavily on whether or not an auxiliary operator (an accessible sequence similar to the main operator) is present in the genome section. Importantly, within our model the extent to which the interconversion rates between search and recognition states depend on the underlying nucleotide sequence is varied. A moderate dependence maximises the capability to distinguish between the main operator and similar sequences. Moreover, these auxiliary operators serve as starting points for DNA looping with the main operator, yielding a spectrum of target detection times spanning several orders of magnitude. Auxiliary operators are shown to act as funnels facilitating target detection by TFs. KW - gene regulatory networks KW - biological physics Y1 - 2015 U6 - https://doi.org/10.1038/srep10072 SN - 2045-2322 VL - 5 IS - 10072 PB - Nature Publishing Group CY - London ER - TY - JOUR A1 - Ghosh, Surya K. A1 - Cherstvy, Andrey G. A1 - Petrov, Eugene P. A1 - Metzler, Ralf T1 - Interactions of rod-like particles on responsive elastic sheets JF - Soft matter N2 - What are the physical laws of the mutual interactions of objects bound to cell membranes, such as various membrane proteins or elongated virus particles? To rationalise this, we here investigate by extensive computer simulations mutual interactions of rod-like particles adsorbed on the surface of responsive elastic two-dimensional sheets. Specifically, we quantify sheet deformations as a response to adhesion of such filamentous particles. We demonstrate that tip-to-tip contacts of rods are favoured for relatively soft sheets, while side-by-side contacts are preferred for stiffer elastic substrates. These attractive orientation-dependent substrate-mediated interactions between the rod-like particles on responsive sheets can drive their aggregation and self-assembly. The optimal orientation of the membrane-bound rods is established via responding to the elastic energy profiles created around the particles. We unveil the phase diagramme of attractive–repulsive rod–rod interactions in the plane of their separation and mutual orientation. Applications of our results to other systems featuring membrane-associated particles are also discussed. Y1 - 2016 U6 - https://doi.org/10.1039/C6SM01522K SN - 1744-6848 SN - 1744-683X PB - RSC CY - London ER - TY - JOUR A1 - Schilde, Uwe A1 - Kelling, Alexandra A1 - Umbreen, Sumaira A1 - Linker, Torsten T1 - Crystal structures of three bicyclic carbohydrate derivatives JF - Acta crystallographica Section E ; Crystallographic communications N2 - The title compounds, [(1R,3R,4R,5R,6S)-4,5-bis(acetyloxy)-7-oxo-2-oxabicyclo- [4.2.0]octan-3-yl]methyl acetate, C14H18O8, (I), [(1S,4R,5S,6R)-5-acetyloxy-7- hydroxyimino-2-oxobicyclo[4.2.0]octan-4-yl acetate, C11H15NO6, (II), and [(3aR,5R,6R,7R,7aS)-6,7-bis(acetyloxy)-2-oxooctahydropyrano[3,2-b]pyrrol-5- yl]methyl acetate, C14H19NO8, (III), are stable bicyclic carbohydrate derivatives. They can easily be synthesized in a few steps from commercially available glycals. As a result of the ring strain from the four-membered rings in (I) and (II), the conformations of the carbohydrates deviate strongly from the ideal chair form. Compound (II) occurs in the boat form. In the five-membered lactam (III), on the other hand, the carbohydrate adopts an almost ideal chair conformation. As a result of the distortion of the sugar rings, the configurations of the three bicyclic carbohydrate derivatives could not be determined from their NMR coupling constants. From our three crystal structure determinations, we were able to establish for the first time the absolute configurations of all new stereocenters of the carbohydrate rings. KW - crystal structure KW - carbohydrate deriv­atives KW - conformation KW - configuration Y1 - 2016 U6 - https://doi.org/10.1107/S2056989016018727 SN - 2056-9890 VL - 72 IS - 12 SP - 1839 EP - 1844 PB - IUCR CY - Chester ER - TY - JOUR A1 - de Carvalho, Sidney J. A1 - Metzler, Ralf A1 - Cherstvy, Andrey G. T1 - Critical adsorption of polyelectrolytes onto planar and convex highly charged surfaces BT - the nonlinear Poisson–Boltzmann approach JF - New journal of physics : the open-access journal for physics N2 - We study the adsorption–desorption transition of polyelectrolyte chains onto planar, cylindrical and spherical surfaces with arbitrarily high surface charge densities by massive Monte Carlo computer simulations. We examine in detail how the well known scaling relations for the threshold transition—demarcating the adsorbed and desorbed domains of a polyelectrolyte near weakly charged surfaces—are altered for highly charged interfaces. In virtue of high surface potentials and large surface charge densities, the Debye–Hückel approximation is often not feasible and the nonlinear Poisson–Boltzmann approach should be implemented. At low salt conditions, for instance, the electrostatic potential from the nonlinear Poisson–Boltzmann equation is smaller than the Debye–Hückel result, such that the required critical surface charge density for polyelectrolyte adsorption σc increases. The nonlinear relation between the surface charge density and electrostatic potential leads to a sharply increasing critical surface charge density with growing ionic strength, imposing an additional limit to the critical salt concentration above which no polyelectrolyte adsorption occurs at all. We contrast our simulations findings with the known scaling results for weak critical polyelectrolyte adsorption onto oppositely charged surfaces for the three standard geometries. Finally, we discuss some applications of our results for some physical–chemical and biophysical systems. KW - polyelectrolyte adsorption KW - electrostatic interactions KW - critical phenomena KW - Debye screening Y1 - 2016 U6 - https://doi.org/10.1088/1367-2630/18/8/083037 SN - 1367-2630 VL - 18 PB - IOP Publ. CY - London ER - TY - JOUR A1 - Schmidt, Joachim A1 - Bechmann, Wolfgang T1 - Zur Anwendung des Skalarprodukts von Kraft und Weg auf reversible Prozesse (Druck-Volumen-Änderung, Dehnung, Elektrostatische Wechselwirkung, Hub) T1 - To the application of the scalar product of force and displacement to reversible processes (pressure-volume change, elongation, electrostatic interaction, raising) BT - die Verwendung äußerer oder systemimmanenter Kräfte BT - the use of external or system-immanent forces N2 - Wir schlagen einen allgemein anwendbaren Algorithmus vor, der unter Verwendung des Skalarprodukts von Kraft und Weg zum richtigen Vorzeichen in den Gleichungen für die Arbeit und die Potentielle Energie bei reversiblen Prozessen (Druck-Volumen-Änderung, Dehnung, Elektrostatische Wechselwirkung, Hub)führt. Wir zeigen, dass es dabei möglich ist, systemimmanente oder externe Kräfte zu benutzen. Wir zeigen, dass bei Verwendung von systemimmanenten Kräften das Skalarprodukt mit negativem Vorzeichen anzusetzen ist. Zudem ist es sehr wichtig, nötige Vorzeichenwechsel bei den einzelnen Schritten zu beachten. Wir betonen dies, weil gelegentlich übersehen wird, dass ein Vorzeichenwechsel nötig ist, wenn das Wegdifferential ds durch das Höhendifferential dh beziehungsweise durch das Abstandsdifferential dx oder dr ersetzt werden muss. KW - Skalarprodukt von Kraft und Weg KW - systemimmanente Kräfte KW - Druck-Volumen-Änderung KW - Dehnung KW - Elektrostatische Wechselwirkung KW - Gravitation KW - scalar product of force and displacement KW - system-immanent forces KW - pressure-volume change KW - elongation KW - electrostatic interaction KW - gravitation Y1 - 2014 U6 - http://nbn-resolving.de/urn/resolver.pl?urn:nbn:de:kobv:517-opus-69732 ER - TY - JOUR A1 - Xu, Pengbo A1 - Zhou, Tian A1 - Metzler, Ralf A1 - Deng, Weihua T1 - Lévy walk dynamics in an external harmonic potential JF - Physical review : E, Statistical, nonlinear, and soft matter physics N2 - Levy walks (LWs) are spatiotemporally coupled random-walk processes describing superdiffusive heat conduction in solids, propagation of light in disordered optical materials, motion of molecular motors in living cells, or motion of animals, humans, robots, and viruses. We here investigate a key feature of LWs-their response to an external harmonic potential. In this generic setting for confined motion we demonstrate that LWs equilibrate exponentially and may assume a bimodal stationary distribution. We also show that the stationary distribution has a horizontal slope next to a reflecting boundary placed at the origin, in contrast to correlated superdiffusive processes. Our results generalize LWs to confining forces and settle some longstanding puzzles around LWs. Y1 - 2020 U6 - https://doi.org/10.1103/PhysRevE.101.062127 SN - 2470-0045 SN - 2470-0053 SN - 1550-2376 SN - 1063-651X SN - 1539-3755 VL - 101 IS - 6 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Quade, Markus A1 - Isele, Thomas A1 - Abel, Markus T1 - Machine learning control BT - explainable and analyzable methods JF - Physica : D, Nonlinear phenomena N2 - Recently, the term explainable AI came into discussion as an approach to produce models from artificial intelligence which allow interpretation. For a long time, symbolic regression has been used to produce explainable and mathematically tractable models. In this contribution, we extend previous work on symbolic regression methods to infer the optimal control of a dynamical system given one or several optimization criteria, or cost functions. In earlier publications, network control was achieved by automated machine learning control using genetic programming. Here, we focus on the subsequent path continuation analysis of the mathematical expressions which result from the machine learning model. In particular, we use AUTO to analyze the solution properties of the controlled oscillator system which served as our model. As a result, we show that there is a considerable advantage of explainable symbolic regression models over less accessible neural networks. In particular, the roadmap of future works may be to integrate such analyses into the optimization loop itself to filter out robust solutions by construction. KW - Explainable AI KW - Machine learning control KW - Dynamical systems KW - Synchronization control KW - Genetic programming Y1 - 2020 U6 - https://doi.org/10.1016/j.physd.2020.132582 SN - 0167-2789 SN - 1872-8022 VL - 412 PB - Elsevier CY - Amsterdam ER - TY - JOUR A1 - Sangian, Danial T1 - Improving the performance of dielectric-elastomer actuators at elevated operating temperatures by means of thermal softening JF - Smart materials and structures N2 - Dielectric elastomer devices operate on the principle of Maxwell stress and their operating performance significantly rely on the elastomer and compliant electrode's electrical and mechanical properties. This paper reports that performing actuation tests at elevated temperatures resulted in an enhanced performance due to the reduction of Young's modulus and the increase of dielectric permittivity. As a result, considerably higher isometric forces and isotonic strains were achieved above the ambient operating temperature. For actuators made of silicone, polyurethane and acrylic elastomers, 166%, 70% and 266% higher isometric forces and 450%, 250% and 54% higher isotonic strains were observed, respectively, when tested at the temperature of 100 degrees C in comparison to ambient temperature values using the same operating voltages. Values of up to 0.4 J kg(-1) and 3.1 W kg(-1) were achieved for the work and power outputs per mass, respectively, on a silicone elastomer driven with a voltage of 1.5 kV at a temperature of 100 degrees C. KW - elevated-temperature effects on the operation of dielectric-elastomer KW - actuators KW - thermally enhanced actuators KW - thermal stimulation of KW - electro-electrets Y1 - 2020 U6 - https://doi.org/10.1088/1361-665X/ab6079 SN - 0964-1726 SN - 1361-665X VL - 29 IS - 2 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Perovic, Milena A1 - Qin, Qing A1 - Oschatz, Martin T1 - From molecular precursors to nanoparticles BT - tailoring the adsorption properties of porous carbon materials by controlled chemical functionalization JF - Advanced functional materials N2 - Nanoporous carbon materials (NCMs) provide the "function" of high specific surface area and thus have large interface area for interactions with surrounding species, which is of particular importance in applications related to adsorption processes. The strength and mechanism of adsorption depend on the pore architecture of the NCMs. In addition, chemical functionalization can be used to induce changes of electron density and/or electron density distribution in the pore walls, thus further modifying the interactions between carbons and guest species. Typical approaches for functionalization of nanoporous materials with regular atomic construction like porous silica, metal-organic frameworks, or zeolites, cannot be applied to NCMs due to their less defined local atomic construction and abundant defects. Therefore, synthetic strategies that offer a higher degree of control over the process of functionalization are needed. Synthetic approaches for covalent functionalization of NCMs, that is, for the incorporation of heteroatoms into the carbon backbone, are critically reviewed with a special focus on strategies following the concept "from molecules to materials." Approaches for coordinative functionalization with metallic species, and the functionalization by nanocomposite formation between pristine carbon materials and heteroatom-containing carbons, are introduced as well. Particular focus is given to the influences of these functionalizations in adsorption-related applications. KW - composites KW - heteroatoms KW - metal species KW - porous carbon materials KW - surface KW - functionalization Y1 - 2020 U6 - https://doi.org/10.1002/adfm.201908371 SN - 1616-301X SN - 1616-3028 VL - 30 IS - 41 PB - Wiley-VCH CY - Weinheim ER - TY - JOUR A1 - Fumani, F. Khastehdel A1 - Nemati, Somayyeh A1 - Mahdavifar, Saeed T1 - Quantum critical lines in the ground state phase diagram of spin-1/2 frustrated transverse-field ising chains JF - Annalen der Physik N2 - This paper focuses on the ground state phase diagram of a 1D spin-1/2 quantum Ising model with competing first and second nearest neighbour interactions known as the axial next nearest neighbour Ising model in the presence of a transverse magnetic field. Here, using quantum correlations, both numerically and analytically, some evidence is provided to clarify the identification of the ground state phase diagram. Local quantum correlations play a crucial role in detecting the critical lines either revealed or hidden by symmetry-breaking. A non-symmetry-breaking disorder transition line can be identified by the first derivative of both entanglement of formation and quantum discord between nearest neighbour spins. In addition, the quantum correlations between the second neighbour spins can also be used to reveal Kosterlitz-Thouless phase transition when their interaction strength grows and becomes closer to the first nearest neighbour one. The results obtained using the Jordan-Wigner transformation confirm the accuracy of the numerical case. KW - axial next nearest neighbour Ising chains KW - quantum correlations KW - quantum KW - phase transitions Y1 - 2020 U6 - https://doi.org/10.1002/andp.202000384 SN - 0003-3804 SN - 1521-3889 VL - 533 IS - 2 PB - Wiley-VCH CY - Weinheim ER - TY - JOUR A1 - Siddiqi, Muhammad Ali A1 - Dörr, Christian A1 - Strydis, Christos T1 - IMDfence BT - architecting a secure protocol for implantable medical devices JF - IEEE access N2 - Over the past decade, focus on the security and privacy aspects of implantable medical devices (IMDs) has intensified, driven by the multitude of cybersecurity vulnerabilities found in various existing devices. However, due to their strict computational, energy and physical constraints, conventional security protocols are not directly applicable to IMDs. Custom-tailored schemes have been proposed instead which, however, fail to cover the full spectrum of security features that modern IMDs and their ecosystems so critically require. In this paper we propose IMDfence, a security protocol for IMD ecosystems that provides a comprehensive yet practical security portfolio, which includes availability, non-repudiation, access control, entity authentication, remote monitoring and system scalability. The protocol also allows emergency access that results in the graceful degradation of offered services without compromising security and patient safety. The performance of the security protocol as well as its feasibility and impact on modern IMDs are extensively analyzed and evaluated. We find that IMDfence achieves the above security requirements at a mere less than 7% increase in total IMD energy consumption, and less than 14 ms and 9 kB increase in system delay and memory footprint, respectively. KW - protocols KW - implants KW - authentication KW - ecosystems KW - remote monitoring KW - scalability KW - authentication protocol KW - battery-depletion attack KW - battery KW - DoS KW - denial-of-service attack KW - IMD KW - implantable medical device KW - non-repudiation KW - smart card KW - zero-power defense Y1 - 2020 U6 - https://doi.org/10.1109/ACCESS.2020.3015686 SN - 2169-3536 VL - 8 SP - 147948 EP - 147964 PB - Institute of Electrical and Electronics Engineers CY - Piscataway ER - TY - JOUR A1 - Laing, Carlo R. A1 - Omel'chenko, Oleh T1 - Moving bumps in theta neuron networks JF - Chaos : an interdisciplinary journal of nonlinear science N2 - We consider large networks of theta neurons on a ring, synaptically coupled with an asymmetric kernel. Such networks support stable "bumps" of activity, which move along the ring if the coupling kernel is asymmetric. We investigate the effects of the kernel asymmetry on the existence, stability, and speed of these moving bumps using continuum equations formally describing infinite networks. Depending on the level of heterogeneity within the network, we find complex sequences of bifurcations as the amount of asymmetry is varied, in strong contrast to the behavior of a classical neural field model. Y1 - 2020 U6 - https://doi.org/10.1063/1.5143261 SN - 1054-1500 SN - 1089-7682 VL - 30 IS - 4 PB - American Institute of Physics CY - Melville ER - TY - JOUR A1 - Mardoukhi, Ahmad A1 - Mardoukhi, Yousof A1 - Hokka, Mikko A1 - Kuokkala, Veli-Tapani T1 - Effects of strain rate and surface cracks on the mechanical behaviour of Balmoral Red granite JF - Philosophical Transactions of the Royal Society of London, Series A : Mathematical, Physical and Engineering Sciences N2 - This work presents a systematic study on the effects of strain rate and surface cracks on the mechanical properties and behaviour of Balmoral Red granite. The tensile behaviour of the rock was studied at low and high strain rates using Brazilian disc samples. Heat shocks were used to produce samples with different amounts of surface cracks. The surface crack patterns were analysed using optical microscopy, and the complexity of the patterns was quantified by calculating the fractal dimensions of the patterns. The strength of the rock clearly drops as a function of increasing fractal dimensions in the studied strain rate range. However, the dynamic strength of the rock drops significantly faster than the quasi-static strength, and, because of this, also the strain rate sensitivity of the rock decreases with increasing fractal dimensions. This can be explained by the fracture behaviour and fragmentation during the dynamic loading, which is more strongly affected by the heat shock than the fragmentation at low strain rates. KW - split Hopkinson pressure bar KW - rock KW - granite KW - dynamic loading KW - fractal dimension KW - surface cracks Y1 - 2017 U6 - https://doi.org/10.1098/rsta.2016.0179 SN - 1364-503X SN - 1471-2962 VL - 375 IS - 2085 PB - Royal Society CY - London ER - TY - JOUR A1 - Ahnen, M. L. A1 - Ansoldi, S. A1 - Antonelli, L. A. A1 - Antoranz, P. A1 - Babic, A. A1 - Banerjee, B. A1 - Bangale, P. A1 - de Almeida, U. Barres A1 - Barrio, J. A. A1 - Gonzalez, J. Becerra A1 - Bednarek, W. A1 - Bernardini, E. A1 - Berti, A. A1 - Biasuzzi, B. A1 - Biland, A. A1 - Blanch, O. A1 - Bonnefoy, S. A1 - Bonnoli, G. A1 - Borracci, F. A1 - Bretz, T. A1 - Buson, S. A1 - Carosi, A. A1 - Chatterjee, A. A1 - Clavero, R. A1 - Colin, P. A1 - Colombo, E. A1 - Contreras, J. L. A1 - Cortina, J. A1 - Covino, S. A1 - Da Vela, P. A1 - Dazzi, F. A1 - De Angelis, A. A1 - De Lotto, B. A1 - Wilhelmi, E. de Ona A1 - Di Pierro, F. A1 - Doert, M. A1 - Dominguez, A. A1 - Prester, D. Dominis A1 - Dorner, D. A1 - Doro, M. A1 - Einecke, S. A1 - Glawion, D. Eisenacher A1 - Elsaesser, D. A1 - Engelkemeier, M. A1 - Ramazani, V. Fallah A1 - Fernandez-Barral, A. A1 - Fidalgo, D. A1 - Fonseca, M. V. A1 - Font, L. A1 - Frantzen, K. A1 - Fruck, C. A1 - Galindo, D. A1 - Lopez, R. J. Garcia A1 - Garczarczyk, M. A1 - Terrats, D. Garrido A1 - Gaug, M. A1 - Giammaria, P. A1 - Godinovic, N. A1 - Gonzalez Munoz, A. A1 - Gora, D. A1 - Guberman, D. A1 - Hadasch, D. A1 - Hahn, A. A1 - Hanabata, Y. A1 - Hayashida, M. A1 - Herrera, J. A1 - Hose, J. A1 - Hrupec, D. A1 - Hughes, G. A1 - Idec, W. A1 - Kodani, K. A1 - Konno, Y. A1 - Kubo, H. A1 - Kushida, J. A1 - La Barbera, A. A1 - Lelas, D. A1 - Lindfors, E. A1 - Lombardi, S. A1 - Longo, F. A1 - Lopez, M. A1 - Lopez-Coto, R. A1 - Majumdar, P. A1 - Makariev, M. A1 - Mallot, K. A1 - Maneva, G. A1 - Manganaro, M. A1 - Mannheim, K. A1 - Maraschi, L. A1 - Marcote, B. A1 - Mariotti, M. A1 - Martinez, M. A1 - Mazin, D. A1 - Menzel, U. A1 - Miranda, J. M. A1 - Mirzoyan, R. A1 - Moralejo, A. A1 - Moretti, E. A1 - Nakajima, D. A1 - Neustroev, V. A1 - Niedzwiecki, A. A1 - Rosillo, M. Nievas A1 - Nilsson, K. A1 - Nishijima, K. A1 - Noda, K. A1 - Nogues, L. A1 - Overkemping, A. A1 - Paiano, S. A1 - Palacio, J. A1 - Palatiello, M. A1 - Paneque, D. A1 - Paoletti, R. A1 - Paredes, J. M. A1 - Paredes-Fortuny, X. A1 - Pedaletti, G. A1 - Peresano, M. A1 - Perri, L. A1 - Persic, M. A1 - Poutanen, J. A1 - Moroni, P. G. Prada A1 - Prandini, E. A1 - Puljak, I. A1 - Reichardt, I. A1 - Rhode, W. A1 - Ribo, M. A1 - Rico, J. A1 - Rodriguez Garcia, J. A1 - Saito, T. A1 - Satalecka, K. A1 - Schroder, S. A1 - Schultz, C. A1 - Schweizer, T. A1 - Shore, S. N. A1 - Sillanpaa, A. A1 - Sitarek, J. A1 - Snidaric, I. A1 - Sobczynska, D. A1 - Stamerra, A. A1 - Steinbring, T. A1 - Strzys, M. A1 - Suric, T. A1 - Takalo, L. A1 - Tavecchio, F. A1 - Temnikov, P. A1 - Terzic, T. A1 - Tescaro, D. A1 - Teshima, M. A1 - Thaele, J. A1 - Torres, D. F. A1 - Toyama, T. A1 - Treves, A. A1 - Vanzo, G. A1 - Verguilov, V. A1 - Vovk, I. A1 - Ward, J. E. A1 - Will, M. A1 - Wu, M. H. A1 - Zanin, R. A1 - Abeysekara, A. U. A1 - Archambault, S. A1 - Archer, A. A1 - Benbow, W. A1 - Bird, R. A1 - Buchovecky, M. A1 - Buckley, J. H. A1 - Bugaev, V. A1 - Connolly, M. P. A1 - Cui, W. A1 - Dickinson, H. J. A1 - Falcone, A. A1 - Feng, Q. A1 - Finley, J. P. A1 - Fleischhack, H. A1 - Flinders, A. A1 - Fortson, L. A1 - Gillanders, G. H. A1 - Griffin, S. A1 - Grube, J. A1 - Huetten, M. A1 - Hanna, D. A1 - Holder, J. A1 - Humensky, T. B. A1 - Kaaret, P. A1 - Kar, P. A1 - Kelley-Hoskins, N. A1 - Kertzman, M. A1 - Kieda, D. A1 - Krause, M. A1 - Krennrich, F. A1 - Lang, M. J. A1 - Maier, G. A1 - McCann, A. A1 - Moriarty, P. A1 - Mukherjee, R. A1 - Nieto, D. A1 - Ong, R. A. A1 - Otte, N. A1 - Park, N. A1 - Perkins, J. A1 - Pichel, A. A1 - Pohl, M. A1 - Popkow, A. A1 - Pueschel, Elisa A1 - Quinn, J. A1 - Ragan, K. A1 - Reynolds, P. T. A1 - Richards, G. T. A1 - Roache, E. A1 - Rovero, A. C. A1 - Rulten, C. A1 - Sadeh, I. A1 - Santander, M. A1 - Sembroski, G. H. A1 - Shahinyan, K. A1 - Telezhinsky, Igor O. A1 - Tucci, J. V. A1 - Tyler, J. A1 - Wakely, S. P. A1 - Weinstein, A. A1 - Wilcox, P. A1 - Wilhelm, Alina A1 - Williams, D. A. A1 - Zitzer, B. A1 - Razzaque, S. A1 - Villata, M. A1 - Raiteri, C. M. A1 - Aller, H. D. A1 - Aller, M. F. A1 - Larionov, V. M. A1 - Arkharov, A. A. A1 - Blinov, D. A. A1 - Efimova, N. V. A1 - Grishina, T. S. A1 - Hagen-Thorn, V. A. A1 - Kopatskaya, E. N. A1 - Larionova, L. V. A1 - Larionova, E. G. A1 - Morozova, D. A. A1 - Troitsky, I. S. A1 - Ligustri, R. A1 - Calcidese, P. A1 - Berdyugin, A. A1 - Kurtanidze, O. M. A1 - Nikolashvili, M. G. A1 - Kimeridze, G. N. A1 - Sigua, L. A. A1 - Kurtanidze, S. O. A1 - Chigladze, R. A. A1 - Chen, W. P. A1 - Koptelova, E. A1 - Sakamoto, T. A1 - Sadun, A. C. A1 - Moody, J. W. A1 - Pace, C. A1 - Pearson, R. A1 - Yatsu, Y. A1 - Mori, Y. A1 - Carraminyana, A. A1 - Carrasco, L. A1 - de la Fuente, E. A1 - Norris, J. P. A1 - Smith, P. S. A1 - Wehrle, A. A1 - Gurwell, M. A. A1 - Zook, A. A1 - Pagani, C. A1 - Perri, M. A1 - Capalbi, M. A1 - Cesarini, A. A1 - Krimm, H. A. A1 - Kovalev, Y. Y. A1 - Kovalev, Yu. A. A1 - Ros, E. A1 - Pushkarev, A. B. A1 - Lister, M. L. A1 - Sokolovsky, K. V. A1 - Kadler, M. A1 - Piner, G. A1 - Lahteenmaki, A. A1 - Tornikoski, M. A1 - Angelakis, E. A1 - Krichbaum, T. P. A1 - Nestoras, I. A1 - Fuhrmann, L. A1 - Zensus, J. A. A1 - Cassaro, P. A1 - Orlati, A. A1 - Maccaferri, G. A1 - Leto, P. A1 - Giroletti, M. A1 - Richards, J. L. A1 - Max-Moerbeck, W. A1 - Readhead, A. C. S. T1 - Multiband variability studies and novel broadband SED modeling of Mrk 501 in 2009 JF - Astronomy and astrophysics : an international weekly journal N2 - Aims. We present an extensive study of the BL Lac object Mrk 501 based on a data set collected during the multi-instrument campaign spanning from 2009 March 15 to 2009 August 1, which includes, among other instruments, MAGIC, VERITAS, Whipple 10 m, and Fermi-LAT to cover the gamma-ray range from 0.1 GeV to 20 TeV; RXTE and Swift to cover wavelengths from UV to hard X-rays; and GASP-WEBT, which provides coverage of radio and optical wavelengths. Optical polarization measurements were provided for a fraction of the campaign by the Steward and St. Petersburg observatories. We evaluate the variability of the source and interband correlations, the gamma-ray flaring activity occurring in May 2009, and interpret the results within two synchrotron self-Compton (SSC) scenarios. Methods. The multiband variability observed during the full campaign is addressed in terms of the fractional variability, and the possible correlations are studied by calculating the discrete correlation function for each pair of energy bands where the significance was evaluated with dedicated Monte Carlo simulations. The space of SSC model parameters is probed following a dedicated grid-scan strategy, allowing for a wide range of models to be tested and offering a study of the degeneracy of model-to-data agreement in the individual model parameters, hence providing a less biased interpretation than the "single-curve SSC model adjustment" typically reported in the literature. Results. We find an increase in the fractional variability with energy, while no significant interband correlations of flux changes are found on the basis of the acquired data set. The SSC model grid-scan shows that the flaring activity around May 22 cannot be modeled adequately with a one-zone SSC scenario (using an electron energy distribution with two breaks), while it can be suitably described within a two (independent) zone SSC scenario. Here, one zone is responsible for the quiescent emission from the averaged 4.5-month observing period, while the other one, which is spatially separated from the first, dominates the flaring emission occurring at X-rays and very-high-energy (> 100 GeV, VHE) gamma-rays. The flaring activity from May 1, which coincides with a rotation of the electric vector polarization angle (EVPA), cannot be satisfactorily reproduced by either a one-zone or a two-independent-zone SSC model, yet this is partially affected by the lack of strictly simultaneous observations and the presence of large flux changes on sub-hour timescales (detected at VHE gamma rays). Conclusions. The higher variability in the VHE emission and lack of correlation with the X-ray emission indicate that, at least during the 4.5-month observing campaign in 2009, the highest energy (and most variable) electrons that are responsible for the VHE gamma rays do not make a dominant contribution to the similar to 1 keV emission. Alternatively, there could be a very variable component contributing to the VHE gamma-ray emission in addition to that coming from the SSC scenario. The studies with our dedicated SSC grid-scan show that there is some degeneracy in both the one-zone and the two-zone SSC scenarios probed, with several combinations of model parameters yielding a similar model-to-data agreement, and some parameters better constrained than others. The observed gamma-ray flaring activity, with the EVPA rotation coincident with the first gamma-ray flare, resembles those reported previously for low frequency peaked blazars, hence suggesting that there are many similarities in the flaring mechanisms of blazars with different jet properties. KW - BL Lacertae objects: individual: Markarian 501 KW - methods: data analysis Y1 - 2017 U6 - https://doi.org/10.1051/0004-6361/201629540 SN - 1432-0746 VL - 603 PB - EDP Sciences CY - Les Ulis ER - TY - JOUR A1 - Xiong, Hui A1 - Mignolet, Benoit A1 - Fang, Li A1 - Osipov, Timur A1 - Wolf, Thomas J. A. A1 - Sistrunk, Emily A1 - Gühr, Markus A1 - Remacle, Francoise A1 - Berrah, Nora T1 - The Role of Super-Atom Molecular Orbitals in Doped Fullerenes in a Femtosecond Intense Laser Field JF - Scientific reports N2 - The interaction of gas phase endohedral fullerene Ho3N@C-80 with intense (0.1-5 x 10(14) W/cm(2)), short (30 fs), 800 nm laser pulses was investigated. The power law dependence of Ho3N@C-80(q+), q = 1-2, was found to be different from that of C-60. Time-dependent density functional theory computations revealed different light-induced ionization mechanisms. Unlike in C-60, in doped fullerenes, the breaking of the cage spherical symmetry makes super atomic molecular orbital (SAMO) states optically active. Theoretical calculations suggest that the fast ionization of the SAMO states in Ho3N@C-80 is responsible for the n = 3 power law for singly charged parent molecules at intensities lower than 1.2 x 10(14) W/cm(2). Y1 - 2017 U6 - https://doi.org/10.1038/s41598-017-00124-9 SN - 2045-2322 VL - 7 PB - Nature Publ. Group CY - London ER - TY - JOUR A1 - Archambault, S. A1 - Archer, A. A1 - Benbow, W. A1 - Bird, R. A1 - Bourbeau, E. A1 - Brantseg, T. A1 - Buchovecky, M. A1 - Buckley, J. H. A1 - Bugaev, V. A1 - Byrum, K. A1 - Cerruti, M. A1 - Christiansen, J. L. A1 - Connolly, M. P. A1 - Cui, W. A1 - Daniel, M. K. A1 - Feng, Q. A1 - Finley, J. P. A1 - Fleischhack, H. A1 - Fortson, L. A1 - Furniss, A. A1 - Geringer-Sameth, A. A1 - Griffin, S. A1 - Grube, J. A1 - Hütten, M. A1 - Hakansson, N. A1 - Hanna, D. A1 - Hervet, O. A1 - Holder, J. A1 - Hughes, G. A1 - Hummensky, B. A1 - Johnson, C. A. A1 - Kaaret, P. A1 - Kar, P. A1 - Kelley-Hoskins, N. A1 - Kertzman, M. A1 - Kieda, D. A1 - Koushiappas, S. A1 - Krause, M. A1 - Krennrich, F. A1 - Lang, M. J. A1 - Lin, T. T. Y. A1 - McArthur, S. A1 - Moriarty, P. A1 - Mukherjee, R. A1 - Nieto, D. A1 - Ong, R. A. A1 - Otte, A. N. A1 - Park, N. A1 - Pohl, M. A1 - Popkow, A. A1 - Pueschel, Elisa A1 - Quinn, J. A1 - Ragan, K. A1 - Reynolds, P. T. A1 - Richards, G. T. A1 - Roache, E. A1 - Rulten, C. A1 - Sadeh, I. A1 - Santander, M. A1 - Sembroski, G. H. A1 - Shahinyan, K. A1 - Smith, A. W. A1 - Staszak, D. A1 - Telezhinsky, Igor O. A1 - Trepanier, S. A1 - Tucci, J. V. A1 - Tyler, J. A1 - Wakely, S. P. A1 - Weinstein, A. A1 - Wilcox, P. A1 - Williams, D. A. A1 - Zitzer, B. T1 - Dark matter constraints from a joint analysis of dwarf Spheroidal galaxy observations with VERITAS JF - Physical review : D, Particles, fields, gravitation, and cosmology N2 - We present constraints on the annihilation cross section of weakly interacting massive particles dark matter based on the joint statistical analysis of four dwarf galaxies with VERITAS. These results are derived from an optimized photon weighting statistical technique that improves on standard imaging atmospheric Cherenkov telescope (IACT) analyses by utilizing the spectral and spatial properties of individual photon events. We report on the results of similar to 230 hours of observations of five dwarf galaxies and the joint statistical analysis of four of the dwarf galaxies. We find no evidence of gamma-ray emission from any individual dwarf nor in the joint analysis. The derived upper limit on the dark matter annihilation cross section from the joint analysis is 1.35 x 10(-23) cm(3) s(-1) at 1 TeV for the bottom quark (b (b) over bar) final state, 2.85 x 10(-24) cm(3) s(-1) at 1 TeV for the tau lepton (tau+tau(-)) final state and 1.32 x 10-25 cm(3) s(-1) at 1 TeV for the gauge boson (gamma gamma) final state. Y1 - 2017 U6 - https://doi.org/10.1103/PhysRevD.95.082001 SN - 2470-0010 SN - 2470-0029 VL - 95 IS - 8 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Leussu, R. A1 - Usoskin, IIlya G. A1 - Valliappan, Senthamizh Pavai A1 - Diercke, Andrea A1 - Arlt, Rainer A1 - Denker, Carsten A1 - Mursula, K. T1 - Wings of the butterfly BT - sunspot groups for 1826-2015 JF - Astronomy and astrophysics : an international weekly journal N2 - The spatio-temporal evolution of sunspot activity, the so-called Maunder butterfly diagram, has been continously available since 1874 using data from the Royal Greenwich Observatory, extended by SOON network data after 1976. Here we present a new extended butterfly diagram of sunspot group occurrence since 1826, using the recently digitized data from Schwabe (1826-1867) and Sporer (1866-1880). The wings of the diagram are separated using a recently developed method based on an analysis of long gaps in sunspot group occurrence in different latitude bands. We define characteristic latitudes, corresponding to the start, end, and the largest extent of the wings (the F, L, and H latitudes). The H latitudes (30 degrees-45 degrees) are highly significantly correlated with the strength of the wings (quantified by the total sum of the monthly numbers of sunspot groups). The F latitudes (20 degrees-30 degrees) depict a weak tendency, especially in the southern hemisphere, to follow the wing strength. The L latitudes (2 degrees-10 degrees) show no clear relation to the wing strength. Overall, stronger cycle wings tend to start at higher latitudes and have a greater wing extent. A strong (5-6)-cycle periodic oscillation is found in the start and end times of the wings and in the overlap and gaps between successive wings of one hemisphere. While the average wing overlap is zero in the southern hemisphere, it is two to three months in the north. A marginally significant oscillation of about ten solar cycles is found in the asymmetry of the L latitudes. The new long database of butterfly wings provides new observational constraints to solar dynamo models that discuss the spatio-temporal distribution of sunspot occurrence over the solar cycle and longer. KW - Sun: activity KW - sunspots KW - history and philosophy of astronomy Y1 - 2017 U6 - https://doi.org/10.1051/0004-6361/201629533 SN - 1432-0746 VL - 599 PB - EDP Sciences CY - Les Ulis ER - TY - JOUR A1 - Rätzel, Dennis A1 - Wilkens, Martin A1 - Menzel, Ralf T1 - Effect of polarization entanglement in photon-photon scattering JF - Physical review : A, Atomic, molecular, and optical physics N2 - It is found that the differential cross section of photon-photon scattering is a function of the degree of polarization entanglement of the two-photon state. A reduced general expression for the differential cross section of photon-photon scattering is derived by applying simple symmetry arguments. An explicit expression is obtained for the example of photon-photon scattering due to virtual electron-positron pairs in quantum electrodynamics. It is shown how the effect in this explicit example can be explained as an effect of quantum interference and that it fits with the idea of distance-dependent forces. Y1 - 2017 U6 - https://doi.org/10.1103/PhysRevA.95.012101 SN - 2469-9926 SN - 2469-9934 VL - 95 IS - 1 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Gong, Chen Chris A1 - Klumpp, Stefan T1 - Modeling sRNA-Regulated Plasmid Maintenance JF - PLoS one N2 - We study a theoretical model for the toxin-antitoxin (hok/sok) mechanism for plasmid maintenance in bacteria. Toxin-antitoxin systems enforce the maintenance of a plasmid through post-segregational killing of cells that have lost the plasmid. Key to their function is the tight regulation of expression of a protein toxin by an sRNA antitoxin. Here, we focus on the nonlinear nature of the regulatory circuit dynamics of the toxin-antitoxin mechanism. The mechanism relies on a transient increase in protein concentration rather than on the steady state of the genetic circuit. Through a systematic analysis of the parameter dependence of this transient increase, we confirm some known design features of this system and identify new ones: for an efficient toxin-antitoxin mechanism, the synthesis rate of the toxin’s mRNA template should be lower that of the sRNA antitoxin, the mRNA template should be more stable than the sRNA antitoxin, and the mRNA-sRNA complex should be more stable than the sRNA antitoxin. Moreover, a short half-life of the protein toxin is also beneficial to the function of the toxin-antitoxin system. In addition, we study a therapeutic scenario in which a competitor mRNA is introduced to sequester the sRNA antitoxin, causing the toxic protein to be expressed. Y1 - 2017 U6 - https://doi.org/10.1371/journal.pone.0169703 SN - 1932-6203 VL - 12 PB - PLoS CY - San Fransisco ER - TY - JOUR A1 - Fandrich, Artur A1 - Buller, Jens A1 - Memczak, Henry A1 - Stoecklein, W. A1 - Hinrichs, K. A1 - Wischerhoff, E. A1 - Schulz, B. A1 - Laschewsky, André A1 - Lisdat, Fred T1 - Responsive Polymer-Electrode Interface-Study of its Thermo- and pH-Sensitivity and the Influence of Peptide Coupling JF - Electrochimica acta : the journal of the International Society of Electrochemistry (ISE) N2 - This study introduces a thermally responsive, polymer-based electrode system. The key component is a surface-attached, temperature-responsive poly(oligoethylene glycol) methacrylate (poly(OEGMA)) type polymer bearing photoreactive benzophenone and carboxy groups containing side chains. The responsive behavior of the polymer in aqueous media has been investigated by turbidimetry measurements. Polymer films are formed on gold substrates by means of the photoreactive 2(dicyclohexylphosphino)benzophenone (DPBP) through photocrosslinking. The electrochemical behavior of the resulting polymer-substrate interface has been investigated in buffered [Fe(CN)6](3-)/[Fe (CN)6](4-)solutions at room temperature and under temperature variation by cyclic voltammetry (CV). The CV experiments show that with increasing temperature structural changes of the polymer layer occur, which alter the output of the electrochemical measurement. Repeated heating/cooling cycles analyzed by CV measurements and pH changes analyzed by quartz crystal microbalance with dissipation monitoring (QCM-D) reveal the reversible nature of the restructuring process. The immobilized films are further modified by covalent coupling of two small biomolecules - a hydrophobic peptide and a more hydrophilic one. These attached components influence the hydrophobicity of the layer in a different way the resulting change of the temperature-caused behavior has been studied by CV indicating a different state of the polymer after coupling of the hydrophobic peptide. KW - Stimuli-responsive materials KW - electroanalysis KW - modified electrode KW - bioreceptors KW - peptides KW - surface modification KW - cyclic voltammetry KW - IR ellipsometry KW - quartz crystal microbalance Y1 - 2017 U6 - https://doi.org/10.1016/j.electacta.2017.01.080 SN - 0013-4686 SN - 1873-3859 VL - 229 SP - 325 EP - 333 PB - Elsevier CY - Oxford ER - TY - JOUR A1 - Zacharias, Michael A1 - Chen, Xuhui A1 - Wagner, Stefan T1 - Attenuation of TeV gamma-rays by the starlight photon field of the host galaxy JF - Monthly notices of the Royal Astronomical Society N2 - The absorption of TeV gamma-ray photons produced in relativistic jets by surrounding soft photon fields is a long-standing problem of jet physics. In some cases, the most likely emission site close to the central black hole is ruled out because of the high opacity caused by strong optical and infrared photon sources, such as the broad-line region. Mostly neglected for jet modelling is the absorption of gamma-rays in the starlight photon field of the host galaxy. Analysing the absorption for arbitrary locations and observation angles of the gamma-ray emission site within the host galaxy, we find that the distance to the galaxy centre, the observation angle, and the distribution of starlight in the galaxy are crucial for the amount of absorption. We derive the absorption value for a sample of 20 TeV-detected blazars with a redshift z(r) < 0.2. The absorption value of the gamma-ray emission located in the galaxy centre may be as high as 20 per cent, with an average value of 6 per cent. This is important in order to determine the intrinsic blazar parameters. We see no significant trends in our sample between the degree of absorption and host properties, such as starlight emissivity, galactic size, half-light radius, and redshift. While the uncertainty of the spectral properties of the extragalactic background light exceeds the effect of absorption by stellar light from the host galaxy in distant objects, the latter is a dominant effect in nearby sources. It may also be revealed in a differential comparison of sources with similar redshifts. KW - opacity KW - radiation mechanisms: non-thermal KW - galaxies: active KW - gamma-rays: galaxies Y1 - 2016 U6 - https://doi.org/10.1093/mnras/stw3032 SN - 0035-8711 SN - 1365-2966 VL - 465 IS - 3 SP - 3767 EP - 3774 PB - Oxford Univ. Press CY - Oxford ER - TY - JOUR A1 - Anielski, Alexander A1 - Barbosa Pfannes, Eva Katharina A1 - Beta, Carsten T1 - Adaptive microfluidic gradient generator for quantitative chemotaxis experiments JF - Review of scientific instruments : a monthly journal devoted to scientific instruments, apparatus, and techniques N2 - Chemotactic motion in a chemical gradient is an essential cellular function that controls many processes in the living world. For a better understanding and more detailed modelling of the underlying mechanisms of chemotaxis, quantitative investigations in controlled environments are needed. We developed a setup that allows us to separately address the dependencies of the chemotactic motion on the average background concentration and on the gradient steepness of the chemoattractant. In particular, both the background concentration and the gradient steepness can be kept constant at the position of the cell while it moves along in the gradient direction. This is achieved by generating a well-defined chemoattractant gradient using flow photolysis. In this approach, the chemoattractant is released by a light-induced reaction from a caged precursor in a microfluidic flow chamber upstream of the cell. The flow photolysis approach is combined with an automated real-time cell tracker that determines changes in the cell position and triggers movement of the microscope stage such that the cell motion is compensated and the cell remains at the same position in the gradient profile. The gradient profile can be either determined experimentally using a caged fluorescent dye or may be alternatively determined by numerical solutions of the corresponding physical model. To demonstrate the function of this adaptive microfluidic gradient generator, we compare the chemotactic motion of Dictyostelium discoideum cells in a static gradient and in a gradient that adapts to the position of the moving cell. Published by AIP Publishing. Y1 - 2017 U6 - https://doi.org/10.1063/1.4978535 SN - 0034-6748 SN - 1089-7623 VL - 88 PB - American Institute of Physics CY - Melville ER - TY - JOUR A1 - Koopman, Wouter-Willem Adriaan A1 - Natali, Marco A1 - Donati, Giovanni P. A1 - Muccini, Michele A1 - Toffanin, Stefano T1 - Charge-exciton interaction rate in organic field-effect transistors by means of transient photoluminescence electromodulated spectroscopy JF - ACS photonics N2 - Organic light-emitting transistors (OLETs) offer a huge potential for the design of highly integrated multifunctional optoelectronic systems and of intense nano scale light sources, such as the long-searched-for electrically pumped organic laser. In order to fulfill these promises, the efficiency and brightness of the current state-of-the-art devices have to be increased significantly. The dominating quenching process limiting the external quantum efficiency in OLETs is charge-exciton interaction. A comprehensive understanding of this quenching process is therefore of paramount importance. The present article reports a systematic investigation of charge-exciton interaction in organic transistors employing time resolved photoluminescence electro-modulation (PLEM) spectroscopy on the picosecond time scale. The results show that the injected charges reduce the exciton radiative recombination in two ways: (i) charges may prevent the generation of excitons and (ii) charges activate a further nonradiative channel for the exciton decay. Moreover, the transient PLEM measurements clearly reveal that not only trapped charges, as already reported in literature, but rather the entire injected charge density contributes to the quenching of the exciton population. KW - photoluminescence quenching KW - charge density KW - exciton dynamics KW - organic KW - field-effect transistor KW - light emission KW - optical spectroscopy Y1 - 2017 U6 - https://doi.org/10.1021/acsphotonics.6b00573 SN - 2330-4022 VL - 4 IS - 2 SP - 282 EP - 291 PB - American Chemical Society CY - Washington, DC ER - TY - JOUR A1 - Sun, Ning-Chen A1 - de Grijs, Richard A1 - Subramanian, Smitha A1 - Cioni, Maria-Rosa L. A1 - Rubele, Stefano A1 - Bekki, Kenji A1 - Ivanov, Valentin D. A1 - Piatti, Andrés E. A1 - Ripepi, Vincenzo T1 - The VMC Survey. XXII. Hierarchical star formation in the 30 Doradus-N158-N159-N160 star-forming complex JF - The astrophysical journal : an international review of spectroscopy and astronomical physics N2 - We study the hierarchical stellar structures in a similar to 1.5 deg(2) area covering the 30. Doradus-N158-N159-N160 starforming complex with the VISTA Survey of. Magellanic Clouds. Based on the young upper main-sequence stars, we find that the surface densities cover a wide range of values, from log(Sigma.pc(2))less than or similar to -2.0 to log(Sigma. pc(2)) greater than or similar to 0.0. Their distributions are highly non-uniform, showing groups that frequently have subgroups inside. The sizes of the stellar groups do not exhibit characteristic values, and range continuously from several parsecs to more than 100. pc; the cumulative size distribution can be well described by a single power law, with the power-law index indicating a projected fractal dimension D-2 = 1.6 +/- 0.3. We suggest that the phenomena revealed here support a scenario of hierarchical star formation. Comparisons with other star-forming regions and galaxies are also discussed. KW - galaxies: clusters: general KW - infrared: stars KW - Magellanic Clouds KW - stars: formation Y1 - 2017 U6 - https://doi.org/10.3847/1538-4357/835/2/171 SN - 0004-637X SN - 1538-4357 VL - 835 IS - 2 PB - Institute of Physics Publ. CY - Bristol ER - TY - JOUR A1 - Warren, Donald C. A1 - Ellison, Donald C. A1 - Barkov, Maxim V. A1 - Nagataki, Shigehiro T1 - Nonlinear Particle Acceleration and Thermal Particles in GRB Afterglows JF - The astrophysical journal : an international review of spectroscopy and astronomical physics N2 - The standard model for GRB afterglow emission treats the accelerated electron population as a simple power law, N(E) proportional to E-p for p greater than or similar to 2. However, in standard Fermi shock acceleration, a substantial fraction of the swept-up particles do not enter the acceleration process at all. Additionally, if acceleration is efficient, then the nonlinear back-reaction of accelerated particles on the shock structure modifies the shape of the nonthermal tail of the particle spectra. Both of these modifications to the standard synchrotron afterglow impact the luminosity, spectra, and temporal variation of the afterglow. To examine the effects of including thermal particles and nonlinear particle acceleration on afterglow emission, we follow a hydrodynamical model for an afterglow jet and simulate acceleration at numerous points during the evolution. When thermal particles are included, we find that the electron population is at no time well fitted by a single power law, though the highest-energy electrons are; if the acceleration is efficient, then the power-law region is even smaller. Our model predicts hard-soft-hard spectral evolution at X-ray energies, as well as an uncoupled X-ray and optical light curve. Additionally, we show that including emission from thermal particles has drastic effects (increases by factors of 100 and 30, respectively) on the observed flux at optical and GeV energies. This enhancement of GeV emission makes afterglow detections by future gamma-ray observatories, such as CTA, very likely. KW - acceleration of particles KW - cosmic rays KW - gamma-ray burst: general KW - shock waves KW - turbulence Y1 - 2017 U6 - https://doi.org/10.3847/1538-4357/aa56c3 SN - 0004-637X SN - 1538-4357 VL - 835 IS - 2 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Liu, Lin A1 - Cherstvy, Andrey G. A1 - Metzler, Ralf T1 - Facilitated Diffusion of Transcription Factor Proteins with Anomalous Bulk Diffusion JF - The journal of physical chemistry : B, Condensed matter, materials, surfaces, interfaces & biophysical chemistry N2 - What are the physical laws of the diffusive search of proteins for their specific binding sites on DNA in the presence of the macromolecular crowding in cells? We performed extensive computer simulations to elucidate the protein target search on DNA. The novel feature is the viscoelastic non-Brownian protein bulk diffusion recently observed experimentally. We examine the influence of the protein-DNA binding affinity and the anomalous diffusion exponent on the target search time. In all cases an optimal search time is found. The relative contribution of intermittent three-dimensional bulk diffusion and one-dimensional sliding of proteins along the DNA is quantified. Our results are discussed in the light of recent single molecule tracking experiments, aiming at a better understanding of the influence of anomalous kinetics of proteins on the facilitated diffusion mechanism. Y1 - 2017 U6 - https://doi.org/10.1021/acs.jpcb.6b12413 SN - 1520-6106 VL - 121 SP - 1284 EP - 1289 PB - American Chemical Society CY - Washington ER - TY - JOUR A1 - Almeida, Leonardo A. A1 - Sana, H. A1 - Taylor, W. A1 - Barbá, Rodolfo A1 - Bonanos, Alceste Z. A1 - Crowther, Paul A1 - Damineli, Augusto A1 - de Koter, A. A1 - de Mink, Selma E. A1 - Evans, C. J. A1 - Gieles, Mark A1 - Grin, Nathan J. A1 - Hénault-Brunet, V. A1 - Langer, Norbert A1 - Lennon, D. A1 - Lockwood, Sean A1 - Maíz Apellániz, Jesús A1 - Moffat, A. F. J. A1 - Neijssel, C. A1 - Norman, C. A1 - Ramírez-Agudelo, O. H. A1 - Richardson, N. D. A1 - Schootemeijer, Abel A1 - Shenar, Tomer A1 - Soszyński, Igor A1 - Tramper, Frank A1 - Vink, J. S. T1 - The tarantula massive binary monitoring BT - I. Observational campaign and OB-type spectroscopic binaries JF - Astronomy and astrophysics : an international weekly journal N2 - Context: Massive binaries play a crucial role in the Universe. Knowing the distributions of their orbital parameters is important for a wide range of topics from stellar feedback to binary evolution channels and from the distribution of supernova types to gravitational wave progenitors, yet no direct measurements exist outside the Milky Way. Aims: The Tarantula Massive Binary Monitoring project was designed to help fill this gap by obtaining multi-epoch radial velocity (RV) monitoring of 102 massive binaries in the 30 Doradus region. Methods: In this paper we analyze 32 FLAMES/GIRAFFE observations of 93 O- and 7 B-type binaries. We performed a Fourier analysis and obtained orbital solutions for 82 systems: 51 single-lined (SB1) and 31 double-lined (SB2) spectroscopic binaries. Results: Overall, the binary fraction and orbital properties across the 30 Doradus region are found to be similar to existing Galactic samples. This indicates that within these domains environmental effects are of second order in shaping the properties of massive binary systems. A small difference is found in the distribution of orbital periods, which is slightly flatter (in log space) in 30 Doradus than in the Galaxy, although this may be compatible within error estimates and differences in the fitting methodology. Also, orbital periods in 30 Doradus can be as short as 1.1 d, somewhat shorter than seen in Galactic samples. Equal mass binaries (q> 0.95) in 30 Doradus are all found outside NGC 2070, the central association that surrounds R136a, the very young and massive cluster at 30 Doradus’s core. Most of the differences, albeit small, are compatible with expectations from binary evolution. One outstanding exception, however, is the fact that earlier spectral types (O2–O7) tend to have shorter orbital periods than later spectral types (O9.2–O9.7). Conclusions: Our results point to a relative universality of the incidence rate of massive binaries and their orbital properties in the metallicity range from solar (Z⊙) to about half solar. This provides the first direct constraints on massive binary properties in massive star-forming galaxies at the Universe’s peak of star formation at redshifts z ~ 1 to 2 which are estimated to have Z ~ 0.5 Z⊙. KW - stars: early-type KW - stars: massive KW - binaries: spectroscopic KW - binaries: close Y1 - 2017 U6 - https://doi.org/10.1051/0004-6361/201629844 SN - 1432-0746 VL - 598 PB - EDP Sciences CY - Les Ulis ER - TY - JOUR A1 - Gorobtsov, O. Yu. A1 - Mercurio, G. A1 - Brenner, G. A1 - Lorenz, Ulf A1 - Gerasimova, N. A1 - Kurta, R. P. A1 - Hieke, F. A1 - Skopintsev, P. A1 - Zaluzhnyy, I. A1 - Lazarev, S. A1 - Dzhigaev, D. A1 - Rose, M. A1 - Singer, A. A1 - Wurth, W. A1 - Vartanyants, I. A. T1 - Statistical properties of a free-electron laser revealed by Hanbury Brown-Twiss interferometry JF - Physical review : A, Atomic, molecular, and optical physics N2 - We present a comprehensive experimental analysis of statistical properties of the self-amplified spontaneous emission free-electron laser (FEL) FLASH by means of Hanbury Brown and Twiss interferometry. The experiments were performed at FEL wavelengths of 5.5, 13.4, and 20.8 nm. We determined the second-order intensity correlation function for all wavelengths and different operation conditions of FLASH. In all experiments a high degree of spatial coherence (above 50%) was obtained. Our analysis performed in spatial and spectral domains provided us with the independent measurements of an average pulse duration of the FEL that were below 60 fs. To explain the complicated behavior of the second-order intensity correlation function we developed an advanced theoretical model that includes the presence of multiple beams and external positional jitter of the FEL pulses. By this analysis we determined that in one of the experiments external positional jitter was about 25% of the beam size. We envision that methods developed in our study will be used widely for analysis and diagnostics of FEL radiation. Y1 - 2017 U6 - https://doi.org/10.1103/PhysRevA.95.023843 SN - 2469-9926 SN - 2469-9934 VL - 95 IS - 2 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Godec, Aljaž A1 - Metzler, Ralf T1 - First passage time statistics for two-channel diffusion JF - Journal of physics : A, Mathematical and theoretical N2 - We present rigorous results for the mean first passage time and first passage time statistics for two-channel Markov additive diffusion in a 3-dimensional spherical domain. Inspired by biophysical examples we assume that the particle can only recognise the target in one of the modes, which is shown to effect a non-trivial first passage behaviour. We also address the scenario of intermittent immobilisation. In both cases we prove that despite the perfectly non-recurrent motion of two-channel Markov additive diffusion in 3 dimensions the first passage statistics at long times do not display Poisson-like behaviour if none of the phases has a vanishing diffusion coefficient. This stands in stark contrast to the standard (one-channel) Markov diffusion counterpart. We also discuss the relevance of our results in the context of cellular signalling. KW - first passage time KW - Markov additive processes KW - Fokker-Planck equation KW - random search processes KW - coupled initial boundary value problem KW - cellular signalling KW - asymptotic analysis Y1 - 2017 U6 - https://doi.org/10.1088/1751-8121/aa5204 SN - 1751-8113 SN - 1751-8121 VL - 50 IS - 8 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Goychuk, Igor T1 - Quantum ergodicity breaking in semi-classical electron transfer dynamics JF - Physical chemistry, chemical physics : a journal of European Chemical Societies N2 - Can the statistical properties of single-electron transfer events be correctly predicted within a common equilibrium ensemble description? This fundamental in nanoworld question of ergodic behavior is scrutinized within a very basic semi-classical curve-crossing problem. It is shown that in the limit of non-adiabatic electron transfer (weak tunneling) well-described by the Marcus-Levich-Dogonadze (MLD) rate the answer is yes. However, in the limit of the so-called solvent-controlled adiabatic electron transfer, a profound breaking of ergodicity occurs. Namely, a common description based on the ensemble reduced density matrix with an initial equilibrium distribution of the reaction coordinate is not able to reproduce the statistics of single-trajectory events in this seemingly classical regime. For sufficiently large activation barriers, the ensemble survival probability in a state remains nearly exponential with the inverse rate given by the sum of the adiabatic curve crossing (Kramers) time and the inverse MLD rate. In contrast, near to the adiabatic regime, the single-electron survival probability is clearly non-exponential, even though it possesses an exponential tail which agrees well with the ensemble description. Initially, it is well described by a Mittag-Leffler distribution with a fractional rate. Paradoxically, the mean transfer time in this classical on the ensemble level regime is well described by the inverse of the nonadiabatic quantum tunneling rate on a single particle level. An analytical theory is developed which perfectly agrees with stochastic simulations and explains our findings. Y1 - 2016 U6 - https://doi.org/10.1039/c6cp07206b SN - 1463-9076 SN - 1463-9084 VL - 19 SP - 3056 EP - 3066 PB - Royal Society of Chemistry CY - Cambridge ER - TY - JOUR A1 - Kunnus, Kristjan A1 - Josefsson, I. A1 - Schreck, Simon Frederik A1 - Quevedo, W. A1 - Miedema, P. S. A1 - Techert, S. A1 - de Groot, F. M. F. A1 - Föhlisch, Alexander A1 - Odelius, M. A1 - Wernet, Ph. T1 - Quantifying covalent interactions with resonant inelastic soft X-ray scattering BT - case study of Ni2+ aqua complex JF - Chemical physics letters N2 - We analyze the effects of covalent interactions in Ni 2p3d resonant inelastic X-ray scattering (RIXS) spectra from aqueous Ni2+ ions and find that the relative RIXS intensities of ligand-to-metal charge-transfer final states with respect to the ligand-field final states reflect the covalent mixing between Ni 3d and water orbitals. Specifically, the experimental intensity ratio at the Ni L-3-edge allows to determine that the Ni 3d orbitals have on average 5.5% of water character. We propose that 2p3d RIXS at the Ni L-3-edge can be utilized to quantify covalency in Ni complexes without the use of external references or simulations. KW - Transition-metal ion KW - Aqueous solution KW - Covalent interaction KW - Resonant inelastic X-ray scattering KW - Ligand-field state KW - Charge-transfer state Y1 - 2016 U6 - https://doi.org/10.1016/j.cplett.2016.12.046 SN - 0009-2614 SN - 1873-4448 VL - 669 SP - 196 EP - 201 PB - Elsevier CY - Amsterdam ER - TY - JOUR A1 - Husemann, Bernd A1 - Bielby, R. A1 - Jahnke, K. A1 - Arrigoni-Battaia, F. A1 - Worseck, Gabor A1 - Shanks, T. A1 - Wardlow, J. A1 - Scholtz, J. T1 - Cosmic dance at z similar to 3 BT - Detecting the host galaxies of the dual AGN system LBQS 0302-0019 and Jil with HAWK-I plus GRAAL JF - Astronomy and astrophysics : an international weekly journal N2 - We recently discovered that the luminous radio-quiet (QSO) LBQS 0302-0019 at z=3.286 is likely accompanied by an obscured AGN at 20 kpc projected distance, which we dubbed Jil. It represents the tightest candidate obscured/unobscured dual AGN system at z >3. To verify the dual AGN scenario we obtained deep K-s band (rest-frame V band) imaging with the VLT/HAWK-I+GRAAL instrument at 0 '.4 resolution during science verification in January 2018. Indeed, we detect the individual host galaxies of the QSO and Jil with estimated stellar masses of log(M-*/M-circle dot)=11.4 +/- 0.5 and log(M-*/M-circle dot)=10.9 +/- 0.5, respectively. Near-IR spectra obtained with VLT-KMOS reveal a clear [O-III] lambda 5007 line detection at the location of Jil which does not contribute significantly to the Ks band flux. Both observations therefore corroborate the dual AGN scenario. A comparison to Illustris cosmological simulations suggests a parent halo mass of log(M-halo/M-*)=13.2 +/- 0.5 for this interacting galaxy system, corresponding to a very massive dark matter halo at that epoch. KW - Galaxies: interactions KW - Galaxies: high-redshift KW - large-scale structure of Universe KW - instrumentation: adaptive optics KW - quasars: individual: LBQS 0302-0018 Y1 - 2018 U6 - https://doi.org/10.1051/0004-6361/201833363 SN - 1432-0746 VL - 614 PB - EDP Sciences CY - Les Ulis ER - TY - JOUR A1 - Sanchez-Ayaso, María de la Estrella A1 - del Valle, Maria Victoria A1 - Marti, Josep A1 - Romero, G. E. A1 - Luque-Escamilla, Pedro Luis T1 - Possible association of two Stellar Bowshocks with Unidentified Fermi Sources JF - The astrophysical journal : an international review of spectroscopy and astronomical physics N2 - The bowshocks of runaway stars had been theoretically proposed as gamma-ray sources. However, this hypothesis has not been confirmed by observations to date. In this paper, we present two runaway stars (lambda Cep and LS 2355) whose bowshocks are coincident with the unidentified Fermi gamma-ray sources 3FLG J2210.1+5925 and 3FGL J1128.7-6232, respectively. After performing a cross-correlation between different catalogs at distinct wavelengths, we found that these bowshocks are the most peculiar objects in the Fermi position ellipses. Then we computed the inverse Compton emission and fitted the Fermi data in order to test the viability of both runaway stars as potential counterparts of the two high-energy sources. We obtained very reasonable values for the fitted parameters of both stars. We also evaluated the possibility for the source 3FGL J1128.7-6232, which is positionally coincident with a H II region, to be the result of background cosmic-ray protons interacting with the matter of the cloud, as well as the probability of a pure chance association. We conclude that the gamma rays from these Fermi sources might be produced in the bowshocks of the considered runaway stars. In such a case, these would be the first sources of this class ever detected at gamma rays. KW - stars: winds, outflows Y1 - 2018 U6 - https://doi.org/10.3847/1538-4357/aac7c7 SN - 0004-637X SN - 1538-4357 VL - 861 IS - 1 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Kegeles, Alexander A1 - Oriti, Daniele A1 - Tomlin, Casey T1 - Inequivalent coherent state representations in group field theory JF - Classical and quantum gravit N2 - In this paper we propose an algebraic formulation of group field theory and consider non-Fock representations based on coherent states. We show that we can construct representations with an infinite number of degrees of freedom on compact manifolds. We also show that these representations break translation symmetry. Since such representations can be regarded as quantum gravitational systems with an infinite number of fundamental pre-geometric building blocks, they may be more suitable for the description of effective geometrical phases of the theory. KW - group field theory KW - quantum gravity KW - quantum field theory KW - spin foam models Y1 - 2018 U6 - https://doi.org/10.1088/1361-6382/aac39f SN - 0264-9381 SN - 1361-6382 VL - 35 IS - 12 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Quade, Markus A1 - Abel, Markus A1 - Kutz, J. Nathan A1 - Brunton, Steven L. T1 - Sparse identification of nonlinear dynamics for rapid model recovery JF - Chaos : an interdisciplinary journal of nonlinear science N2 - Big data have become a critically enabling component of emerging mathematical methods aimed at the automated discovery of dynamical systems, where first principles modeling may be intractable. However, in many engineering systems, abrupt changes must be rapidly characterized based on limited, incomplete, and noisy data. Many leading automated learning techniques rely on unrealistically large data sets, and it is unclear how to leverage prior knowledge effectively to re-identify a model after an abrupt change. In this work, we propose a conceptual framework to recover parsimonious models of a system in response to abrupt changes in the low-data limit. First, the abrupt change is detected by comparing the estimated Lyapunov time of the data with the model prediction. Next, we apply the sparse identification of nonlinear dynamics (SINDy) regression to update a previously identified model with the fewest changes, either by addition, deletion, or modification of existing model terms. We demonstrate this sparse model recovery on several examples for abrupt system change detection in periodic and chaotic dynamical systems. Our examples show that sparse updates to a previously identified model perform better with less data, have lower runtime complexity, and are less sensitive to noise than identifying an entirely new model. The proposed abrupt-SINDy architecture provides a new paradigm for the rapid and efficient recovery of a system model after abrupt changes. Y1 - 2018 U6 - https://doi.org/10.1063/1.5027470 SN - 1054-1500 SN - 1089-7682 VL - 28 IS - 6 PB - American Institute of Physics CY - Melville ER - TY - JOUR A1 - Ye, S. -Y. A1 - Kurth, William S. A1 - Hospodarsky, George B. A1 - Persoon, Ann M. A1 - Gurnett, Don A. A1 - Morooka, Michiko A1 - Wahlund, Jan-Erik A1 - Hsu, Hsiang-Wen A1 - Seiss, Martin A1 - Srama, Ralf T1 - Cassini RPWS dust observation near the Janus/Epimetheus orbit JF - Journal of geophysical research : Space physics N2 - During the Ring Grazing orbits near the end of Cassini mission, the spacecraft crossed the equatorial plane near the orbit of Janus/Epimetheus (similar to 2.5 Rs). This region is populated with dust particles that can be detected by the Radio and Plasma Wave Science (RPWS) instrument via an electric field antenna signal. Analysis of the voltage waveforms recorded on the RPWS antennas provides estimations of the density and size distribution of the dust particles. Measured RPWS profiles, fitted with Lorentzian functions, are shown to be mostly consistent with the Cosmic Dust Analyzer, the dedicated dust instrument on board Cassini. The thickness of the dusty ring varies between 600 and 1,000 km. The peak location shifts north and south within 100 km of the ring plane, likely a function of the precession phase of Janus orbit. KW - Saturn KW - dust KW - ring Y1 - 2018 U6 - https://doi.org/10.1029/2017JA025112 SN - 2169-9380 SN - 2169-9402 VL - 123 IS - 6 SP - 4952 EP - 4960 PB - American Geophysical Union CY - Washington ER - TY - JOUR A1 - Estrada, Ernesto A1 - Delvenne, Jean-Charles A1 - Hatano, Naomichi A1 - Mateos, Jose L. A1 - Metzler, Ralf A1 - Riascos, Alejandro P. A1 - Schaub, Michael T. T1 - Random multi-hopper model BT - super-fast random walks on graphs JF - Journal of Complex Networks N2 - We develop a mathematical model considering a random walker with long-range hops on arbitrary graphs. The random multi-hopper can jump to any node of the graph from an initial position, with a probability that decays as a function of the shortest-path distance between the two nodes in the graph. We consider here two decaying functions in the form of Laplace and Mellin transforms of the shortest-path distances. We prove that when the parameters of these transforms approach zero asymptotically, the hitting time in the multi-hopper approaches the minimum possible value for a normal random walker. We show by computational experiments that the multi-hopper explores a graph with clusters or skewed degree distributions more efficiently than a normal random walker. We provide computational evidences of the advantages of the random multi-hopper model with respect to the normal random walk by studying deterministic, random and real-world networks. Y1 - 2018 U6 - https://doi.org/10.1093/comnet/cnx043 SN - 2051-1310 SN - 2051-1329 VL - 6 IS - 3 SP - 382 EP - 403 PB - Oxford Univ. Press CY - Oxford ER - TY - JOUR A1 - Wetterich, Sebastian A1 - Schirrmeiste, Lutz A1 - Nazarova, Larisa B. A1 - Palagushkina, Olga A1 - Bobrov, Anatoly A1 - Pogosyan, Lilit A1 - Savelieva, Larisa A1 - Syrykh, Liudmila A1 - Matthes, Heidrun A1 - Fritz, Michael A1 - Günther, Frank A1 - Opel, Thomas A1 - Meyer, Hanno T1 - Holocene thermokarst and pingo development in the Kolyma Lowland (NE Siberia) JF - Permafrost and Periglacial Processes N2 - Ground ice and sedimentary records of a pingo exposure reveal insights into Holocene permafrost, landscape and climate dynamics. Early to mid-Holocene thermokarst lake deposits contain rich floral and faunal paleoassemblages, which indicate lake shrinkage and decreasing summer temperatures (chironomid-based T-July) from 10.5 to 3.5 cal kyr BP with the warmest period between 10.5 and 8 cal kyr BP. Talik refreezing and pingo growth started about 3.5 cal kyr BP after disappearance of the lake. The isotopic composition of the pingo ice (delta O-18 - 17.1 +/- 0.6 parts per thousand, delta D -144.5 +/- 3.4 parts per thousand, slope 5.85, deuterium excess -7.7 +/- 1.5 parts per thousand) point to the initial stage of closed-system freezing captured in the record. A differing isotopic composition within the massive ice body was found (delta O-18 - 21.3 +/- 1.4 parts per thousand, delta D -165 +/- 11.5 parts per thousand, slope 8.13, deuterium excess 4.9 +/- 3.2 parts per thousand), probably related to the infill of dilation cracks by surface water with quasi-meteoric signature. Currently inactive syngenetic ice wedges formed in the thermokarst basin after lake drainage. The pingo preserves traces of permafrost response to climate variations in terms of ground-ice degradation (thermokarst) during the early and mid-Holocene, and aggradation (wedge-ice and pingo-ice growth) during the late Holocene. KW - bioindicators KW - cryolithology KW - hydrochemistry KW - Khalerchinskaya tundra KW - stable water isotopes Y1 - 2018 U6 - https://doi.org/10.1002/ppp.1979 SN - 1045-6740 SN - 1099-1530 VL - 29 IS - 3 SP - 182 EP - 198 PB - Wiley CY - Hoboken ER - TY - JOUR A1 - Keles, Engin T1 - Spectral signature of atmospheric winds in high-resolution transit observations JF - Monthly Notices of the Royal Astronomical Society N2 - The study of exoplanet atmospheres showed large diversity compared to the planets in our Solar system. Especially Jupiter-type exoplanets orbiting their host star in close orbits, the so-called hot and ultra-hot Jupiters, have been studied in detail due to their enhanced atmospheric signature. Due to their tidally locked status, the temperature difference between the day- and nightside triggers atmospheric winds that can lead to various fingerprints in the observations. Spatially resolved absorption lines during transit such as sodium (Na) could be a good tracer for such winds. Different works resolved the Na absorption lines on different exoplanets which show different line widths. Assuming that this could be attributed to such zonal jet streams, this work models the effect of such winds on synthetic absorption lines. For this, transiting Jupiter-type planets with rotational velocities similar to hot and ultra-hot Jupiter are considered. The investigation shows that high wind velocities could reproduce the broadening of Na-line profiles inferred in different high-resolution transit observations. There is a tendency that the broadening values decrease for planets with lower equilibrium temperature. This could be explained by atmospheric drag induced by the ionization of alkali lines that slow down the zonal jet streams, favouring their existence on hot Jupiter rather than ultra-hot Jupiter. Y1 - 2021 U6 - https://doi.org/10.1093/mnras/stab099 VL - 502 IS - 1 SP - 1456 EP - 1468 PB - Oxford Univ. Press CY - Oxford ER - TY - JOUR A1 - Holzmeier, Fabian A1 - Wolf, Thomas J. A. A1 - Gienger, Christian A1 - Wagner, Isabella A1 - Bozek, J. A1 - Nandi, S. A1 - Nicolas, C. A1 - Fischer, Ingo A1 - Gühr, Markus A1 - Fink, Reinhold F. T1 - Normal and resonant Auger spectroscopy of isocyanic acid, HNCO JF - The journal of chemical physics : bridges a gap between journals of physics and journals of chemistr N2 - In this paper, we investigate HNCO by resonant and nonresonant Auger electron spectroscopy at the K-edges of carbon, nitrogen, and oxygen, employing soft X-ray synchrotron radiation. In comparison with the isosteric but linear CO2 molecule, spectra of the bent HNCO molecule are similar but more complex due to its reduced symmetry, wherein the degeneracy of the π-orbitals is lifted. Resonant Auger electron spectra are presented at different photon energies over the first core-excited 1s → 10a′ resonance. All Auger electron spectra are assigned based on ab initio configuration interaction computations combined with the one-center approximation for Auger intensities and moment theory to consider vibrational motion. The calculated spectra were scaled by a newly introduced energy scaling factor, and generally, good agreement is found between experiment and theory for normal as well as resonant Auger electron spectra. A comparison of resonant Auger spectra with nonresonant Auger structures shows a slight broadening as well as a shift of the former spectra between −8 and −9 eV due to the spectating electron. Since HNCO is a small molecule and contains the four most abundant atoms of organic molecules, the reported Auger electron decay spectra will provide a benchmark for further theoretical approaches in the computation of core electron spectra. Y1 - 2018 U6 - https://doi.org/10.1063/1.5030621 SN - 0021-9606 SN - 1089-7690 VL - 149 IS - 3 PB - American Institute of Physics CY - Melville ER - TY - JOUR A1 - Grätz, Fabio M. A1 - Seiss, Martin A1 - Spahn, Frank T1 - Formation of moon-induced gaps in dense planetary rings BT - application to the rings of saturn JF - The astrophysical journal : an international review of spectroscopy and astronomical physics N2 - We develop an axisymmetric diffusion model to describe radial density profiles in the vicinity of tiny moons embedded in planetary rings. Our diffusion model accounts for the gravitational scattering of the ring particles by an embedded moon and for the viscous diffusion of the ring matter back into the gap. With test particle simulations, we show that the scattering of the ring particles passing the moon is larger for small impact parameters than estimated by Goldreich & Tremaine and Namouni. This is significant for modeling the Keeler gap. We apply our model to the gaps of the moons Pan and Daphnis embedded in the outer A ring of Saturn with the aim to estimate the shear viscosity of the ring in the vicinity of the Encke and Keeler gap. In addition, we analyze whether tiny icy moons whose dimensions lie below Cassini's resolution capabilities would be able to explain the gap structure of the C ring and the Cassini division. KW - diffusion KW - planets and satellites: rings KW - scattering Y1 - 2018 U6 - https://doi.org/10.3847/1538-4357/aace00 SN - 0004-637X SN - 1538-4357 VL - 862 IS - 2 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - He, Yongli A1 - Huang, Jianping A1 - Li, Dongdong A1 - Xie, Yongkun A1 - Zhang, Guolong A1 - Qi, Yulei A1 - Wang, Shanshan A1 - Totz, Sonja Juliana T1 - Comparison of the effect of land-sea thermal contrast on interdecadal variations in winter and summer blockings JF - Climate dynamics : observational, theoretical and computational research on the climate system N2 - The influence of winter and summer land-sea surface thermal contrast on blocking for 1948-2013 is investigated using observations and the coupled model intercomparison project outputs. The land-sea index (LSI) is defined to measure the changes of zonal asymmetric thermal forcing under global warming. The summer LSI shows a slower increasing trend than winter during this period. For the positive of summer LSI, the EP flux convergence induced by the land-sea thermal forcing in the high latitude becomes weaker than normal, which induces positive anomaly of zonal-mean westerly and double-jet structure. Based on the quasiresonance amplification mechanism, the narrow and reduced westerly tunnel between two jet centers provides a favor environment for more frequent blocking. Composite analysis demonstrates that summer blocking shows an increasing trend of event numbers and a decreasing trend of durations. The numbers of the short-lived blocking persisting for 5-9 days significantly increases and the numbers of the long-lived blocking persisting for longer than 10 days has a weak increase than that in negative phase of summer LSI. The increasing transient wave activities induced by summer LSI is responsible for the decreasing duration of blockings. The increasing blocking due to summer LSI can further strengthen the continent warming and increase the summer LSI, which forms a positive feedback. The opposite dynamical effect of LSI on summer and winter blocking are discussed and found that the LSI-blocking negative feedback partially reduces the influence of the above positive feedback and induce the weak summer warming rate. KW - Land-sea thermal contrast KW - Blocking KW - Asymmetric warming KW - Double-jet Y1 - 2017 U6 - https://doi.org/10.1007/s00382-017-3954-9 SN - 0930-7575 SN - 1432-0894 VL - 51 IS - 4 SP - 1275 EP - 1294 PB - Springer CY - New York ER - TY - JOUR A1 - Leitner, T. A1 - Josefsson, Ida A1 - Mazza, T. A1 - Miedema, Piter S. A1 - Schröder, H. A1 - Beye, Martin A1 - Kunnus, Kristjan A1 - Schreck, S. A1 - Düsterer, Stefan A1 - Föhlisch, Alexander A1 - Meyer, M. A1 - Odelius, Michael A1 - Wernet, Philippe T1 - Time-resolved electron spectroscopy for chemical analysis of photodissociation BT - Photoelectron spectra of Fe(CO)(5), Fe(CO)(4), and Fe(CO)(3) JF - The journal of chemical physics : bridges a gap between journals of physics and journals of chemistr N2 - The prototypical photoinduced dissociation of Fe(CO)(5) in the gas phase is used to test time-resolved x-ray photoelectron spectroscopy for studying photochemical reactions. Upon one-photon excitation at 266 nm, Fe(CO)(5) successively dissociates to Fe(CO)(4) and Fe(CO)(3) along a pathway where both fragments retain the singlet multiplicity of Fe(CO)(5). The x-ray free-electron laser FLASH is used to probe the reaction intermediates Fe(CO)(4) and Fe(CO)(3) with time-resolved valence and core-level photoelectron spectroscopy, and experimental results are interpreted with ab initio quantum chemical calculations. Changes in the valence photoelectron spectra are shown to reflect changes in the valenceorbital interactions upon Fe-CO dissociation, thereby validating fundamental theoretical concepts in Fe-CO bonding. Chemical shifts of CO 3 sigma inner-valence and Fe 3 sigma core-level binding energies are shown to correlate with changes in the coordination number of the Fe center. We interpret this with coordination-dependent charge localization and core-hole screening based on calculated changes in electron densities upon core-hole creation in the final ionic states. This extends the established capabilities of steady-state electron spectroscopy for chemical analysis to time-resolved investigations. It could also serve as a benchmark for howcharge and spin density changes in molecular dissociation and excited-state dynamics are expressed in valence and core-level photoelectron spectroscopy. Published by AIP Publishing. Y1 - 2018 U6 - https://doi.org/10.1063/1.5035149 SN - 0021-9606 SN - 1089-7690 VL - 149 IS - 4 PB - American Institute of Physics CY - Melville ER - TY - JOUR A1 - Olson, R. A1 - An, Soon-Il A1 - Fan, Y. A1 - Evans, J. P. A1 - Caesar, Levke T1 - North Atlantic observations sharpen meridional overturning projections JF - Climate dynamics : observational, theoretical and computational research on the climate system N2 - Atlantic Meridional Overturning Circulation (AMOC) projections are uncertain due to both model errors, as well as internal climate variability. An AMOC slowdown projected by many climate models is likely to have considerable effects on many aspects of global and North Atlantic climate. Previous studies to make probabilistic AMOC projections have broken new ground. However, they do not drift-correct or cross-validate the projections, and do not fully account for internal variability. Furthermore, they consider a limited subset of models, and ignore the skill of models at representing the temporal North Atlantic dynamics. We improve on previous work by applying Bayesian Model Averaging to weight 13 Coupled Model Intercomparison Project phase 5 models by their skill at modeling the AMOC strength, and its temporal dynamics, as approximated by the northern North-Atlantic temperature-based AMOC Index. We make drift-corrected projections accounting for structural model errors, and for the internal variability. Cross-validation experiments give approximately correct empirical coverage probabilities, which validates our method. Our results present more evidence that AMOC likely already started slowing down. While weighting considerably moderates and sharpens our projections, our results are at low end of previously published estimates. We project mean AMOC changes between periods 1960-1999 and 2060-2099 of -4.0 Sv and -6.8 Sv for RCP4.5 and RCP8.5 emissions scenarios respectively. The corresponding average 90% credible intervals for our weighted experiments are [-7.2, -1.2] and [-10.5, -3.7] Sv respectively for the two scenarios. KW - Atlantic Meridional Overturning Circulation KW - Climate modeling KW - Bayesian Model Averaging KW - Model structural error KW - Probabilistic projections Y1 - 2017 U6 - https://doi.org/10.1007/s00382-017-3867-7 SN - 0930-7575 SN - 1432-0894 VL - 50 IS - 11-12 SP - 4171 EP - 4188 PB - Springer CY - New York ER - TY - JOUR A1 - Muzahid, S. A1 - Fonseca, G. A1 - Roberts, A. A1 - Rosenwasser, B. A1 - Richter, Philipp A1 - Narayanan, A. A1 - Churchill, C. A1 - Charlton, J. T1 - COS-Weak: probing the CGM using analogues of weak Mg II absorbers at z < 0.3 JF - Monthly notices of the Royal Astronomical Society N2 - We present a sample of 34 weak metal line absorbers at z < 0.3 selected by the simultaneous >3σ detections of the Si iiλ1260 and C iiλ1334 absorption lines, with Wr(SiII)<0.2 Å and Wr(CII)<0.3 Å, in archival HST/COS spectra. Our sample increases the number of known low-z ‘weak absorbers’ by a factor of >5. The column densities of H i and low-ionization metal lines obtained from Voigt profile fitting are used to build simple photoionization models. The inferred densities and line-of-sight thicknesses of the absorbers are in the ranges of −3.3 < log nH/cm−3 < −2.4 and ∼1 pc–50 kpc (median ≈500 pc), respectively. Most importantly, 85 per cent (50 per cent) of these absorbers show a metallicity of [Si/H]>−1.0(0.0)⁠. The fraction of systems showing near-/supersolar metallicity in our sample is significantly higher than in the H i-selected sample of Wotta et al., and the galaxy-selected sample of Prochaska et al., of absorbers probing the circum-galactic medium at similar redshift. A search for galaxies has revealed a significant galaxy-overdensity around these weak absorbers compared to random positions with a median impact parameter of 166 kpc from the nearest galaxy. Moreover, we find the presence of multiple galaxies in ≈80 per cent of the cases, suggesting group environments. The observed dN/dz of 0.8 ± 0.2 indicates that such metal-enriched, compact, dense structures are ubiquitous in the haloes of low-z group galaxies. We suggest that these are transient structures that are related to galactic outflows and/or stripping of metal-rich gas from galaxies. KW - galaxies: formation KW - galaxies: haloes KW - quasar: absorption line Y1 - 2018 U6 - https://doi.org/10.1093/mnras/sty529 SN - 0035-8711 SN - 1365-2966 VL - 476 IS - 4 SP - 4965 EP - 4986 PB - Oxford Univ. Press CY - Oxford ER - TY - JOUR A1 - Marino, Raffaella Anna A1 - Cantalupo, Sebastiano A1 - Lilly, Simon J. A1 - Gallego, Sofia G. A1 - Straka, Lorrie A. A1 - Borisova, Elena A1 - Pezzulli, Gabriele A1 - Bacon, Roland A1 - Brinchmann, Jarle A1 - Carollo, C. Marcella A1 - Caruana, Joseph A1 - Conseil, Simon A1 - Contini, Thierry A1 - Diener, Catrina A1 - Finley, Hayley A1 - Inami, Hanae A1 - Leclercq, Floriane A1 - Muzahid, Sowgat A1 - Richard, Johan A1 - Schaye, Joop A1 - Wendt, Martin A1 - Wisotzki, Lutz T1 - Dark Galaxy Candidates at Redshift similar to 3.5 Detected with MUSE JF - The astrophysical journal : an international review of spectroscopy and astronomical physics N2 - Recent theoretical models suggest that the early phase of galaxy formation could involve an epoch when galaxies are gas rich but inefficient at forming stars: a "dark galaxy" phase. Here, we report the results of our Multi-Unit Spectroscopic Explorer (MUSE) survey for dark galaxies fluorescently illuminated by quasars at z > 3. Compared to previous studies which are based on deep narrowband (NB) imaging, our integral field survey provides a nearly uniform sensitivity coverage over a large volume in redshift space around the quasars as well as full spectral information at each location. Thanks to these unique features, we are able to build control samples at large redshift distances from the quasars using the same data taken under the same conditions. By comparing the rest-frame equivalent width (EW0) distributions of the Ly alpha sources detected in proximity to the quasars and in control samples, we detect a clear correlation between the locations of high-EW0 objects and the quasars. This correlation is not seen in other properties, such as Ly alpha luminosities or volume overdensities, suggesting the possible fluorescent nature of at least some of these objects. Among these, we find six sources without continuum counterparts and EW0 limits larger than 240 angstrom that are the best candidates for dark galaxies in our survey at z > 3.5. The volume densities and properties, including inferred gas masses and star formation efficiencies, of these dark galaxy candidates are similar to those of previously detected candidates at z approximate to 2.4 in NB surveys. Moreover, if the most distant of these are fluorescently illuminated by the quasar, our results also provide a lower limit of t - 60 Myr on the quasar lifetime. KW - galaxies: formation KW - galaxies: high-redshift KW - galaxies: star formation KW - intergalactic medium KW - quasars: emission lines KW - quasars: general Y1 - 2018 U6 - https://doi.org/10.3847/1538-4357/aab6aa SN - 0004-637X SN - 1538-4357 VL - 859 IS - 1 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Totz, Sonja Juliana A1 - Löber, Jakob A1 - Totz, Jan Frederik A1 - Engel, Harald T1 - Control of transversal instabilities in reaction-diffusion systems JF - New journal of physics : the open-access journal for physics N2 - In two-dimensional reaction-diffusion systems, local curvature perturbations on traveling waves are typically damped out and vanish. However, if the inhibitor diffuses much faster than the activator, transversal instabilities can arise, leading from flat to folded, spatio-temporally modulated waves and to spreading spiral turbulence. Here, we propose a scheme to induce or inhibit these instabilities via a spatio-temporal feedback loop. In a piecewise-linear version of the FitzHugh-Nagumo model, transversal instabilities and spiral turbulence in the uncontrolled system are shown to be suppressed in the presence of control, thereby stabilizing plane wave propagation. Conversely, in numerical simulations with the modified Oregonator model for the photosensitive Belousov-Zhabotinsky reaction, which does not exhibit transversal instabilities on its own, we demonstrate the feasibility of inducing transversal instabilities and study the emerging wave patterns in a well-controlled manner. KW - traveling waves KW - control KW - transversal instabilities Y1 - 2018 U6 - https://doi.org/10.1088/1367-2630/aabce5 SN - 1367-2630 VL - 20 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Nunez Valdez, Maribel A1 - Efthimiopoulos, Ilias A1 - Taran, Michail A1 - Mueller, Jan A1 - Bykova, Elena A1 - McCammon, Catherine A1 - Koch-Müller, Monika A1 - Wilke, Max T1 - Evidence for a pressure-induced spin transition in olivine-type LiFePO4 triphylite JF - Physical review : B, Condensed matter and materials physics N2 - We present a combination of first-principles and experimental results regarding the structural and magnetic properties of olivine-type LiFePO4 under pressure. Our investigations indicate that the starting Pbnm phase of LiFePO4 persists up to 70 GPa. Further compression leads to an isostructural transition in the pressure range of 70-75 GPa, inconsistent with a former theoretical study. Considering our first-principles prediction for a high-spin to low-spin transition of Fe2+ close to 72 GPa, we attribute the experimentally observed isostructural transition to a change in the spin state of Fe2+ in LiFePO4. Compared to relevant Fe-bearing minerals, LiFePO4 exhibits the largest onset pressure for a pressure-induced spin state transition. Y1 - 2018 U6 - https://doi.org/10.1103/PhysRevB.97.184405 SN - 2469-9950 SN - 2469-9969 VL - 97 IS - 18 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Vafin, Sergei A1 - Lazar, M. A1 - Fichtner, H. A1 - Schlickeiser, R. A1 - Drillisch, M. T1 - Solar wind temperature anisotropy constraints from streaming instabilities JF - Astronomy and astrophysics : an international weekly journal N2 - Due to the relatively low rate of particle-particle collisions in the solar wind, kinetic instabilities (e.g., the mirror and firehose) play an important role in regulating large deviations from temperature isotropy. These instabilities operate in the high beta(parallel to) > 1 plasmas, and cannot explain the other limits of the temperature anisotropy reported by observations in the low beta beta(parallel to) < 1 regimes. However, the instability conditions are drastically modified in the presence of streaming (or counterstreaming) components, which are ubiquitous in space plasmas. These effects have been analyzed for the solar wind conditions in a large interval of heliospheric distances, 0.3-2.5 AU. It was found that proton counter-streams are much more crucial for plasma stability than electron ones. Moreover, new instability thresholds can potentially explain all observed bounds on the temperature anisotropy, and also the level of differential streaming in the solar wind. KW - solar wind KW - instabilities KW - waves KW - turbulence Y1 - 2018 U6 - https://doi.org/10.1051/0004-6361/201731852 SN - 1432-0746 VL - 613 PB - EDP Sciences CY - Les Ulis ER -