TY - JOUR A1 - Giewekemeyer, K. A1 - Krueger, S. P. A1 - Kalbfleisch, S. A1 - Bartels, Meike A1 - Beta, Carsten A1 - Salditt, T. T1 - X-ray propagation microscopy of biological cells using waveguides as a quasipoint source JF - Physical review : A, Atomic, molecular, and optical physics N2 - We have used x-ray waveguides as highly confining optical elements for nanoscale imaging of unstained biological cells using the simple geometry of in-line holography. The well-known twin-image problem is effectively circumvented by a simple and fast iterative reconstruction. The algorithm which combines elements of the classical Gerchberg-Saxton scheme and the hybrid-input-output algorithm is optimized for phase-contrast samples, well-justified for imaging of cells at multi-keV photon energies. The experimental scheme allows for a quantitative phase reconstruction from a single holographic image without detailed knowledge of the complex illumination function incident on the sample, as demonstrated for freeze-dried cells of the eukaryotic amoeba Dictyostelium discoideum. The accessible resolution range is explored by simulations, indicating that resolutions on the order of 20 nm are within reach applying illumination times on the order of minutes at present synchrotron sources. Y1 - 2011 U6 - https://doi.org/10.1103/PhysRevA.83.023804 SN - 1050-2947 VL - 83 IS - 2 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Oskinova, Lida A1 - Hamann, Wolf-Rainer A1 - Cassinelli, Joseph P. A1 - Brown, John C. A1 - Todt, Helge Tobias T1 - X-ray emission from massive stars with magnetic fields JF - Astronomische Nachrichten = Astronomical notes N2 - We investigate the connections between the magnetic fields and the X-ray emission from massive stars. Our study shows that the X-ray properties of known strongly magnetic stars are diverse: while some comply to the predictions of the magnetically confined wind model, others do not. We conclude that strong, hard, and variable X-ray emission may be a sufficient attribute of magnetic massive stars, but it is not a necessary one. We address the general properties of X-ray emission from "normal" massive stars, especially the long standing mystery about the correlations between the parameters of X-ray emission and fundamental stellar properties. The recent development in stellar structure modeling shows that small-scale surface magnetic fields may be common. We suggest a "hybrid" scenario which could explain the X-ray emission from massive stars by a combination of magnetic mechanisms on the surface and shocks in the stellar wind. The magnetic mechanisms and the wind shocks are triggered by convective motions in sub-photospheric layers. This scenario opens the door for a natural explanation of the well established correlation between bolometric and X-ray luminosities. KW - stars: magnetic fields KW - stars: mass-loss KW - stars: winds, outflows KW - stars: Wolf-Rayet KW - techniques: spectroscopic KW - X-rays: stars Y1 - 2011 U6 - https://doi.org/10.1002/asna.201111602 SN - 0004-6337 VL - 332 IS - 9-10 SP - 988 EP - 993 PB - Wiley-Blackwell CY - Malden ER - TY - JOUR A1 - Fiehler, Katja A1 - Bannert, Michael M. A1 - Bischoff, Matthias A1 - Blecker, Carlo A1 - Stark, Rudolf A1 - Vaitl, Dieter A1 - Franz, Volker H. A1 - Roesler, Frank T1 - Working memory maintenance of grasp-target information in the human posterior parietal cortex JF - NeuroImage : a journal of brain function N2 - Event-related functional magnetic resonance imaging was applied to identify cortical areas involved in maintaining target information in working memory used for an upcoming grasping action. Participants had to grasp with their thumb and index finger of the dominant right hand three-dimensional objects of different size and orientation. Reaching-to-grasp movements were performed without visual feedback either immediately after object presentation or after a variable delay of 2-12 s. The right inferior parietal cortex demonstrated sustained neural activity throughout the delay, which overlapped with activity observed during encoding of the grasp target. Immediate and delayed grasping activated similar motor-related brain areas and showed no differential activity. The results suggest that the right inferior parietal cortex plays an important functional role in working memory maintenance of grasp-related information. Moreover, our findings confirm the assumption that brain areas engaged in maintaining information are also involved in encoding the same information, and thus extend previous findings on working memory function of the posterior parietal cortex in saccadic behavior to reach-to-grasp movements. Y1 - 2011 U6 - https://doi.org/10.1016/j.neuroimage.2010.09.080 SN - 1053-8119 VL - 54 IS - 3 SP - 2401 EP - 2411 PB - Elsevier CY - San Diego ER - TY - JOUR A1 - Aliu, E. A1 - Arlen, T. A1 - Aune, T. A1 - Beilicke, M. A1 - Benbow, W. A1 - Boettcher, Markus A1 - Bouvier, A. A1 - Bradbury, S. M. A1 - Buckley, J. H. A1 - Bugaev, V. A1 - Cannon, A. A1 - Cesarini, A. A1 - Ciupik, L. A1 - Collins-Hughes, E. A1 - Connolly, M. P. A1 - Cui, W. A1 - Dickherber, R. A1 - Errando, M. A1 - Falcone, A. A1 - Finley, J. P. A1 - Fortson, L. A1 - Furniss, A. A1 - Galante, N. A1 - Gall, D. A1 - Gillanders, G. H. A1 - Godambe, S. A1 - Griffin, S. A1 - Grube, J. A1 - Gyuk, G. A1 - Hanna, D. A1 - Holder, J. A1 - Huan, H. A1 - Hughes, G. A1 - Hui, C. M. A1 - Humensky, T. B. A1 - Kaaret, P. A1 - Karlsson, N. A1 - Kertzman, M. A1 - Kieda, D. A1 - Krawczynski, H. A1 - Krennrich, F. A1 - Madhavan, A. S. A1 - Maier, G. A1 - Majumdar, P. A1 - McArthur, S. A1 - McCann, A. A1 - Moriarty, P. A1 - Mukherjee, R. A1 - Ong, R. A. A1 - Orr, M. A1 - Otte, A. N. A1 - Park, N. A1 - Perkins, J. S. A1 - Pichel, A. A1 - Pohl, Martin A1 - Prokoph, H. A1 - Quinn, J. A1 - Ragan, K. A1 - Reyes, L. C. A1 - Reynolds, P. T. A1 - Roache, E. A1 - Rose, H. J. A1 - Ruppel, J. A1 - Saxon, D. B. A1 - Schroedter, M. A1 - Sembroski, G. H. A1 - Skole, C. A1 - Smith, A. W. A1 - Staszak, D. A1 - Tesic, G. A1 - Theiling, M. A1 - Thibadeau, S. A1 - Tsurusaki, K. A1 - Tyler, J. A1 - Varlotta, A. A1 - Vincent, S. A1 - Vivier, M. A1 - Wakely, S. P. A1 - Ward, J. E. A1 - Weinstein, A. A1 - Weisgarber, T. A1 - Williams, D. A. T1 - Veritas observations of unusual extragalactic transient swift J164449.3+573451 JF - The astrophysical journal : an international review of spectroscopy and astronomical physics ; Part 2, Letters N2 - We report on very high energy (>100 GeV) gamma-ray observations of Swift J164449.3+573451, an unusual transient object first detected by the Swift Observatory and later detected by multiple radio, optical, and X-ray observatories. A total exposure of 28 hr was obtained on Swift J164449.3+573451 with the Very Energetic Radiation Imaging Telescope Array System ( VERITAS) during 2011 March 28-April 15. We do not detect the source and place a differential upper limit on the emission at 500 GeV during these observations of 1.4 x 10(-12) erg cm(-2) s(-1) (99% confidence level). We also present time-resolved upper limits and use a flux limit averaged over the X-ray flaring period to constrain various emission scenarios that can accommodate both the radio-through-X-ray emission detected from the source and the lack of detection by VERITAS. KW - accretion, accretion disks KW - galaxies: active KW - gamma rays: galaxies KW - radiation mechanisms: non-thermal Y1 - 2011 U6 - https://doi.org/10.1088/2041-8205/738/2/L30 SN - 2041-8205 VL - 738 IS - 2 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Acciari, V. A. A1 - Aliu, E. A1 - Arlen, T. A1 - Aune, T. A1 - Beilicke, M. A1 - Benbow, W. A1 - Bradbury, S. M. A1 - Buckley, J. H. A1 - Bugaev, V. A1 - Byrum, K. A1 - Cannon, A. A1 - Cesarini, A. A1 - Ciupik, L. A1 - Collins-Hughes, E. A1 - Connolly, M. P. A1 - Cui, W. A1 - Dickherber, R. A1 - Duke, C. A1 - Errando, M. A1 - Falcone, A. A1 - Finley, J. P. A1 - Finnegan, G. A1 - Fortson, L. A1 - Furniss, A. A1 - Galante, N. A1 - Gall, D. A1 - Gillanders, G. H. A1 - Godambe, S. A1 - Griffin, S. A1 - Grube, J. A1 - Guenette, R. A1 - Gyuk, G. A1 - Hanna, D. A1 - Holder, J. A1 - Hughes, G. A1 - Hui, C. M. A1 - Humensky, T. B. A1 - Kaaret, P. A1 - Karlsson, N. A1 - Kertzman, M. A1 - Kieda, D. A1 - Krawczynski, H. A1 - Krennrich, F. A1 - Lang, M. J. A1 - LeBohec, S. A1 - Maier, G. A1 - Majumdar, P. A1 - McArthur, S. A1 - McCann, A. A1 - Moriarty, P. A1 - Mukherjee, R. A1 - Ong, R. A. A1 - Orr, M. A1 - Otte, A. N. A1 - Park, N. A1 - Perkins, J. S. A1 - Pohl, Martin A1 - Prokoph, H. A1 - Quinn, J. A1 - Ragan, K. A1 - Reyes, L. C. A1 - Reynolds, P. T. A1 - Roache, E. A1 - Rose, H. J. A1 - Ruppel, J. A1 - Saxon, D. B. A1 - Schroedter, M. A1 - Sembroski, G. H. A1 - Senturk, G. D. A1 - Smith, A. W. A1 - Staszak, D. A1 - Tesic, G. A1 - Theiling, M. A1 - Thibadeau, S. A1 - Tsurusaki, K. A1 - Varlotta, A. A1 - Vassiliev, V. V. A1 - Vincent, S. A1 - Vivier, M. A1 - Wakely, S. P. A1 - Ward, J. E. A1 - Weekes, T. C. A1 - Weinstein, A. A1 - Weisgarber, T. A1 - Williams, D. A. A1 - Zitzer, B. T1 - VERITAS OBSERVATIONS OF THE TeV BINARY LS I+61 degrees 303 DURING 2008-2010 JF - The astrophysical journal : an international review of spectroscopy and astronomical physics N2 - We present the results of observations of the TeV binary LS I + 61 degrees 303 with the VERITAS telescope array between 2008 and 2010, at energies above 300 GeV. In the past, both ground-based gamma-ray telescopes VERITAS and MAGIC have reported detections of TeV emission near the apastron phases of the binary orbit. The observations presented here show no strong evidence for TeV emission during these orbital phases; however, during observations taken in late 2010, significant emission was detected from the source close to the phase of superior conjunction (much closer to periastron passage) at a 5.6 standard deviation (5.6 sigma) post-trials significance. In total, between 2008 October and 2010 December a total exposure of 64.5 hr was accumulated with VERITAS on LS I + 61 degrees 303, resulting in an excess at the 3.3 sigma significance level for constant emission over the entire integrated data set. The flux upper limits derived for emission during the previously reliably active TeV phases (i.e., close to apastron) are less than 5% of the Crab Nebula flux in the same energy range. This result stands in apparent contrast to previous observations by both MAGIC and VERITAS which detected the source during these phases at 10% of the Crab Nebula flux. During the two year span of observations, a large amount of X-ray data were also accrued on LS I + 61 degrees 303 by the Swift X-ray Telescope and the Rossi X-ray Timing Explorer Proportional Counter Array. We find no evidence for a correlation between emission in the X-ray and TeV regimes during 20 directly overlapping observations. We also comment on data obtained contemporaneously by the Fermi Large Area Telescope. KW - binaries: general KW - gamma rays: general KW - X-rays: binaries Y1 - 2011 U6 - https://doi.org/10.1088/0004-637X/738/1/3 SN - 0004-637X VL - 738 IS - 1 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Acciari, V. A. A1 - Aliu, E. A1 - Arlen, T. A1 - Aune, T. A1 - Beilicke, M. A1 - Benbow, W. A1 - Bradbury, S. M. A1 - Buckley, J. H. A1 - Bugaev, V. A1 - Byrum, K. A1 - Cannon, A. A1 - Cesarini, A. A1 - Christiansen, J. L. A1 - Ciupik, L. A1 - Collins-Hughes, E. A1 - Connolly, M. P. A1 - Cui, W. A1 - Duke, C. A1 - Errando, M. A1 - Falcone, A. A1 - Finley, J. P. A1 - Finnegan, G. A1 - Fortson, L. A1 - Furniss, A. A1 - Galante, N. A1 - Gall, D. A1 - Godambe, S. A1 - Griffin, S. A1 - Grube, J. A1 - Guenette, R. A1 - Gyuk, G. A1 - Hanna, D. A1 - Holder, J. A1 - Hughes, G. A1 - Hui, C. M. A1 - Humensky, T. B. A1 - Jackson, D. J. A1 - Kaaret, P. A1 - Karlsson, N. A1 - Kertzman, M. A1 - Kieda, D. A1 - Krawczynski, H. A1 - Krennrich, F. A1 - Lang, M. J. A1 - Madhavan, A. S. A1 - Maier, G. A1 - McArthur, S. A1 - McCann, A. A1 - Moriarty, P. A1 - Newbold, M. D. A1 - Ong, R. A. A1 - Orr, M. A1 - Otte, A. N. A1 - Park, N. A1 - Perkins, J. S. A1 - Pohl, Martin A1 - Prokoph, H. A1 - Quinn, J. A1 - Ragan, K. A1 - Reyes, L. C. A1 - Reynolds, P. T. A1 - Roache, E. A1 - Rose, H. J. A1 - Ruppel, J. A1 - Saxon, D. B. A1 - Schroedter, M. A1 - Sembroski, G. H. A1 - Sentuerk, G. D. A1 - Smith, A. W. A1 - Staszak, D. A1 - Swordy, S. P. A1 - Tesic, G. A1 - Theiling, M. A1 - Thibadeau, S. A1 - Tsurusaki, K. A1 - Varlotta, A. A1 - Vassiliev, V. V. A1 - Vincent, S. A1 - Vivier, M. A1 - Wakely, S. P. A1 - Ward, J. E. A1 - Weekes, T. C. A1 - Weinstein, A. A1 - Weisgarber, T. A1 - Williams, D. A. A1 - Wood, M. T1 - Veritas observations of gamma-ray bursts detected by swift JF - The astrophysical journal : an international review of spectroscopy and astronomical physics N2 - We present the results of 16 Swift-triggered Gamma-ray burst (GRB) follow-up observations taken with the Very Energetic Radiation Imaging Telescope Array System (VERITAS) telescope array from 2007 January to 2009 June. The median energy threshold and response time of these observations were 260 GeV and 320 s, respectively. Observations had an average duration of 90 minutes. Each burst is analyzed independently in two modes: over the whole duration of the observations and again over a shorter timescale determined by the maximum VERITAS sensitivity to a burst with a t(-1.5) time profile. This temporal model is characteristic of GRB afterglows with high-energy, long-lived emission that have been detected by the Large Area Telescope on board the Fermi satellite. No significant very high energy (VHE) gamma-ray emission was detected and upper limits above the VERITAS threshold energy are calculated. The VERITAS upper limits are corrected for gamma-ray extinction by the extragalactic background light and interpreted in the context of the keV emission detected by Swift. For some bursts the VHE emission must have less power than the keV emission, placing constraints on inverse Compton models of VHE emission. KW - astroparticle physics KW - gamma-ray burst: general Y1 - 2011 U6 - https://doi.org/10.1088/0004-637X/743/1/62 SN - 0004-637X VL - 743 IS - 1 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Arhammar, C. A1 - Pietzsch, Annette A1 - Bock, Nicolas A1 - Holmstroem, Erik A1 - Araujo, C. Moyses A1 - Grasjo, Johan A1 - Zhao, Shuxi A1 - Green, Sara A1 - Peery, T. A1 - Hennies, Franz A1 - Amerioun, Shahrad A1 - Föhlisch, Alexander A1 - Schlappa, Justine A1 - Schmitt, Thorsten A1 - Strocov, Vladimir N. A1 - Niklasson, Gunnar A. A1 - Wallace, Duane C. A1 - Rubensson, Jan-Erik A1 - Johansson, Borje A1 - Ahuja, Rajeev C. T1 - Unveiling the complex electronic structure of amorphous metal oxides JF - Proceedings of the National Academy of Sciences of the United States of America N2 - Amorphous materials represent a large and important emerging area of material's science. Amorphous oxides are key technological oxides in applications such as a gate dielectric in Complementary metal-oxide semiconductor devices and in Silicon-Oxide-Nitride-Oxide-Silicon and TANOS (TaN-Al2O3-Si3N4-SiO2-Silicon) flash memories. These technologies are required for the high packing density of today's integrated circuits. Therefore the investigation of defect states in these structures is crucial. In this work we present X-ray synchrotron measurements, with an energy resolution which is about 5-10 times higher than is attainable with standard spectrometers, of amorphous alumina. We demonstrate that our experimental results are in agreement with calculated spectra of amorphous alumina which we have generated by stochastic quenching. This first principles method, which we have recently developed, is found to be superior to molecular dynamics in simulating the rapid gas to solid transition that takes place as this material is deposited for thin film applications. We detect and analyze in detail states in the band gap that originate from oxygen pairs. Similar states were previously found in amorphous alumina by other spectroscopic methods and were assigned to oxygen vacancies claimed to act mutually as electron and hole traps. The oxygen pairs which we probe in this work act as hole traps only and will influence the information retention in electronic devices. In amorphous silica oxygen pairs have already been found, thus they may be a feature which is characteristic also of other amorphous metal oxides. KW - stochastic quench KW - X-ray absorption spectroscopy KW - ab initio KW - coating Y1 - 2011 U6 - https://doi.org/10.1073/pnas.1019698108 SN - 0027-8424 VL - 108 IS - 16 SP - 6355 EP - 6360 PB - National Acad. of Sciences CY - Washington ER - TY - JOUR A1 - Qiu, Xunlin A1 - Gerhard, Reimund A1 - Mellinger, Axel T1 - Turning polymer foams or polymer-film systems into ferroelectrets dielectric barrier discharges in voids JF - IEEE transactions on dielectrics and electrical insulation N2 - Polymer foams and void-containing polymer-film systems with internally charged voids combine large piezoelectricity with mechanical flexibility and elastic compliance. This new class of soft materials (often called ferro-or piezoelectrets) has attracted considerable attention from science and industry. It has been found that the voids can be internally charged by means of dielectric barrier discharges (DBDs) under high electric fields. The charged voids can be considered as man-made macroscopic dipoles. Depending on the ferroelectret structure and the pressure of the internal gas, the voids may be highly compressible. Consequently, very large dipole-moment changes can be induced by mechanical or electrical stresses, leading to large piezoelectricity. DBD charging of the voids is a critical process for rendering polymer foams piezoelectric. Thus a comprehensive exploration of DBD charging is essential for the understanding and the optimization of piezoelectricity in ferroelectrets. Recent studies show that DBDs in the voids are triggered when the internal electric field reaches a threshold value according to Townsend's model of Paschen breakdown. During the DBDs, charges of opposite polarity are generated and trapped at the top and bottom internal surfaces of the gas-filled voids, respectively. The deposited charges induce an electric field opposite to the externally applied one and thus extinguish the DBDs. Back discharges may eventually be triggered when the external voltage is reduced or turned off. In order to optimize the efficiency of DBD charging, the geometry (in particular the height) of the voids, the type of gas and its pressure inside the voids are essential factors to be considered and to be optimized. In addition, the influence of the plasma treatment on the internal void surfaces during the DBDs should be taken into consideration. KW - Ferroelectret KW - piezoelectret KW - dielectric barrier discharge (DBD) KW - effective polarization KW - man-made dipole Y1 - 2011 U6 - https://doi.org/10.1109/TDEI.2011.5704490 SN - 1070-9878 VL - 18 IS - 1 SP - 34 EP - 42 PB - Inst. of Electr. and Electronics Engineers CY - Piscataway ER - TY - JOUR A1 - Pontius, N. A1 - Kachel, T. A1 - Schüssler-Langeheine, C. A1 - Schlotter, W. F. A1 - Beye, Martin A1 - Sorgenfrei, Nomi A1 - Chang, C. F. A1 - Föhlisch, Alexander A1 - Wurth, W. A1 - Metcalf, P. A1 - Leonov, I. A1 - Yaresko, A. A1 - Stojanovic, N. A1 - Berglund, Martin A1 - Guerassimova, N. A1 - Duesterer, S. A1 - Redlin, H. A1 - Duerr, H. A. T1 - Time-resolved resonant soft x-ray diffraction with free-electron lasers femtosecond dynamics across the Verwey transition in magnetite JF - Applied physics letters N2 - Resonant soft x-ray diffraction (RSXD) with femtosecond (fs) time resolution is a powerful tool for disentangling the interplay between different degrees of freedom in strongly correlated electron materials. It allows addressing the coupling of particular degrees of freedom upon an external selective perturbation, e. g., by an optical or infrared laser pulse. Here, we report a time-resolved RSXD experiment from the prototypical correlated electron material magnetite using soft x-ray pulses from the free-electron laser FLASH in Hamburg. We observe ultrafast melting of the charge-orbital order leading to the formation of a transient phase, which has not been observed in equilibrium. Y1 - 2011 U6 - https://doi.org/10.1063/1.3584855 SN - 0003-6951 VL - 98 IS - 18 PB - American Institute of Physics CY - Melville ER - TY - JOUR A1 - Blakesley, James C. A1 - Schubert, Marcel A1 - Steyrleuthner, Robert A1 - Chen, Zhihua A1 - Facchetti, Antonio A1 - Neher, Dieter T1 - Time-of-flight measurements and vertical transport in a high electron-mobility polymer JF - Applied physics letters N2 - We investigate charge transport in a high-electron mobility polymer, poly(N, N-bis 2-octyldodecyl-naphthalene-1,4,5,8-bis dicarboximide-2,6-diyl-alt-5,5-2,2-bithiophene) [P(NDI2OD-T2), Polyera ActivInk (TM) N2200]. Time-of-flight measurements reveal electron mobilities approaching those measured in field-effect transistors, the highest ever recorded in a conjugated polymer using this technique. The modest temperature dependence and weak dispersion of the transients indicate low energetic disorder in this material. Steady-state electron-only current measurements reveal a barrier to injection of about 300 meV. We propose that this barrier is located within the P(NDI2OD-T2) film and arises from molecular orientation effects. Y1 - 2011 U6 - https://doi.org/10.1063/1.3657827 SN - 0003-6951 VL - 99 IS - 18 PB - American Institute of Physics CY - Melville ER - TY - JOUR A1 - Fang, Peng A1 - Wang, Feipeng A1 - Wirges, Werner A1 - Gerhard, Reimund A1 - Basso, Heitor Cury T1 - Three-layer piezoelectrets from fluorinated ethylene-propylene (FEP) copolymer films JF - Applied physics : A, Materials science & processing N2 - A process for preparing three-layer piezoelectrets from fluorinated ethylene-propylene (FEP) copolymer films is introduced. Samples are made from commercial FEP films by means of laser cutting, laser bonding, electrode evaporation, and high-field poling. The observed dielectric-resonance spectra demonstrate the piezoelectricity of the FEP sandwiches. Piezoelectric d (33) coefficients up to a few hundred pC/N are achieved. Charging at elevated temperatures can increase the thermal stability of the piezoelectrets. Isothermal experiments for approximately 15 min demonstrate that samples charged at 140A degrees C keep their piezoelectric activity up to at least 120A degrees C and retain 70% of their initial d (33) even at 130A degrees C. Acoustical measurements show a relatively flat frequency response in the range between 300 Hz and 20 kHz. Y1 - 2011 U6 - https://doi.org/10.1007/s00339-010-6008-2 SN - 0947-8396 SN - 1432-0630 VL - 103 IS - 2 SP - 455 EP - 461 PB - Springer CY - New York ER - TY - JOUR A1 - Evans, Nancy Remage A1 - DeGioia-Eastwood, Kathleen A1 - Gagne, Marc A1 - Townsley, Leisa A1 - Broos, Patrick S. A1 - Wolk, Scott J. A1 - Naze, Yael A1 - Corcoran, Michael A1 - Oskinova, Lida A1 - Moffat, Anthony F. J. A1 - Wang, Junfeng A1 - Walborn, Nolan R. T1 - The search for low-mass companions of b stars in the Carina Nebula cluster trumpler 16 JF - The astrophysical journal : an international review of spectroscopy and astronomical physics ; Supplement series N2 - We have developed lists of likely B3-A0 stars (called "late B" stars) in the young cluster Trumpler 16. The following criteria were used: location within 3' of eta Car, an appropriate V and B - V combination, and proper motion (where available). Color and magnitude cuts have been made assuming an E(B - V) = 0.55 mag +/- 0.1, which is a good approximation close to the center of Trumpler 16. These lists have been cross-correlated with X-ray sources found in the Chandra Carina Complex Project. Previous studies have shown that only very rarely (if at all) do late main-sequence B stars produce X-rays. We present evidence that the X-ray-detected sources are binaries with low-mass companions, since stars less massive than 1.4 M-circle dot are strong X-ray sources at the age of the cluster. Both the median X-ray energies and X-ray luminosities of these sources are in good agreement with values for typical low-mass coronal X-ray sources. We find that 39% of the late B stars based on a list with proper motions have low-mass companions. Similarly, 32% of a sample without proper motions have low-mass companions. We discuss the X-ray detection completeness. These results on low-mass companions of intermediate-mass stars are complementary to spectroscopic and interferometric results and probe new parameter space of low-mass companions at all separations. They do not support a steeply rising distribution of mass ratios to low masses for intermediate-mass (5 M-circle dot) primaries, such as would be found by random pairing from the initial mass function. KW - open clusters and associations: individual (Trumpler 16) KW - stars: massive Y1 - 2011 U6 - https://doi.org/10.1088/0067-0049/194/1/13 SN - 0067-0049 VL - 194 IS - 1 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Martin, Maria A. A1 - Winkelmann, Ricarda A1 - Haseloff, M. A1 - Albrecht, Tanja A1 - Bueler, Ed A1 - Khroulev, C. A1 - Levermann, Anders T1 - The Potsdam parallel ice sheet model (PISM-PIK) - Part 2: Dynamic equilibrium simulation of the Antarctic ice sheet JF - The Cryosphere : TC ; an interactive open access journal of the European Geosciences Union N2 - We present a dynamic equilibrium simulation of the ice sheet-shelf system on Antarctica with the Potsdam Parallel Ice Sheet Model (PISM-PIK). The simulation is initialized with present-day conditions for bed topography and ice thickness and then run to steady state with constant present-day surface mass balance. Surface temperature and sub-shelf basal melt distribution are parameterized. Grounding lines and calving fronts are free to evolve, and their modeled equilibrium state is compared to observational data. A physically-motivated calving law based on horizontal spreading rates allows for realistic calving fronts for various types of shelves. Steady-state dynamics including surface velocity and ice flux are analyzed for whole Antarctica and the Ronne-Filchner and Ross ice shelf areas in particular. The results show that the different flow regimes in sheet and shelves, and the transition zone between them, are captured reasonably well, supporting the approach of superposition of SIA and SSA for the representation of fast motion of grounded ice. This approach also leads to a natural emergence of sliding-dominated flow in stream-like features in this new 3-D marine ice sheet model. Y1 - 2011 U6 - https://doi.org/10.5194/tc-5-727-2011 SN - 1994-0416 VL - 5 IS - 3 SP - 727 EP - 740 PB - Copernicus CY - Göttingen ER - TY - JOUR A1 - Winkelmann, Ricarda A1 - Martin, Maria A. A1 - Haseloff, Monika A1 - Albrecht, Torsten A1 - Bueler, Ed A1 - Khroulev, C. A1 - Levermann, Anders T1 - The Potsdam parallel ice sheet model (PISM-PIK) - Part 1: Model description JF - The Cryosphere : TC ; an interactive open access journal of the European Geosciences Union N2 - We present the Potsdam Parallel Ice Sheet Model (PISM-PIK), developed at the Potsdam Institute for Climate Impact Research to be used for simulations of large-scale ice sheet-shelf systems. It is derived from the Parallel Ice Sheet Model (Bueler and Brown, 2009). Velocities are calculated by superposition of two shallow stress balance approximations within the entire ice covered region: the shallow ice approximation (SIA) is dominant in grounded regions and accounts for shear deformation parallel to the geoid. The plug-flow type shallow shelf approximation (SSA) dominates the velocity field in ice shelf regions and serves as a basal sliding velocity in grounded regions. Ice streams can be identified diagnostically as regions with a significant contribution of membrane stresses to the local momentum balance. All lateral boundaries in PISM-PIK are free to evolve, including the grounding line and ice fronts. Ice shelf margins in particular are modeled using Neumann boundary conditions for the SSA equations, reflecting a hydrostatic stress imbalance along the vertical calving face. The ice front position is modeled using a subgrid-scale representation of calving front motion (Albrecht et al., 2011) and a physically-motivated calving law based on horizontal spreading rates. The model is tested in experiments from the Marine Ice Sheet Model Intercomparison Project (MISMIP). A dynamic equilibrium simulation of Antarctica under present-day conditions is presented in Martin et al. (2011). Y1 - 2011 U6 - https://doi.org/10.5194/tc-5-715-2011 SN - 1994-0416 VL - 5 IS - 3 SP - 715 EP - 726 PB - Copernicus CY - Göttingen ER - TY - JOUR A1 - Richter, Philipp A1 - Krause, F. A1 - Fechner, Cora A1 - Charlton, Jane C. A1 - Murphy, M. T. T1 - The neutral gas extent of galaxies as derived from weak intervening Ca II absorbers JF - Astronomy and astrophysics : an international weekly journal N2 - We present a systematic study of weak intervening CaII absorbers at low redshift (z < 0.5), based on the analysis of archival high-resolution (R >= 45 000) optical spectra of 304 quasars and active galactic nuclei observed with VLT/UVES. Along a total redshift path of Delta z approximate to 100 we detected 23 intervening CaII absorbers in both the CaII H & K lines, with rest frame equivalent widths W-r,W-3934 = 15-799 m angstrom and column densities log N(CaII) = 11.25-13.04 (obtained by fitting Voigt-profile components). We obtain a bias-corrected number density of weak intervening CaII absorbers of dN/dz = 0.117 +/- 0.044 at < z(abs)> = 0.35 for absorbers with log N(CaII) >= 11.65 (W-r,W-3934 >= 32 m angstrom). This is similar to 2.6 times the value obtained for damped Lyman alpha absorbers (DLAs) at low redshift. All CaII absorbers in our sample show associated absorption by other low ions such as MgII and FeII; 45 percent of them have associated NaI absorption. From ionization modelling we conclude that intervening CaII absorption with log N(CaII) >= 11.5 arises in DLAs, sub-DLAs and Lyman-limit systems (LLS) at HI column densities of log N(HI) >= 17.4. Using supplementary HI information for nine of the absorbers we find that the CaII/HI ratio decreases strongly with increasing HI column density, indicating a column-density-dependent dust depletion of Ca. The observed column density distribution function of CaII absorption components follows a relatively steep power law, f(N) proportional to N-beta, with a slope of -beta = -1.68, which again points towards an enhanced dust depletion in high column density systems. The relatively large cross section of these absorbers together with the frequent detection of CaII absorption in high-velocity clouds (HVCs) in the halo of the Milky Way suggests that a considerable fraction of the intervening CaII systems trace (partly) neutral gas structures in the halos and circumgalactic environment of galaxies (i.e., they are HVC analogs). Based on the recently measured detection rate of CaII absorption in the Milky Way HVCs we estimate that the mean (projected) CaII covering fraction of galaxies and their gaseous halos is < f(c,CaII)> = 0.33. Using this value and considering all galaxies with luminosities L >= 0.05 L-star we calculate that the characteristic radial extent of (partly) neutral gas clouds with log N(HI) >= 17.4 around low-redshift galaxies is R-HVC approximate to 55 kpc. KW - galaxies: halos KW - galaxies: formation KW - galaxies: ISM KW - intergalactic medium KW - quasars: absorption lines Y1 - 2011 U6 - https://doi.org/10.1051/0004-6361/201015566 SN - 0004-6361 VL - 528 IS - 4 PB - EDP Sciences CY - Les Ulis ER - TY - JOUR A1 - Hundertmark, Michaela A1 - Dimova, Rumiana A1 - Lengefeld, Jan A1 - Seckler, Robert A1 - Hincha, Dirk K. T1 - The intrinsically disordered late embryogenesis abundant protein LEA18 from Arabidopsis thaliana modulates membrane stability through binding and folding JF - Biochimica et biophysica acta : Biomembranes N2 - Intrinsically disordered proteins (IDPs) constitute a substantial part of cellular proteomes. late embryogenesis abundant (LEA) proteins are mostly predicted to be IDPs associated with dehydration tolerance in many plant, animal and bacterial species. Their functions, however, are largely unexplored and also their structure and interactions with potential target molecules have only recently been experimentally investigated in a small number of proteins. Here, we report on the structure and interactions with membranes of the Pfam LEA_1 protein LEA18 from the higher plant Arabidopsis thaliana. This functionally uncharacterized positively charged protein specifically aggregated and destabilized negatively charged liposomes. Isothermal titration calorimetry showed binding of the protein to both charged and uncharged membranes. LEA18 alone was largely unstructured in solution. While uncharged membranes had no influence on the secondary structure of LEA18, the protein partially folded into beta-sheet structure in the presence of negatively charged liposomes. These data suggest that LEA18 does not function as a membrane stabilizing protein, as suggested for other LEA proteins. Instead, a possible function of LEA18 could be the composition-dependent modulation of membrane stability, e.g., during signaling or vesicle-mediated transport. KW - Intrinsically disordered protein KW - Late embryogenesis abundant protein KW - Membrane stability KW - Protein-membrane interaction KW - Protein folding Y1 - 2011 U6 - https://doi.org/10.1016/j.bbamem.2010.09.010 SN - 0005-2736 VL - 1808 IS - 1 SP - 446 EP - 453 PB - Elsevier CY - Amsterdam ER - TY - JOUR A1 - Winkel, B. A1 - Ben Bekhti, Nadya A1 - Darmstaedter, V. A1 - Floeer, L. A1 - Kerp, J. A1 - Richter, Philipp T1 - The high-velocity cloud complex Galactic center negative as seen by EBHIS and GASS I. Cloud catalog and global properties JF - Astronomy and astrophysics : an international weekly journal N2 - Using Milky Way data of the new Effelsberg-Bonn HI Survey (EBHIS) and the Galactic All-Sky Survey (GASS), we present a revised picture of the high-velocity cloud (HVC) complex Galactic center negative (GCN). Owing to the higher angular resolution of these surveys compared to previous studies (e.g., the Leiden Dwingeloo Survey), we resolve complex GCN into lots of individual tiny clumps, that mostly have relatively broad line widths of more than 15 km s(-1). We do not detect a diffuse extended counterpart, which is unusual for an HVC complex. In total 243 clumps were identified and parameterized which allows us to statistically analyze the data. Cold-line components (i.e.,Delta upsilon(fwhm) < 7.5 km s(-1)) are found in about 5% only of the identified cloudlets. Our analysis reveals that complex GCN is likely built up of several subpopulations that do not share a common origin. Furthermore, complex GCN might be a prime example for warm-gas accretion onto the Milky Way, where neutral HI clouds are not stable against interaction with the Milky Way gas halo and become ionized prior to accretion. KW - ISM: clouds KW - Galaxy: halo Y1 - 2011 U6 - https://doi.org/10.1051/0004-6361/201117357 SN - 0004-6361 VL - 533 IS - 18 PB - EDP Sciences CY - Les Ulis ER - TY - JOUR A1 - Delahaye, T. A1 - Fiasson, A. A1 - Pohl, Martin A1 - Salati, P. T1 - The GeV-TeV Galactic gamma-ray diffuse emission I. Uncertainties in the predictions of the hadronic component JF - Astronomy and astrophysics : an international weekly journal N2 - Context. The Galactic gamma-ray diffuse emission is currently observed in the GeV-TeV energy range with unprecedented accuracy by the Fermi satellite. Understanding this component is crucial because it provides a background to many different signals, such as extragalactic sources or annihilating dark matter. It is timely to reinvestigate how it is calculated and to assess the various uncertainties that are likely to affect the accuracy of the predictions. Aims. The Galactic gamma-ray diffuse emission is mostly produced above a few GeV by the interactions of cosmic ray primaries impinging on the interstellar material. The theoretical error on that component is derived by exploring various potential sources of uncertainty. Particular attention is paid to cosmic ray propagation. Nuclear cross sections, the proton and helium fluxes at the Earth's position, the Galactic radial profile of supernova remnants, and the hydrogen distribution can also severely affect the signal. Methods. The propagation of cosmic ray species throughout the Galaxy is described in the framework of a semi-analytic two-zone diffusion/convection model. The gamma-ray flux is reliably and quickly determined. This allows conversion of the constraints set by the boron-to-carbon data into a theoretical uncertainty on the diffuse emission. New deconvolutions of the HI and CO sky maps are also used to get the hydrogen distribution within the Galaxy. Results. The thickness of the cosmic ray diffusive halo is found to have a significant effect on the Galactic gamma-ray diffuse emission, while the interplay between diffusion and convection has little influence on the signal. The uncertainties related to nuclear cross sections and to the primary cosmic ray fluxes at the Earth are significant. The radial distribution of supernova remnants along the Galactic plane turns out to be a key ingredient. As expected, the predictions are extremely sensitive to the spatial distribution of hydrogen within the Milky Way. Conclusions. Most of the sources of uncertainty are likely to be reduced in the near future. The stress should be put (i) on better determination of the thickness of the cosmic ray diffusive halo; and (ii) on refined observations of the radial profile of supernova remnants. KW - gamma rays: diffuse background KW - cosmic rays KW - methods: analytical KW - gamma rays: ISM Y1 - 2011 U6 - https://doi.org/10.1051/0004-6361/201116647 SN - 0004-6361 VL - 531 IS - 4 PB - EDP Sciences CY - Les Ulis ER - TY - JOUR A1 - Worseck, Gabor A1 - Prochaska, J. Xavier A1 - McQuinn, Matthew A1 - Dall'Aglio, Aldo A1 - Fechner, Cora A1 - Hennawi, Joseph F. A1 - Reimers, Dieter A1 - Richter, Philipp A1 - Wisotzki, Lutz T1 - The end of Helium Reionization at z similar or equal to 2.7 Inferred from cosmic variance in HST/COS He II Ly alpha Absorption spectra JF - The astrophysical journal : an international review of spectroscopy and astronomical physics ; Part 2, Letters N2 - We report on the detection of strongly varying intergalactic He II absorption in HST/COS spectra of two z(em) similar or equal to 3 quasars. From our homogeneous analysis of the He II absorption in these and three archival sightlines, we find a marked increase in the mean He II effective optical depth from similar or equal to 1 at z similar or equal to 2.3 to greater than or similar to 5 at z similar or equal to 3.2, but with a large scatter of 2 less than or similar to tau(eff, He II) less than or similar to 5 at 2.7 < z < 3 on scales of similar to 10 proper Mpc. This scatter is primarily due to fluctuations in the He II fraction and the He II-ionizing background, rather than density variations that are probed by the coeval Hi forest. Semianalytic models of He II absorption require a strong decrease in the He II-ionizing background to explain the strong increase of the absorption at z greater than or similar to 2.7, probably indicating He II reionization was incomplete at z(reion) greater than or similar to 2.7. Likewise, recent three-dimensional numerical simulations of He II reionization qualitatively agree with the observed trend only if He II reionization completes at z(reion) similar or equal to 2.7 or even below, as suggested by a large tau(eff, He II) greater than or similar to 3 in two of our five sightlines at z < 2.8. By doubling the sample size at 2.7 less than or similar to z less than or similar to 3, our newly discovered He II sightlines for the first time probe the diversity of the second epoch of reionization when helium became fully ionized. KW - dark ages, reionization, first stars KW - diffuse radiation KW - intergalactic medium KW - quasars: absorption lines KW - quasars: individual (SDSS J092447.36+485242.8, SDSS J110155.74+105302.3) Y1 - 2011 U6 - https://doi.org/10.1088/2041-8205/733/2/L24 SN - 2041-8205 VL - 733 IS - 2 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Tremblay, Jean Christophe A1 - Monturet, Serge A1 - Saalfrank, Peter T1 - The Effects of electron-hole pair coupling on the infrared laser-controlled vibrational excitation of NO on Au(111) JF - The journal of physical chemistry : A, Molecules, spectroscopy, kinetics, environment & general theory N2 - In this work, we present theoretical simulations of laser-driven vibrational control of NO adsorbed on a gold surface. Our goal is to tailor laser pulses to selectively excite specific modes and vibrational eigenstates, as well as to favor photodesorption of the adsorbed molecule. To this end, various control schemes and algorithms are applied. For adsorbates at metallic surfaces, the creation of electron hole pairs in the substrate is known to play a dominant role in the transfer of energy from the system to the surroundings. These nonadiabatic couplings are included perturbatively in our reduced density matrix simulations using a generalization of the state-resolved position-dependent anharmonic rate model we recently introduced. An extension of the reduced density matrix is also proposed to provide a sound model for photodesorption in dissipative systems. Y1 - 2011 U6 - https://doi.org/10.1021/jp205902k SN - 1089-5639 VL - 115 IS - 39 SP - 10698 EP - 10707 PB - American Chemical Society CY - Washington ER - TY - JOUR A1 - Hübener, Robert A1 - Kruszynska, Caroline A1 - Hartmann, Lorenz A1 - Duer, Wolfgang A1 - Plenio, Martin B. A1 - Eisert, Jens T1 - Tensor network methods with graph enhancement JF - Physical review : B, Condensed matter and materials physics N2 - We present applications of the renormalization algorithm with graph enhancement (RAGE). This analysis extends the algorithms and applications given for approaches based on matrix product states introduced in [Phys. Rev. A 79, 022317 (2009)] to other tensor-network states such as the tensor tree states (TTS) and projected entangled pair states. We investigate the suitability of the bare TTS to describe ground states, showing that the description of certain graph states and condensed-matter models improves. We investigate graph-enhanced tensor-network states, demonstrating that in some cases (disturbed graph states and for certain quantum circuits) the combination of weighted graph states with TTS can greatly improve the accuracy of the description of ground states and time-evolved states. We comment on delineating the boundary of the classically efficiently simulatable states of quantum many-body systems. Y1 - 2011 U6 - https://doi.org/10.1103/PhysRevB.84.125103 SN - 1098-0121 VL - 84 IS - 12 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Koseska, Aneta A1 - Volkov, Evgenii A1 - Kurths, Jürgen T1 - Synthetic multicellular oscillatory systems controlling protein dynamics with genetic circuits JF - Physica scripta : an international journal for experimental and theoretical physics N2 - Synthetic biology is a relatively new research discipline that combines standard biology approaches with the constructive nature of engineering. Thus, recent efforts in the field of synthetic biology have given a perspective to consider cells as 'programmable matter'. Here, we address the possibility of using synthetic circuits to control protein dynamics. In particular, we show how intercellular communication and stochasticity can be used to manipulate the dynamical behavior of a population of coupled synthetic units and, in this manner, finely tune the expression of specific proteins of interest, e.g. in large bioreactors. Y1 - 2011 U6 - https://doi.org/10.1088/0031-8949/84/04/045007 SN - 0031-8949 VL - 84 IS - 4 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Huang, Tingwen A1 - Chen, Guanrong A1 - Kurths, Jürgen T1 - Synchronization of chaotic of chaotic systems with time-varying coupöing delays JF - Discrete and continuous dynamical systems : a journal bridging mathematics and sciences ; Series B, Mathematical modelling, analysis and computations N2 - In this paper, we study the complete synchronization of a class of time-varying delayed coupled chaotic systems using feedback control. In terms of Linear Matrix Inequalities, a sufficient condition is obtained through using a Lyapunov-Krasovskii functional and differential equation in equalities. The conditions can be easily verified and implemented. We present two simulation examples to illustrate the effectiveness of the proposed method. KW - Synchronization KW - Chaotic System KW - Time-varying Delay Y1 - 2011 U6 - https://doi.org/10.3934/dcdsb.2011.16.1071 SN - 1531-3492 VL - 16 IS - 4 SP - 1071 EP - 1082 PB - American Institute of Mathematical Sciences CY - Springfield ER - TY - JOUR A1 - Sepp, T. A1 - Tempel, E. A1 - Gramann, M. A1 - Nurmi, P. A1 - Haupt, Michael T1 - Studying the patterns of the universe JF - Baltic astronomy N2 - The SDSS galaxy catalog is one of the best databases for galaxy distribution studies. The SDSS DR8 data is used to construct the galaxy cluster catalog. We construct the clusters from the calculated luminosity density field and identify denser regions. Around these peak regions we construct galaxy clusters. Another interesting question in cosmology is how observable galaxy structures are connected to underlying dark matter distribution. To study this we compare the SDSS DR7 galaxy group catalog with galaxy groups obtained from the semi-analytical Millennium N-Body simulation. Specifically, we compare the group richness, virial radius, maximum separation and velocity dispersion distributions and find a relatively good agreement between the mock catalog and observations. This strongly supports the idea, that the dark matter distribution and galaxies in the semi-analytical models and observations are very closely linked. KW - galaxies: groups, clusters KW - cosmology: dark matter, large-scale structure of the Universe Y1 - 2011 SN - 1392-0049 VL - 20 IS - 2 SP - 309 EP - 312 PB - Institute of Theoretical Physics and Astronomy CY - Moletai ER - TY - JOUR A1 - Kollosche, Matthias A1 - Stoyanov, Hristiyan A1 - Laflamme, Simon A1 - Kofod, Guggi T1 - Strongly enhanced sensitivity in elastic capacitive strain sensors JF - Journal of materials chemistry N2 - Strain sensors based on dielectric elastomer capacitors function by the direct coupling of mechanical deformations with the capacitance. The coupling can be improved by enhancing the relative permittivity of the dielectric elastomer. Here, this is carried out through the grafting of conducting polymer (poly-aniline) to the elastomer backbone, leading to molecular composites. An enhancement in capacitance response of 46 times is observed. This could help to extend the possible range of miniaturization towards even smaller device features. Y1 - 2011 U6 - https://doi.org/10.1039/c0jm03786a SN - 0959-9428 VL - 21 IS - 23 SP - 8292 EP - 8294 PB - Royal Society of Chemistry CY - Cambridge ER - TY - JOUR A1 - Mulansky, Mario A1 - Ahnert, Karsten A1 - Pikovskij, Arkadij A1 - Shepelyansky, Dima L. T1 - Strong and weak chaos in weakly nonintegrable many-body hamiltonian systems JF - Journal of statistical physics N2 - We study properties of chaos in generic one-dimensional nonlinear Hamiltonian lattices comprised of weakly coupled nonlinear oscillators by numerical simulations of continuous-time systems and symplectic maps. For small coupling, the measure of chaos is found to be proportional to the coupling strength and lattice length, with the typical maximal Lyapunov exponent being proportional to the square root of coupling. This strong chaos appears as a result of triplet resonances between nearby modes. In addition to strong chaos we observe a weakly chaotic component having much smaller Lyapunov exponent, the measure of which drops approximately as a square of the coupling strength down to smallest couplings we were able to reach. We argue that this weak chaos is linked to the regime of fast Arnold diffusion discussed by Chirikov and Vecheslavov. In disordered lattices of large size we find a subdiffusive spreading of initially localized wave packets over larger and larger number of modes. The relations between the exponent of this spreading and the exponent in the dependence of the fast Arnold diffusion on coupling strength are analyzed. We also trace parallels between the slow spreading of chaos and deterministic rheology. KW - Lyapunov exponent KW - Arnold diffusion KW - Chaos spreading Y1 - 2011 U6 - https://doi.org/10.1007/s10955-011-0335-3 SN - 0022-4715 VL - 145 IS - 5 SP - 1256 EP - 1274 PB - Springer CY - New York ER - TY - JOUR A1 - Gruber, W. A1 - Chakravarty, S. A1 - Baehtz, C. A1 - Leitenberger, Wolfram A1 - Bruns, M. A1 - Kobler, A. A1 - Kübel, Christian A1 - Schmidt, H. T1 - Strain relaxation and vacancy creation in thin platinum films JF - Physical review letters N2 - Synchrotron based combined in situ x-ray diffractometry and reflectometry is used to investigate the role of vacancies for the relaxation of residual stress in thin metallic Pt films. From the experimentally determined relative changes of the lattice parameter a and of the film thickness L the modification of vacancy concentration and residual strain was derived as a function of annealing time at 130 degrees C. The results indicate that relaxation of strain resulting from compressive stress is accompanied by the creation of vacancies at the free film surface. This proves experimentally the postulated dominant role of vacancies for stress relaxation in thin metal films close to room temperature. Y1 - 2011 U6 - https://doi.org/10.1103/PhysRevLett.107.265501 SN - 0031-9007 VL - 107 IS - 26 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Stich, Michael A1 - Beta, Carsten T1 - Standing waves in a complex Ginzburg-Landau equation with time-delay feedback JF - Discrete and continuous dynamical systems : a journal bridging mathematics and sciences N2 - Standing waves are studied as solutions of a complex Ginsburg-Landau equation subjected to local and global time-delay feedback terms. The onset of standing waves is studied at the instability of the homogeneous periodic solution with respect to spatially periodic perturbations. The solution of this spatiotemporal wave pattern is given and is compared to the homogeneous periodic solution. KW - pattern formation KW - reaction-diffusion system KW - control Y1 - 2011 SN - 1078-0947 SN - 1553-5231 IS - 1 SP - 1329 EP - 1334 PB - American Institute of Mathematical Sciences CY - Springfield ER - TY - JOUR A1 - Rychkov, Dmitry A1 - Gerhard, Reimund T1 - Stabilization of positive charge on polytetrafluoroethylene electret films treated with titanium-tetrachloride vapor JF - Applied physics letters N2 - The surface of polytetrafluoroethylene films was treated with titanium-tetrachloride vapor. The treatment was carried out in a flow reactor by means of molecular-layer deposition, a method from the arsenal of chemical nanotechnology. X-ray photoelectron spectroscopy reveals that such a treatment results in considerable changes in the chemical composition at and near the surface of the fluoropolymer film. Both, defluorination and oxidation of the surface were observed. At the same time, samples treated with titanium tetrachloride show a significant enhancement in the thermal stability of the positive homocharge. The thermally stimulated surface-potential-decay curves were observed to shift to higher temperatures by more than 100 degrees C. Y1 - 2011 U6 - https://doi.org/10.1063/1.3565166 SN - 0003-6951 VL - 98 IS - 12 PB - American Institute of Physics CY - Melville ER - TY - JOUR A1 - Kalbitz, Rene A1 - Frübing, Peter A1 - Gerhard, Reimund A1 - Taylor, D. M. T1 - Stability of polarization in organic ferroelectric metal-insulator-semiconductor structures JF - Applied physics letters N2 - Dielectric measurements have been carried out on all-organic metal-insulator-semiconductor structures with the ferroelectric polymer poly(vinylidenefluoride-trifluoroethylene) as the gate insulator. It is shown that the polarization states remain stable after poling with accumulation and depletion voltage. However, negative charge trapped at the semiconductor-insulator interface during the depletion cycle masks the negative shift in flatband voltage expected during the sweep to accumulation voltages. Y1 - 2011 U6 - https://doi.org/10.1063/1.3543632 SN - 0003-6951 VL - 98 IS - 3 PB - American Institute of Physics CY - Melville ER - TY - JOUR A1 - Pietzsch, Annette A1 - Sun, Y. -P. A1 - Hennies, Franz A1 - Rinkevicius, Z. A1 - Karlsson, Hans O. A1 - Schmitt, Thorsten A1 - Strocov, Vladimir N. A1 - Andersson, Joakim A1 - Kennedy, B. A1 - Schlappa, J. A1 - Föhlisch, Alexander A1 - Rubensson, Jan-Erik A1 - Gel'mukhanov, F. T1 - Spatial quantum beats in vibrational resonant inelastic soft X-ray scattering at dissociating states in oxygen JF - Physical review letters N2 - Resonant inelastic soft x-ray scattering (RIXS) spectra excited at the 1 sigma(g) -> 3 sigma(u) resonance in gas-phase O-2 show excitations due to the nuclear degrees of freedom with up to 35 well-resolved discrete vibronic states and a continuum due to the kinetic energy distribution of the separated atoms. The RIXS profile demonstrates spatial quantum beats caused by two interfering wave packets with different momenta as the atoms separate. Thomson scattering strongly affects both the spectral profile and the scattering anisotropy. Y1 - 2011 U6 - https://doi.org/10.1103/PhysRevLett.106.153004 SN - 0031-9007 VL - 106 IS - 15 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Navirian, Hengameh A. A1 - Herzog, Marc A1 - Goldshteyn, J. A1 - Leitenberger, Wolfram A1 - Vrejoiu, Ionella A1 - Khakhulin, D. A1 - Wulff, M. A1 - Shayduk, Roman A1 - Gaal, P. A1 - Bargheer, Matias T1 - Shortening x-ray pulses for pump-probe experiments at synchrotrons JF - Journal of applied physics N2 - We implemented an experimental scheme for ultrafast x-ray diffraction at storage rings based on a laser-driven Bragg-switch that shortens the x-ray pulses emitted from an undulator. The increased time-resolution is demonstrated by observing changes of intensity, position and width of the diffraction peaks of a La(0.7)Sr(0.3)MnO(3)/SrTiO(3) superlattice sample after optical excitation, i.e., by quantitatively measuring the propagation of an expansion wave through the sample. These experimental transients with timescales of 35 to 60 ps evidence a reduction of the x-ray pulse duration by a factor of two. Y1 - 2011 U6 - https://doi.org/10.1063/1.3601057 SN - 0021-8979 VL - 109 IS - 12 PB - American Institute of Physics CY - Melville ER - TY - JOUR A1 - Schaefer, Edith A1 - Westendorf, Christian A1 - Bodenschatz, Eberhard A1 - Beta, Carsten A1 - Geil, Burkhard A1 - Janshoff, Andreas T1 - Shape oscillations of dictyostelium discoideum cells on ultramicroelectrodes monitored by impedance analysis JF - Small Y1 - 2011 U6 - https://doi.org/10.1002/smll.201001955 SN - 1613-6810 VL - 7 IS - 6 SP - 723 EP - 726 PB - Wiley-Blackwell CY - Malden ER - TY - JOUR A1 - Pikovskij, Arkadij A1 - Fishman, Shmuel T1 - Scaling properties of weak chaos in nonlinear disordered lattices JF - Physical review : E, Statistical, nonlinear and soft matter physics N2 - We study the discrete nonlinear Schrodinger equation with a random potential in one dimension. It is characterized by the length, the strength of the random potential, and the field density that determines the effect of nonlinearity. Following the time evolution of the field and calculating the largest Lyapunov exponent, the probability of the system to be regular is established numerically and found to be a scaling function of the parameters. This property is used to calculate the asymptotic properties of the system in regimes beyond our computational power. Y1 - 2011 U6 - https://doi.org/10.1103/PhysRevE.83.025201 SN - 1539-3755 SN - 1550-2376 VL - 83 IS - 2 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Mulansky, Mario A1 - Ahnert, Karsten A1 - Pikovskij, Arkadij T1 - Scaling of energy spreading in strongly nonlinear disordered lattices JF - Physical review : E, Statistical, nonlinear and soft matter physics N2 - To characterize a destruction of Anderson localization by nonlinearity, we study the spreading behavior of initially localized states in disordered, strongly nonlinear lattices. Due to chaotic nonlinear interaction of localized linear or nonlinear modes, energy spreads nearly subdiffusively. Based on a phenomenological description by virtue of a nonlinear diffusion equation, we establish a one-parameter scaling relation between the velocity of spreading and the density, which is confirmed numerically. From this scaling it follows that for very low densities the spreading slows down compared to the pure power law. Y1 - 2011 U6 - https://doi.org/10.1103/PhysRevE.83.026205 SN - 1539-3755 VL - 83 IS - 2 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Koenig, Tobias A1 - Goldenberg, Leonid M. A1 - Kulikovska, Olga A1 - Kulikovsky, Lazar A1 - Stumpe, Joachim A1 - Santer, Svetlana T1 - Reversible structuring of photosensitive polymer films by surface plasmon near field radiation JF - Soft matter N2 - We report on the fabrication and characterisation of a novel type of hybrid azo-modified photosensitive polymer film with a nanoscale metallic structuring integrated into the substrate. The metal structures permit to generate surface plasmon near fields when irradiated by UV-light from the rear without directly illuminating the polymer. This allows establishment of a localized, complex-shape intensity distribution at sub-wavelength resolution with a corresponding impact on the photosensitive polymer. The possibilities of exploiting this setup are manifold. We find that just by using the change of polarization of the incident light as means of control, the topography can be driven to change between various patterns reversibly. These results are confirmed by numerical simulations and compared with in situ recorded topography changes. Y1 - 2011 U6 - https://doi.org/10.1039/c0sm01164a SN - 1744-683X VL - 7 IS - 9 SP - 4174 EP - 4178 PB - Royal Society of Chemistry CY - Cambridge ER - TY - JOUR A1 - Montoya, Marisa A1 - Born, Andreas A1 - Levermann, Anders T1 - Reversed North Atlantic gyre dynamics in present and glacial climates JF - Climate dynamics : observational, theoretical and computational research on the climate system N2 - The dynamics of the North Atlantic subpolar gyre (SPG) are assessed under present and glacial boundary conditions by investigating the SPG sensitivity to surface wind-stress changes in a coupled climate model. To this end, the gyre transport is decomposed in Ekman, thermohaline, and bottom transports. Surface wind-stress variations are found to play an important indirect role in SPG dynamics through their effect on water-mass densities. Our results suggest the existence of two dynamically distinct regimes of the SPG, depending on the absence or presence of deep water formation (DWF) in the Nordic Seas and a vigorous Greenland-Scotland ridge (GSR) overflow. In the first regime, the GSR overflow is weak and the SPG strength increases with wind-stress as a result of enhanced outcropping of isopycnals in the centre of the SPG. As soon as a vigorous GSR overflow is established, its associated positive density anomalies on the southern GSR slope reduce the SPG strength. This has implications for past glacial abrupt climate changes, insofar as these can be explained through latitudinal shifts in North Atlantic DWF sites and strengthening of the North Atlantic current. Regardless of the ultimate trigger, an abrupt shift of DWF into the Nordic Seas could result both in a drastic reduction of the SPG strength and a sudden reversal in its sensitivity to wind-stress variations. Our results could provide insight into changes in the horizontal ocean circulation during abrupt glacial climate changes, which have been largely neglected up to now in model studies. Y1 - 2011 U6 - https://doi.org/10.1007/s00382-009-0729-y SN - 0930-7575 VL - 36 IS - 5-6 SP - 1107 EP - 1118 PB - Springer CY - New York ER - TY - THES A1 - Osterloh, Lukas T1 - Retrieving aerosol microphysical properties from multiwavelength Lidar Data Y1 - 2011 CY - Potsdam ER - TY - JOUR A1 - Blakesley, James C. A1 - Neher, Dieter T1 - Relationship between energetic disorder and open-circuit voltage in bulk heterojunction organic solar cells JF - Physical review : B, Condensed matter and materials physics N2 - We simulate organic bulk heterojunction solar cells. The effects of energetic disorder are incorporated through a Gaussian or exponential model of density of states. Analytical models of open-circuit voltage (V(OC)) are derived from the splitting of quasi-Fermi potentials. Their predictions are backed up by more complex numerical device simulations including effects such as carrier-density-dependent charge-carrier mobilities. It is predicted that the V(OC) depends on: (1) the donor-acceptor energy gap; (2) charge-carrier recombination rates; (3) illumination intensity; (4) the contact work functions (if not in the pinning regime); and (5) the amount of energetic disorder. A large degree of energetic disorder, or a high density of traps, is found to cause significant reductions in V(OC). This can explain why V(OC) is often less than expected in real devices. Energetic disorder also explains the nonideal temperature and intensity dependence of V(OC) and the superbimolecular recombination rates observed in many real bulk heterojunction solar cells. Y1 - 2011 U6 - https://doi.org/10.1103/PhysRevB.84.075210 SN - 1098-0121 VL - 84 IS - 7 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Blaha, Karen A. A1 - Pikovskij, Arkadij A1 - Rosenblum, Michael A1 - Clark, Matthew T. A1 - Rusin, Craig G. A1 - Hudson, John L. T1 - Reconstruction of two-dimensional phase dynamics from experiments on coupled oscillators JF - Physical review : E, Statistical, nonlinear and soft matter physics N2 - Phase models are a powerful method to quantify the coupled dynamics of nonlinear oscillators from measured data. We use two phase modeling methods to quantify the dynamics of pairs of coupled electrochemical oscillators, based on the phases of the two oscillators independently and the phase difference, respectively. We discuss the benefits of the two-dimensional approach relative to the one-dimensional approach using phase difference. We quantify the dependence of the coupling functions on the coupling magnitude and coupling time delay. We show differences in synchronization predictions of the two models using a toy model. We show that the two-dimensional approach reveals behavior not detected by the one-dimensional model in a driven experimental oscillator. This approach is broadly applicable to quantify interactions between nonlinear oscillators, especially where intrinsic oscillator sensitivity and coupling evolve with time. Y1 - 2011 U6 - https://doi.org/10.1103/PhysRevE.84.046201 SN - 1539-3755 VL - 84 IS - 4 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Fechner, Cora T1 - Reconstructing the intergalactic UV background with QSO absorption lines JF - Astronomy and astrophysics : an international weekly journal N2 - We present a new approach to observationally constraining the spectral energy distribution of the intergalactic UV background by studying metal absorption systems. We study single-component metal line systems that exhibit various well-measured species. Among the observed transitions, at least two ratios of ionization stages from the same element are required, e. g. C III/C IV and Si III/Si IV. For each system photoionization models are constructed by varying the spectrum of the ionizing radiation. The spectral energy distribution can then be constrained by comparing the models with the observed column density ratios. Extensive tests with artificial absorbers show that the spectrum of the ionizing radiation cannot be reconstructed unambiguously, but it is possible to constrain the main characteristics of the spectrum. Furthermore, the resulting physical parameters of the absorber, such as ionization parameter, metallicity, and relative abundances, may depend strongly on the adopted ionizing spectrum. Even in case of well-fitting models, the uncertainties can be as high as similar to 0.5 dex for the ionization parameter and up to similar to 1.5 dex for the metallicity. Therefore, it is essential to know the hardness of the UV background when estimating the metallicity of the intergalactic medium. Applying the procedure to a small sample of 3 observed single-component metal line systems yields a soft ionizing radiation at z > 2 and a slightly harder spectrum at z < 2. The resulting energy distributions exhibit strong He II Lya re-emission features, suggesting that reprocessing by intergalactic He II is important. Comparing the observed systems to UV background spectra from the literature indicates that a recent model that includes sawtooth modulation due to reprocessing by intergalactic He II with delayed helium reionization fits the investigated systems very well. KW - intergalactic medium KW - quasars: absorption lines KW - diffuse radiation Y1 - 2011 U6 - https://doi.org/10.1051/0004-6361/201117080 SN - 0004-6361 VL - 532 IS - 2 PB - EDP Sciences CY - Les Ulis ER - TY - JOUR A1 - Kralemann, Björn A1 - Pikovskij, Arkadij A1 - Rosenblum, Michael T1 - Reconstructing phase dynamics of oscillator networks JF - Chaos : an interdisciplinary journal of nonlinear science N2 - We generalize our recent approach to the reconstruction of phase dynamics of coupled oscillators from data [B. Kralemann et al., Phys. Rev. E 77, 066205 (2008)] to cover the case of small networks of coupled periodic units. Starting from a multivariate time series, we first reconstruct genuine phases and then obtain the coupling functions in terms of these phases. Partial norms of these coupling functions quantify directed coupling between oscillators. We illustrate the method by different network motifs for three coupled oscillators and for random networks of five and nine units. We also discuss nonlinear effects in coupling. Y1 - 2011 U6 - https://doi.org/10.1063/1.3597647 SN - 1054-1500 VL - 21 IS - 2 PB - American Institute of Physics CY - Melville ER - TY - JOUR A1 - Grass, T. D. A1 - dos Santos, Francisca E. A. A1 - Pelster, Axel T1 - Real-time Ginzburg-Landau theory for bosons in optical lattices JF - Laser physics N2 - Within the Schwinger-Keldysh formalism we derive a Ginzburg-Landau theory for the Bose-Hubbard model which describes the real-time dynamics of the complex order parameter field. Analyzing the excitations in the vicinity of the quantum phase transitions it turns out that particle/hole dispersions in the Mott phase map continuously onto corresponding amplitude/phase excitations in the superfluid phase. Furthermore, in the superfluid phase we find a sound mode, which is in accordance with recent Bragg spectroscopy measurements in the Bogoliubov regime, as well as an additional gapped mode, which seems to have been detected via lattice modulation. Y1 - 2011 U6 - https://doi.org/10.1134/S1054660X11150096 SN - 1054-660X SN - 1555-6611 VL - 21 IS - 8 SP - 1459 EP - 1463 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Zhirov, O. V. A1 - Pikovskij, Arkadij A1 - Shepelyansky, Dima L. T1 - Quantum vacuum of strongly nonlinear lattices JF - Physical review : E, Statistical, nonlinear and soft matter physics N2 - We study the properties of classical and quantum strongly nonlinear chains by means of extensive numerical simulations. Due to strong nonlinearity, the classical dynamics of such chains remains chaotic at arbitrarily low energies. We show that the collective excitations of classical chains are described by sound waves whose decay rate scales algebraically with the wave number with a generic exponent value. The properties of the quantum chains are studied by the quantum Monte Carlo method and it is found that the low-energy excitations are well described by effective phonon modes with the sound velocity dependent on an effective Planck constant. Our results show that at low energies the quantum effects lead to a suppression of chaos and drive the system to a quasi-integrable regime of effective phonon modes. Y1 - 2011 U6 - https://doi.org/10.1103/PhysRevE.83.016202 SN - 1539-3755 VL - 83 IS - 1 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Turner, Sarah T. A1 - Pingel, Patrick A1 - Steyrleuthner, Robert A1 - Crossland, Edward J. W. A1 - Ludwigs, Sabine A1 - Neher, Dieter T1 - Quantitative analysis of bulk heterojunction films using linear absorption spectroscopy and solar cell performance JF - Advanced functional materials N2 - A fundamental understanding of the relationship between the bulk morphology and device performance is required for the further development of bulk heterojunction organic solar cells. Here, non-optimized (chloroform cast) and nearly optimized (solvent-annealed o-dichlorobenzene cast) P3HT:PCBM blend films treated over a range of annealing temperatures are studied via optical and photovoltaic device measurements. Parameters related to the P3HT aggregate morphology in the blend are obtained through a recently established analytical model developed by F. C. Spano for the absorption of weakly interacting H-aggregates. Thermally induced changes are related to the glass transition range of the blend. In the chloroform prepared devices, the improvement in device efficiency upon annealing within the glass transition range can be attributed to the growth of P3HT aggregates, an overall increase in the percentage of chain crystallinity, and a concurrent increase in the hole mobilities. Films treated above the glass transition range show an increase in efficiency and fill factor not only associated with the change in chain crystallinity, but also with a decrease in the energetic disorder. On the other hand, the properties of the P3HT phase in the solvent-annealed o-dichlorobenzene cast blends are almost indistinguishable from those of the corresponding pristine P3HT layer and are only weakly affected by thermal annealing. Apparently, slow drying of the blend allows the P3HT chains to crystallize into large domains with low degrees of intra- and interchain disorder. This morphology appears to be most favorable for the efficient generation and extraction of charges. KW - Organic electronics KW - morphology KW - solar cells KW - mobility KW - absorption spectroscopy Y1 - 2011 U6 - https://doi.org/10.1002/adfm.201101583 SN - 1616-301X VL - 21 IS - 24 SP - 4640 EP - 4652 PB - Wiley-VCH CY - Weinheim ER - TY - JOUR A1 - Müller, Matthias M. A1 - Haakh, Harald R. A1 - Calarco, Tommaso A1 - Koch, Christiane P. A1 - Henkel, Carsten T1 - Prospects for fast Rydberg gates on an atom chip JF - Quantum information processing N2 - Atom chips are a promising candidate for a scalable architecture for quantum information processing provided a universal set of gates can be implemented with high fidelity. The difficult part in achieving universality is the entangling two-qubit gate. We consider a Rydberg phase gate for two atoms trapped on a chip and employ optimal control theory to find the shortest gate that still yields a reasonable gate error. Our parameters correspond to a situation where the Rydberg blockade regime is not yet reached. We discuss the role of spontaneous emission and the effect of noise from the chip surface on the atoms in the Rydberg state. KW - Optimal control KW - Phase gate KW - Rydberg atoms KW - Cavity quantum electrodynamics Y1 - 2011 U6 - https://doi.org/10.1007/s11128-011-0296-0 SN - 1570-0755 VL - 10 IS - 6 SP - 771 EP - 792 PB - Springer CY - New York ER - TY - JOUR A1 - Baushev, Anton N. T1 - Principal properties of the velocity distribution of dark matter particles on the outskirts of the Solar system JF - Monthly notices of the Royal Astronomical Society N2 - The velocity distribution of the dark matter particles on the outskirts of the Solar system remains unclear. We suggest to determine it using experimentally found properties of the oldest halo objects. Indeed, the oldest halo stars and globular clusters form a collisionless system, as well as dark matter particles do, and they evolved in the same gravitational field. If we accept this analogy, we can show that the velocity distribution of the dark matter particles should be highly anisotropic and have a sharp maximum near upsilon similar to 500 km s(-1). The distribution is totally different from the Maxwell one. We analyse the influence of the distribution function on the results of dark matter detection experiments. It is found that the direct detection signal should differ noticeably from the one calculated from the Maxwell distribution with similar or equal to 220 km s(-1), which is conventional for direct detection experiments (the ratio depends on the detector properties and typically falls within the range between 6 and 0.2). Moreover, the sharp distinction from the Maxwell distribution can be very essential to the observations of dark matter annihilation. KW - elementary particles KW - methods: analytical KW - dark matter Y1 - 2011 U6 - https://doi.org/10.1111/j.1745-3933.2011.01125.x SN - 0035-8711 VL - 417 IS - 1 SP - L83 EP - L87 PB - Wiley-Blackwell CY - Malden ER - TY - JOUR A1 - Sun, Zhuanlan A1 - Zhang, Xiaoqing A1 - Xia, Zhongfu A1 - Qiu, Xunlin A1 - Wirges, Werner A1 - Gerhard, Reimund A1 - Zeng, Changchun A1 - Zhang, Chuck A1 - Wang, Ben T1 - Polarization and piezoelectricity in polymer films with artificial void structure JF - Applied physics : A, Materials science & processing N2 - Laminated polymer-film systems with well-defined void structures were prepared from fluoroethylenepropylene (FEP) and polytetrafluoroethylene (PTFE) layers. First the PTFE films were patterned and then fusion-bonded with the FEP films. The laminates were subjected to either corona or contact charging in order to obtain the desired piezoelectricity. The build-up of the "macro-dipoles" in the laminated films was studied by recording the electric hysteresis loops. The resulting electro-mechanical properties were investigated by means of dielectric resonance spectroscopy (DRS) and direct measurements of the stress-strain relationship. Moreover, the thermal stability of the piezoelectric d (33) coefficient was investigated at elevated temperatures and via thermally stimulated discharge (TSD) current measurements in short circuit. For 150 mu m thick laminated films, consisting of one 25 mu m thick PTFE layer, two 12.5 mu m thick FEP layers, and a void of 100 mu m height, the critical voltage necessary for the build-up of the "macro-dipoles" in the inner voids was approximately 1400 V, which agrees with the value calculated from the Paschen Law. A quasi-static piezoelectric d (33) coefficient up to 300 pC/N was observed after corona charging. The mechanical properties of the film systems are highly anisotropic. At room temperature, the Young's moduli of the laminated film system are around 0.37 MPa in the thickness direction and 274 MPa in the lateral direction, respectively. Using these values, the theoretical shape anisotropy ratio of the void was calculated, which agrees well with experimental observation. Compared with films that do not exhibit structural regularity, the laminates showed improved thermal stability of the d (33) coefficients. The thermal stability of d (33) can be further improved by pre-aging. E.g., the reduction of the d (33) value in the sample pre-aged at 150A degrees C for 5 h was less than 5% after annealing for 30 h at a temperature of 90A degrees C. Y1 - 2011 U6 - https://doi.org/10.1007/s00339-011-6481-2 SN - 0947-8396 VL - 105 IS - 1 SP - 197 EP - 205 PB - Springer CY - New York ER - TY - JOUR A1 - Kuznetsov, Sergey P. T1 - Plykin type attractor in electronic device simulated in MULTISIM JF - Chaos : an interdisciplinary journal of nonlinear science N2 - An electronic device is suggested representing a non-autonomous dynamical system with hyperbolic chaotic attractor of Plykin type in the stroboscopic map, and the results of its simulation with software package NI MULTISIM are considered in comparison with numerical integration of the underlying differential equations. A main practical advantage of electronic devices of this kind is their structural stability that means insensitivity of the chaotic dynamics in respect to variations of functions and parameters of elements constituting the system as well as to interferences and noises. Y1 - 2011 U6 - https://doi.org/10.1063/1.3646903 SN - 1054-1500 VL - 21 IS - 4 PB - American Institute of Physics CY - Melville ER - TY - JOUR A1 - Schenk, Paul A1 - Hamilton, Douglas P. A1 - Johnson, Robert E. A1 - McKinnon, William B. A1 - Paranicas, Chris A1 - Schmidt, Jürgen A1 - Showalter, Mark R. T1 - Plasma, plumes and rings saturn system dynamics as recorded in global color patterns on its midsize icy satellites JF - Icarus : international journal of solar system studies N2 - New global maps of the five inner midsize icy saturnian satellites, Mimas, Enceladus, Tethys, Dione, and Rhea, have been constructed in three colors (UV, Green and near-IR) at resolutions of 1 km/pixel. The maps reveal prominent global patterns common to several of these satellites but also three major color features unique to specific satellites or satellite subgroups. The most common features among the group are first-order global asymmetries in color properties. This pattern, expressed on Tethys, Dione and Rhea, takes the form of a similar to 1.4-1.8 times enhancement in redness (expressed as IR/UV ratio) of the surface at the center of the trailing hemisphere of motion, and a similar though significantly weaker IR/UV enhancement at the center of the leading hemisphere. The peak in redness on the trailing hemisphere also corresponds to a known decrease in albedo. These double hemispheric asymmetries are attributable to plasma and E-ring grain bombardment on the trailing and leading hemispheres, respectively, for the outer three satellites Tethys, Dione and Rhea, whereas as E-ring bombardment may be focused on the trailing hemisphere of Mimas due to its orbital location interior to Enceladus. The maps also reveal three major deviations from these basic global patterns. We observe the previously known dark bluish leading hemisphere equatorial band on Tethys but have also discovered a similar band on Mimas. Similar in shape, both features match the surface patterns expected for irradiation of the surface by incident MeV electrons that drift in a direction opposite to the plasma flow. The global asymmetry on Enceladus is offset similar to 40 degrees to the west compared to the other satellites. We do not consider Enceladus in detail here, but the global distribution of bluish material can be shown to match the deposition pattern predicted for plume fallback onto the surface (Kempf, S., Beckmann, U., Schmidt, S. [2010]. Icarus 206, 446-457. doi:10.1016/j.icarus.2009.09.016). E-ring deposition on Enceladus thus appears to mask or prevent the formation of the lenses and hemispheric asymmetries we see on the other satellites. Finally, we observe a chain of discrete bluish splotches along the equator of Rhea. Unlike the equatorial bands of Tethys and Mimas, these splotches form a very narrow great circle <= 10-km wide (north-to-south) and appear to be related to surface disruption, exposing fresh, bluish ice on older crater rims. This feature is unique to Rhea and may have formed by impact onto its surface of orbiting material. KW - Satellites, Surfaces KW - Saturn, Satellites KW - Saturn, Rings KW - Enceladus KW - Satellites, Composition KW - Magnetospheres Y1 - 2011 U6 - https://doi.org/10.1016/j.icarus.2010.08.016 SN - 0019-1035 VL - 211 IS - 1 SP - 740 EP - 757 PB - Elsevier CY - San Diego ER - TY - BOOK A1 - Rabe, Thorid T1 - Physikdidaktische Lehrerprofessionalisierung zwischen Anspruch und Wirklichkeit : Antrittsvorlesung 2011-06-08 N2 - Physiklehrer bestimmen durch die Gestaltung des Unterrichts und damit durch ihr professionelles Handeln maßgeblich mit, wie die individuellen Lernprozesse der Schüler zu Inhalten der Physik ablaufen. Für die Entwicklung ihrer professionellen Handlungskompetenz müssen zukünftige Physiklehrer einerseits physikalisches, physikdidaktisches und pädagogisches Wissen erwerben und andererseits motiviert sein, dieses Wissen auch anzuwenden. In ihrer Vorlesung geht Thorid Rabe der Frage nach, welche physikdidaktischen Kompetenzen Studierende im Rahmen der universitären Ausbildung erwerben sollten. Am Beispiel der Lehrveranstaltung "Physikalische Schulexperimente" zeigt sie, wie physikdidaktische Theorie und praktisches Lehrerhandeln aufeinander bezogen werden können. Zudem wird sie ein Forschungsprojekt vorstellen, das einem bisher vernachlässigten Aspekt professioneller Handlungskompetenz nachgeht, nämlich den domänenspezifischen Selbstwirksamkeitserwartungen - dem Zutrauen in sich selbst, als Physiklehrer angemessen und erfolgreich handeln zu können. Y1 - 2011 UR - http://info.ub.uni-potsdam.de/multimedia/show_multimediafile.php?mediafile_id=548 PB - Univ.-Bibl. CY - Potsdam ER - TY - JOUR A1 - Green, Luci M. A1 - Kliem, Bernhard A1 - Wallace, A. J. T1 - Photospheric flux cancellation and associated flux rope formation and eruption JF - Astronomy and astrophysics : an international weekly journal N2 - Aims. We study an evolving bipolar active region that exhibits flux cancellation at the internal polarity inversion line, the formation of a soft X-ray sigmoid along the inversion line and a coronal mass ejection. The aim is to investigate the quantity of flux cancellation that is involved in flux rope formation in the time period leading up to the eruption. Methods. The active region is studied using its extreme ultraviolet and soft X-ray emissions as it evolves from a sheared arcade to flux rope configuration. The evolution of the photospheric magnetic field is described and used to estimate how much flux is reconnected into the flux rope. Results. About one third of the active region flux cancels at the internal polarity inversion line in the 2.5 days leading up to the eruption. In this period, the coronal structure evolves from a weakly to a highly sheared arcade and then to a sigmoid that crosses the inversion line in the inverse direction. These properties suggest that a flux rope has formed prior to the eruption. The amount of cancellation implies that up to 60% of the active region flux could be in the body of the flux rope. We point out that only part of the cancellation contributes to the flux in the rope if the arcade is only weakly sheared, as in the first part of the evolution. This reduces the estimated flux in the rope to similar to 30% or less of the active region flux. We suggest that the remaining discrepancy between our estimate and the limiting value of similar to 10% of the active region flux, obtained previously by the flux rope insertion method, results from the incomplete coherence of the flux rope, due to nonuniform cancellation along the polarity inversion line. A hot linear feature is observed in the active region which rises as part of the eruption and then likely traces out the field lines close to the axis of the flux rope. The flux cancellation and changing magnetic connections at one end of this feature suggest that the flux rope reaches coherence by reconnection immediately before and early in the impulsive phase of the associated flare. The sigmoid is destroyed in the eruption but reforms quickly, with the amount of cancellation involved being much smaller than in the course of its original formation. KW - Sun: activity KW - Sun: coronal mass ejections (CMEs) KW - magnetic fields KW - magnetic reconnection KW - Sun: photosphere KW - Sun: magnetic topology Y1 - 2011 U6 - https://doi.org/10.1051/0004-6361/201015146 SN - 0004-6361 VL - 526 IS - 2 PB - EDP Sciences CY - Les Ulis ER - TY - JOUR A1 - Schuh, Christian A1 - Lomadze, Nino A1 - Rühe, Jürgen A1 - Kopyshev, Alexey A1 - Santer, Svetlana T1 - Photomechanical degrafting of Azo-functionalized Poly(methacrylic acid) (PMAA) brushes JF - The journal of physical chemistry : B, Condensed matter, materials, surfaces, interfaces & biophysical chemistry N2 - We report on the preparation and characterization of photosensitive polymer brushes. The brushes are synthesized through polymer analogous attachment of azobenzene groups to surface-attached poly(methacrylic acid) (PMAA) chains. The topography of the photosensitive brushes shows a strong reaction upon irradiation with UV light. While homogeneous illumination leaves the polymer topography unchanged, irradiation of the samples with interference patterns with periodically varying light intensity leads to the formation of surface relief gratings (SRG). The height of the stripes of the grating can be controlled by adjusting the irradiation time. The SRG pattern can be erased through solvent treatment when the periodicity of the stripe pattern is less than the length of the fully stretched polymer chains. In the opposite case, photomechanical scission of receding polymer chains is observed during SRG formation, and the inscribed patterns are permanent. Y1 - 2011 U6 - https://doi.org/10.1021/jp2041229 SN - 1520-6106 VL - 115 IS - 35 SP - 10431 EP - 10438 PB - American Chemical Society CY - Washington ER - TY - JOUR A1 - Kniepert, Juliane A1 - Schubert, Marcel A1 - Blakesley, James C. A1 - Neher, Dieter T1 - Photogeneration and recombination in P3HT/PCBM solar cells probed by time-delayed collection field experiments JF - The journal of physical chemistry letters N2 - Time-delayed collection field (TDCF) experiments are performed on bulk heterojunction solar cells comprised of a blend of poly(3-hexylthiophene) and [6,6]-phenyl C-71 butyric acid methyl ester. TDCF is analogous to a pump-probe experiment using optical excitation and an electrical probe with a resolution of < 100 ns. The number of free charge carriers extracted after a short delay is found to be independent of the electric field during illumination. Also, experiments performed with a variable delay between the optical excitation and the electrical probe do not reveal any evidence for the generation of charge via field-assisted dissociation of bound long-lived polaron pairs. Photocurrent transients are well fitted by computational drift diffusion simulations with only direct generation of free charge carriers. With increasing delay times between pump and probe, two loss mechanisms are identified; first, charge-carriers are swept out of the device by the internal electric field, and second, bimolecular recombination of the remaining carriers takes place with a reduced recombination coefficient. Y1 - 2011 U6 - https://doi.org/10.1021/jz200155b SN - 1948-7185 VL - 2 IS - 7 SP - 700 EP - 705 PB - American Chemical Society CY - Washington ER - TY - JOUR A1 - Schmidt, Hans-Jürgen T1 - Perihelion advance for orbits with large eccentricities in the Schwarzschild black hole JF - Physical review : D, Particles, fields, gravitation, and cosmology N2 - We deduce a new formula for the perihelion advance Theta of a test particle in the Schwarzschild black hole by applying a newly developed nonlinear transformation within the Schwarzschild space-time. By this transformation we are able to apply the well-known formula valid in the weak-field approximation near infinity also to trajectories in the strong-field regime near the horizon of the black hole. The resulting formula has the structure Theta = c(1) - c(2) ln(c(3)(2) - e(2)) with positive constants c(1,2,3) depending on the angular momentum of the test particle. It is especially useful for orbits with large eccentricities e < c(3) < 1 showing that Theta -> infinity as e -> c(3). Y1 - 2011 U6 - https://doi.org/10.1103/PhysRevD.83.124010 SN - 1550-7998 VL - 83 IS - 12 PB - American Physical Society CY - College Park ER - TY - GEN A1 - Qiu, Xunlin T1 - Patterned piezo-, pyro-, and ferroelectricity of poled polymer electrets T2 - Journal of applied physics Y1 - 2011 U6 - https://doi.org/10.1063/1.3638069 SN - 0021-8979 VL - 110 IS - 5 PB - American Institute of Physics CY - Melville ER - TY - JOUR A1 - Straube, Arthur V. A1 - Pikovskij, Arkadij T1 - Pattern formation induced by time-dependent advection JF - Mathematical modelling of natural phenomena N2 - We study pattern-forming instabilities in reaction-advection-diffusion systems. We develop an approach based on Lyapunov-Bloch exponents to figure out the impact of a spatially periodic mixing flow on the stability of a spatially homogeneous state. We deal with the flows periodic in space that may have arbitrary time dependence. We propose a discrete in time model, where reaction, advection, and diffusion act as successive operators, and show that a mixing advection can lead to a pattern-forming instability in a two-component system where only one of the species is advected. Physically, this can be explained as crossing a threshold of Turing instability due to effective increase of one of the diffusion constants. KW - pattern formation KW - reaction-advection-diffusion equation Y1 - 2011 U6 - https://doi.org/10.1051/mmnp/20116107 SN - 0973-5348 VL - 6 IS - 1 SP - 138 EP - 148 PB - EDP Sciences CY - Les Ulis ER - TY - JOUR A1 - Pohl, Martin A1 - Eichler, David T1 - Origin of ultra-high-energy galactic cosmic rays the isotropy problem JF - The astrophysical journal : an international review of spectroscopy and astronomical physics N2 - We study the propagation of ultra-high-energy cosmic rays (UHECRs) in the Galaxy, concentrating on the energy range below the ankle in the spectrum at 4 EeV. A Monte Carlo method, based on analytical solutions to the time-dependent diffusion problem, is used to account for intermittency by placing sources at random locations. Assuming a source population that scales with baryon mass density or star formation (e.g., long GRB), we derive constraints arising from intermittency and the observational limits on the composition and anisotropy. It is shown that the composition and anisotropy at 10(18) eV are difficult to reproduce and require that either (1) the particle mean free path is much smaller than a gyroradius, implying the escape time is very long, (2) the composition is heavier than suggested by recent Auger data, (3) the ultra-high-energy sub-ankle component is mostly extragalactic, or (4) we are living in a rare lull in the UHECR production, and the current UHECR intensity is far below the Galactic time average. We therefore recommend a strong observational focus on determining the UHECR composition around 10(18) eV. KW - cosmic rays KW - gamma-ray burst: general Y1 - 2011 U6 - https://doi.org/10.1088/0004-637X/742/2/114 SN - 0004-637X VL - 742 IS - 2 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Ilnytskyi, Jaroslav M. A1 - Neher, Dieter A1 - Saphiannikova, Marina T1 - Opposite photo-induced deformations in azobenzene-containing polymers with different molecular architecture molecular dynamics study JF - The journal of chemical physics : bridges a gap between journals of physics and journals of chemistr N2 - Photo-induced deformations in azobenzene-containing polymers (azo-polymers) are central to a number of applications, such as optical storage and fabrication of diffractive elements. The microscopic nature of the underlying opto-mechanical coupling is yet not clear. In this study, we address the experimental finding that the scenario of the effects depends on molecular architecture of the used azo-polymer. Typically, opposite deformations in respect to the direction of light polarization are observed for liquid crystalline and amorphous azo-polymers. In this study, we undertake molecular dynamics simulations of two different models that mimic these two types of azo-polymers. We employ hybrid force field modeling and consider only trans-isomers of azobenzene, represented as Gay-Berne sites. The effect of illumination on the orientation of the chromophores is considered on the level of orientational hole burning and emphasis is given to the resulting deformation of the polymer matrix. We reproduce deformations of opposite sign for the two models being considered here and discuss the relevant microscopic mechanisms in both cases. KW - amorphous state KW - light polarisation KW - liquid crystal polymers KW - molecular dynamics method KW - optical hole burning KW - photochemistry Y1 - 2011 U6 - https://doi.org/10.1063/1.3614499 SN - 0021-9606 VL - 135 IS - 4 PB - American Institute of Physics CY - Melville ER - TY - JOUR A1 - Abdo, A. A. A1 - Ackermann, Margit A1 - Ajello, M. A1 - Allafort, A. J. A1 - Baldini, L. A1 - Ballet, J. A1 - Barbiellini, G. A1 - Baring, M. G. A1 - Bastieri, D. A1 - Bellazzini, R. A1 - Berenji, B. A1 - Blandford, R. D. A1 - Bloom, E. D. A1 - Bonamente, E. A1 - Borgland, A. W. A1 - Bouvier, A. A1 - Brandt, T. J. A1 - Bregeon, Johan A1 - Brigida, M. A1 - Bruel, P. A1 - Buehler, R. A1 - Buson, S. A1 - Caliandro, G. A. A1 - Cameron, R. A. A1 - Caraveo, P. A. A1 - Casandjian, J. M. A1 - Cecchi, C. A1 - Chaty, S. A1 - Chekhtman, A. A1 - Cheung, C. C. A1 - Chiang, J. A1 - Cillis, A. N. A1 - Ciprini, S. A1 - Claus, R. A1 - Cohen-Tanugi, J. A1 - Conrad, Jan A1 - Corbel, S. A1 - Cutini, S. A1 - de Angelis, A. A1 - de Palma, F. A1 - Dermer, C. D. A1 - Digel, S. W. A1 - do Couto e Silva, E. A1 - Drell, P. S. A1 - Drlica-Wagner, A. A1 - Dubois, R. A1 - Dumora, D. A1 - Favuzzi, C. A1 - Ferrara, E. C. A1 - Fortin, P. A1 - Frailis, M. A1 - Fukazawa, Y. A1 - Fukui, Y. A1 - Funk, S. A1 - Fusco, P. A1 - Gargano, F. A1 - Gasparrini, D. A1 - Gehrels, N. A1 - Germani, S. A1 - Giglietto, N. A1 - Giordano, F. A1 - Giroletti, M. A1 - Glanzman, T. A1 - Godfrey, G. A1 - Grenier, I. A. A1 - Grondin, M. -H. A1 - Guiriec, S. A1 - Hadasch, D. A1 - Hanabata, Y. A1 - Harding, A. K. A1 - Hayashida, M. A1 - Hayashi, K. A1 - Hays, E. A1 - Horan, D. A1 - Jackson, M. S. A1 - Johannesson, G. A1 - Johnson, A. S. A1 - Kamae, T. A1 - Katagiri, H. A1 - Kataoka, J. A1 - Kerr, M. A1 - Knoedlseder, J. A1 - Kuss, M. A1 - Lande, J. A1 - Latronico, L. A1 - Lee, S. -H. A1 - Lemoine-Goumard, M. A1 - Longo, F. A1 - Loparco, F. A1 - Lovellette, M. N. A1 - Lubrano, P. A1 - Madejski, G. M. A1 - Makeev, A. A1 - Mazziotta, Mario Nicola A1 - McEnery, J. E. A1 - Michelson, P. F. A1 - Mignani, R. P. A1 - Mitthumsiri, W. A1 - Mizuno, T. A1 - Moiseev, A. A. A1 - Monte, C. A1 - Monzani, M. E. A1 - Morselli, A. A1 - Moskalenko, I. V. A1 - Murgia, S. A1 - Naumann-Godo, M. A1 - Nolan, P. L. A1 - Norris, J. P. A1 - Nuss, E. A1 - Ohsugi, T. A1 - Okumura, A. A1 - Orlando, E. A1 - Ormes, J. F. A1 - Paneque, D. A1 - Parent, D. A1 - Pelassa, V. A1 - Pesce-Rollins, M. A1 - Pierbattista, M. A1 - Piron, F. A1 - Pohl, Martin A1 - Porter, T. A. A1 - Raino, S. A1 - Rando, R. A1 - Razzano, M. A1 - Reimer, O. A1 - Reposeur, T. A1 - Ritz, S. A1 - Romani, R. W. A1 - Roth, M. A1 - Sadrozinski, H. F. -W. A1 - Parkinson, P. M. Saz A1 - Sgro, C. A1 - Smith, D. A. A1 - Smith, P. D. A1 - Spandre, G. A1 - Spinelli, P. A1 - Strickman, M. S. A1 - Tajima, H. A1 - Takahashi, H. A1 - Takahashi, T. A1 - Tanaka, T. A1 - Thayer, J. G. A1 - Thayer, J. B. A1 - Thompson, D. J. A1 - Tibaldo, L. A1 - Tibolla, O. A1 - Torres, D. F. A1 - Tosti, G. A1 - Tramacere, A. A1 - Troja, E. A1 - Uchiyama, Y. A1 - Vandenbroucke, J. A1 - Vasileiou, V. A1 - Vianello, G. A1 - Vilchez, N. A1 - Vitale, V. A1 - Waite, A. P. A1 - Wang, P. A1 - Winer, B. L. A1 - Wood, K. S. A1 - Yamamoto, H. A1 - Yamazaki, R. A1 - Yang, Z. A1 - Ziegler, M. T1 - Observations of the young supernova remnant RX J1713.7-3946 with the fermi large area telescope JF - The astrophysical journal : an international review of spectroscopy and astronomical physics N2 - We present observations of the young supernova remnant (SNR) RX J1713.7-3946 with the Fermi Large Area Telescope (LAT). We clearly detect a source positionally coincident with the SNR. The source is extended with a best-fit extension of 0 degrees.55 +/- 0 degrees.04 matching the size of the non-thermal X-ray and TeV gamma-ray emission from the remnant. The positional coincidence and the matching extended emission allow us to identify the LAT source with SNR RX J1713.7-3946. The spectrum of the source can be described by a very hard power law with a photon index of Gamma = 1.5 +/- 0.1 that coincides in normalization with the steeper H. E. S. S.-detected gamma-ray spectrum at higher energies. The broadband gamma-ray emission is consistent with a leptonic origin as the dominant mechanism for the gamma-ray emission. KW - acceleration of particles KW - gamma rays: general KW - gamma rays: ISM KW - ISM: individual objects (RX J1713.7-3946) KW - ISM: supernova remnants KW - radiation mechanisms: non-thermal Y1 - 2011 U6 - https://doi.org/10.1088/0004-637X/734/1/28 SN - 0004-637X VL - 734 IS - 1 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Donges, Jonathan A1 - Donner, Reik Volker A1 - Trauth, Martin H. A1 - Marwan, Norbert A1 - Schellnhuber, Hans Joachim A1 - Kurths, Jürgen T1 - Nonlinear detection of paleoclimate-variability transitions possibly related to human evolution JF - Proceedings of the National Academy of Sciences of the United States of America N2 - Potential paleoclimatic driving mechanisms acting on human evolution present an open problem of cross-disciplinary scientific interest. The analysis of paleoclimate archives encoding the environmental variability in East Africa during the past 5 Ma has triggered an ongoing debate about possible candidate processes and evolutionary mechanisms. In this work, we apply a nonlinear statistical technique, recurrence network analysis, to three distinct marine records of terrigenous dust flux. Our method enables us to identify three epochs with transitions between qualitatively different types of environmental variability in North and East Africa during the (i) Middle Pliocene (3.35-3.15 Ma B. P.), (ii) Early Pleistocene (2.25-1.6 Ma B. P.), and (iii) Middle Pleistocene (1.1-0.7 Ma B. P.). A deeper examination of these transition periods reveals potential climatic drivers, including (i) large-scale changes in ocean currents due to a spatial shift of the Indonesian throughflow in combination with an intensification of Northern Hemisphere glaciation, (ii) a global reorganization of the atmospheric Walker circulation induced in the tropical Pacific and Indian Ocean, and (iii) shifts in the dominating temporal variability pattern of glacial activity during the Middle Pleistocene, respectively. A reexamination of the available fossil record demonstrates statistically significant coincidences between the detected transition periods and major steps in hominin evolution. This result suggests that the observed shifts between more regular and more erratic environmental variability may have acted as a trigger for rapid change in the development of humankind in Africa. KW - African climate KW - Plio-Pleistocene KW - climate-driven evolution KW - dynamical transitions KW - nonlinear time series analysis Y1 - 2011 U6 - https://doi.org/10.1073/pnas.1117052108 SN - 0027-8424 VL - 108 IS - 51 SP - 20422 EP - 20427 PB - National Acad. of Sciences CY - Washington ER - TY - JOUR A1 - Prosen, Tomaz A1 - Ilievski, Enej T1 - Nonequilibrium phase transition in a periodically driven XY spin chain JF - Physical review letters N2 - We present a general formulation of Floquet states of periodically time-dependent open Markovian quasifree fermionic many-body systems in terms of a discrete Lyapunov equation. Illustrating the technique, we analyze periodically kicked XY spin-1/2 chain which is coupled to a pair of Lindblad reservoirs at its ends. A complex phase diagram is reported with reentrant phases of long range and exponentially decaying spin-spin correlations as some of the system's parameters are varied. The structure of phase diagram is reproduced in terms of counting nontrivial stationary points of Floquet quasiparticle dispersion relation. Y1 - 2011 U6 - https://doi.org/10.1103/PhysRevLett.107.060403 SN - 0031-9007 VL - 107 IS - 6 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Hoban, Matty J. A1 - Campbell, Earl T. A1 - Loukopoulos, Klearchos A1 - Browne, Dan E. T1 - Non-adaptive measurement-based quantum computation and multi-party Bell inequalities JF - New journal of physics : the open-access journal for physics N2 - Quantum correlations exhibit behaviour that cannot be resolved with a local hidden variable picture of the world. In quantum information, they are also used as resources for information processing tasks, such as measurement-based quantum computation (MQC). In MQC, universal quantum computation can be achieved via adaptive measurements on a suitable entangled resource state. In this paper, we look at a version of MQC in which we remove the adaptivity of measurements and aim to understand what computational abilities remain in the resource. We show that there are explicit connections between this model of computation and the question of non-classicality in quantum correlations. We demonstrate this by focusing on deterministic computation of Boolean functions, in which natural generalizations of the Greenberger-Horne-Zeilinger paradox emerge; we then explore probabilistic computation via, which multipartite Bell inequalities can be defined. We use this correspondence to define families of multi-party Bell inequalities, which we show to have a number of interesting contrasting properties. Y1 - 2011 U6 - https://doi.org/10.1088/1367-2630/13/2/023014 SN - 1367-2630 VL - 13 IS - 1 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Lisso, Janina A1 - Schröder, Florian A1 - Fisahn, Joachim A1 - Muessig, Carsten T1 - NFX1-LIKE2 (NFXL2) Suppresses Abscisic Acid Accumulation and Stomatal Closure in Arabidopsis thaliana JF - PLoS one N2 - The NFX1-LIKE1 (NFXL1) and NFXL2 genes were identified as regulators of salt stress responses. The NFXL1 protein is a nuclear factor that positively affects adaptation to salt stress. The nfxl1-1 loss-of-function mutant displayed reduced survival rates under salt and high light stress. In contrast, the nfxl2-1 mutant, defective in the NFXL2 gene, and NFXL2-antisense plants exhibited enhanced survival under these conditions. We show here that the loss of NFXL2 function results in abscisic acid (ABA) overaccumulation, reduced stomatal conductance, and enhanced survival under drought stress. The nfxl2-1 mutant displayed reduced stomatal aperture under all conditions tested. Fusicoccin treatment, exposition to increasing light intensities, and supply of decreasing CO2 concentrations demonstrated full opening capacity of nfxl2-1 stomata. Reduced stomatal opening presumably is a consequence of elevated ABA levels. Furthermore, seedling growth, root growth, and stomatal closure were hypersensitive to exogenous ABA. The enhanced ABA responses may contribute to the improved drought stress resistance of the mutant. Three NFXL2 splice variants were cloned and named NFXL2-78, NFXL2-97, and NFXL2-100 according to the molecular weight of the putative proteins. Translational fusions to the green fluorescent protein suggest nuclear localisation of the NFXL2 proteins. Stable expression of the NFXL2-78 splice variant in nfxl2-1 plants largely complemented the mutant phenotype. Our data show that NFXL2 controls ABA levels and suppresses ABA responses. NFXL2 may prevent unnecessary and costly stress adaptation under favourable conditions. Y1 - 2011 U6 - https://doi.org/10.1371/journal.pone.0026982 SN - 1932-6203 VL - 6 IS - 11 PB - PLoS CY - San Fransisco ER - TY - JOUR A1 - Levnajic, Zoran A1 - Pikovskij, Arkadij T1 - Network reconstruction from random phase resetting JF - Physical review letters N2 - We propose a novel method of reconstructing the topology and interaction functions for a general oscillator network. An ensemble of initial phases and the corresponding instantaneous frequencies is constructed by repeating random phase resets of the system dynamics. The desired details of network structure are then revealed by appropriately averaging over the ensemble. The method is applicable for a wide class of networks with arbitrary emergent dynamics, including full synchrony. Y1 - 2011 U6 - https://doi.org/10.1103/PhysRevLett.107.034101 SN - 0031-9007 VL - 107 IS - 3 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Shayduk, Roman A1 - Navirian, Hengameh A1 - Leitenberger, Wolfram A1 - Goldshteyn, Jevgenij A1 - Vrejoiu, Ionela A1 - Weinelt, Martin A1 - Gaal, Peter A1 - Herzog, Marc A1 - von Korff Schmising, Clemens A1 - Bargheer, Matias T1 - Nanoscale heat transport studied by high-resolution time-resolved x-ray diffraction JF - New journal of physics : the open-access journal for physics N2 - We report on synchrotron-based high-repetition rate ultrafast x-ray diffraction (UXRD) experiments monitoring the transport of heat from an epitaxial La(0.7)Sr(0.3)MnO(3)/SrTiO(3) superlattice (SL) into the substrate on timescales from 100 ps to 4 mu s. Transient thermal lattice expansion was determined with an accuracy of 10(-7), corresponding to a sensitivity to temperature changes down to 0.01 K. We follow the heat flow within the SL and into the substrate after the impulsive laser heating leads to a small temperature rise of Delta T = 6 K. The transient lattice temperature can be simulated very well using the bulk heat conductivities. This contradicts the interpretation of previous UXRD measurements, which predicted a long-lasting expansion of SrRuO(3) for more than 200 ps. The disagreement could be resolved by assuming that the heat conductivity changes in the first hundred picoseconds. Y1 - 2011 U6 - https://doi.org/10.1088/1367-2630/13/9/093032 SN - 1367-2630 VL - 13 IS - 11 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Aliu, E. A1 - Aune, T. A1 - Beilicke, M. A1 - Benbow, W. A1 - Boettcher, Markus A1 - Bouvier, A. A1 - Bradbury, S. M. A1 - Buckley, J. H. A1 - Bugaev, V. A1 - Cannon, A. A1 - Cesarini, A. A1 - Ciupik, L. A1 - Connolly, M. P. A1 - Cui, W. A1 - Decerprit, G. A1 - Dickherber, R. A1 - Duke, C. A1 - Errando, M. A1 - Falcone, A. A1 - Feng, Q. A1 - Finnegan, G. A1 - Fortson, L. A1 - Furniss, A. A1 - Galante, N. A1 - Gall, D. A1 - Gillanders, G. H. A1 - Godambe, S. A1 - Griffin, S. A1 - Grube, J. A1 - Gyuk, G. A1 - Hanna, D. A1 - Hivick, B. A1 - Holder, J. A1 - Huan, H. A1 - Hughes, G. A1 - Hui, C. M. A1 - Humensky, T. B. A1 - Kaaret, P. A1 - Karlsson, N. A1 - Kertzman, M. A1 - Kieda, D. A1 - Krawczynski, H. A1 - Krennrich, F. A1 - Maier, G. A1 - Majumdar, P. A1 - McArthur, S. A1 - McCann, A. A1 - Moriarty, P. A1 - Mukherjee, R. A1 - Nelson, T. A1 - Ong, R. A. A1 - Orr, M. A1 - Otte, A. N. A1 - Park, N. A1 - Perkins, J. S. A1 - Pichel, A. A1 - Pohl, Martin A1 - Prokoph, H. A1 - Quinn, J. A1 - Ragan, K. A1 - Reyes, L. C. A1 - Reynolds, P. T. A1 - Roache, E. A1 - Rose, H. J. A1 - Ruppel, J. A1 - Saxon, D. B. A1 - Sembroski, G. H. A1 - Skole, C. A1 - Smith, A. W. A1 - Staszak, D. A1 - Tesic, G. A1 - Theiling, M. A1 - Thibadeau, S. A1 - Tsurusaki, K. A1 - Tyler, J. A1 - Varlotta, A. A1 - Vassiliev, V. V. A1 - Wakely, S. P. A1 - Weekes, T. C. A1 - Weinstein, A. A1 - Williams, D. A. A1 - Zitzer, B. A1 - Ciprini, S. A1 - Fumagalli, M. A1 - Kaplan, K. A1 - Paneque, D. A1 - Prochaska, J. X. T1 - Multiwavelenght observations of the previously unidentified blzar RX J0648.7+1516 JF - The astrophysical journal : an international review of spectroscopy and astronomical physics N2 - We report on the VERITAS discovery of very high energy (VHE) gamma-ray emission above 200 GeV from the high-frequency-peaked BL Lac (HBL) object RX J0648.7+1516 (GB J0648+1516), associated with 1FGL J0648.8+1516. The photon spectrum above 200 GeV is fitted by a power law dN/dE = F-0(E/E-0)(-Gamma) with a photon index Gamma of 4.4 +/- 0.8(stat) +/- 0.3(syst) and a flux normalization F-0 of (2.3 +/- 0.5(stat) +/- 1.2(sys)) x 10(-11) TeV-1 cm(-2) s(-1) with E-0 = 300 GeV. No VHE variability is detected during VERITAS observations of RX J0648.7+1516 between 2010 March 4 and April 15. Following the VHE discovery, the optical identification and spectroscopic redshift were obtained using the Shane 3 m Telescope at the Lick Observatory, showing the unidentified object to be a BL Lac type with a redshift of z = 0.179. Broadband multiwavelength observations contemporaneous with the VERITAS exposure period can be used to subclassify the blazar as an HBL object, including data from the MDM observatory, Swift-UVOT, and X-Ray Telescope, and continuous monitoring at photon energies above 1 GeV from the Fermi Large Area Telescope (LAT). We find that in the absence of undetected, high-energy rapid variability, the one-zone synchrotron self-Compton (SSC) model overproduces the high-energy gamma-ray emission measured by the Fermi-LAT over 2.3 years. The spectral energy distribution can be parameterized satisfactorily with an external-Compton or lepto-hadronic model, which have two and six additional free parameters, respectively, compared to the one-zone SSC model. KW - BL Lacertae objects: individual (RX J0648.7+1516, 1FGL J0648.8+1516, VER J0648+152) KW - gamma rays: galaxies Y1 - 2011 U6 - https://doi.org/10.1088/0004-637X/742/2/127 SN - 0004-637X VL - 742 IS - 2 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Kofod, Guggi A1 - Stoyanov, Hristiyan A1 - Gerhard, Reimund T1 - Multilayer coaxial fiber dielectric elastomers for actuation and sensing JF - Applied physics : A, Materials science & processing N2 - A simple dip-coating technique was employed to manufacture coaxial actuators with multiple layers of alternating dielectric and conducting layers. A thin rubber string was coated with an electrode-insulator-electrode structure, giving rise to a thin, fiber-like actuator with coaxial geometry. The process was repeated to achieve a compact multilayer actuator with up to three coaxial dielectric layers. Mechanical and electromechanical characterization of the actuators is presented, showing actuation strains up to 8% and proper voltage-thickness scaling behavior. Also presented is a capacitance vs. extension plot, demonstrating that these structures can be used for compact and accurate capacitive strain sensing. Y1 - 2011 U6 - https://doi.org/10.1007/s00339-010-6066-5 SN - 0947-8396 SN - 1432-0630 VL - 102 IS - 3 SP - 577 EP - 581 PB - Springer CY - New York ER - TY - JOUR A1 - Gerhardt, Matthias A1 - Groeger, Gillian A1 - MacCarthy, Niall T1 - Monopolar vs. bipolar subretinal stimulation-An in vitro study JF - Journal of neuroscience methods N2 - This study uses an in vitro rd10 mouse model to quantify and compare the ability of the monopolar and the (concentric) bipolar electrode configurations for subretinal stimulation. To allow for results which can be directly compared an identical region of the retina was stimulated due to the circumstance that the bipolar electrode configuration allows also for monopolar stimulation, if the concentric counter-electrode is set potential-free (floating). A ganglion cell, located centrally over the bipolar electrode configuration was selected to extracellularly record action potentials during stimulation. To analyse the recorded action potentials, we introduce a new method which combines the advantages of (a) singular value decomposition (SVD) for weighting similar modulation patterns with which the recorded action potentials are characterized and (b) multi curve fitting to identify a common threshold level, required to finally assemble a strength-duration relationship (SDR). By directly comparing the obtained SDR curves, we found that the efficiency of stimulation with the monopolar electrode configuration is significantly higher than with the bipolar electrode configuration. All obtained SDR curves were fitted using the Lapicque model to estimate the chronaxie times and the rheobase currents. Liquid inclusions, eventually separating the retina from the electrodes are discussed to be a major cause for low ganglion cell responses during stimulation with the bipolar electrode configuration. KW - SVD KW - Subretinal KW - Electrodes KW - Monopolar KW - Bipolar KW - Retina KW - Ganglion KW - Cells Y1 - 2011 U6 - https://doi.org/10.1016/j.jneumeth.2011.04.017 SN - 0165-0270 VL - 199 IS - 1 SP - 26 EP - 34 PB - Elsevier CY - Amsterdam ER - TY - JOUR A1 - Malic, E. A1 - Weber, C. A1 - Richter, M. A1 - Atalla, V. A1 - Klamroth, Tillmann A1 - Saalfrank, Peter A1 - Reich, Sebastian A1 - Knorr, A. T1 - Microscopic model of the optical absorption of carbon nanotubes functionalized with molecular spiropyran photoswitches JF - Physical review letters N2 - The adsorption of molecules to the surface of carbon nanostructures opens a new field of hybrid systems with distinct and controllable properties. We present a microscopic study of the optical absorption in carbon nanotubes functionalized with molecular spiropyran photoswitches. The switching process induces a change in the dipole moment leading to a significant coupling to the charge carriers in the nanotube. As a result, the absorption spectra of functionalized tubes reveal a considerable redshift of transition energies depending on the switching state of the spiropyran molecule. Our results suggest that carbon nanotubes are excellent substrates for the optical readout of spiropyran-based molecular switches. The gained insights can be applied to other noncovalently functionalized one-dimensional nanostructures in an externally induced dipole field. Y1 - 2011 U6 - https://doi.org/10.1103/PhysRevLett.106.097401 SN - 0031-9007 VL - 106 IS - 9 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Beta, Carsten A1 - Bodenschatz, Eberhard T1 - Microfluidic tools for quantitative studies of eukaryotic chemotaxis JF - European journal of cell biology N2 - Over the past decade, microfluidic techniques have been established as a versatile platform to perform live cell experiments under well-controlled conditions. To investigate the directional responses of cells, stable concentration profiles of chemotactic factors can be generated in microfluidic gradient mixers that provide a high degree of spatial control. However, the times for built-up and switching of gradient profiles are in general too slow to resolve the intracellular protein translocation events of directional sensing of eukaryotes. Here, we review an example of a conventional microfluidic gradient mixer as well as the novel flow photolysis technique that achieves an increased temporal resolution by combining the photo-activation of caged compounds with the advantages of microfluidic chambers. KW - Eukaryotic chemotaxis KW - Dictyostelium discoideum KW - Microfluidics KW - Caged compounds KW - Numerical simulations Y1 - 2011 U6 - https://doi.org/10.1016/j.ejcb.2011.05.006 SN - 0171-9335 VL - 90 IS - 10 SP - 811 EP - 816 PB - Elsevier CY - Jena ER - TY - JOUR A1 - Khader, Patrick H. A1 - Pachur, Thorsten A1 - Meier, Stefanie A1 - Bien, Siegfried A1 - Jost, Kerstin A1 - Roesler, Frank T1 - Memory-based decision-making with heuristics evidence for a controlled activation of memory representations JF - Journal of cognitive neuroscience N2 - Many of our daily decisions are memory based, that is, the attribute information about the decision alternatives has to be recalled. Behavioral studies suggest that for such decisions we often use simple strategies (heuristics) that rely on controlled and limited information search. It is assumed that these heuristics simplify decision-making by activating long-term memory representations of only those attributes that are necessary for the decision. However, from behavioral studies alone, it is unclear whether using heuristics is indeed associated with limited memory search. The present study tested this assumption by monitoring the activation of specific long-term-memory representations with fMRI while participants made memory-based decisions using the "take-the-best" heuristic. For different decision trials, different numbers and types of information had to be retrieved and processed. The attributes consisted of visual information known to be represented in different parts of the posterior cortex. We found that the amount of information required for a decision was mirrored by a parametric activation of the dorsolateral PFC. Such a parametric pattern was also observed in all posterior areas, suggesting that activation was not limited to those attributes required for a decision. However, the posterior increases were systematically modulated by the relative importance of the information for making a decision. These findings suggest that memory-based decision-making is mediated by the dorsolateral PFC, which selectively controls posterior storage areas. In addition, the systematic modulations of the posterior activations indicate a selective boosting of activation of decision-relevant attributes. Y1 - 2011 SN - 0898-929X VL - 23 IS - 11 SP - 3540 EP - 3554 PB - MIT Press CY - Cambridge ER - TY - JOUR A1 - Mizuno, Yosuke A1 - Pohl, Martin A1 - Niemiec, Jacek A1 - Zhang, Bing A1 - Nishikawa, Ken-Ichi A1 - Hardee, Philip E. T1 - Magnetic-field amplification by turbulence in a relativistic shockpropagating through an inhomogeneous medium JF - The astrophysical journal : an international review of spectroscopy and astronomical physics N2 - We perform two-dimensional relativistic magnetohydrodynamic simulations of a mildly relativistic shock propagating through an inhomogeneous medium. We show that the postshock region becomes turbulent owing to preshock density inhomogeneity, and the magnetic field is strongly amplified due to the stretching and folding of field lines in the turbulent velocity field. The amplified magnetic field evolves into a filamentary structure in two-dimensional simulations. The magnetic energy spectrum is flatter than the Kolmogorov spectrum and indicates that a so-called small-scale dynamo is occurring in the postshock region. We also find that the amount of magnetic-field amplification depends on the direction of the mean preshock magnetic field, and the timescale of magnetic-field growth depends on the shock strength. KW - gamma-ray burst: general KW - magnetohydrodynamics (MHD) KW - methods: numerical KW - relativistic processes KW - shock waves KW - turbulence Y1 - 2011 U6 - https://doi.org/10.1088/0004-637X/726/2/62 SN - 0004-637X VL - 726 IS - 2 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Schoeller, M. A1 - Hubrig, Swetlana A1 - Ilyin, Ilya A1 - Kharchenko, N. V. A1 - Briquet, Maryline A1 - Gonzalez, J. F. A1 - Langer, Norbert A1 - Oskinova, Lida T1 - Magnetic field studies of massive main sequence stars JF - Astronomische Nachrichten = Astronomical notes N2 - We report on the status of our spectropolarimetric observations of massive stars. During the last years, we have discovered magnetic fields in many objects of the upper main sequence, including Be stars, beta Cephei and Slowly Pulsating B stars, and a dozen O stars. Since the effects of those magnetic fields have been found to be substantial by recent models, we are looking into their impact on stellar rotation, pulsation, stellar winds, and chemical abundances. Accurate studies of the age, environment, and kinematic characteristics of the magnetic stars are also promising to give us new insight into the origin of the magnetic fields. Furthermore, longer time series of magnetic field measurements allow us to observe the temporal variability of the magnetic field and to deduce the stellar rotation period and the magnetic field geometry. Studies of the magnetic field in massive stars are indispensable to understand the conditions controlling the presence of those fields and their implications on the stellar physical parameters and evolution. KW - stars: early-type KW - stars: magnetic fields KW - stars: kinematics KW - techniques: polarimetric Y1 - 2011 U6 - https://doi.org/10.1002/asna.201111606 SN - 0004-6337 VL - 332 IS - 9-10 SP - 994 EP - 997 PB - Wiley-Blackwell CY - Malden ER - TY - JOUR A1 - Schmah, Tanya A1 - Marwan, Norbert A1 - Thomsen, Jesper Skovhus A1 - Saparin, Peter T1 - Long range node-strut analysis of trabecular bone microarchitecture JF - Medical physics : the international journal of medical physics research and practice N2 - Purpose: We present a new morphometric measure of trabecular bone microarchitecture, called mean node strength (NdStr), which is part of a newly developed approach called long range nodestrut analysis. Our general aim is to describe and quantify the apparent "latticelike" microarchitecture of the trabecular bone network. Methods: Similar in some ways to the topological node-strut analysis introduced by Garrahan et al. [J. Microsc. 142, 341-349 (1986)], our method is distinguished by an emphasis on long-range trabecular connectivity. Thus, while the topological classification of a pixel (after skeletonization) as a node, strut, or terminus, can be determined from the 3 x 3 neighborhood of that pixel, our method, which does not involve skeletonization, takes into account a much larger neighborhood. In addition, rather than giving a discrete classification of each pixel as a node, strut, or terminus, our method produces a continuous variable, node strength. The node strength is averaged over a region of interest to produce the mean node strength of the region. Results: We have applied our long range node-strut analysis to a set of 26 high-resolution peripheral quantitative computed tomography (pQCT) axial images of human proximal tibiae acquired 17 mm below the tibial plateau. We found that NdStr has a strong positive correlation with trabecular volumetric bone mineral density (BMD). After an exponential transformation, we obtain a Pearson's correlation coefficient of r - 0.97. Qualitative comparison of images with similar BMD but with very different NdStr values suggests that the latter measure has successfully quantified the prevalence of the "latticelike" microarchitecture apparent in the image. Moreover, we found a strong correlation (r - 0.62) between NdStr and the conventional node-terminus ratio (Nd/Tm) of Garrahan et al. The Nd/Tm ratios were computed using traditional histomorphometry performed on bone biopsies obtained at the same location as the pQCT scans. Conclusions: The newly introduced morphometric measure allows a quantitative assessment of the long-range connectivity of trabecular bone. One advantage of this method is that it is based on pQCT images that can be obtained noninvasively from patients, i.e., without having to obtain a bone biopsy from the patient. KW - trabecular bone KW - osteoporosis KW - structure analysis KW - histomorphometry KW - pQCT Y1 - 2011 U6 - https://doi.org/10.1118/1.3622600 SN - 0094-2405 VL - 38 IS - 9 SP - 5003 EP - 5011 PB - American Association of Physicists in Medicine CY - Melville ER - TY - JOUR A1 - Filimon, Marlena A1 - Kopf, Ilona A1 - Schmidt, Dietrich A. A1 - Bruendermann, Erik A1 - Rühe, Jürgen A1 - Santer, Svetlana A1 - Havenith, Martina T1 - Local chemical composition of nanophase-separated polymer brushes JF - Physical chemistry, chemical physics : a journal of European Chemical Societies N2 - Using scattering scanning nearfield infrared microscopy (s-SNIM), we have imaged the nanoscale phase separation of mixed polystyrene-poly(methyl methacrylate) (PS-PMMA) brushes and investigated changes in the top layer as a function of solvent exposure. We deduce that the top-layer of the mixed brushes is composed primarily of PMMA after exposure to acetone, while after exposure to toluene this changes to PS. Access to simultaneously measured topographic and chemical information allows direct correlation of the chemical morphology of the sample with topographic information. Our results demonstrate the potential of s-SNIM for chemical mapping based on distinct infrared absorption properties of polymers with a high spatial resolution of 80 nm x 80 nm. Y1 - 2011 U6 - https://doi.org/10.1039/c0cp02756a SN - 1463-9076 VL - 13 IS - 24 SP - 11620 EP - 11626 PB - Royal Society of Chemistry CY - Cambridge ER - TY - JOUR A1 - Janotta, Peter A1 - Gogolin, Christian A1 - Barrett, Jonathan A1 - Brunner, Nicolas T1 - Limits on nonlocal correlations from the structure of the local state space JF - New journal of physics : the open-access journal for physics N2 - The outcomes of measurements on entangled quantum systems can be nonlocally correlated. However, while it is easy to write down toy theories allowing arbitrary nonlocal correlations, those allowed in quantum mechanics are limited. Quantum correlations cannot, for example, violate a principle known as macroscopic locality, which implies that they cannot violate Tsirelson's bound. This paper shows that there is a connection between the strength of nonlocal correlations in a physical theory and the structure of the state spaces of individual systems. This is illustrated by a family of models in which local state spaces are regular polygons, where a natural analogue of a maximally entangled state of two systems exists. We characterize the nonlocal correlations obtainable from such states. The family allows us to study the transition between classical, quantum and super-quantum correlations by varying only the local state space. We show that the strength of nonlocal correlations-in particular whether the maximally entangled state violates Tsirelson's bound or not-depends crucially on a simple geometric property of the local state space, known as strong self-duality. This result is seen to be a special case of a general theorem, which states that a broad class of entangled states in probabilistic theories-including, by extension, all bipartite classical and quantum states-cannot violate macroscopic locality. Finally, our results show that models exist that are locally almost indistinguishable from quantum mechanics, but can nevertheless generate maximally nonlocal correlations. Y1 - 2011 U6 - https://doi.org/10.1088/1367-2630/13/6/063024 SN - 1367-2630 VL - 13 IS - 23 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Lomadze, Nino A1 - Kopyshev, Alexey A1 - Rühe, Jürgen A1 - Santer, Svetlana T1 - Light-Induced chain scission in photosensitive polymer brushes JF - Macromolecules : a publication of the American Chemical Society N2 - We report on a process inducing photomechanical fracture of chemical bonds in photosensitive PMAA polymer brushes. The photosensitive PMAA polymer brushes were prepared by covalent attachment of azobenzene groups to poly(methylacrylic acid) (PMAA) chains generated by surface-initiated polymerization. While homogeneous irradiation leaves the polymer topography unchanged, the azo-PMAA brushes show a strong response upon irradiation with UV interference patterns. The photoisomerization process in the surface-attached polymer films results in the irreversible formation of surface relief gratings (SRG), which are strongly enhanced upon washing with a good solvent for the polymer. The photomechanical forces during mass transport induced by the irradiation lead to the scission of covalent bounds and accordingly to a degrafting of the polymer chains in areas where the polymer is receding from. It is observed that the number of ruptured chains depends strongly on the amount of azo side chains in the polymer. Y1 - 2011 U6 - https://doi.org/10.1021/ma201016q SN - 0024-9297 VL - 44 IS - 18 SP - 7372 EP - 7377 PB - American Chemical Society CY - Washington ER - TY - JOUR A1 - Valleriani, Angelo A1 - Zhang, Gong A1 - Nagar, Apoorva A1 - Ignatova, Zoya A1 - Lipowsky, Reinhard T1 - Length-dependent translation of messenger RNA by ribosomes JF - Physical review : E, Statistical, nonlinear and soft matter physics N2 - A simple measure for the efficiency of protein synthesis by ribosomes is provided by the steady state amount of protein per messenger RNA (mRNA), the so-called translational ratio, which is proportional to the translation rate. Taking the degradation of mRNA into account, we show theoretically that both the translation rate and the translational ratio decrease with increasing mRNA length, in agreement with available experimental data for the prokaryote Escherichia coli. We also show that, compared to prokaryotes, mRNA degradation in eukaryotes leads to a less rapid decrease of the translational ratio. This finding is consistent with the fact that, compared to prokaryotes, eukaryotes tend to have longer proteins. Y1 - 2011 U6 - https://doi.org/10.1103/PhysRevE.83.042903 SN - 1539-3755 VL - 83 IS - 4 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Floss, Gereon A1 - Klamroth, Tillmann A1 - Saalfrank, Peter T1 - Laser-controlled switching of molecular arrays in an dissipative environment JF - Physical review : B, Condensed matter and materials physics N2 - The optical switching of molecular ensembles in a dissipative environment is a subject of various fields of chemical physics and physical chemistry. Here we try to switch arrays of molecules from a stable collective ground state to a state in which all molecules have been transferred to another stable higher-energy configuration. In our model switching proceeds through electronically excited intermediates which are coherently coupled to each other through dipolar interactions, and which decay incoherently within a finite lifetime by coupling to a dissipative environment. The model is quite general, but parameters are chosen to roughly resemble the all-trans -> all-cis isomerization of an array of azobenzene molecules on a surface. Using analytical and optimal control pulses and the concept of "laser distillation," we demonstrate that for various aggregates (dimers up to hexamers), controlled and complete switching should be possible. Y1 - 2011 U6 - https://doi.org/10.1103/PhysRevB.83.104301 SN - 1098-0121 VL - 83 IS - 10 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Sun, Y. -P. A1 - Hennies, Franz A1 - Pietzsch, Annette A1 - Kennedy, B. A1 - Schmitt, Thorsten A1 - Strocov, Vladimir N. A1 - Andersson, Joakim A1 - Berglund, Martin A1 - Rubensson, Jan-Erik A1 - Aidas, K. A1 - Gel'mukhanov, F. A1 - Odelius, Michael A1 - Föhlisch, Alexander T1 - Intramolecular soft modes and intermolecular interactions in liquid acetone JF - Physical review : B, Condensed matter and materials physics N2 - Resonant inelastic x-ray scattering spectra excited at the O1s(-1)pi* resonance of liquid acetone are presented. Scattering to the electronic ground state shows a resolved vibrational progression where the dominant contribution is due to the C-O stretching mode, thus demonstrating a unique sensitivity of the method to the local potential energy surface in complex molecular systems. For scattering to electronically excited states, soft vibrational modes and, to a smaller extent, intermolecular interactions give a broadening, which blurs the vibrational fine structure. It is predicted that environmental broadening is dominant in aqueous acetone. Y1 - 2011 U6 - https://doi.org/10.1103/PhysRevB.84.132202 SN - 1098-0121 VL - 84 IS - 13 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Sun, Y-P A1 - Pietzsch, Annette A1 - Hennies, Franz A1 - Rinkevicius, Z. A1 - Karlsson, Hans O. A1 - Schmitt, Thorsten A1 - Strocov, Vladimir N. A1 - Andersson, Joakim A1 - Kennedy, B. A1 - Schlappa, J. A1 - Föhlisch, Alexander A1 - Gel'mukhanov, F. A1 - Rubensson, Jan-Erik T1 - Internal symmetry and selection rules in resonant inelastic soft x-ray scattering JF - Journal of physics : B, Atomic, molecular and optical physics N2 - Resonant inelastic soft x-ray scattering spectra excited at the dissociative 1 sigma(g) -> 3 sigma(u) resonance in gas-phase O(2) are presented and discussed in terms of state-of-the-art molecular theory. A new selection rule due to internal spin coupling is established, facilitating a deep analysis of the valence excited final states. Furthermore, it is found that a commonly accepted symmetry selection rule due to orbital parity breaks down, as the core hole and excited electron swap parity, thereby opening the symmetry forbidden 3 sigma(g) decay channel. Y1 - 2011 U6 - https://doi.org/10.1088/0953-4075/44/16/161002 SN - 0953-4075 VL - 44 IS - 16 PB - IOP Publ. Ltd. CY - Bristol ER - TY - THES A1 - Matthes, Heidrun T1 - Interaction of land surface processes and the atmophere in the Arctic - senitivities and extremes Y1 - 2011 CY - Potsdam ER - TY - JOUR A1 - Abdo, A. A. A1 - Ackermann, Margit A1 - Ajello, M. A1 - Allafort, A. J. A1 - Baldini, L. A1 - Ballet, J. A1 - Barbiellini, G. A1 - Baring, M. G. A1 - Bastieri, D. A1 - Bechtol, K. C. A1 - Bellazzini, R. A1 - Berenji, B. A1 - Blandford, R. D. A1 - Bloom, E. D. A1 - Bonamente, E. A1 - Borgland, A. W. A1 - Bouvier, A. A1 - Brandt, T. J. A1 - Bregeon, Johan A1 - Brez, A. A1 - Brigida, M. A1 - Bruel, P. A1 - Buehler, R. A1 - Buson, S. A1 - Caliandro, G. A. A1 - Cameron, R. A. A1 - Cannon, A. A1 - Caraveo, P. A. A1 - Carrigan, Svenja A1 - Casandjian, J. M. A1 - Cavazzuti, E. A1 - Cecchi, C. A1 - Celik, O. A1 - Charles, E. A1 - Chekhtman, A. A1 - Cheung, C. C. A1 - Chiang, J. A1 - Ciprini, S. A1 - Claus, R. A1 - Cohen-Tanugi, J. A1 - Conrad, Jan A1 - Cutini, S. A1 - Dermer, C. D. A1 - de Palma, F. A1 - do Couto e Silva, E. A1 - Drell, P. S. A1 - Dubois, R. A1 - Dumora, D. A1 - Favuzzi, C. A1 - Fegan, S. J. A1 - Ferrara, E. C. A1 - Focke, W. B. A1 - Fortin, P. A1 - Frailis, M. A1 - Fuhrmann, L. A1 - Fukazawa, Y. A1 - Funk, S. A1 - Fusco, P. A1 - Gargano, F. A1 - Gasparrini, D. A1 - Gehrels, N. A1 - Germani, S. A1 - Giglietto, N. A1 - Giordano, F. A1 - Giroletti, M. A1 - Glanzman, T. A1 - Godfrey, G. A1 - Grenier, I. A. A1 - Guillemot, L. A1 - Guiriec, S. A1 - Hayashida, M. A1 - Hays, E. A1 - Horan, D. A1 - Hughes, R. E. A1 - Johannesson, G. A1 - Johnson, A. S. A1 - Johnson, W. N. A1 - Kadler, M. A1 - Kamae, T. A1 - Katagiri, H. A1 - Kataoka, J. A1 - Knoedlseder, J. A1 - Kuss, M. A1 - Lande, J. A1 - Latronico, L. A1 - Lee, S. -H. A1 - Lemoine-Goumard, M. A1 - Longo, F. A1 - Loparco, F. A1 - Lott, B. A1 - Lovellette, M. N. A1 - Lubrano, P. A1 - Madejski, G. M. A1 - Makeev, A. A1 - Max-Moerbeck, W. A1 - Mazziotta, Mario Nicola A1 - McEnery, J. E. A1 - Mehault, J. A1 - Michelson, P. F. A1 - Mitthumsiri, W. A1 - Mizuno, T. A1 - Moiseev, A. A. A1 - Monte, C. A1 - Monzani, M. E. A1 - Morselli, A. A1 - Moskalenko, I. V. A1 - Murgia, S. A1 - Naumann-Godo, M. A1 - Nishino, S. A1 - Nolan, P. L. A1 - Norris, J. P. A1 - Nuss, E. A1 - Ohsugi, T. A1 - Okumura, A. A1 - Omodei, N. A1 - Orlando, E. A1 - Ormes, J. F. A1 - Paneque, D. A1 - Panetta, J. H. A1 - Parent, D. A1 - Pavlidou, V. A1 - Pearson, T. J. A1 - Pelassa, V. A1 - Pepe, M. A1 - Pesce-Rollins, M. A1 - Piron, F. A1 - Porter, T. A. A1 - Raino, S. A1 - Rando, R. A1 - Razzano, M. A1 - Readhead, A. A1 - Reimer, A. A1 - Reimer, O. A1 - Richards, J. L. A1 - Ripken, J. A1 - Ritz, S. A1 - Roth, M. A1 - Sadrozinski, H. F. -W. A1 - Sanchez, D. A1 - Sander, A. A1 - Scargle, J. D. A1 - Sgro, C. A1 - Siskind, E. J. A1 - Smith, P. D. A1 - Spandre, G. A1 - Spinelli, P. A1 - Stawarz, L. A1 - Stevenson, M. A1 - Strickman, M. S. A1 - Sokolovsky, K. V. A1 - Suson, D. J. A1 - Takahashi, H. A1 - Takahashi, T. A1 - Tanaka, T. A1 - Thayer, J. B. A1 - Thayer, J. G. A1 - Thompson, D. J. A1 - Tibaldo, L. A1 - Torres, F. A1 - Tosti, G. A1 - Tramacere, A. A1 - Uchiyama, Y. A1 - Usher, T. L. A1 - Vandenbroucke, J. A1 - Vasileiou, V. A1 - Vilchez, N. A1 - Vitale, V. A1 - Waite, A. P. A1 - Wang, P. A1 - Wehrle, A. E. A1 - Winer, B. L. A1 - Wood, K. S. A1 - Yang, Z. A1 - Ylinen, T. A1 - Zensus, J. A. A1 - Ziegler, M. A1 - Aleksic, J. A1 - Antonelli, L. A. A1 - Antoranz, P. A1 - Backes, Michael A1 - Barrio, J. A. A1 - Gonzalez, J. Becerra A1 - Bednarek, W. A1 - Berdyugin, A. A1 - Berger, K. A1 - Bernardini, E. A1 - Biland, A. A1 - Blanch Bigas, O. A1 - Bock, R. K. A1 - Boller, A. A1 - Bonnoli, G. A1 - Bordas, Pol A1 - Tridon, D. Borla A1 - Bosch-Ramon, Valentin A1 - Bose, D. A1 - Braun, I. A1 - Bretz, T. A1 - Camara, M. A1 - Carmona, E. A1 - Carosi, A. A1 - Colin, P. A1 - Colombo, E. A1 - Contreras, J. L. A1 - Cortina, J. A1 - Covino, S. A1 - Dazzi, F. A1 - de Angelis, A. A1 - del Pozo, E. De Cea A1 - De Lotto, B. A1 - De Maria, M. A1 - De Sabata, F. A1 - Mendez, C. Delgado A1 - Ortega, A. Diago A1 - Doert, M. A1 - Dominguez, A. A1 - Prester, Dijana Dominis A1 - Dorner, D. A1 - Doro, M. A1 - Elsaesser, D. A1 - Ferenc, D. A1 - Fonseca, M. V. A1 - Font, L. A1 - Lopen, R. J. Garcia A1 - Garczarczyk, M. A1 - Gaug, M. A1 - Giavitto, G. A1 - Godinovi, N. A1 - Hadasch, D. A1 - Herrero, A. A1 - Hildebrand, D. A1 - Hoehne-Moench, D. A1 - Hose, J. A1 - Hrupec, D. A1 - Jogler, T. A1 - Klepser, S. A1 - Kraehenbuehl, T. A1 - Kranich, D. A1 - Krause, J. A1 - La Barbera, A. A1 - Leonardo, E. A1 - Lindfors, E. A1 - Lombardi, S. A1 - Lopez, M. A1 - Lorenz, E. A1 - Majumdar, P. A1 - Makariev, E. A1 - Maneva, G. A1 - Mankuzhiyil, N. A1 - Mannheim, K. A1 - Maraschi, L. A1 - Mariotti, M. A1 - Martinez, M. A1 - Mazin, D. A1 - Meucci, M. A1 - Miranda, J. M. A1 - Mirzoyan, R. A1 - Miyamoto, H. A1 - Moldon, J. A1 - Moralejo, A. A1 - Nieto, D. A1 - Nilsson, K. A1 - Orito, R. A1 - Oya, I. A1 - Paoletti, R. A1 - Paredes, J. M. A1 - Partini, S. A1 - Pasanen, M. A1 - Pauss, F. A1 - Pegna, R. G. A1 - Perez-Torres, M. A. A1 - Persic, M. A1 - Peruzzo, J. A1 - Pochon, J. A1 - Moroni, P. G. Prada A1 - Prada, F. A1 - Prandini, E. A1 - Puchades, N. A1 - Puljak, I. A1 - Reichardt, T. A1 - Reinthal, R. A1 - Rhode, W. A1 - Ribo, M. A1 - Rico, J. A1 - Rissi, M. A1 - Ruegamer, S. A1 - Saggion, A. A1 - Saito, K. A1 - Saito, T. Y. A1 - Salvati, M. A1 - Sanchez-Conde, M. A1 - Satalecka, K. A1 - Scalzotto, V. A1 - Scapin, V. A1 - Schultz, C. A1 - Schweizer, T. A1 - Shayduk, M. A1 - Shore, S. N. A1 - Sierpowska-Bartosik, A. A1 - Sillanpaa, A. A1 - Sitarek, J. A1 - Sobczynska, D. A1 - Spanier, F. A1 - Spiro, S. A1 - Stamerra, A. A1 - Steinke, B. A1 - Storz, J. A1 - Strah, N. A1 - Struebig, J. C. A1 - Suric, T. A1 - Takalo, L. O. A1 - Tavecchio, F. A1 - Temnikov, P. A1 - Terzic, T. A1 - Tescaro, D. A1 - Teshima, M. A1 - Vankov, H. A1 - Wagner, R. M. A1 - Weitzel, Q. A1 - Zabalza, V. A1 - Zandanel, F. A1 - Zanin, R. A1 - Acciari, V. A. A1 - Arlen, T. A1 - Aune, T. A1 - Benbow, W. A1 - Boltuch, D. A1 - Bradbury, S. M. A1 - Buckley, J. H. A1 - Bugaev, V. A1 - Cannon, A. A1 - Cesarini, A. A1 - Ciupik, L. A1 - Cui, W. A1 - Dickherber, R. A1 - Errando, M. A1 - Falcone, A. A1 - Finley, J. P. A1 - Finnegan, G. A1 - Fortson, L. A1 - Furniss, A. A1 - Galante, N. A1 - Gall, D. A1 - Gillanders, G. H. A1 - Godambe, S. A1 - Grube, J. A1 - Guenette, R. A1 - Gyuk, G. A1 - Hanna, D. A1 - Holder, J. A1 - Huang, D. A1 - Hui, C. M. A1 - Humensky, T. B. A1 - Kaaret, P. A1 - Karlsson, N. A1 - Kertzman, M. A1 - Kieda, D. A1 - Konopelko, A. A1 - Krawczynski, H. A1 - Krennrich, F. A1 - Lang, M. J. A1 - Maier, G. A1 - McArthur, S. A1 - McCann, A. A1 - McCutcheon, M. A1 - Moriarty, P. A1 - Mukherjee, R. A1 - Ong, R. A1 - Otte, N. A1 - Pandel, D. A1 - Perkins, J. S. A1 - Pichel, A. A1 - Pohl, M. A1 - Quinn, J. A1 - Ragan, K. A1 - Reyes, L. C. A1 - Reynolds, P. T. A1 - Roache, E. A1 - Rose, H. J. A1 - Rovero, A. C. A1 - Schroedter, M. A1 - Sembroski, G. H. A1 - Senturk, G. D. A1 - Steele, D. A1 - Swordy, S. P. A1 - Tesic, G. A1 - Theiling, M. A1 - Thibadeau, S. A1 - Varlotta, A. A1 - Vincent, S. A1 - Wakely, S. P. A1 - Ward, J. E. A1 - Weekes, T. C. A1 - Weinstein, A. A1 - Weisgarber, T. A1 - Williams, D. A. A1 - Wood, M. A1 - Zitzer, B. A1 - Villata, M. A1 - Raiteri, C. M. A1 - Aller, H. D. A1 - Aller, M. F. A1 - Arkharov, A. A. A1 - Blinov, D. A. A1 - Calcidese, P. A1 - Chen, W. P. A1 - Efimova, N. V. A1 - Kimeridze, G. A1 - Konstantinova, T. S. A1 - Kopatskaya, E. N. A1 - Koptelova, E. A1 - Kurtanidze, O. M. A1 - Kurtanidze, S. O. A1 - Lahteenmaki, A. A1 - Larionov, V. M. A1 - Larionova, E. G. A1 - Larionova, L. V. A1 - Ligustri, R. A1 - Morozova, D. A. A1 - Nikolashvili, M. G. A1 - Sigua, L. A. A1 - Troitsky, I. S. A1 - Angelakis, E. A1 - Capalbi, M. A1 - Carraminana, A. A1 - Carrasco, L. A1 - Cassaro, P. A1 - de la Fuente, E. A1 - Gurwell, M. A. A1 - Kovalev, Y. Y. A1 - Kovalev, Yu. A. A1 - Krichbaum, T. P. A1 - Krimm, H. A. A1 - Leto, Paolo A1 - Lister, M. L. A1 - Maccaferri, G. A1 - Moody, J. W. A1 - Mori, Y. A1 - Nestoras, I. A1 - Orlati, A. A1 - Pagani, C. A1 - Pace, C. A1 - Pearson, R. A1 - Perri, M. A1 - Piner, B. G. A1 - Pushkarev, A. B. A1 - Ros, E. A1 - Sadun, A. C. A1 - Sakamoto, T. A1 - Tornikoski, M. A1 - Yatsu, Y. A1 - Zook, A. T1 - Insights into the high-energy gamma-Ray emission of markarian 501 fromextensive multifrequency observations in the fermi era JF - The astrophysical journal : an international review of spectroscopy and astronomical physics N2 - We report on the gamma-ray activity of the blazar Mrk 501 during the first 480 days of Fermi operation. We find that the average Large Area Telescope (LAT) gamma-ray spectrum of Mrk 501 can be well described by a single power-law function with a photon index of 1.78 +/- 0.03. While we observe relatively mild flux variations with the Fermi-LAT (within less than a factor of two), we detect remarkable spectral variability where the hardest observed spectral index within the LAT energy range is 1.52 +/- 0.14, and the softest one is 2.51 +/- 0.20. These unexpected spectral changes do not correlate with the measured flux variations above 0.3 GeV. In this paper, we also present the first results from the 4.5 month long multifrequency campaign (2009 March 15-August 1) on Mrk 501, which included the Very Long Baseline Array (VLBA), Swift, RXTE, MAGIC, and VERITAS, the F-GAMMA, GASP-WEBT, and other collaborations and instruments which provided excellent temporal and energy coverage of the source throughout the entire campaign. The extensive radio to TeV data set from this campaign provides us with the most detailed spectral energy distribution yet collected for this source during its relatively low activity. The average spectral energy distribution of Mrk 501 is well described by the standard one-zone synchrotron self-Compton (SSC) model. In the framework of this model, we find that the dominant emission region is characterized by a size less than or similar to 0.1 pc (comparable within a factor of few to the size of the partially resolved VLBA core at 15-43 GHz), and that the total jet power (similar or equal to 10(44) erg s(-1)) constitutes only a small fraction (similar to 10(-3)) of the Eddington luminosity. The energy distribution of the freshly accelerated radiating electrons required to fit the time-averaged data has a broken power-law form in the energy range 0.3 GeV-10 TeV, with spectral indices 2.2 and 2.7 below and above the break energy of 20 GeV. We argue that such a form is consistent with a scenario in which the bulk of the energy dissipation within the dominant emission zone of Mrk 501 is due to relativistic, proton-mediated shocks. We find that the ultrarelativistic electrons and mildly relativistic protons within the blazar zone, if comparable in number, are in approximate energy equipartition, with their energy dominating the jet magnetic field energy by about two orders of magnitude. KW - acceleration of particles KW - BL Lacertae objects: general KW - BL Lacertae objects: individual (Mrk 501) KW - galaxies: active KW - gamma rays: general KW - radiation mechanisms: non-thermal Y1 - 2011 U6 - https://doi.org/10.1088/0004-637X/727/2/129 SN - 0004-637X VL - 727 IS - 2 PB - IOP Publ. Ltd. CY - Bristol ER - TY - JOUR A1 - Schuch, Norbert A1 - Harrison, Sarah K. A1 - Osborne, Tobias J. A1 - Eisert, Jens T1 - Information propagation for interacting-particle systems JF - Physical review : A, Atomic, molecular, and optical physics N2 - We study the speed at which information propagates through systems of interacting quantum particles moving on a regular lattice and show that for a certain class of initial conditions there exists a maximum speed of sound at which information can propagate. Our argument applies equally to quantum spins, bosons such as in the Bose-Hubbard model, fermions, anyons, and general mixtures thereof, on arbitrary lattices of any dimension. It also pertains to dissipative dynamics on the lattice, and generalizes to the continuum for quantum fields. Our result can be seen as an analog of the Lieb-Robinson bound for strongly correlated models. Y1 - 2011 U6 - https://doi.org/10.1103/PhysRevA.84.032309 SN - 1050-2947 VL - 84 IS - 3 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Kar, Parimal A1 - Lipowsky, Reinhard A1 - Knecht, Volker T1 - Importance of polar solvation for cross-reactivity of antibody and its variants with steroids JF - The journal of physical chemistry : B, Condensed matter, materials, surfaces, interfaces & biophysical chemistry N2 - Understanding the factors determining the binding of ligands to receptors in detail is essential for rational drug design. Here, the free energies of binding of the steroids progesterone (PRG) and 5 beta-androstane-3,17-dione (SAD) to the Diels-Alderase antibody 1E9, as well as the Leu(H47)Trp/Arg(H100)Trp 1E9 double mutant (1E9dm) and the corresponding single mutants, have been estimated and decomposed using the molecular mechanics-Poisson-Boltzmann surface area (MM-PBSA) method. Also the difference in binding free energies between the PRG-1E9dm complex and the complex of PRG with the antiprogesterone antibody DB3 have been evaluated and decomposed. The steroids bind less strongly to 1E9 than to DB3, but the mutations tend to improve the steroid affinity, in quantitative agreement with experimental data. Although the complexes formed by PRG or SAD with 1E9dm and by PRG with DB3 have similar affinity, the binding mechanisms are different. Reduced Waals for SAD-1E9dm versus PRG-1E9dm or for PRG-1E9dm versus PRG-DB3 are energetically compensated by an increased solvation of polar groups, partly contrasting previous conclusions based on structural inspection. Our study illustrates that deducing binding mechanisms from structural models alone can be misleading. Therefore, taking into account solvation effects as in MM-PBSA calculations is essential to elucidate molecular recognition. Y1 - 2011 U6 - https://doi.org/10.1021/jp201538t SN - 1520-6106 VL - 115 IS - 23 SP - 7661 EP - 7669 PB - American Chemical Society CY - Washington ER - TY - JOUR A1 - Douce, Laurent A1 - Suisse, Jean-Moise A1 - Guillon, Daniel A1 - Taubert, Andreas T1 - Imidazolium-based liquid crystals a modular platform for versatile new materials with finely tuneable properties and behaviour JF - Liquid crystals : an international journal of science and technology N2 - Ionic liquid Crystals constitute highly versatile materials that have drawn much interest these past few years in the fields of academic research and industrial development. In this respect, the present article is intended as an update of K. Binnemans review published in 2005, but focusing exclusively on the imidazolium cation - the most widely studied. Herein, imidazolium-containing thermotropic liquid crystalline materials will be sorted by molecular structure (mono-, bis-, poly-imidazolium compounds, with symmetrical and non-symmetrical structures) and discussed. Their physico-chemical properties will be exposed in order to adduce the relevancy and potential of the imidazolium platform in various fields of research. KW - imidazolium KW - liquid crystal KW - ionic liquid Y1 - 2011 U6 - https://doi.org/10.1080/02678292.2011.610474 SN - 0267-8292 VL - 38 IS - 11-12 SP - 1653 EP - 1661 PB - Routledge, Taylor & Francis Group CY - Abingdon ER - TY - JOUR A1 - Turukina, L. V. A1 - Pikovskij, Arkadij T1 - Hyperbolic chaos in a system of resonantly coupled weakly nonlinear oscillators JF - Modern physics letters : A, Particles and fields, gravitation, cosmology, nuclear physics N2 - We show that a hyperbolic chaos can be observed in resonantly coupled oscillators near a Hopf bifurcation, described by normal-form-type equations for complex amplitudes. The simplest example consists of four oscillators, comprising two alternatively activated, due to an external periodic modulation, pairs. In terms of the stroboscopic Poincare map, the phase differences change according to an expanding Bernoulli map that depends on the coupling type. Several examples of hyperbolic chaos for different types of coupling are illustrated numerically. KW - Coupled oscillators KW - Hyperbolic chaos Y1 - 2011 U6 - https://doi.org/10.1016/j.physleta.2011.02.017 SN - 0375-9601 VL - 375 IS - 11 SP - 1407 EP - 1411 PB - Elsevier CY - Amsterdam ER - TY - JOUR A1 - Seiss, Martin A1 - Spahn, Frank T1 - Hydrodynamics of saturn's dense rings JF - Mathematical modelling of natural phenomena N2 - The space missions Voyager and Cassini together with earthbound observations revealed a wealth of structures in Saturn's rings. There are, for example, waves being excited at ring positions which are in orbital resonance with Saturn's moons. Other structures can be assigned to embedded moons like empty gaps, moon induced wakes or S-shaped propeller features. Furthermore, irregular radial structures are observed in the range from 10 meters until kilometers. Here some of these structures will be discussed in the frame of hydrodynamical modeling of Saturn's dense rings. For this purpose we will characterize the physical properties of the ring particle ensemble by mean field quantities and point to the special behavior of the transport coefficients. We show that unperturbed rings can become unstable and how diffusion acts in the rings. Additionally, the alternative streamline formalism is introduced to describe perturbed regions of dense rings with applications to the wake damping and the dispersion relation of the density waves. KW - granular gas KW - instabilities KW - hydrodynamics KW - planetary rings Y1 - 2011 U6 - https://doi.org/10.1051/mmnp/20116409 SN - 0973-5348 SN - 1760-6101 VL - 6 IS - 4 SP - 191 EP - 218 PB - EDP Sciences CY - Les Ulis ER - TY - JOUR A1 - Jewitt, David A1 - Weaver, Harold A1 - Mutchler, Max A1 - Larson, Stephen A1 - Agarwal, Jessica T1 - Hubble space telescope observations of main-belt comet (596) scheila JF - The astrophysical journal : an international review of spectroscopy and astronomical physics ; Part 2, Letters N2 - We present Hubble Space Telescope Observations of (596) Scheila during its recent dust outburst. The nucleus remained point-like with absolute magnitude H(V) = 8.85 +/- 0.02 in our data, equal to the pre-outburst value, with no secondary fragments of diameter >= 100m (for assumed albedos 0.04). We find a coma having a peak scattering cross section similar to 2.2x10(4) km(2), corresponding to a mass in micron-sized particles of similar to 4x10(7) kg. The particles are deflected by solar radiation pressure on projected spatial scales similar to 2x10(4) km, in the sunward direction, and swept from the vicinity of the nucleus on timescales of weeks. The coma fades by similar to 30% between observations on UT 2010 December 27 and 2011 January 4. The observed mass loss is inconsistent with an origin either by rotational instability of the nucleus or by electrostatic ejection of regolith charged by sunlight. Dust ejection could be caused by the sudden but unexplained exposure of buried ice. However, the data are most simply explained by the impact, at similar to 5 km s(-1), of a previously unknown asteroid similar to 35m in diameter. KW - comets: general KW - comets: individual ((596) Scheila) KW - minor planets, asteroids: general Y1 - 2011 U6 - https://doi.org/10.1088/2041-8205/733/1/L4 SN - 2041-8205 VL - 733 IS - 1 PB - IOP Publ. Ltd. CY - Bristol ER - TY - GEN A1 - Gerhard, Reimund T1 - Honoring Professor Gerhard M. Sessler on his 80th Birthday (15th of February 2011) T2 - IEEE transactions on dielectrics and electrical insulation Y1 - 2011 U6 - https://doi.org/10.1109/TDEI.2011.5704485 SN - 1070-9878 VL - 18 IS - 1 SP - 1 EP - 2 PB - Inst. of Electr. and Electronics Engineers CY - Piscataway ER - TY - JOUR A1 - Kuehn, Sergei A1 - Pingel, Patrick A1 - Breusing, Markus A1 - Fischer, Thomas A1 - Stumpe, Joachim A1 - Neher, Dieter A1 - Elsaesser, Thomas T1 - High-Resolution Near-Field Optical Investigation of Crystalline Domains in Oligomeric PQT-12 Thin Films JF - Advanced functional materials N2 - The structure and morphology on different length scales dictate both the electrical and optical properties of organic semiconductor thin films. Using a combination of spectroscopic methods, including scanning near-field optical microscopy, we study the domain structure and packing quality of highly crystalline thin films of oligomeric PQT-12 with 100 nanometer spatial resolution. The pronounced optical anisotropy of these layers measured by polarized light microscopy facilitates the identification of regions with uniform molecular orientation. We find that a hierarchical order on three different length scales exists in these layers, made up of distinct well-ordered dichroic areas at the ten-micrometer-scale, which are sub-divided into domains with different molecular in-plane orientation. These serve as a template for the formation of smaller needle-like crystallites at the layer surface. A high degree of crystalline order is believed to be the cause of the rather high field-effect mobility of these layers of 10(-3) cm 2 V(-1) s(-1), whereas it is limited by the presence of domain boundaries at macroscopic distances. Y1 - 2011 U6 - https://doi.org/10.1002/adfm.201001978 SN - 1616-301X VL - 21 IS - 5 SP - 860 EP - 868 PB - Wiley-Blackwell CY - Malden ER - TY - JOUR A1 - Robinson, Alexander A1 - Calov, Reinhard A1 - Ganopolski, Andrey T1 - Greenland ice sheet model parameters constrained using simulations of the Eemian Interglacial JF - Climate of the past : an interactive open access journal of the European Geosciences Union N2 - Using a new approach to force an ice sheet model, we performed an ensemble of simulations of the Greenland Ice Sheet evolution during the last two glacial cycles, with emphasis on the Eemian Interglacial. This ensemble was generated by perturbing four key parameters in the coupled regional climate-ice sheet model and by introducing additional uncertainty in the prescribed "background" climate change. The sensitivity of the surface melt model to climate change was determined to be the dominant driver of ice sheet instability, as reflected by simulated ice sheet loss during the Eemian Interglacial period. To eliminate unrealistic parameter combinations, constraints from present-day and paleo information were applied. The constraints include (i) the diagnosed present-day surface mass balance partition between surface melting and ice discharge at the margin, (ii) the modeled present-day elevation at GRIP; and (iii) the modeled elevation reduction at GRIP during the Eemian. Using these three constraints, a total of 360 simulations with 90 different model realizations were filtered down to 46 simulations and 20 model realizations considered valid. The paleo constraint eliminated more sensitive melt parameter values, in agreement with the surface mass balance partition assumption. The constrained simulations resulted in a range of Eemian ice loss of 0.4-4.4m sea level equivalent, with a more likely range of about 3.7-4.4m sea level if the GRIP delta O-18 isotope record can be considered an accurate proxy for the precipitation-weighted annual mean temperatures. Y1 - 2011 U6 - https://doi.org/10.5194/cp-7-381-2011 SN - 1814-9324 VL - 7 IS - 2 SP - 381 EP - 396 PB - Copernicus CY - Göttingen ER - TY - JOUR A1 - Abel, M. W. A1 - Shepelyansky, Dima L. T1 - Google matrix of business process management JF - The European physical journal : B, Condensed matter and complex systems N2 - Development of efficient business process models and determination of their characteristic properties are subject of intense interdisciplinary research. Here, we consider a business process model as a directed graph. Its nodes correspond to the units identified by the modeler and the link direction indicates the causal dependencies between units. It is of primary interest to obtain the stationary flow on such a directed graph, which corresponds to the steady-state of a firm during the business process. Following the ideas developed recently for the World Wide Web, we construct the Google matrix for our business process model and analyze its spectral properties. The importance of nodes is characterized by PageRank and recently proposed CheiRank and 2DRank, respectively. The results show that this two-dimensional ranking gives a significant information about the influence and communication properties of business model units. We argue that the Google matrix method, described here, provides a new efficient tool helping companies to make their decisions on how to evolve in the exceedingly dynamic global market. Y1 - 2011 U6 - https://doi.org/10.1140/epjb/e2010-10710-y SN - 1434-6028 VL - 84 IS - 4 SP - 493 EP - 500 PB - Springer CY - New York ER - TY - JOUR A1 - Sanhueza-Pino, Katia A1 - Korup, Oliver A1 - Hetzel, Ralf A1 - Munack, Henry A1 - Weidinger, Johannes T. A1 - Dunning, Stuart A. A1 - Ormukov, Cholponbek A1 - Kubik, Peter W. T1 - Glacial advances constrained by Be-10 exposure dating of bedrock landslides, Kyrgyz Tien Shan JF - Quaternary research : an interdisciplinary journal N2 - Numerous large landslide deposits occur in the Tien Shan, a tectonically active intraplate orogen in Central Asia. Yet their significance in Quaternary landscape evolution and natural hazard assessment remains unresolved due to the lack of "absolute" age constraints. Here we present the first Be-10 exposure ages for three prominent (>10(7) m(3)) bedrock landslides that blocked major rivers and formed lakes, two of which subsequently breached, in the northern Kyrgyz Tien Shan. Three Be-10 ages reveal that one landslide in the Alamyedin River occurred at 11-15 ka, which is consistent with two C-14 ages of gastropod shells from reworked loess capping the landslide. One large landslide in Aksu River is among the oldest documented in semi-arid continental interiors, with a Be-10 age of 63-67 ka. The Ukok River landslide deposit(s) yielded variable Be-10 ages, which may result from multiple landslides, and inheritance of Be-10. Two Be-10 ages of 8.2 and 5.9 ka suggest that one major landslide occurred in the early to mid-Holocene, followed by at least one other event between 1.5 and 0.4 ka. Judging from the regional glacial chronology, all three landslides have occurred between major regional glacial advances. Whereas Alamyedin and Ukok can be considered as postglacial in this context, Aksu is of interglacial age. None of the landslide deposits show traces of glacial erosion, hence their locations and I Be ages mark maximum extents and minimum ages of glacial advances, respectively. Using toe-to-headwall altitude ratios of 0.4-0.5, we reconstruct minimum equilibrium-line altitudes that exceed previous estimates by as much as 400 m along the moister northern fringe of the Tien Shan. Our data show that deposits from large landslides can provide valuable spatio-temporal constraints for glacial advances in landscapes where moraines and glacial deposits have low preservation potential. (C) 2011 University of Washington. Published by Elsevier Inc. All rights reserved. KW - Landslide KW - Rock avalanche KW - Be-10 exposure dating KW - Quaternary glaciations KW - Tien Shan Y1 - 2011 U6 - https://doi.org/10.1016/j.yqres.2011.06.013 SN - 0033-5894 VL - 76 IS - 3 SP - 295 EP - 304 PB - Elsevier CY - San Diego ER - TY - JOUR A1 - Sun, Zhongkui A1 - Yang, Xiaoli T1 - Generating and enhancing lag synchronization of chaotic systems by white noise JF - Chaos : an interdisciplinary journal of nonlinear science N2 - In this paper, we study the crucial impact of white noise on lag synchronous regime in a pair of time-delay unidirectionally coupled systems. Our result demonstrates that merely via white-noise-based coupling lag synchronization could be achieved between the coupled systems (chaotic or not). And it is also demonstrated that a conventional lag synchronous regime can be enhanced by white noise. Sufficient conditions are further proved mathematically for noise-inducing and noise-enhancing lag synchronization, respectively. Additionally, the influence of parameter mismatch on the proposed lag synchronous regime is studied, by which we announce the robustness and validity of the new strategy. Two numerical examples are provided to illustrate the validity and some possible applications of the theoretical result. Y1 - 2011 U6 - https://doi.org/10.1063/1.3623440 SN - 1054-1500 SN - 1089-7682 VL - 21 IS - 3 PB - American Institute of Physics CY - Melville ER - TY - JOUR A1 - Schmidt, Hans-Jürgen T1 - Gauss-Bonnet lagrangian G lnG and cosmological exact solutions JF - Physical review : D, Particles, fields, gravitation, and cosmology N2 - For the Lagrangian L = G lnG where G is the Gauss-Bonnet curvature scalar we deduce the field equation and solve it in closed form for 3-flat Friedmann models using a state-finder parametrization. Further we show that among all Lagrangians F(G) this L is the only one not having the form G(r) with a real constant r but possessing a scale-invariant field equation. This turns out to be one of its analogies to f(R) theories in two-dimensional space-time. In the appendix, we systematically list several formulas for the decomposition of the Riemann tensor in arbitrary dimensions n, which are applied in the main deduction for n = 4. Y1 - 2011 U6 - https://doi.org/10.1103/PhysRevD.83.083513 SN - 1550-7998 VL - 83 IS - 8 PB - American Physical Society CY - College Park ER - TY - JOUR A1 - Acciari, V. A. A1 - Aliu, E. A1 - Araya, M. A1 - Arlen, T. A1 - Aune, T. A1 - Beilicke, M. A1 - Benbow, W. A1 - Bradbury, S. M. A1 - Buckley, J. H. A1 - Bugaev, V. A1 - Byrum, K. A1 - Cannon, A. A1 - Cesarini, A. A1 - Ciupik, L. A1 - Collins-Hughes, E. A1 - Cui, W. A1 - Dickherber, R. A1 - Duke, C. A1 - Falcone, A. A1 - Finley, J. P. A1 - Fortson, L. A1 - Furniss, A. A1 - Galante, N. A1 - Gall, D. A1 - Godambe, S. A1 - Griffin, S. A1 - Guenette, R. A1 - Gyuk, G. A1 - Hanna, D. A1 - Holder, J. A1 - Hughes, G. A1 - Hui, C. M. A1 - Humensky, T. B. A1 - Imran, A. A1 - Kaaret, P. A1 - Kertzman, M. A1 - Krawczynski, H. A1 - Krennrich, F. A1 - Madhavan, A. S. A1 - Maier, G. A1 - Majumdar, P. A1 - McArthur, S. A1 - Moriarty, P. A1 - Ong, R. A. A1 - Otte, A. N. A1 - Pandel, D. A1 - Park, N. A1 - Perkins, J. S. A1 - Pohl, Martin A1 - Prokoph, H. A1 - Quinn, J. A1 - Ragan, K. A1 - Reyes, L. C. A1 - Reynolds, P. T. A1 - Roache, E. A1 - Rose, H. J. A1 - Saxon, D. B. A1 - Sembroski, G. H. A1 - Sentuerk, G. D. A1 - Smith, A. W. A1 - Tesic, G. A1 - Theiling, M. A1 - Thibadeau, S. A1 - Varlotta, A. A1 - Vincent, S. A1 - Vivier, M. A1 - Wakely, S. P. A1 - Ward, J. E. A1 - Weekes, T. C. A1 - Weinstein, A. A1 - Weisgarber, T. A1 - Weng, S. A1 - Williams, D. A. A1 - Wood, M. A1 - Zitzer, B. T1 - Gamma-ray observations of the Be/Pulsar binary 1A 0535+262 during a Giant X-Ray outburst JF - The astrophysical journal : an international review of spectroscopy and astronomical physics N2 - Giant X-ray outbursts, with luminosities of about 10(37) erg s(-1), are observed roughly every five years from the nearby Be/pulsar binary 1A 0535+262. In this article, we present observations of the source with VERITAS at very high energies (VHEs; E > 100 GeV) triggered by the X-ray outburst in 2009 December. The observations started shortly after the onset of the outburst and provided comprehensive coverage of the episode, as well as the 111 day binary orbit. No VHE emission is evident at any time. We also examined data from the contemporaneous observations of 1A 0535+262 with the Fermi/Large Area Telescope at high-energy photons (E > 0.1 GeV) and failed to detect the source at GeV energies. The X-ray continua measured with the Swift/X-Ray Telescope and the RXTE/PCA can be well described by the combination of blackbody and Comptonized emission from thermal electrons. Therefore, the gamma-ray and X-ray observations suggest the absence of a significant population of non-thermal particles in the system. This distinguishes 1A 0535+262 from those Be X-ray binaries (such as PSR B1259-63 and LS I +61 degrees 303) that have been detected at GeV-TeV energies. We discuss the implications of the results on theoretical models. KW - acceleration of particles KW - binaries: general KW - gamma rays: general KW - stars: individual (1A 0535+262) Y1 - 2011 U6 - https://doi.org/10.1088/0004-637X/733/2/96 SN - 0004-637X VL - 733 IS - 2 PB - IOP Publ. Ltd. CY - Bristol ER - TY - THES A1 - Dosche, Carsten T1 - Funktionale Farbstoffe und ihre Photophysik und Anwendung in komplexen Matrizes Y1 - 2011 CY - Potsdam ER - TY - JOUR A1 - Berenstein, Igal A1 - Beta, Carsten T1 - Flow-induced control of chemical turbulence JF - The journal of chemical physics : bridges a gap between journals of physics and journals of chemistr N2 - We report spatiotemporal chaos in the Oregonator model of the Belousov-Zhabotinsky reaction. Spatiotemporal chaos spontaneously develops in a regime, where the underlying local dynamics show stable limit cycle oscillations (diffusion-induced turbulence). We show that spatiotemporal chaos can be suppressed by a unidirectional flow in the system. With increasing flow velocity, we observe a transition scenario from spatiotemporal chaos via a regime of travelling waves to a stationary steady state. At large flow velocities, we recover the known regime of flow distributed oscillations. KW - chaos KW - chemical equilibrium KW - chemically reactive flow KW - reaction kinetics theory KW - spatiotemporal phenomena KW - turbulence Y1 - 2011 U6 - https://doi.org/10.1063/1.3656248 SN - 0021-9606 VL - 135 IS - 16 PB - American Institute of Physics CY - Melville ER -