TY - JOUR A1 - Siegmund, Nicole A1 - Panebianco, Juan E. A1 - Avecilla, Fernando A1 - Iturri, Laura Antonela A1 - Sommer, Michael A1 - Buschiazzo, Daniel A1 - Funk, Roger T1 - From gustiness to dustiness BT - the impact of wind gusts on particulate matter emissions in field experiments in La Pampa, Argentina JF - Atmosphere N2 - This study delivers the first empirical data-driven analysis of the impact of turbulence induced gustiness on the fine dust emissions from a measuring field. For quantification of the gust impact, a new measure, the Gust uptake Efficiency (GuE) is introduced. GuE provides a percentage of over- or under-proportional dust uptake due to gust activity during a wind event. For the three analyzed wind events, GuE values of up to 150% could be found, yet they significantly differed per particle size class with a tendency for lower values for smaller particles. In addition, a high-resolution correlation analysis among 31 particle size classes and wind speed was conducted; it revealed strong negative correlation coefficients for very small particles and positive correlations for bigger particles, where 5 mu m appears to be an empirical threshold dividing both directions. We conclude with a number of suggestions for further investigations: an optimized field experiment setup, a new particle size ratio (PM1/PM0.5 in addition to PM10/PM2.5), as well as a comprehensive data-driven search for an optimal wind gust definition in terms of soil erosivity. KW - wind gusts KW - wind erosion KW - particle uptake KW - dust plumes Y1 - 2022 U6 - https://doi.org/10.3390/atmos13081173 SN - 2073-4433 VL - 13 IS - 8 PB - MDPI CY - Basel ER - TY - JOUR A1 - Funk, Roger A1 - Busse, Jaqueline A1 - Siegmund, Nicole A1 - Sommer, Michael A1 - Iturri, Laura Antonela A1 - Panebianco, Juan E. A1 - Avecilla, Fernando A1 - Buschiazzo, Daniel T1 - Phytoliths in particulate matter released by wind erosion on arable land in La Pampa, Argentina JF - Frontiers in environmental science N2 - Silicon (Si) is considered a beneficial element in plant nutrition, but its importance on ecosystems goes far beyond that. Various forms of silicon are found in soils, of which the phytogenic pool plays a decisive role due to its good availability. This Si returns to the soil through the decomposition of plant residues, where they then participate in the further cycle as biogenic amorphous silica (bASi) or so-called phytoliths. These have a high affinity for water, so that the water holding capacity and water availability of soils can be increased even by small amounts of ASi. Agricultural land is a considerable global dust source, and dust samples from arable land have shown in cloud formation experiments a several times higher ice nucleation activity than pure mineral dust. Here, particle sizes in the particulate matter fractions (PM) are important, which can travel long distances and reach high altitudes in the atmosphere. Based on this, the research question was whether phytoliths could be detected in PM samples from wind erosion events, what are the main particle sizes of phytoliths and whether an initial quantification was possible.Measurements of PM concentrations were carried out at a wind erosion measuring field in the province La Pampa, Argentina. PM were sampled during five erosion events with Environmental Dust Monitors (EDM). After counting and classifying all particles with diameters between 0.3 and 32 mu m in the EDMs, they are collected on filters. The filters were analyzed by Scanning Electron Microscopy and Energy Dispersive X-Ray analysis (SEM-EDX) to investigate single or ensembles of particles regarding composition and possible origins.The analyses showed up to 8.3 per cent being phytoliths in the emitted dust and up to 25 per cent of organic origin. Particles of organic origin are mostly in the coarse dust fraction, whereas phytoliths are predominately transported in the finer dust fractions. Since phytoliths are both an important source of Si as a plant nutrient and are also involved in soil C fixation, their losses from arable land via dust emissions should be considered and its specific influence on atmospheric processes should be studied in detail in the future. KW - dust KW - dust composition KW - particulate matter KW - scanning electron microscope KW - (SEM) analysis KW - phytolith Y1 - 2022 U6 - https://doi.org/10.3389/fenvs.2022.969898 SN - 2296-665X VL - 10 PB - Frontiers Media CY - Lausanne ER -