TY  - JOUR
A1  - Kiel, Mareike
A1  - Möhwald, Helmuth
A1  - Bargheer, Matias
T1  - Broadband measurements of the transient optical complex dielectric function of a nanoparticle/polymer composite upon ultrafast excitation
JF  - Physical review : B, Condensed matter and materials physics
N2  - We determined experimentally the complex transient optical dielectric function of a well-characterized polyelectrolyte/gold-nanoparticle composite system over a broad spectral range upon short pulse laser excitation by simultaneously measuring the time-dependent reflectance and transmittance of white light pulses with femtosecond pump-probe spectroscopy. We extracted directly the ultrafast changes in the real and imaginary parts of the effective dielectric function, epsilon(eff)(r) (omega,t)and epsilon(eff)(i) (omega,t), from the experiment. This complete experimental set of information on the time-dependent complex dielectric function challenges theories modeling the transient dielectric function of gold particles and the effective medium.
Y1  - 2011
U6  - https://doi.org/10.1103/PhysRevB.84.165121
SN  - 1098-0121
VL  - 84
IS  - 16
PB  - American Physical Society
CY  - College Park
ER  -