TY  - JOUR
A1  - Abouzar, Maryam H.
A1  - Poghossian, Arshak
A1  - Cherstvy, Andrey G.
A1  - Pedraza, Angela M.
A1  - Ingebrandt, Sven
A1  - Schöning, Michael J.
T1  - Label-free electrical detection of DNA by means of field-effect nanoplate capacitors experiments and modeling
JF  - Physica status solidi : A, Applications and materials science
N2  - Label-free electrical detection of consecutive deoxyribonucleic acid (DNA) hybridization/denaturation by means of an array of individually addressable field-effect-based nanoplate silicon-on-insulator (SOI) capacitors modified with gold nanoparticles (Au-NP) is investigated. The proposed device detects charge changes on Au-NP/DNA hybrids induced by the hybridization or denaturation event. DNA hybridization was performed in a high ionic-strength solution to provide a high hybridization efficiency. On the other hand, to reduce the screening of the DNA charge by counter ions and to achieve a high sensitivity, the sensor signal induced by the hybridization and denaturation events was measured in a low ionic-strength solution. High sensor signals of about 120, 90, and 80 mV were registered after the DNA hybridization, denaturation, and re-hybridization events, respectively. Fluorescence microscopy has been applied as reference method to verify the DNA immobilization, hybridization, and denaturation processes. An electrostatic charge-plane model for potential changes at the gate surface of a nanoplate field-effect sensor induced by the DNA hybridization has been developed taking into account both the Debye length and the distance of the DNA charge from the gate surface.
KW  - DNA
KW  - field-effect
KW  - gold nanoparticle
KW  - label-free detection
KW  - nanoplate capacitor
Y1  - 2012
U6  - https://doi.org/10.1002/pssa.201100710
SN  - 1862-6300
VL  - 209
IS  - 5
SP  - 925
EP  - 934
PB  - Wiley-VCH
CY  - Weinheim
ER  - 
TY  - JOUR
A1  - Abramowski, Attila
A1  - Acero, F.
A1  - Aharonian, Felix A.
A1  - Akhperjanian, A. G.
A1  - Anton, Gisela
A1  - Balzer, Arnim
A1  - Barnacka, Anna
A1  - de Almeida, U. Barres
A1  - Becherini, Yvonne
A1  - Becker, J.
A1  - Behera, B.
A1  - Bernlöhr, K.
A1  - Birsin, E.
A1  - Biteau, Jonathan
A1  - Bochow, A.
A1  - Boisson, Catherine
A1  - Bolmont, J.
A1  - Bordas, Pol
A1  - Brucker, J.
A1  - Brun, Francois
A1  - Brun, Pierre
A1  - Bulik, Tomasz
A1  - Buesching, I.
A1  - Carrigan, Svenja
A1  - Casanova, Sabrina
A1  - Cerruti, M.
A1  - Chadwick, Paula M.
A1  - Charbonnier, A.
A1  - Chaves, Ryan C. G.
A1  - Cheesebrough, A.
A1  - Clapson, A. C.
A1  - Coignet, G.
A1  - Cologna, Gabriele
A1  - Conrad, Jan
A1  - Dalton, M.
A1  - Daniel, M. K.
A1  - Davids, I. D.
A1  - Degrange, B.
A1  - Deil, C.
A1  - Dickinson, H. J.
A1  - Djannati-Ataï, A.
A1  - Domainko, W.
A1  - Drury, L. O'C.
A1  - Dubus, G.
A1  - Dutson, K.
A1  - Dyks, J.
A1  - Dyrda, M.
A1  - Egberts, Kathrin
A1  - Eger, P.
A1  - Espigat, P.
A1  - Fallon, L.
A1  - Farnier, C.
A1  - Fegan, S.
A1  - Feinstein, F.
A1  - Fernandes, M. V.
A1  - Fiasson, A.
A1  - Fontaine, G.
A1  - Foerster, A.
A1  - Fuessling, M.
A1  - Gallant, Y. A.
A1  - Gast, H.
A1  - Gerard, L.
A1  - Gerbig, D.
A1  - Giebels, B.
A1  - Glicenstein, J. F.
A1  - Glueck, B.
A1  - Goret, P.
A1  - Goering, D.
A1  - Haeffner, S.
A1  - Hague, J. D.
A1  - Hampf, D.
A1  - Hauser, M.
A1  - Heinz, S.
A1  - Heinzelmann, G.
A1  - Henri, G.
A1  - Hermann, G.
A1  - Hinton, James Anthony
A1  - Hoffmann, A.
A1  - Hofmann, W.
A1  - Hofverberg, P.
A1  - Holler, M.
A1  - Horns, D.
A1  - Jacholkowska, A.
A1  - de Jager, O. C.
A1  - Jahn, C.
A1  - Jamrozy, M.
A1  - Jung, I.
A1  - Kastendieck, M. A.
A1  - Katarzynski, K.
A1  - Katz, U.
A1  - Kaufmann, S.
A1  - Keogh, D.
A1  - Khangulyan, D.
A1  - Khelifi, B.
A1  - Klochkov, D.
A1  - Kluzniak, W.
A1  - Kneiske, T.
A1  - Komin, Nu.
A1  - Kosack, K.
A1  - Kossakowski, R.
A1  - Laffon, H.
A1  - Lamanna, G.
A1  - Lennarz, D.
A1  - Lohse, T.
A1  - Lopatin, A.
A1  - Lu, C. -C.
A1  - Marandon, V.
A1  - Marcowith, Alexandre
A1  - Masbou, J.
A1  - Maurin, D.
A1  - Maxted, N.
A1  - Mayer, M.
A1  - McComb, T. J. L.
A1  - Medina, M. C.
A1  - Mehault, J.
A1  - Moderski, R.
A1  - Moulin, Emmanuel
A1  - Naumann, C. L.
A1  - Naumann-Godo, M.
A1  - de Naurois, M.
A1  - Nedbal, D.
A1  - Nekrassov, D.
A1  - Nguyen, N.
A1  - Nicholas, B.
A1  - Niemiec, J.
A1  - Nolan, S. J.
A1  - Ohm, S.
A1  - Wilhelmi, E. de Ona
A1  - Opitz, B.
A1  - Ostrowski, M.
A1  - Oya, I.
A1  - Panter, M.
A1  - Arribas, M. Paz
A1  - Pedaletti, G.
A1  - Pelletier, G.
A1  - Petrucci, P. -O.
A1  - Pita, S.
A1  - Puehlhofer, G.
A1  - Punch, M.
A1  - Quirrenbach, A.
A1  - Raue, M.
A1  - Rayner, S. M.
A1  - Reimer, A.
A1  - Reimer, O.
A1  - Renaud, M.
A1  - de los Reyes, R.
A1  - Rieger, F.
A1  - Ripken, J.
A1  - Rob, L.
A1  - Rosier-Lees, S.
A1  - Rowell, G.
A1  - Rudak, B.
A1  - Rulten, C. B.
A1  - Ruppel, J.
A1  - Sahakian, V.
A1  - Sanchez, David M.
A1  - Santangelo, A.
A1  - Schlickeiser, R.
A1  - Schoeck, F. M.
A1  - Schulz, A.
A1  - Schwanke, U.
A1  - Schwarzburg, S.
A1  - Schwemmer, S.
A1  - Sheidaei, F.
A1  - Skilton, J. L.
A1  - Sol, H.
A1  - Spengler, G.
A1  - Stawarz, L.
A1  - Steenkamp, R.
A1  - Stegmann, Christian
A1  - Stinzing, F.
A1  - Stycz, K.
A1  - Sushch, Iurii
A1  - Szostek, A.
A1  - Tavernet, J. -P.
A1  - Terrier, R.
A1  - Tluczykont, M.
A1  - Valerius, K.
A1  - van Eldik, C.
A1  - Vasileiadis, G.
A1  - Venter, C.
A1  - Vialle, J. P.
A1  - Viana, A.
A1  - Vincent, P.
A1  - Voelk, H. J.
A1  - Volpe, F.
A1  - Vorobiov, S.
A1  - Vorster, M.
A1  - Wagner, S. J.
A1  - Ward, M.
A1  - White, R.
A1  - Wierzcholska, A.
A1  - Zacharias, M.
A1  - Zajczyk, A.
A1  - Zdziarski, A. A.
A1  - Zech, Alraune
A1  - Zechlin, H. -S.
A1  - Aleksic, J.
A1  - Antonelli, L. A.
A1  - Antoranz, P.
A1  - Backes, Michael
A1  - Barrio, J. A.
A1  - Bastieri, D.
A1  - Becerra Gonzalez, J.
A1  - Bednarek, W.
A1  - Berdyugin, A.
A1  - Berger, K.
A1  - Bernardini, E.
A1  - Biland, A.
A1  - Blanch Bigas, O.
A1  - Bock, R. K.
A1  - Boller, A.
A1  - Bonnoli, G.
A1  - Tridon, D. Borla
A1  - Braun, I.
A1  - Bretz, T.
A1  - Canellas, A.
A1  - Carmona, E.
A1  - Carosi, A.
A1  - Colin, P.
A1  - Colombo, E.
A1  - Contreras, J. L.
A1  - Cortina, J.
A1  - Cossio, L.
A1  - Covino, S.
A1  - Dazzi, F.
A1  - De Angelis, A.
A1  - De Cea del Pozo, E.
A1  - De Lotto, B.
A1  - Delgado Mendez, C.
A1  - Diago Ortega, A.
A1  - Doert, M.
A1  - Dominguez, A.
A1  - Prester, Dijana Dominis
A1  - Dorner, D.
A1  - Doro, M.
A1  - Elsaesser, D.
A1  - Ferenc, D.
A1  - Fonseca, M. V.
A1  - Font, L.
A1  - Fruck, C.
A1  - Garcia Lopez, R. J.
A1  - Garczarczyk, M.
A1  - Garrido, D.
A1  - Giavitto, G.
A1  - Godinovic, N.
A1  - Hadasch, D.
A1  - Haefner, D.
A1  - Herrero, A.
A1  - Hildebrand, D.
A1  - Hoehne-Moench, D.
A1  - Hose, J.
A1  - Hrupec, D.
A1  - Huber, B.
A1  - Jogler, T.
A1  - Klepser, S.
A1  - Kraehenbuehl, T.
A1  - Krause, J.
A1  - La Barbera, A.
A1  - Lelas, D.
A1  - Leonardo, E.
A1  - Lindfors, E.
A1  - Lombardi, S.
A1  - Lopez, M.
A1  - Lorenz, E.
A1  - Makariev, M.
A1  - Maneva, G.
A1  - Mankuzhiyil, N.
A1  - Mannheim, K.
A1  - Maraschi, L.
A1  - Mariotti, M.
A1  - Martinez, M.
A1  - Mazin, D.
A1  - Meucci, M.
A1  - Miranda, J. M.
A1  - Mirzoyan, R.
A1  - Miyamoto, H.
A1  - Moldon, J.
A1  - Moralejo, A.
A1  - Munar, P.
A1  - Nieto, D.
A1  - Nilsson, K.
A1  - Orito, R.
A1  - Oya, I.
A1  - Paneque, D.
A1  - Paoletti, R.
A1  - Pardo, S.
A1  - Paredes, J. M.
A1  - Partini, S.
A1  - Pasanen, M.
A1  - Pauss, F.
A1  - Perez-Torres, M. A.
A1  - Persic, M.
A1  - Peruzzo, L.
A1  - Pilia, M.
A1  - Pochon, J.
A1  - Prada, F.
A1  - Moroni, P. G. Prada
A1  - Prandini, E.
A1  - Puljak, I.
A1  - Reichardt, I.
A1  - Reinthal, R.
A1  - Rhode, W.
A1  - Ribo, M.
A1  - Rico, J.
A1  - Ruegamer, S.
A1  - Saggion, A.
A1  - Saito, K.
A1  - Saito, T. Y.
A1  - Salvati, M.
A1  - Satalecka, K.
A1  - Scalzotto, V.
A1  - Scapin, V.
A1  - Schultz, C.
A1  - Schweizer, T.
A1  - Shayduk, M.
A1  - Shore, S. N.
A1  - Sillanpaa, A.
A1  - Sitarek, J.
A1  - Sobczynska, D.
A1  - Spanier, F.
A1  - Spiro, S.
A1  - Stamerra, A.
A1  - Steinke, B.
A1  - Storz, J.
A1  - Strah, N.
A1  - Suric, T.
A1  - Takalo, L.
A1  - Takami, H.
A1  - Tavecchio, F.
A1  - Temnikov, P.
A1  - Terzic, T.
A1  - Tescaro, D.
A1  - Teshima, M.
A1  - Thom, M.
A1  - Tibolla, O.
A1  - Torres, D. F.
A1  - Treves, A.
A1  - Vankov, H.
A1  - Vogler, P.
A1  - Wagner, R. M.
A1  - Weitzel, Q.
A1  - Zabalza, V.
A1  - Zandanel, F.
A1  - Zanin, R.
A1  - Arlen, T.
A1  - Aune, T.
A1  - Beilicke, M.
A1  - Benbow, W.
A1  - Bouvier, A.
A1  - Bradbury, S. M.
A1  - Buckley, J. H.
A1  - Bugaev, V.
A1  - Byrum, K.
A1  - Cannon, A.
A1  - Cesarini, A.
A1  - Ciupik, L.
A1  - Connolly, M. P.
A1  - Cui, W.
A1  - Dickherber, R.
A1  - Duke, C.
A1  - Errando, M.
A1  - Falcone, A.
A1  - Finley, J. P.
A1  - Finnegan, G.
A1  - Fortson, L.
A1  - Furniss, A.
A1  - Galante, N.
A1  - Gall, D.
A1  - Godambe, S.
A1  - Griffin, S.
A1  - Grube, J.
A1  - Gyuk, G.
A1  - Hanna, D.
A1  - Holder, J.
A1  - Huan, H.
A1  - Hui, C. M.
A1  - Kaaret, P.
A1  - Karlsson, N.
A1  - Kertzman, M.
A1  - Khassen, Y.
A1  - Kieda, D.
A1  - Krawczynski, H.
A1  - Krennrich, F.
A1  - Lang, M. J.
A1  - LeBohec, S.
A1  - Maier, G.
A1  - McArthur, S.
A1  - McCann, A.
A1  - Moriarty, P.
A1  - Mukherjee, R.
A1  - Nunez, P. D.
A1  - Ong, R. A.
A1  - Orr, M.
A1  - Otte, A. N.
A1  - Park, N.
A1  - Perkins, J. S.
A1  - Pichel, A.
A1  - Pohl, Martin
A1  - Prokoph, H.
A1  - Ragan, K.
A1  - Reyes, L. C.
A1  - Reynolds, P. T.
A1  - Roache, E.
A1  - Rose, H. J.
A1  - Ruppel, J.
A1  - Schroedter, M.
A1  - Sembroski, G. H.
A1  - Sentuerk, G. D.
A1  - Telezhinsky, Igor O.
A1  - Tesic, G.
A1  - Theiling, M.
A1  - Thibadeau, S.
A1  - Varlotta, A.
A1  - Vassiliev, V. V.
A1  - Vivier, M.
A1  - Wakely, S. P.
A1  - Weekes, T. C.
A1  - Williams, D. A.
A1  - Zitzer, B.
A1  - de Almeida, U. Barres
A1  - Cara, M.
A1  - Casadio, C.
A1  - Cheung, C. C.
A1  - McConville, W.
A1  - Davies, F.
A1  - Doi, A.
A1  - Giovannini, G.
A1  - Giroletti, M.
A1  - Hada, K.
A1  - Hardee, P.
A1  - Harris, D. E.
A1  - Junor, W.
A1  - Kino, M.
A1  - Lee, N. P.
A1  - Ly, C.
A1  - Madrid, J.
A1  - Massaro, F.
A1  - Mundell, C. G.
A1  - Nagai, H.
A1  - Perlman, E. S.
A1  - Steele, I. A.
A1  - Walker, R. C.
A1  - Wood, D. L.
T1  - The 2010 very high energy gamma-ray flare and 10 years ofmulti-wavelength oservations of M 87
JF  - The astrophysical journal : an international review of spectroscopy and astronomical physics
N2  - The giant radio galaxy M 87 with its proximity (16 Mpc), famous jet, and very massive black hole ((3-6) x 10(9) M-circle dot) provides a unique opportunity to investigate the origin of very high energy (VHE; E > 100 GeV) gamma-ray emission generated in relativistic outflows and the surroundings of supermassive black holes. M 87 has been established as a VHE gamma-ray emitter since 2006. The VHE gamma-ray emission displays strong variability on timescales as short as a day. In this paper, results from a joint VHE monitoring campaign on M 87 by the MAGIC and VERITAS instruments in 2010 are reported. During the campaign, a flare at VHE was detected triggering further observations at VHE (H.E.S.S.), X-rays (Chandra), and radio (43 GHz Very Long Baseline Array, VLBA). The excellent sampling of the VHE gamma-ray light curve enables one to derive a precise temporal characterization of the flare: the single, isolated flare is well described by a two-sided exponential function with significantly different flux rise and decay times of tau(rise)(d) = (1.69 +/- 0.30) days and tau(decay)(d) = (0.611 +/- 0.080) days, respectively. While the overall variability pattern of the 2010 flare appears somewhat different from that of previous VHE flares in 2005 and 2008, they share very similar timescales (similar to day), peak fluxes (Phi(>0.35 TeV) similar or equal to (1-3) x 10(-11) photons cm(-2) s(-1)), and VHE spectra. VLBA radio observations of 43 GHz of the inner jet regions indicate no enhanced flux in 2010 in contrast to observations in 2008, where an increase of the radio flux of the innermost core regions coincided with a VHE flare. On the other hand, Chandra X-ray observations taken similar to 3 days after the peak of the VHE gamma-ray emission reveal an enhanced flux from the core (flux increased by factor similar to 2; variability timescale <2 days). The long-term (2001-2010) multi-wavelength (MWL) light curve of M 87, spanning from radio to VHE and including data from Hubble Space Telescope, Liverpool Telescope, Very Large Array, and European VLBI Network, is used to further investigate the origin of the VHE gamma-ray emission. No unique, common MWL signature of the three VHE flares has been identified. In the outer kiloparsec jet region, in particular in HST-1, no enhanced MWL activity was detected in 2008 and 2010, disfavoring it as the origin of the VHE flares during these years. Shortly after two of the three flares (2008 and 2010), the X-ray core was observed to be at a higher flux level than its characteristic range (determined from more than 60 monitoring observations: 2002-2009). In 2005, the strong flux dominance of HST-1 could have suppressed the detection of such a feature. Published models for VHE gamma-ray emission from M 87 are reviewed in the light of the new data.
KW  - galaxies: active
KW  - galaxies: individual (M 87)
KW  - galaxies: jets
KW  - galaxies: nuclei
KW  - gamma rays: galaxies
KW  - radiation mechanisms: non-thermal
Y1  - 2012
U6  - https://doi.org/10.1088/0004-637X/746/2/151
SN  - 0004-637X
VL  - 746
IS  - 2
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Adamcik, Jozef
A1  - Jeon, Jae-Hyung
A1  - Karczewski, Konrad J.
A1  - Metzler, Ralf
A1  - Dietler, Giovanni
T1  - Quantifying supercoiling-induced denaturation bubbles in DNA
JF  - Soft matter
N2  - In both eukaryotic and prokaryotic DNA sequences of 30-100 base-pairs rich in AT base-pairs have been identified at which the double helix preferentially unwinds. Such DNA unwinding elements are commonly associated with origins for DNA replication and transcription, and with chromosomal matrix attachment regions. Here we present a quantitative study of local DNA unwinding based on extensive single DNA plasmid imaging. We demonstrate that long-lived single-stranded denaturation bubbles exist in negatively supercoiled DNA, at the expense of partial twist release. Remarkably, we observe a linear relation between the degree of supercoiling and the bubble size, in excellent agreement with statistical modelling. Furthermore, we obtain the full distribution of bubble sizes and the opening probabilities at varying salt and temperature conditions. The results presented herein underline the important role of denaturation bubbles in negatively supercoiled DNA for biological processes such as transcription and replication initiation in vivo.
Y1  - 2012
U6  - https://doi.org/10.1039/c2sm26089a
SN  - 1744-683X
VL  - 8
IS  - 33
SP  - 8651
EP  - 8658
PB  - Royal Society of Chemistry
CY  - Cambridge
ER  - 
TY  - JOUR
A1  - Al-Sa'di, Mahmoud
A1  - Jaiser, Frank
A1  - Bagnich, Sergey A.
A1  - Unger, Thomas
A1  - Blakesley, James C.
A1  - Wilke, Andreas
A1  - Neher, Dieter
T1  - Electrical and optical simulations of a polymer-based phosphorescent organic light-emitting diode with high efficiency
JF  - Journal of polymer science : B, Polymer physics
N2  - A comprehensive numerical device simulation of the electrical and optical characteristics accompanied with experimental measurements of a new highly efficient system for polymer-based light-emitting diodes doped with phosphorescent dyes is presented. The system under investigation comprises an electron transporter attached to a polymer backbone blended with an electronically inert small molecule and an iridium-based green phosphorescent dye which serves as both emitter and hole transporter. The device simulation combines an electrical and an optical model. Based on the known highest occupied molecular orbital (HOMO) and lowest unoccupied molecular orbital (LUMO) levels of all components as well as the measured electrical and optical characteristics of the devices, we model the emissive layer as an effective medium using the dye's HOMO as hole transport level and the polymer LUMO as electron transport level. By fine-tuning the injection barriers at the electron and hole-injecting contact, respectively, in simulated devices, unipolar device characteristics were fitted to the experimental data. Simulations using the so-obtained set of parameters yielded very good agreement to the measured currentvoltage, luminancevoltage characteristics, and the emission profile of entire bipolar light-emitting diodes, without additional fitting parameters. The simulation was used to gain insight into the physical processes and the mechanisms governing the efficiency of the organic light-emitting diode, including the position and extent of the recombination zone, carrier concentration profiles, and field distribution inside the device. The simulations show that the device is severely limited by hole injection, and that a reduction of the hole-injection barrier would improve the device efficiency by almost 50%.
KW  - conjugated polymers
KW  - high performance polymers
KW  - organic electronics
KW  - organic light-emitting diode
KW  - simulations
KW  - TCAD
Y1  - 2012
U6  - https://doi.org/10.1002/polb.23158
SN  - 0887-6266
VL  - 50
IS  - 22
SP  - 1567
EP  - 1576
PB  - Wiley-Blackwell
CY  - Hoboken
ER  - 
TY  - JOUR
A1  - Albrecht, Steve
A1  - Janietz, Silvia
A1  - Schindler, Wolfram
A1  - Frisch, Johannes
A1  - Kurpiers, Jona
A1  - Kniepert, Juliane
A1  - Inal, Sahika
A1  - Pingel, Patrick
A1  - Fostiropoulos, Konstantinos
A1  - Koch, Norbert
A1  - Neher, Dieter
T1  - Fluorinated Copolymer PCPDTBT with enhanced open-circuit voltage and reduced recombination for highly efficient polymer solar cells
JF  - Journal of the American Chemical Society
N2  - A novel fluorinated copolymer (F-PCPDTBT) is introduced and shown to exhibit significantly higher power conversion efficiency in bulk heterojunction solar cells with PC70BM compared to the well-known low-band-gap polymer PCPDTBT. Fluorination lowers the polymer HOMO level, resulting in high open-circuit voltages well exceeding 0.7 V. Optical spectroscopy and morphological studies with energy-resolved transmission electron microscopy reveal that the fluorinated polymer aggregates more strongly in pristine and blended layers, with a smaller amount of additives needed to achieve optimum device performance. Time-delayed collection field and charge extraction by linearly increasing voltage are used to gain insight into the effect of fluorination on the field dependence of free charge-carrier generation and recombination. F-PCPDTBT is shown to exhibit a significantly weaker field dependence of free charge-carrier generation combined with an overall larger amount of free charges, meaning that geminate recombination is greatly reduced. Additionally, a 3-fold reduction in non-geminate recombination is measured compared to optimized PCPDTBT blends. As a consequence of reduced non-geminate recombination, the performance of optimized blends of fluorinated PCPDTBT with PC70BM is largely determined by the field dependence of free-carrier generation, and this field dependence is considerably weaker compared to that of blends comprising the non-fluorinated polymer. For these optimized blends, a short-circuit current of 14 mA/cm(2), an open-circuit voltage of 0.74 V, and a fill factor of 58% are achieved, giving a highest energy conversion efficiency of 6.16%. The superior device performance and the low band-gap render this new polymer highly promising for the construction of efficient polymer-based tandem solar cells.
Y1  - 2012
U6  - https://doi.org/10.1021/ja305039j
SN  - 0002-7863
VL  - 134
IS  - 36
SP  - 14932
EP  - 14944
PB  - American Chemical Society
CY  - Washington
ER  - 
TY  - JOUR
A1  - Albrecht, Steve
A1  - Schaefer, Sebastian
A1  - Lange, Ilja
A1  - Yilmaz, Seyfullah
A1  - Dumsch, Ines
A1  - Allard, Sybille
A1  - Scherf, Ullrich
A1  - Hertwig, Andreas
A1  - Neher, Dieter
T1  - Light management in PCPDTBT:PC70BM solar cells: A comparison of standard and inverted device structures
JF  - Organic electronics : physics, materials and applications
N2  - We compare standard and inverted bulk heterojunction solar cells composed of PCPDTBT:PC70BM blends. Inverted devices comprising 100 nm thick active layers exhibited short circuit currents of 15 mA/cm(2), 10% larger than in corresponding standard devices. Modeling of the optical field distribution in the different device stacks proved that this enhancement originates from an increased absorption of incident light in the active layer. Internal quantum efficiencies (IQEs) were obtained from the direct comparison of experimentally derived and modeled currents for different layer thicknesses, yielding IQEs of similar to 70% for a layer thickness of 100 nm. Simulations predict a significant increase of the light harvesting efficiency upon increasing the layer thickness to 270 nm. However, a continuous deterioration of the photovoltaic properties with layer thickness was measured for both device architectures, attributed to incomplete charge extraction. On the other hand, our optical modeling suggests that inverted devices based on PCPDTBT should be able to deliver high power conversion efficiencies (PCEs) of more than 7% provided that recombination losses can be reduced.
KW  - Organic solar cells
KW  - Inverted solar cells
KW  - PCPDTBT
KW  - Low band-gap
KW  - Optical modeling
Y1  - 2012
U6  - https://doi.org/10.1016/j.orgel.2011.12.019
SN  - 1566-1199
VL  - 13
IS  - 4
SP  - 615
EP  - 622
PB  - Elsevier
CY  - Amsterdam
ER  - 
TY  - JOUR
A1  - Albrecht, Steve
A1  - Schindler, Wolfram
A1  - Kurpiers, Jona
A1  - Kniepert, Juliane
A1  - Blakesley, James C.
A1  - Dumsch, Ines
A1  - Allard, Sybille
A1  - Fostiropoulos, Konstantinos
A1  - Scherf, Ullrich
A1  - Neher, Dieter
T1  - On the field dependence of free charge carrier generation and recombination in blends of PCPDTBT/PC70BM influence of solvent additives
JF  - The journal of physical chemistry letters
N2  - We have applied time-delayed collection field (TDCF) and charge extraction by linearly increasing voltage (CELIV) to investigate the photogeneration, transport, and recombination of charge carriers in blends composed of PCPDTBT/PC70BM processed with and without the solvent additive diiodooctane. The results suggest that the solvent additive has severe impacts on the elementary processes involved in the photon to collected electron conversion in these blends. First, a pronounced field dependence of the free carrier generation is found for both blends, where the field dependence is stronger without the additive. Second, the fate of charge carriers in both blends can be described with a rather high bimolecular recombination coefficients, which increase with decreasing internal field. Third, the mobility is three to four times higher with the additive. Both blends show a negative field dependence of mobility, which we suggest to cause bias-dependent recombination coefficients.
Y1  - 2012
U6  - https://doi.org/10.1021/jz3000849
SN  - 1948-7185
VL  - 3
IS  - 5
SP  - 640
EP  - 645
PB  - American Chemical Society
CY  - Washington
ER  - 
TY  - JOUR
A1  - Albrecht, Torsten
A1  - Levermann, Anders
T1  - Fracture field for large-scale ice dynamics
JF  - Journal of glaciology
N2  - Recent observations and modeling studies emphasize the crucial role of fracture mechanics for the stability of ice shelves and thereby the evolution of ice sheets. Here we introduce a macroscopic fracture-density field into a prognostic continuum ice-flow model and compute its evolution incorporating the initiation and growth of fractures as well as their advection with two-dimensional ice flow. To a first approximation, fracture growth is assumed to depend on the spreading rate only, while fracture initiation is defined in terms of principal stresses. The inferred fracture-density fields compare well with observed elongate surface structures. Since crevasses and other deep-reaching fracture structures have been shown to influence the overall ice-shelf dynamics, we propose the fracture-density field introduced here be used as a measure for ice softening and decoupling of the ice flow in fracture-weakened zones. This may yield more accurate and realistic velocity patterns in prognostic simulations. Additionally, the memory of past fracture events links the calving front to the upstream dynamics. Thus the fracture-density field proposed here may be employed in fracture-based calving parameterizations. The aim of this study is to introduce the field and investigate which of the observed surface structures can be reproduced by the simplest physically motivated fracture source terms.
Y1  - 2012
U6  - https://doi.org/10.3189/2012JoG11J191
SN  - 0022-1430
SN  - 1727-5652
VL  - 58
IS  - 207
SP  - 165
EP  - 176
PB  - International Glaciological Society
CY  - Cambridge
ER  - 
TY  - JOUR
A1  - Aliu, E.
A1  - Archambault, S.
A1  - Arlen, T.
A1  - Aune, T.
A1  - Beilicke, M.
A1  - Benbow, W.
A1  - Boettcher, Markus
A1  - Bouvier, A.
A1  - Bradbury, S. M.
A1  - Buckley, J. H.
A1  - Bugaev, V.
A1  - Byrum, K.
A1  - Cannon, A.
A1  - Cesarini, A.
A1  - Ciupik, L.
A1  - Collins-Hughes, E.
A1  - Connolly, M. P.
A1  - Coppi, P.
A1  - Cui, W.
A1  - Decerprit, G.
A1  - Dickherber, R.
A1  - Dumm, J.
A1  - Errando, Manel
A1  - Falcone, A.
A1  - Feng, Q.
A1  - Finley, J. P.
A1  - Finnegan, G.
A1  - Fortson, L.
A1  - Furniss, A.
A1  - Galante, N.
A1  - Gall, D.
A1  - Godambe, S.
A1  - Griffin, S.
A1  - Grube, J.
A1  - Gyuk, G.
A1  - Hanna, D.
A1  - Hawkins, K.
A1  - Holder, J.
A1  - Huan, H.
A1  - Hughes, G.
A1  - Humensky, T. B.
A1  - Kaaret, P.
A1  - Karlsson, N.
A1  - Kertzman, M.
A1  - Khassen, Y.
A1  - Kieda, D.
A1  - Krawczynski, H.
A1  - Krennrich, F.
A1  - Lang, M. J.
A1  - Lee, K.
A1  - Madhavan, A. S.
A1  - Maier, G.
A1  - Majumdar, P.
A1  - McArthur, S.
A1  - McCann, A.
A1  - Moriarty, P.
A1  - Mukherjee, Reshmi
A1  - Ong, R. A.
A1  - Orr, M.
A1  - Otte, A. N.
A1  - Palma, N.
A1  - Park, N.
A1  - Perkins, J. S.
A1  - Pichel, A.
A1  - Pohl, Martin
A1  - Prokoph, H.
A1  - Quinn, J.
A1  - Ragan, K.
A1  - Reyes, L. C.
A1  - Reynolds, P. T.
A1  - Roache, E.
A1  - Rose, H. J.
A1  - Ruppel, J.
A1  - Saxon, D. B.
A1  - Schroedter, M.
A1  - Sembroski, G. H.
A1  - Sentuerk, G. D.
A1  - Smith, A. W.
A1  - Staszak, D.
A1  - Telezhinsky, Igor O.
A1  - Tesic, G.
A1  - Theiling, M.
A1  - Thibadeau, S.
A1  - Tsurusaki, K.
A1  - Varlotta, A.
A1  - Vivier, M.
A1  - Wakely, S. P.
A1  - Ward, J. E.
A1  - Weekes, T. C.
A1  - Weinstein, A.
A1  - Weisgarber, T.
A1  - Williams, D. A.
A1  - Zitzer, B.
A1  - Fortin, P.
A1  - Horan, D.
T1  - Disovery of high-energy and very high energy gamma-ray emission from the blazar RBS 0413
JF  - The astrophysical journal : an international review of spectroscopy and astronomical physics
N2  - We report on the discovery of high-energy (HE; E > 0.1 GeV) and very high energy (VHE; E > 100 GeV) gamma-ray emission from the high-frequency-peaked BL Lac object RBS 0413. VERITAS, a ground-based gamma-ray observatory, detected VHE. rays from RBS 0413 with a statistical significance of 5.5 standard deviations (sigma) and a gamma-ray flux of (1.5 +/- 0.6(stat) +/- 0.7(syst)) x 10(-8) photons m(-2) s(-1) (similar to 1% of the Crab Nebula flux) above 250 GeV. The observed spectrum can be described by a power law with a photon index of 3.18 +/- 0.68(stat) +/- 0.30(syst). Contemporaneous observations with the Large Area Telescope (LAT) on the Fermi Gamma-ray Space Telescope detected HE gamma rays from RBS 0413 with a (stat)istical significance of more than 9 sigma, a power-law photon index of 1.57 +/- 0.12(stat-0.12sys')(+0.11) and a gamma-ray flux between 300 MeV and 300 GeV of (1.64 +/- 0.43(stat-0.22sys)(+ 0.31)) x 10(-5) photons m(-2) s(-1). We present the results from Fermi-LAT and VERITAS, including a spectral energy distribution modeling of the gamma-ray, quasi-simultaneous X-ray (Swift-XRT), ultraviolet (Swift-UVOT), and R-band optical (MDM) data. We find that, if conditions close to equipartition are required, both the combined synchrotron self-Compton/external-Compton and the lepto-hadronic models are preferred over a pure synchrotron self-Compton model.
KW  - BL Lacertae objects: individual (RBS 0413-VER J0319+187)
KW  - gamma rays: galaxies
Y1  - 2012
U6  - https://doi.org/10.1088/0004-637X/750/2/94
SN  - 0004-637X
VL  - 750
IS  - 2
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Aliu, E.
A1  - Archambault, S.
A1  - Arlen, T.
A1  - Aune, T.
A1  - Beilicke, M.
A1  - Benbow, W.
A1  - Boettcher, Markus
A1  - Bouvier, A.
A1  - Buckley, J. H.
A1  - Bugaev, V.
A1  - Cesarini, A.
A1  - Ciupik, L.
A1  - Collins-Hughes, E.
A1  - Connolly, M. P.
A1  - Cui, W.
A1  - Dickherber, R.
A1  - Duke, C.
A1  - Dumm, J.
A1  - Errando, M.
A1  - Falcone, A.
A1  - Federici, Simone
A1  - Feng, Q.
A1  - Finley, J. P.
A1  - Finnegan, G.
A1  - Fortson, L.
A1  - Furniss, A.
A1  - Galante, N.
A1  - Gall, D.
A1  - Godambe, S.
A1  - Griffin, S.
A1  - Grube, J.
A1  - Gyuk, G.
A1  - Hanna, D.
A1  - Holder, J.
A1  - Huan, H.
A1  - Kaaret, P.
A1  - Karlsson, N.
A1  - Khassen, Y.
A1  - Kieda, D.
A1  - Krawczynski, H.
A1  - Krennrich, F.
A1  - Lee, K.
A1  - Madhavan, A. S.
A1  - Maier, G.
A1  - Majumdar, P.
A1  - McArthur, S.
A1  - McCann, A.
A1  - Moriarty, P.
A1  - Mukherjee, R.
A1  - Nelson, T.
A1  - de Bhroithe, A. O'Faolain
A1  - Ong, R. A.
A1  - Orr, M.
A1  - Otte, A. N.
A1  - Park, N.
A1  - Perkins, J. S.
A1  - Pichel, A.
A1  - Pohl, Martin
A1  - Prokoph, H.
A1  - Quinn, J.
A1  - Ragan, K.
A1  - Reyes, L. C.
A1  - Reynolds, P. T.
A1  - Roache, E.
A1  - Saxon, D. B.
A1  - Sembroski, G. H.
A1  - Staszak, D.
A1  - Telezhinsky, Igor O.
A1  - Tesic, G.
A1  - Theiling, M.
A1  - Thibadeau, S.
A1  - Tsurusaki, K.
A1  - Varlotta, A.
A1  - Vassiliev, V. V.
A1  - Vincent, S.
A1  - Vivier, M.
A1  - Wakely, S. P.
A1  - Weekes, T. C.
A1  - Weinstein, A.
A1  - Welsing, R.
A1  - Williams, D. A.
A1  - Zitzer, B.
A1  - Fortin, P.
A1  - Horan, D.
A1  - Fumagalli, M.
A1  - Kaplan, K.
A1  - Prochaska, J. X.
T1  - Veritas observations of six bright, hard-spectrum fermi-lat blazars
JF  - The astrophysical journal : an international review of spectroscopy and astronomical physics
N2  - We report on VERITAS very high energy (VHE; E >= 100 GeV) observations of six blazars selected from the Fermi Large Area Telescope First Source Catalog (1FGL). The gamma-ray emission from 1FGL sources was extrapolated up to the VHE band, taking gamma-ray absorption by the extragalactic background light into account. This allowed the selection of six bright, hard-spectrum blazars that were good candidate TeV emitters. Spectroscopic redshift measurements were attempted with the Keck Telescope for the targets without Sloan Digital Sky Survey spectroscopic data. No VHE emission is detected during the observations of the six sources described here. Corresponding TeV upper limits are presented, along with contemporaneous Fermi observations and non-concurrent Swift UVOT and X-Ray Telescope data. The blazar broadband spectral energy distributions (SEDs) are assembled and modeled with a single-zone synchrotron self-Compton model. The SED built for each of the six blazars shows a synchrotron peak bordering between the intermediate-and high-spectrum-peak classifications, with four of the six resulting in particle-dominated emission regions.
KW  - BL Lacertae objects: general
KW  - gamma rays: galaxies
Y1  - 2012
U6  - https://doi.org/10.1088/0004-637X/759/2/102
SN  - 0004-637X
VL  - 759
IS  - 2
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  -