TY - JOUR A1 - Varykhalov, Andrei A1 - Shikin, A. M. A1 - Gudat, Wolfgang A1 - Moras, P. A1 - Grazioli, C. A1 - Carbone, C. A1 - Rader, Oliver T1 - Probing the ground state electronic structure of a correlated electron system by quantum well states: Ag/ Ni(111) N2 - The ground state electronic properties of the strongly correlated transition metal Ni are usually not accessible from the excitation spectra measured in photoelectron spectroscopy. We show that the bottom of the Ni d band along [111] can be probed through the energy dependence of the phase of quantum-well states in Ag/Ni(111). Our model description of the quantum-well energies measured by angle-resolved photoemission determines the bottom of the Lambda(1) d band of Ni as 2.6 eV, in full agreement with standard local density theory and at variance with the values of 1.7-1.8 eV from direct angle-resolved photoemission experiments of Ni Y1 - 2005 SN - 0031-9007 ER - TY - JOUR A1 - Rader, Oliver A1 - Pampuch, Carsten A1 - Shikin, A. M. A1 - Gudat, Wolfgang A1 - Okabayashi, J. A1 - Mizokawa, T. A1 - Fujimori, A. A1 - Hayashi, T. A1 - Tanaka, M. A1 - Tanaka, A. A1 - Kimura, A. T1 - Resonant photoemission of Ga1-xMnxAs at the Mn L edge N2 - Ga1-xMnxAs, x=0.043, has been grown ex situ on GaAs(100) by low-temperature molecular-beam epitaxy. On the reprepared p(1x1) surface, resonant photoemission of the valence band shows a 20-fold enhancement of the Mn 3d contribution at the L-3 edge. The difference spectrum is similar to our previously obtained resonant photoemission at the Mn M edge, in particular a strong satellite appears and no clear Fermi edge ruling out strong Mn 3d weight at the valence-band maximum. The x-ray absorption lineshape differs from previous publications. Our calculation based on a configuration-interaction cluster model reproduces the x-ray absorption and the L-3 on-resonance photoemission spectrum for model parameters Delta, U-dd, and (pdsigma) consistent with our previous work and shows the same spectral shape on and off resonance thus rendering resonant photoemission measured at the L-3 edge representative of the Mn 3d contribution. At the same time, the results are more bulk sensitive due to a probing depth about twice as large as for photoemission at the Mn M edge. The confirmation of our previous results obtained at the M edge calls recent photoemission results into question which report the absence of the satellite and good agreement with local-density theory Y1 - 2004 ER - TY - JOUR A1 - Clark, Oliver J. A1 - Freyse, Friedrich A1 - Yashina, L. V. A1 - Rader, Oliver A1 - Sanchez-Barriga, Jaime T1 - Robust behavior and spin-texture stability of the topological surface state in Bi2Se3 upon deposition of gold JF - npj quantum materials N2 - The Dirac point of a topological surface state (TSS) is protected against gapping by time-reversal symmetry. Conventional wisdom stipulates, therefore, that only through magnetisation may a TSS become gapped. However, non-magnetic gaps have now been demonstrated in Bi2Se3 systems doped with Mn or In, explained by hybridisation of the Dirac cone with induced impurity resonances. Recent photoemission experiments suggest that an analogous mechanism applies even when Bi2Se3 is surface dosed with Au. Here, we perform a systematic spin- and angle-resolved photoemission study of Au-dosed Bi2Se3. Although there are experimental conditions wherein the TSS appears gapped due to unfavourable photoemission matrix elements, our photon-energy-dependent spectra unambiguously demonstrate the robustness of the Dirac cone against high Au coverage. We further show how the spin textures of the TSS and its accompanying surface resonances remain qualitatively unchanged following Au deposition, and discuss the mechanism underlying the suppression of the spectral weight. KW - Electronic properties and materials KW - Topological matter Y1 - 2022 U6 - https://doi.org/10.1038/s41535-022-00443-9 SN - 2397-4648 VL - 7 IS - 1 PB - Nature Publishing Group CY - London ER - TY - GEN A1 - Hlawenka, Peter A1 - Siemensmeyer, Konrad A1 - Weschke, Eugen A1 - Varykhalov, Andrei A1 - Sánchez-Barriga, Jaime A1 - Shitsevalova, Natalya Y. A1 - Dukhnenko, A.V. A1 - Filipov, V. B. A1 - Gabáni, Slavomir A1 - Flachbart, Karol A1 - Rader, Oliver A1 - Rienks, Emile D. L. T1 - Samarium hexaboride is a trivial surface conductor T2 - Postprints der Universität Potsdam : Mathematisch-Naturwissenschaftliche Reihe N2 - SmB6 is predicted to be the first member of the intersection of topological insulators and Kondo insulators, strongly correlated materials in which the Fermi level lies in the gap of a many-body resonance that forms by hybridization between localized and itinerant states. While robust, surface-only conductivity at low temperature and the observation of surface states at the expected high symmetry points appear to confirm this prediction, we find both surface states at the (100) surface to be topologically trivial. We find the (Gamma) over bar state to appear Rashba split and explain the prominent (X) over bar state by a surface shift of the many-body resonance. We propose that the latter mechanism, which applies to several crystal terminations, can explain the unusual surface conductivity. While additional, as yet unobserved topological surface states cannot be excluded, our results show that a firm connection between the two material classes is still outstanding. T3 - Zweitveröffentlichungen der Universität Potsdam : Mathematisch-Naturwissenschaftliche Reihe - 612 KW - topological Kondo-insulator KW - SmB 6 KW - photoemission KW - states KW - gap Y1 - 2019 U6 - http://nbn-resolving.de/urn/resolver.pl?urn:nbn:de:kobv:517-opus4-424213 SN - 1866-8372 IS - 612 ER - TY - JOUR A1 - Hlawenka, Peter A1 - Siemensmeyer, Konrad A1 - Weschke, Eugen A1 - Varykhalov, Andrei A1 - Sanchez-Barriga, Jaime A1 - Shitsevalova, Natalya Y. A1 - Dukhnenko, A. V. A1 - Filipov, V. B. A1 - Gabani, Slavomir A1 - Flachbart, Karol A1 - Rader, Oliver A1 - Rienks, Emile D. L. T1 - Samarium hexaboride is a trivial surface conductor JF - Nature Communications N2 - SmB6 is predicted to be the first member of the intersection of topological insulators and Kondo insulators, strongly correlated materials in which the Fermi level lies in the gap of a many-body resonance that forms by hybridization between localized and itinerant states. While robust, surface-only conductivity at low temperature and the observation of surface states at the expected high symmetry points appear to confirm this prediction, we find both surface states at the (100) surface to be topologically trivial. We find the (Gamma) over bar state to appear Rashba split and explain the prominent (X) over bar state by a surface shift of the many-body resonance. We propose that the latter mechanism, which applies to several crystal terminations, can explain the unusual surface conductivity. While additional, as yet unobserved topological surface states cannot be excluded, our results show that a firm connection between the two material classes is still outstanding. Y1 - 2018 U6 - https://doi.org/10.1038/s41467-018-02908-7 SN - 2041-1723 VL - 9 PB - Nature Publ. Group CY - London ER - TY - JOUR A1 - Varykhalov, Andrei A1 - Rader, Oliver A1 - Gudat, Wolfgang T1 - Structure and quantum-size effects in a surface carbide : W(110)/C-R(15 X 3) N2 - Results of the combined investigation of atomic and electronic structure of the W(110)/C-R(15x3) surface carbide are reported. A variety of experimental techniques has been involved such as scanning tunneling microscopy (STM), low-energy electron diffraction, x-ray photoelectron spectroscopy, and angle-resolved photoemission (ARPES). Distance-dependent STM measurements show a nontrivial geometrical behavior in the topography data, demonstrating five different patterns representing the superstructure at different values of the tip-surface separation. Atomic resolution was achieved at lower tunneling gap resistance. An unexpected spatial asymmetry in the distribution of the local density of states across the surface unit cell has been observed as well. Photoelectron spectroscopy of C1s and W4f core levels clarifies the nature of the chemical bonding in the system. The band mapping with ARPES provides information on the wave- vector dependence of the electronic states. Notable quantum size and superlattice effects were discovered in the dispersion of the valence-band states. The experimental data suggests an apparent one-dimensional character of the electronic structure. Lateral quantization and umklapp scattering are proposed as explanation. Finally, based on photoemission and STM measurements, an improved crystallographic model of the tungsten surface carbide is introduced Y1 - 2005 SN - 1098-0121 ER -