TY  - JOUR
A1  - Wolf, Thomas J. A.
A1  - Parrish, Robert M.
A1  - Myhre, Rolf H.
A1  - Martinez, Todd J.
A1  - Koch, Henrik
A1  - Gühr, Markus
T1  - Observation of Ultrafast Intersystem Crossing in Thymine by Extreme Ultraviolet Time-Resolved Photoelectron Spectroscopy
JF  - The journal of physical chemistry : A, Molecules, spectroscopy, kinetics, environment & general theory
N2  - We studied the photoinduced ultrafast relaxation dynamics of the nucleobase thymine using gas-phase time-resolved photoelectron spectroscopy. By employing extreme ultraviolet pulses from high harmonic generation for photoionization, we substantially extend our spectral observation window with respect to previous studies. This enables us to follow relaxation of the excited state population all the way to low-lying electronic states including the ground state. In thymine, we observe relaxation from the optically bright (1)pi pi* state of thymine to a dark (1)n pi* state within 80 +/- 30 fs. The (1)n pi* state relaxes further within 3.5 +/- 0.3 ps to a low-lying electronic state. By comparison with quantum chemical simulations, we can unambiguously assign its spectroscopic signature to the (3)pi pi* state. Hence, our study draws a comprehensive picture of the relaxation mechanism of thymine including ultrafast intersystem crossing to the triplet manifold.
Y1  - 2019
U6  - https://doi.org/10.1021/acs.jpca.9b05573
SN  - 1089-5639
SN  - 1520-5215
VL  - 123
IS  - 32
SP  - 6897
EP  - 6903
PB  - American Chemical Society
CY  - Washington
ER  - 
TY  - JOUR
A1  - Rinaldi, G.
A1  - Formisano, M.
A1  - Kappel, David
A1  - Capaccioni, F.
A1  - Bockelee-Morvan, D.
A1  - Cheng, Y-C
A1  - Vincent, J-B
A1  - Deshapriya, P.
A1  - Arnold, G.
A1  - Capria, M. T.
A1  - Ciarniello, M.
A1  - De Sanctis, M. C.
A1  - Doose, L.
A1  - Erard, S.
A1  - Federico, C.
A1  - Filacchione, G.
A1  - Fink, U.
A1  - Leyrat, C.
A1  - Longobardo, A.
A1  - Magni, G.
A1  - Mighorini, A.
A1  - Mottola, S.
A1  - Naletto, G.
A1  - Raponi, A.
A1  - Taylor, F.
A1  - Tosi, F.
A1  - Tozzi, G. P.
A1  - Salatti, M.
T1  - Analysis of night-side dust activity on comet 67P observed by VIRTIS-M
BT  - a new method to constrain the thermal inertia on the surface
JF  - Astronomy and astrophysics : an international weekly journal
N2  - On 2015 July 18, near perihelion at a heliocentric distance of 1.28 au, the Visible InfraRed Thermal Imaging Spectrometer (VIRTIS-M) on board the Rosetta spacecraft had the opportunity of observing dust activity in the inner coma with a view of the night side (shadowed side) of comet 67P/Churyumov-Gerasimenko. At the time of the measurements we present here, we observe a dust plume that originates on the far side of the nucleus. We are able to identify the approximate location of its source at the boundary between the Hapi and Anuket regions, and we find that it has been in darkness for some hours before the observation. Assuming that this time span is equal to the conductive time scale, we obtain a thermal inertia in the range 25-36 W K-1 m(-2) s(-1/2). These thermal inertia values can be used to verify with a 3D finite-element method (REM) numerical code whether the surface and subsurface temperatures agree with the values found in the literature. We explored three different configurations: (1) a layer of water ice mixed with dust beneath a dust mantle of 5 mm with thermal inertia of 36 J m(-2) K-1 S-0.5 ; (2) the same structure, but with thermal inertia of 100 J m(-2) K-1 S-0.5; (3) an ice-dust mixture that is directly exposed. Of these three configurations, the first seems to be the most reasonable, both for the low thermal inertia and for the agreement with the surface and subsurface temperatures that have been found for the comet 67P/Churyumov-Gerasimenko. The spectral properties of the plume show that the visible dust color ranged from 16 +/- 4.8%/100 nm to 13 +/- 2.6%/100 nm, indicating that this plume has no detectable color gradient. The morphology of the plume can be classified as a narrow jet that has an estimated total ejected mass of between 6 and 19 tons when we assume size distribution indices between -2.5 and -3.
KW  - comets: general
KW  - comets: individual: 67P/Churyumov-Gerasimenko
KW  - infrared: planetary systems
Y1  - 2019
U6  - https://doi.org/10.1051/0004-6361/201834907
SN  - 1432-0746
VL  - 630
PB  - EDP Sciences
CY  - Les Ulis
ER  - 
TY  - JOUR
A1  - Tubiana, C.
A1  - Rinaldi, G.
A1  - Guettler, C.
A1  - Snodgrass, C.
A1  - Shi, X.
A1  - Hu, X.
A1  - Marschall, R.
A1  - Fulle, M.
A1  - Bockeele-Morvan, D.
A1  - Naletto, G.
A1  - Capaccioni, F.
A1  - Sierks, H.
A1  - Arnold, G.
A1  - Barucci, M. A.
A1  - Bertaux, J-L
A1  - Bertini, I
A1  - Bodewits, D.
A1  - Capria, M. T.
A1  - Ciarniello, M.
A1  - Cremonese, G.
A1  - Crovisier, J.
A1  - Da Deppo, V
A1  - Debei, S.
A1  - De Cecco, M.
A1  - Deller, J.
A1  - De Sanctis, M. C.
A1  - Davidsson, B.
A1  - Doose, L.
A1  - Erard, S.
A1  - Filacchione, G.
A1  - Fink, U.
A1  - Formisano, M.
A1  - Fornasier, S.
A1  - Gutierrez, P. J.
A1  - Ip, W-H
A1  - Ivanovski, S.
A1  - Kappel, David
A1  - Keller, H. U.
A1  - Kolokolova, L.
A1  - Koschny, D.
A1  - Krueger, H.
A1  - La Forgia, F.
A1  - Lamy, P. L.
A1  - Lara, L. M.
A1  - Lazzarin, M.
A1  - Levasseur-Regourd, A. C.
A1  - Lin, Z-Y
A1  - Longobardo, A.
A1  - Lopez-Moreno, J. J.
A1  - Marzari, F.
A1  - Migliorini, A.
A1  - Mottola, S.
A1  - Rodrigo, R.
A1  - Taylor, F.
A1  - Toth, I
A1  - Zakharov, V
T1  - Diurnal variation of dust and gas production in comet 67P/Churyumov-Gerasimenko at the inbound equinox as seen by OSIRIS and VIRTIS-M on board Rosetta
JF  - Astronomy and astrophysics : an international weekly journal
N2  - Context. On 27 April 2015, when comet 67P/Churyumov-Gerasimenko was at 1.76 au from the Sun and moving toward perihelion, the OSIRIS and VIRTIS-M instruments on board the Rosetta spacecraft simultaneously observed the evolving dust and gas coma during a complete rotation of the comet. Aims. We aim to characterize the spatial distribution of dust, H2O, and CO2 gas in the inner coma. To do this, we performed a quantitative analysis of the release of dust and gas and compared the observed H2O production rate with the rate we calculated using a thermophysical model. Methods. For this study we selected OSIRIS WAC images at 612 nm (dust) and VIRTIS-M image cubes at 612 nm, 2700 nm (H2O emission band), and 4200 nm (CO2 emission band). We measured the average signal in a circular annulus to study the spatial variation around the comet, and in a sector of the annulus to study temporal variation in the sunward direction with comet rotation, both at a fixed distance of 3.1 km from the comet center. Results. The spatial correlation between dust and water, both coming from the sunlit side of the comet, shows that water is the main driver of dust activity in this time period. The spatial distribution of CO2 is not correlated with water and dust. There is no strong temporal correlation between the dust brightness and water production rate as the comet rotates. The dust brightness shows a peak at 0 degrees subsolar longitude, which is not pronounced in the water production. At the same epoch, there is also a maximum in CO2 production. An excess of measured water production with respect to the value calculated using a simple thermophysical model is observed when the head lobe and regions of the southern hemisphere with strong seasonal variations are illuminated (subsolar longitude 270 degrees-50 degrees). A drastic decrease in dust production when the water production (both measured and from the model) displays a maximum occurs when typical northern consolidated regions are illuminated and the southern hemisphere regions with strong seasonal variations are instead in shadow (subsolar longitude 50 degrees-90 degrees). Possible explanations of these observations are presented and discussed.
KW  - comets: general
KW  - comets: individual: 67P/Churyumov-Gerasimenko
KW  - methods: data analysis
Y1  - 2019
U6  - https://doi.org/10.1051/0004-6361/201834869
SN  - 1432-0746
VL  - 630
PB  - EDP Sciences
CY  - Les Ulis
ER  - 
TY  - JOUR
A1  - Baran, Andrzej S.
A1  - Telting, J. H.
A1  - Jeffery, C. Simon
A1  - Ostensen, R. H.
A1  - Vos, Joris
A1  - Reed, M. D.
A1  - Vŭcković, Maja
T1  - K2 observations of the sdBV plus dM/bd binaries PHL457 and EQPsc
JF  - Monthly notices of the Royal Astronomical Society
N2  - We present an analysis of two pulsating subdwarf B stars PHL 457 and EQ Psc observed during the K2 mission. The K2 light curves of both stars show variation consistent with irradiation of a cooler companion by the hot subdwarf. They also show higher frequency oscillations consistent with pulsation. Using new spectroscopic data, we measured the radial velocity, effective temperature, surface gravity, and helium abundance of both hot subdwarfs as a function of orbital phase. We confirm the previously published spectroscopic orbit of PHL 457, and present the first spectroscopic orbit of EQ Psc. The orbital periods are 0.313 and 0.801 d, respectively. For EQPsc, we find a strong correlation between T-eff and orbital phase, due to contribution of light from the irradiated companion. We calculated amplitude spectra, identified significant pulsation frequencies, and searched for multiplets and asymptotic period spacings. By means of multiplets and period spacing, we identified the degrees of several pulsation modes in each star. The g-mode multiplets indicate subsynchronous core rotation with periods of 4.6 d (PHL 457) and 9.4 d (EQ Psc). We made spectral energy disctribution (SED) fits of PHL 457 and EQ Psc using available broad-band photometry and Gaia data. While the SED of PHL 457 shows no evidence of a cool companion, the SED for EQPsc clearly shows an infrared (IR) access consistent with a secondary with a temperature of about 6800K and a radius of 0.23 R-circle dot. This is the first detection of an IR access in any sdB + dM binary.
KW  - binaries: general
KW  - stars: individual (PHL 457, EQ Psc)
KW  - stars: oscillations (including pulsations)
Y1  - 2019
U6  - https://doi.org/10.1093/mnras/stz2209
SN  - 0035-8711
SN  - 1365-2966
VL  - 489
IS  - 2
SP  - 1556
EP  - 1571
PB  - Oxford Univ. Press
CY  - Oxford
ER  - 
TY  - GEN
A1  - Lazarian, Alexander
A1  - Yan, Huirong
T1  - Erratum: Superdiffusion of Cosmic Rays: Implications for Cosmic Ray Acceleration (The American Astronomical Society. - Vol. 784, (2014), 38)
T2  - The astrophysical journal : an international review of spectroscopy and astronomical physics
N2  - Diffusion of cosmic rays (CRs) is the key process for understanding their propagation and acceleration. We employ the description of spatial separation of magnetic field lines in magnetohydrodynamic turbulence in Lazarian & Vishniac to quantify the divergence of the magnetic field on scales less than the injection scale of turbulence and show that this divergence induces superdiffusion of CR in the direction perpendicular to the mean magnetic field. The perpendicular displacement squared increases, not as the distance x along the magnetic field, which is the case for a regular diffusion, but as the x 3 for freely streaming CRs. The dependence changes to x 3/2 for the CRs propagating diffusively along the magnetic field. In the latter case, we show that it is important to distinguish the perpendicular displacement with respect to the mean field and to the local magnetic field. We consider how superdiffusion changes the acceleration of CRs in shocks and show how it decreases efficiency of the CRs acceleration in perpendicular shocks. We also demonstrate that in the case when the small-scale magnetic field is generated in the pre-shock region, an efficient acceleration can take place for the CRs streaming without collisions along the magnetic loops.
Y1  - 2019
U6  - https://doi.org/10.3847/1538-4357/ab50ba
SN  - 0004-637X
SN  - 1538-4357
VL  - 885
IS  - 2
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Eliazar, Iddo
A1  - Metzler, Ralf
A1  - Reuveni, Shlomi
T1  - Poisson-process limit laws yield Gumbel max-min and min-max
JF  - Physical review : E, Statistical, nonlinear and soft matter physics
N2  - “A chain is only as strong as its weakest link” says the proverb. But what about a collection of statistically identical chains: How long till all chains fail? The answer to this question is given by the max-min of a matrix whose (i,j)entry is the failure time of link j of chain i: take the minimum of each row, and then the maximum of the rows' minima. The corresponding min-max is obtained by taking the maximum of each column, and then the minimum of the columns' maxima. The min-max applies to the storage of critical data. Indeed, consider multiple backup copies of a set of critical data items, and consider the (i,j) matrix entry to be the time at which item j on copy i is lost; then, the min-max is the time at which the first critical data item is lost. In this paper we address random matrices whose entries are independent and identically distributed random variables. We establish Poisson-process limit laws for the row's minima and for the columns' maxima. Then, we further establish Gumbel limit laws for the max-min and for the min-max. The limit laws hold whenever the entries' distribution has a density, and yield highly applicable approximation tools and design tools for the max-min and min-max of large random matrices. A brief of the results presented herein is given in: Gumbel central limit theorem for max-min and min-max
Y1  - 2019
U6  - https://doi.org/10.1103/PhysRevE.100.022129
SN  - 2470-0045
SN  - 2470-0053
VL  - 100
IS  - 2
PB  - American Physical Society
CY  - College Park
ER  - 
TY  - JOUR
A1  - Eliazar, Iddo
A1  - Metzler, Ralf
A1  - Reuveni, Shlomi
T1  - Gumbel central limit theorem for max-min and min-max
JF  - Physical review : E, Statistical, nonlinear and soft matter physics
N2  - The max-min and min-max of matrices arise prevalently in science and engineering. However, in many real-world situations the computation of the max-min and min-max is challenging as matrices are large and full information about their entries is lacking. Here we take a statistical-physics approach and establish limit laws—akin to the central limit theorem—for the max-min and min-max of large random matrices. The limit laws intertwine random-matrix theory and extreme-value theory, couple the matrix dimensions geometrically, and assert that Gumbel statistics emerge irrespective of the matrix entries' distribution. Due to their generality and universality, as well as their practicality, these results are expected to have a host of applications in the physical sciences and beyond.
Y1  - 2019
U6  - https://doi.org/10.1103/PhysRevE.100.020104
SN  - 2470-0045
SN  - 2470-0053
VL  - 100
IS  - 2
PB  - American Physical Society
CY  - College Park
ER  - 
TY  - JOUR
A1  - Soupiona, Ourania
A1  - Samaras, Stefanos
A1  - Ortiz-Amezcua, Pablo
A1  - Böckmann, Christine
A1  - Papayannis, Alexandros D.
A1  - Moreira, Gregori De Arruda
A1  - Benavent-Oltra, Jose Antonio
A1  - Guerrero-Rascado, Juan Luis
A1  - Bedoya-Velásquez, Andres Esteban
A1  - Olmo-Reyes, Francisco José
A1  - Román, Roberto
A1  - Kokkalis, Panagiotis
A1  - Mylonaki, Maria
A1  - Alados-Arboledas, Lucas
A1  - Papanikolaou, Christina Anna
A1  - Foskinis, Romanos
T1  - Retrieval of optical and microphysical properties of transported Saharan dust over Athens and Granada based on multi-wavelength Raman lidar measurements: Study of the mixing processes
JF  - Atmospheric environment : air pollution ; emissions, transport and dispersion, transformation, deposition effects, micrometeorology, urban atmosphere, global atmosphere
N2  - In this paper we extract the aerosol microphysical properties for a collection of mineral dust cases measured by multi-wavelength depolarization Raman lidar systems located at the National Technical University of Athens (NTUA, Athens, Greece) and the Andalusian Institute for Earth System Research (IISTA-CEAMA, Granada, Spain). The lidar-based retrievals were carried out with the Spheroidal Inversion eXperiments software tool (SphInX) developed at the University of Potsdam (Germany). The software uses regularized inversion of a two-dimensional enhancement of the Mie model based on the spheroid-particle approximation with the aspect ratio determining the particle shape. The selection of the cases was based on the transport time from the source regions to the measuring sites. The aerosol optical depth as measured by AERONET ranged from 0.27 to 0.54 (at 500 nm) depending on the intensity of each event. Our analysis showed the hourly mean particle linear depolarization ratio and particle lidar ratio values at 532 nm ranging from 11 to 34% and from 42 to 79 sr respectively, depending on the mixing status, the corresponding air mass pathways and their transport time. Cases with shorter transport time showed good agreement in terms of the optical and SphInX-retrieved microphysical properties between Athens and Granada providing a complex refractive index value equal to 1.4 + 0.004i. On the other hand, the results for cases with higher transport time deviated from the aforementioned ones as well as from each other, providing, in particular, an imaginary part of the refractive index ranging from 0.002 to 0.005. Reconstructions of two-dimensional shape-size distributions for each selected layer showed that the dominant effective particle shape was prolate with diverse spherical contributions. The retrieved volume concentrations reflect overall the intensity of the episodes.
Y1  - 2019
U6  - https://doi.org/10.1016/j.atmosenv.2019.116824
SN  - 1352-2310
SN  - 1873-2844
VL  - 214
PB  - Elsevier
CY  - Oxford
ER  - 
TY  - JOUR
A1  - Pittarello, Lidia
A1  - Goderis, Steven
A1  - Soens, Bastien
A1  - McKibbin, Seann J.
A1  - Giuli, Gabriele
A1  - Bariselli, Federico
A1  - Dias, Bruno
A1  - Helber, Bernd
A1  - Lepore, Giovanni Orazio
A1  - Vanhaecke, Frank
A1  - Köberl, Christian
A1  - Magin, Thierry E.
A1  - Claeys, Philippe
T1  - Meteoroid atmospheric entry investigated with plasma flow experiments: Petrography and geochemistry of the recovered material
JF  - Icarus : international journal of solar system studies
N2  - Melting experiments attempting to reproduce some of the processes affecting asteroidal and cometary material during atmospheric entry have been performed in a high enthalpy facility. For the first time with the specific experimental setup, the resulting material has been recovered, studied, and compared with natural analogues, focusing on the thermal and redox reactions triggered by interaction between the melt and the atmospheric gases under high temperature and low pressure conditions. Experimental conditions were tested across a range of parameters, such as heat flux, experiment duration, and pressure, using two types of sample holders materials, namely cork and graphite. A basalt served as asteroidal analog and to calibrate the experiments, before melting a H5 ordinary chondrite meteorite. The quenched melt recovered after the experiments has been analyzed by mu-XRF, EDS-SEM, EMPA, LA-ICP-MS, and XANES spectroscopy. The glass formed from the basalt is fairly homogeneous, depleted in highly volatile elements (e.g., Na, K), relatively enriched in moderately siderophile elements (e.g., Co, Ni), and has reached an equilibrium redox state with a lower Fe3+/Fe-tot ratio than that in the starting material. Spherical objects, enriched in SiO2, Na2O and K2O, were observed, inferring condensation from the vaporized material. Despite instantaneous quenching, the melt formed from the ordinary chondrite shows extensive crystallization of mostly olivine and magnetite, the latter indicative of oxygen fugacity compatible with presence of both Fe2+ and Fe3+. Similar features have been observed in natural meteorite fusion crusts and in micrometeorites, implying that, at least in terms of maximum temperature reached and chemical reactions, the experiments have successfully reproduced the conditions likely encountered by extraterrestrial material following atmospheric entry.
KW  - Melting experiments
KW  - Atmospheric entry
KW  - Meteorites
KW  - Fusion crust
KW  - Redox
Y1  - 2019
U6  - https://doi.org/10.1016/j.icarus.2019.04.033
SN  - 0019-1035
SN  - 1090-2643
VL  - 331
SP  - 170
EP  - 178
PB  - Elsevier
CY  - San Diego
ER  - 
TY  - JOUR
A1  - Poeschel, Thorsten
A1  - Brilliantov, Nikolai V.
A1  - Formella, Arno
T1  - Impact of high-energy tails on granular gas properties
JF  - Physical review : E, Statistical, nonlinear and soft matter physics
N2  - The velocity distribution function of granular gases in the homogeneous cooling state as well as some heated granular gases decays for large velocities as f proportional to exp(-const x nu). That is, its high-energy tail is overpopulated as compared with the Maxwell distribution. At the present time, there is no theory to describe the influence of the tail on the kinetic characteristics of granular gases. We develop an approach to quantify the overpopulated tail and analyze its impact on granular gas properties, in particular on the cooling coefficient. We observe and explain anomalously slow relaxation of the velocity distribution function to its steady state.
Y1  - 2006
U6  - https://doi.org/10.1103/PhysRevE.74.041302
SN  - 1539-3755
SN  - 1550-2376
VL  - 74
IS  - 4
PB  - The American Physical Society
CY  - College Park
ER  -