TY  - JOUR
A1  - Navirian, Hengameh A.
A1  - Herzog, Marc
A1  - Goldshteyn, J.
A1  - Leitenberger, Wolfram
A1  - Vrejoiu, Ionella
A1  - Khakhulin, D.
A1  - Wulff, M.
A1  - Shayduk, Roman
A1  - Gaal, P.
A1  - Bargheer, Matias
T1  - Shortening x-ray pulses for pump-probe experiments at synchrotrons
JF  - Journal of applied physics
N2  - We implemented an experimental scheme for ultrafast x-ray diffraction at storage rings based on a laser-driven Bragg-switch that shortens the x-ray pulses emitted from an undulator. The increased time-resolution is demonstrated by observing changes of intensity, position and width of the diffraction peaks of a La(0.7)Sr(0.3)MnO(3)/SrTiO(3) superlattice sample after optical excitation, i.e., by quantitatively measuring the propagation of an expansion wave through the sample. These experimental transients with timescales of 35 to 60 ps evidence a reduction of the x-ray pulse duration by a factor of two.
Y1  - 2011
U6  - https://doi.org/10.1063/1.3601057
SN  - 0021-8979
VL  - 109
IS  - 12
PB  - American Institute of Physics
CY  - Melville
ER  - 
TY  - JOUR
A1  - Kar, Parimal
A1  - Lipowsky, Reinhard
A1  - Knecht, Volker
T1  - Importance of polar solvation for cross-reactivity of antibody and its variants with steroids
JF  - The journal of physical chemistry : B, Condensed matter, materials, surfaces, interfaces & biophysical chemistry
N2  - Understanding the factors determining the binding of ligands to receptors in detail is essential for rational drug design. Here, the free energies of binding of the steroids progesterone (PRG) and 5 beta-androstane-3,17-dione (SAD) to the Diels-Alderase antibody 1E9, as well as the Leu(H47)Trp/Arg(H100)Trp 1E9 double mutant (1E9dm) and the corresponding single mutants, have been estimated and decomposed using the molecular mechanics-Poisson-Boltzmann surface area (MM-PBSA) method. Also the difference in binding free energies between the PRG-1E9dm complex and the complex of PRG with the antiprogesterone antibody DB3 have been evaluated and decomposed. The steroids bind less strongly to 1E9 than to DB3, but the mutations tend to improve the steroid affinity, in quantitative agreement with experimental data. Although the complexes formed by PRG or SAD with 1E9dm and by PRG with DB3 have similar affinity, the binding mechanisms are different. Reduced Waals for SAD-1E9dm versus PRG-1E9dm or for PRG-1E9dm versus PRG-DB3 are energetically compensated by an increased solvation of polar groups, partly contrasting previous conclusions based on structural inspection. Our study illustrates that deducing binding mechanisms from structural models alone can be misleading. Therefore, taking into account solvation effects as in MM-PBSA calculations is essential to elucidate molecular recognition.
Y1  - 2011
U6  - https://doi.org/10.1021/jp201538t
SN  - 1520-6106
VL  - 115
IS  - 23
SP  - 7661
EP  - 7669
PB  - American Chemical Society
CY  - Washington
ER  - 
TY  - JOUR
A1  - Postberg, Frank
A1  - Schmidt, J.
A1  - Hillier, J.
A1  - Kempf, Sascha
A1  - Srama, Ralf
T1  - A salt-water reservoir as the source of a compositionally stratified plume on Enceladus
JF  - Nature : the international weekly journal of science
N2  - The discovery of a plume of water vapour and ice particles emerging from warm fractures ('tiger stripes') in Saturn's small, icy moon Enceladus(1-6) raised the question of whether the plume emerges from a subsurface liquid source(6-8) or from the decomposition of ice(9-12). Previous compositional analyses of particles injected by the plume into Saturn's diffuse E ring have already indicated the presence of liquid water(8), but the mechanisms driving the plume emission are still debated(13). Here we report an analysis of the composition of freshly ejected particles close to the sources. Salt-rich ice particles are found to dominate the total mass flux of ejected solids (more than 99 per cent) but they are depleted in the population escaping into Saturn's E ring. Ice grains containing organic compounds are found to be more abundant in dense parts of the plume. Whereas previous Cassini observations were compatible with a variety of plume formation mechanisms, these data eliminate or severely constrain non-liquid models and strongly imply that a salt-water reservoir with a large evaporating surface(7,8) provides nearly all of the matter in the plume.
Y1  - 2011
U6  - https://doi.org/10.1038/nature10175
SN  - 0028-0836
VL  - 474
IS  - 7353
SP  - 620
EP  - 622
PB  - Nature Publ. Group
CY  - London
ER  - 
TY  - JOUR
A1  - Baumgärtel, Hellmut
T1  - A Characteristic decay semigroup for the resonances of trace class perturbations with analyticity conditions of semibounded hamiltonians
JF  - International journal of theoretical physic
N2  - To asymptotic complete scattering systems {M(+) + V, M(+)} on H(+) := L(2)(R(+), K, d lambda), where M(+) is the multiplication operator on H(+) and V is a trace class operator with analyticity conditions, a decay semigroup is associated such that the spectrum of the generator of this semigroup coincides with the set of all resonances (poles of the analytic continuation of the scattering matrix into the lower half plane across the positive half line), i.e. the decay semigroup yields a "time-dependent" characterization of the resonances. As a counterpart a "spectral characterization" is mentioned which is due to the "eigenvalue-like" properties of resonances.
KW  - Resonances
KW  - Scattering theory
KW  - Lax-Phillips theory
KW  - Decay semigroups
Y1  - 2011
U6  - https://doi.org/10.1007/s10773-010-0533-9
SN  - 0020-7748
VL  - 50
IS  - 7
SP  - 2002
EP  - 2008
PB  - Springer
CY  - New York
ER  - 
TY  - JOUR
A1  - Delahaye, T.
A1  - Fiasson, A.
A1  - Pohl, Martin
A1  - Salati, P.
T1  - The GeV-TeV Galactic gamma-ray diffuse emission I. Uncertainties in the predictions of the hadronic component
JF  - Astronomy and astrophysics : an international weekly journal
N2  - Context. The Galactic gamma-ray diffuse emission is currently observed in the GeV-TeV energy range with unprecedented accuracy by the Fermi satellite. Understanding this component is crucial because it provides a background to many different signals, such as extragalactic sources or annihilating dark matter. It is timely to reinvestigate how it is calculated and to assess the various uncertainties that are likely to affect the accuracy of the predictions.
 Aims. The Galactic gamma-ray diffuse emission is mostly produced above a few GeV by the interactions of cosmic ray primaries impinging on the interstellar material. The theoretical error on that component is derived by exploring various potential sources of uncertainty. Particular attention is paid to cosmic ray propagation. Nuclear cross sections, the proton and helium fluxes at the Earth's position, the Galactic radial profile of supernova remnants, and the hydrogen distribution can also severely affect the signal.
 Methods. The propagation of cosmic ray species throughout the Galaxy is described in the framework of a semi-analytic two-zone diffusion/convection model. The gamma-ray flux is reliably and quickly determined. This allows conversion of the constraints set by the boron-to-carbon data into a theoretical uncertainty on the diffuse emission. New deconvolutions of the HI and CO sky maps are also used to get the hydrogen distribution within the Galaxy.
 Results. The thickness of the cosmic ray diffusive halo is found to have a significant effect on the Galactic gamma-ray diffuse emission, while the interplay between diffusion and convection has little influence on the signal. The uncertainties related to nuclear cross sections and to the primary cosmic ray fluxes at the Earth are significant. The radial distribution of supernova remnants along the Galactic plane turns out to be a key ingredient. As expected, the predictions are extremely sensitive to the spatial distribution of hydrogen within the Milky Way.
 Conclusions. Most of the sources of uncertainty are likely to be reduced in the near future. The stress should be put (i) on better determination of the thickness of the cosmic ray diffusive halo; and (ii) on refined observations of the radial profile of supernova remnants.
KW  - gamma rays: diffuse background
KW  - cosmic rays
KW  - methods: analytical
KW  - gamma rays: ISM
Y1  - 2011
U6  - https://doi.org/10.1051/0004-6361/201116647
SN  - 0004-6361
VL  - 531
IS  - 4
PB  - EDP Sciences
CY  - Les Ulis
ER  - 
TY  - JOUR
A1  - Kappel, Marcel
A1  - Abel, Markus
A1  - Gerhard, Reimund
T1  - Characterization and calibration of piezoelectric polymers in situ measurements of body vibrations
JF  - Review of scientific instruments : a monthly journal devoted to scientific instruments, apparatus, and techniques
N2  - Piezoelectric polymers are known for their flexibility in applications, mainly due to their bending ability, robustness, and variable sensor geometry. It is an optimal material for minimal-invasive investigations in vibrational systems, e.g., for wood, where acoustical impedance matches particularly well. Many applications may be imagined, e. g., monitoring of buildings, vehicles, machinery, alarm systems, such that our investigations may have a large impact on technology. Longitudinal piezoelectricity converts mechanical vibrations normal to the polymer-film plane into an electrical signal, and the respective piezoelectric coefficient needs to be carefully determined in dependence on the relevant material parameters. In order to evaluate efficiency and durability for piezopolymers, we use polyvinylidene fluoride and measure the piezoelectric coefficient with respect to static pressure, amplitude of the dynamically applied force, and long-term stability. A known problem is the slow relaxation of the material towards equilibrium, if the external pressure changes; here, we demonstrate how to counter this problem with careful calibration. Since our focus is on acoustical measurements, we determine accurately the frequency response curve - for acoustics probably the most important characteristic. Eventually, we show that our piezopolymer transducers can be used as a calibrated acoustical sensors for body vibration measurements on a wooden musical instrument, where it is important to perform minimal-invasive measurements. A comparison with the simultaneously recorded airborne sound yields important insight of the mechanism of sound radiation in comparison with the sound propagating in the material. This is especially important for transient signals, where not only the long-living eigenmodes contribute to the sound radiation. Our analyses support that piezopolymer sensors can be employed as a general tool for the determination of the internal dynamics of vibrating systems.
KW  - acoustic transducers
KW  - calibration
KW  - durability
KW  - electric sensing devices
KW  - piezoelectricity
KW  - polymers
Y1  - 2011
U6  - https://doi.org/10.1063/1.3607435
SN  - 0034-6748
VL  - 82
IS  - 7
PB  - American Institute of Physics
CY  - Melville
ER  - 
TY  - JOUR
A1  - Lueck, S.
A1  - Pikovskij, Arkadij
T1  - Dynamics of multi-frequency oscillator ensembles with resonant coupling
JF  - Modern physics letters : A, Particles and fields, gravitation, cosmology, nuclear physics
N2  - We study dynamics of populations of resonantly coupled oscillators having different frequencies. Starting from the coupled van der Pol equations we derive the Kuramoto-type phase model for the situation, where the natural frequencies of two interacting subpopulations are in relation 2 : 1. Depending on the parameter of coupling, ensembles can demonstrate fully synchronous clusters, partial synchrony (only one subpopulation synchronizes), or asynchrony in both subpopulations. Theoretical description of the dynamics based on the Watanabe-Strogatz approach is developed.
KW  - Oscillator populations
KW  - Kuramoto model
KW  - Resonant interaction
Y1  - 2011
U6  - https://doi.org/10.1016/j.physleta.2011.06.016
SN  - 0375-9601
VL  - 375
IS  - 28-29
SP  - 2714
EP  - 2719
PB  - Elsevier
CY  - Amsterdam
ER  - 
TY  - JOUR
A1  - Levnajic, Zoran
A1  - Pikovskij, Arkadij
T1  - Network reconstruction from random phase resetting
JF  - Physical review letters
N2  - We propose a novel method of reconstructing the topology and interaction functions for a general oscillator network. An ensemble of initial phases and the corresponding instantaneous frequencies is constructed by repeating random phase resets of the system dynamics. The desired details of network structure are then revealed by appropriately averaging over the ensemble. The method is applicable for a wide class of networks with arbitrary emergent dynamics, including full synchrony.
Y1  - 2011
U6  - https://doi.org/10.1103/PhysRevLett.107.034101
SN  - 0031-9007
VL  - 107
IS  - 3
PB  - American Physical Society
CY  - College Park
ER  - 
TY  - JOUR
A1  - Rivnay, Jonathan
A1  - Steyrleuthner, Robert
A1  - Jimison, Leslie H.
A1  - Casadei, Alberto
A1  - Chen, Zhihua
A1  - Toney, Michael F.
A1  - Facchetti, Antonio
A1  - Neher, Dieter
A1  - Salleo, Alberto
T1  - Drastic control of texture in a high performance n-Type polymeric semiconductor and implications for charge transport
JF  - Macromolecules : a publication of the American Chemical Society
N2  - Control of crystallographic texture from mostly face-on to edge-on is observed for the film morphology of the n-type semicrystalline polymer [N,N-9-bis(2-octyldodecyl)naphthalene-1,4,5,8-bis(dicarboximide)-2,6-diy1]alt-5,59-(2,29-bithiophene)}, P(NDI2OD-T2), when annealing the film to the polymer melting point followed by slow cooling to ambient temperature. A variety of X-ray diffraction analyses, including pole figure construction and Fourier transform peak shape deconvolution, are employed to quantify the texture change, relative degree of crystallinity and lattice order. We find that annealing the polymer film to the melt leads to a shift from 77.5% face-on to 94.6% edge-on lamellar texture as well as to a 2-fold increase in crystallinity and a 40% decrease in intracrystallite cumulative disorder. The texture change results in a significant drop in the electron-only diode current density through the film thickness upon melt annealing while little change is observed in the in-plane transport of bottom gated thin film transistors. This suggests that the texture change is prevalent in the film interior and that either the (bottom) surface structure is different from the interior structure or the intracrystalline order and texture play a secondary role in transistor transport for this material.
Y1  - 2011
U6  - https://doi.org/10.1021/ma200864s
SN  - 0024-9297
VL  - 44
IS  - 13
SP  - 5246
EP  - 5255
PB  - American Chemical Society
CY  - Washington
ER  - 
TY  - JOUR
A1  - Gerhardt, Matthias
A1  - Groeger, Gillian
A1  - MacCarthy, Niall
T1  - Monopolar vs. bipolar subretinal stimulation-An in vitro study
JF  - Journal of neuroscience methods
N2  - This study uses an in vitro rd10 mouse model to quantify and compare the ability of the monopolar and the (concentric) bipolar electrode configurations for subretinal stimulation. To allow for results which can be directly compared an identical region of the retina was stimulated due to the circumstance that the bipolar electrode configuration allows also for monopolar stimulation, if the concentric counter-electrode is set potential-free (floating). A ganglion cell, located centrally over the bipolar electrode configuration was selected to extracellularly record action potentials during stimulation. To analyse the recorded action potentials, we introduce a new method which combines the advantages of (a) singular value decomposition (SVD) for weighting similar modulation patterns with which the recorded action potentials are characterized and (b) multi curve fitting to identify a common threshold level, required to finally assemble a strength-duration relationship (SDR). By directly comparing the obtained SDR curves, we found that the efficiency of stimulation with the monopolar electrode configuration is significantly higher than with the bipolar electrode configuration. All obtained SDR curves were fitted using the Lapicque model to estimate the chronaxie times and the rheobase currents. Liquid inclusions, eventually separating the retina from the electrodes are discussed to be a major cause for low ganglion cell responses during stimulation with the bipolar electrode configuration.
KW  - SVD
KW  - Subretinal
KW  - Electrodes
KW  - Monopolar
KW  - Bipolar
KW  - Retina
KW  - Ganglion
KW  - Cells
Y1  - 2011
U6  - https://doi.org/10.1016/j.jneumeth.2011.04.017
SN  - 0165-0270
VL  - 199
IS  - 1
SP  - 26
EP  - 34
PB  - Elsevier
CY  - Amsterdam
ER  - 
TY  - JOUR
A1  - Qiu, Xunlin
A1  - Wirges, Werner
A1  - Gerhard, Reimund
T1  - Beneficial and detrimental fatigue effects of dielectric barrier discharges on the piezoelectricity of polypropylene ferroelectrets
JF  - Journal of applied physics
N2  - Cellular polypropylene (PP) ferroelectrets combine a large piezoelectricity with mechanical flexibility and elastic compliance. Their charging process represents a series of dielectric barrier discharges (DBDs) that generate a cold plasma with numerous active species and thus modify the inner polymer surfaces of the foam cells. Both the threshold for the onset of DBDs and the piezoelectricity of ferroelectrets are sensitive to repeated DBDs in the voids. It is found that the threshold voltage is approximately halved and the charging efficiency is clearly improved after only 10(3) DBD cycles. However, plasma modification of the inner surfaces from repeated DBDs deteriorates the chargeability of the voids, leading to a significant reduction of the piezoelectricity in ferroelectrets. After a significant waiting period, the chargeability of previously fatigued voids shows a partial recovery. The plasma modification is, however, detrimental to the stability of the deposited charges and thus also of the macroscopic dipoles and of the piezoelectricity. Fatigue from only 10(3) DBD cycles already results in significantly less stable piezoelectricity in cellular PP ferroelectrets. The fatigue rate as a function of the number of voltage cycles follows a stretched exponential. Fatigue from repeated DBDs can be avoided if most of the gas molecules inside the voids are removed via a suitable evacuation process.
Y1  - 2011
U6  - https://doi.org/10.1063/1.3610507
SN  - 0021-8979
SN  - 1089-7550
VL  - 110
IS  - 2
PB  - American Institute of Physics
CY  - Melville
ER  - 
TY  - JOUR
A1  - Komarov, Maxim
A1  - Pikovskij, Arkadij
T1  - Effects of nonresonant interaction in ensembles of phase oscillators
JF  - Physical review : E, Statistical, nonlinear and soft matter physics
N2  - We consider general properties of groups of interacting oscillators, for which the natural frequencies are not in resonance. Such groups interact via nonoscillating collective variables like the amplitudes of the order parameters defined for each group. We treat the phase dynamics of the groups using the Ott-Antonsen ansatz and reduce it to a system of coupled equations for the order parameters. We describe different regimes of cosynchrony in the groups. For a large number of groups, heteroclinic cycles, corresponding to a sequential synchronous activity of groups and chaotic states where the order parameters oscillate irregularly, are possible.
Y1  - 2011
U6  - https://doi.org/10.1103/PhysRevE.84.016210
SN  - 1539-3755
VL  - 84
IS  - 1
PB  - American Physical Society
CY  - College Park
ER  - 
TY  - JOUR
A1  - Ilnytskyi, Jaroslav M.
A1  - Neher, Dieter
A1  - Saphiannikova, Marina
T1  - Opposite photo-induced deformations in azobenzene-containing polymers with different molecular architecture molecular dynamics study
JF  - The journal of chemical physics : bridges a gap between journals of physics and journals of chemistr
N2  - Photo-induced deformations in azobenzene-containing polymers (azo-polymers) are central to a number of applications, such as optical storage and fabrication of diffractive elements. The microscopic nature of the underlying opto-mechanical coupling is yet not clear. In this study, we address the experimental finding that the scenario of the effects depends on molecular architecture of the used azo-polymer. Typically, opposite deformations in respect to the direction of light polarization are observed for liquid crystalline and amorphous azo-polymers. In this study, we undertake molecular dynamics simulations of two different models that mimic these two types of azo-polymers. We employ hybrid force field modeling and consider only trans-isomers of azobenzene, represented as Gay-Berne sites. The effect of illumination on the orientation of the chromophores is considered on the level of orientational hole burning and emphasis is given to the resulting deformation of the polymer matrix. We reproduce deformations of opposite sign for the two models being considered here and discuss the relevant microscopic mechanisms in both cases.
KW  - amorphous state
KW  - light polarisation
KW  - liquid crystal polymers
KW  - molecular dynamics method
KW  - optical hole burning
KW  - photochemistry
Y1  - 2011
U6  - https://doi.org/10.1063/1.3614499
SN  - 0021-9606
VL  - 135
IS  - 4
PB  - American Institute of Physics
CY  - Melville
ER  - 
TY  - JOUR
A1  - Levnajic, Zoran
T1  - Emergent multistability and frustration in phase-repulsive networks of oscillators
JF  - Physical review : E, Statistical, nonlinear and soft matter physics
N2  - The collective dynamics of oscillator networks with phase-repulsive coupling is studied, considering various network sizes and topologies. The notion of link frustration is introduced to characterize and quantify the network dynamical states. In opposition to widely studied phase-attractive case, the properties of final dynamical states in our model critically depend on the network topology. In particular, each network's total frustration value is intimately related to its topology. Moreover, phase-repulsive networks in general display multiple final frustration states, whose statistical and stability properties are uniquely identifying them.
Y1  - 2011
U6  - https://doi.org/10.1103/PhysRevE.84.016231
SN  - 1539-3755
VL  - 84
IS  - 1
PB  - American Physical Society
CY  - College Park
ER  - 
TY  - JOUR
A1  - Grass, T. D.
A1  - dos Santos, Francisca E. A.
A1  - Pelster, Axel
T1  - Real-time Ginzburg-Landau theory for bosons in optical lattices
JF  - Laser physics
N2  - Within the Schwinger-Keldysh formalism we derive a Ginzburg-Landau theory for the Bose-Hubbard model which describes the real-time dynamics of the complex order parameter field. Analyzing the excitations in the vicinity of the quantum phase transitions it turns out that particle/hole dispersions in the Mott phase map continuously onto corresponding amplitude/phase excitations in the superfluid phase. Furthermore, in the superfluid phase we find a sound mode, which is in accordance with recent Bragg spectroscopy measurements in the Bogoliubov regime, as well as an additional gapped mode, which seems to have been detected via lattice modulation.
Y1  - 2011
U6  - https://doi.org/10.1134/S1054660X11150096
SN  - 1054-660X
SN  - 1555-6611
VL  - 21
IS  - 8
SP  - 1459
EP  - 1463
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Fechner, Cora
T1  - Reconstructing the intergalactic UV background with QSO absorption lines
JF  - Astronomy and astrophysics : an international weekly journal
N2  - We present a new approach to observationally constraining the spectral energy distribution of the intergalactic UV background by studying metal absorption systems. We study single-component metal line systems that exhibit various well-measured species. Among the observed transitions, at least two ratios of ionization stages from the same element are required, e. g. C III/C IV and Si III/Si IV. For each system photoionization models are constructed by varying the spectrum of the ionizing radiation. The spectral energy distribution can then be constrained by comparing the models with the observed column density ratios. Extensive tests with artificial absorbers show that the spectrum of the ionizing radiation cannot be reconstructed unambiguously, but it is possible to constrain the main characteristics of the spectrum. Furthermore, the resulting physical parameters of the absorber, such as ionization parameter, metallicity, and relative abundances, may depend strongly on the adopted ionizing spectrum. Even in case of well-fitting models, the uncertainties can be as high as similar to 0.5 dex for the ionization parameter and up to similar to 1.5 dex for the metallicity. Therefore, it is essential to know the hardness of the UV background when estimating the metallicity of the intergalactic medium. Applying the procedure to a small sample of 3 observed single-component metal line systems yields a soft ionizing radiation at z > 2 and a slightly harder spectrum at z < 2. The resulting energy distributions exhibit strong He II Lya re-emission features, suggesting that reprocessing by intergalactic He II is important. Comparing the observed systems to UV background spectra from the literature indicates that a recent model that includes sawtooth modulation due to reprocessing by intergalactic He II with delayed helium reionization fits the investigated systems very well.
KW  - intergalactic medium
KW  - quasars: absorption lines
KW  - diffuse radiation
Y1  - 2011
U6  - https://doi.org/10.1051/0004-6361/201117080
SN  - 0004-6361
VL  - 532
IS  - 2
PB  - EDP Sciences
CY  - Les Ulis
ER  - 
TY  - JOUR
A1  - Bagnich, Sergey A.
A1  - Unger, Th.
A1  - Jaiser, Frank
A1  - Neher, Dieter
A1  - Thesen, M. W.
A1  - Krüger, H.
T1  - Efficient green electrophosphorescence based on ambipolar nonconjugated polymers evaluation of transport and emission properties
JF  - Journal of applied physics
N2  - New materials for polymer organic light-emitting diodes based on a polymer matrix doped with phosphorescent dyes are presented. The matrix system is based on a polystyrene backbone bearing either electron or hole transporting units at the 4-position of each repeat unit. Random copolymers and polymer blend systems of the homopolymers are prepared, both with 62 wt.% electron transporting and 38 wt.% hole transporting moieties. Adding a green electrophosphorescent dye to the polymer matrix leads to efficient electroluminescence with a maximum current efficiency of 35 cd/A and a maximum external quantum efficiency of up to 10%. The mobilities of electrons and holes in the dye-doped copolymer, as measured by transient electroluminescence, are around 5 x 10(-5) and 5 x 10(-6) cm(2)/Vs, respectively, while the blend of the two homopolymers exhibits slightly lower mobilities of both types of carriers. Despite the pronounced imbalance of charge transport, the device performance is almost entirely limited by the phosphorescence efficiency of the dye, implying balanced flow of holes and electrons into the active region. Also, devices made with either the copolymer or the blend yielded very similar device efficiencies, despite the noticeable difference in electron and hole mobility. It is proposed that electrons are efficiently blocked at the interlayer and that the so-formed space charge assists the balanced injection of holes.
Y1  - 2011
U6  - https://doi.org/10.1063/1.3618681
SN  - 0021-8979
SN  - 1089-7550
VL  - 110
IS  - 3
PB  - American Institute of Physics
CY  - Melville
ER  - 
TY  - JOUR
A1  - Prosen, Tomaz
A1  - Ilievski, Enej
T1  - Nonequilibrium phase transition in a periodically driven XY spin chain
JF  - Physical review letters
N2  - We present a general formulation of Floquet states of periodically time-dependent open Markovian quasifree fermionic many-body systems in terms of a discrete Lyapunov equation. Illustrating the technique, we analyze periodically kicked XY spin-1/2 chain which is coupled to a pair of Lindblad reservoirs at its ends. A complex phase diagram is reported with reentrant phases of long range and exponentially decaying spin-spin correlations as some of the system's parameters are varied. The structure of phase diagram is reproduced in terms of counting nontrivial stationary points of Floquet quasiparticle dispersion relation.
Y1  - 2011
U6  - https://doi.org/10.1103/PhysRevLett.107.060403
SN  - 0031-9007
VL  - 107
IS  - 6
PB  - American Physical Society
CY  - College Park
ER  - 
TY  - JOUR
A1  - Zakrevskyy, Yuriy
A1  - Kopyshev, Alexey
A1  - Lomadze, Nino
A1  - Morozova, Elena
A1  - Lysyakova, Liudmila
A1  - Kasyanenko, Nina
A1  - Santer, Svetlana
T1  - DNA compaction by azobenzene-containing surfactant
JF  - Physical review : E, Statistical, nonlinear and soft matter physics
N2  - We report on the interaction of cationic azobenzene-containing surfactant with DNA investigated by absorption and fluorescence spectroscopy, dynamic light scattering, and atomic force microscopy. The properties of the surfactant can be controlled with light by reversible switching of the azobenzene unit, incorporated into the surfactant tail, between a hydrophobic trans (visible irradiation) and a hydrophilic cis (UV irradiation) configuration. The influence of the trans-cis isomerization of the azobenzene on the compaction process of DNA molecules and the role of both isomers in the formation and colloidal stability of DNA-surfactant complexes is discussed. It is shown that the trans isomer plays a major role in the DNA compaction process. The influence of the cis isomer on the DNA coil configuration is rather small. The construction of a phase diagram of the DNA concentration versus surfactant/DNA charge ratio allows distancing between three major phases: colloidally stable and unstable compacted globules, and extended coil conformation. There is a critical concentration of DNA above which the compacted globules can be hindered from aggregation and precipitation by adding an appropriate amount of the surfactant in the trans configuration. This is because of the compensation of hydrophobicity of the globules with an increasing amount of the surfactant. Below the critical DNA concentration, the compacted globules are colloidally stable and can be reversibly transferred with light to an extended coil state.
Y1  - 2011
U6  - https://doi.org/10.1103/PhysRevE.84.021909
SN  - 1539-3755
VL  - 84
IS  - 2
PB  - American Physical Society
CY  - College Park
ER  - 
TY  - JOUR
A1  - Schütz, Nadine
A1  - Holschneider, Matthias
T1  - Detection of trend changes in time series using Bayesian inference
JF  - Physical review : E, Statistical, nonlinear and soft matter physics
N2  - Change points in time series are perceived as isolated singularities where two regular trends of a given signal do not match. The detection of such transitions is of fundamental interest for the understanding of the system's internal dynamics or external forcings. In practice observational noise makes it difficult to detect such change points in time series. In this work we elaborate on a Bayesian algorithm to estimate the location of the singularities and to quantify their credibility. We validate the performance and sensitivity of our inference method by estimating change points of synthetic data sets. As an application we use our algorithm to analyze the annual flow volume of the Nile River at Aswan from 1871 to 1970, where we confirm a well-established significant transition point within the time series.
Y1  - 2011
U6  - https://doi.org/10.1103/PhysRevE.84.021120
SN  - 1539-3755
SN  - 1550-2376
VL  - 84
IS  - 2
PB  - American Physical Society
CY  - College Park
ER  - 
TY  - JOUR
A1  - Blakesley, James C.
A1  - Neher, Dieter
T1  - Relationship between energetic disorder and open-circuit voltage in bulk heterojunction organic solar cells
JF  - Physical review : B, Condensed matter and materials physics
N2  - We simulate organic bulk heterojunction solar cells. The effects of energetic disorder are incorporated through a Gaussian or exponential model of density of states. Analytical models of open-circuit voltage (V(OC)) are derived from the splitting of quasi-Fermi potentials. Their predictions are backed up by more complex numerical device simulations including effects such as carrier-density-dependent charge-carrier mobilities. It is predicted that the V(OC) depends on: (1) the donor-acceptor energy gap; (2) charge-carrier recombination rates; (3) illumination intensity; (4) the contact work functions (if not in the pinning regime); and (5) the amount of energetic disorder. A large degree of energetic disorder, or a high density of traps, is found to cause significant reductions in V(OC). This can explain why V(OC) is often less than expected in real devices. Energetic disorder also explains the nonideal temperature and intensity dependence of V(OC) and the superbimolecular recombination rates observed in many real bulk heterojunction solar cells.
Y1  - 2011
U6  - https://doi.org/10.1103/PhysRevB.84.075210
SN  - 1098-0121
VL  - 84
IS  - 7
PB  - American Physical Society
CY  - College Park
ER  - 
TY  - JOUR
A1  - Burylko, Oleksandr
A1  - Pikovskij, Arkadij
T1  - Desynchronization transitions in nonlinearly coupled phase oscillators
JF  - Physica :D, Nonlinear phenomena
N2  - We consider the nonlinear extension of the Kuramoto model of globally coupled phase oscillators where the phase shift in the coupling function depends on the order parameter. A bifurcation analysis of the transition from fully synchronous state to partial synchrony is performed. We demonstrate that for small ensembles it is typically mediated by stable cluster states, that disappear with creation of heteroclinic cycles, while for a larger number of oscillators a direct transition from full synchrony to a periodic or a quasiperiodic regime occurs.
KW  - Coupled oscillators
KW  - Oscillator ensembles
KW  - Kuramoto model
KW  - Nonlinear coupling
KW  - Bifurcations
Y1  - 2011
U6  - https://doi.org/10.1016/j.physd.2011.05.016
SN  - 0167-2789
VL  - 240
IS  - 17
SP  - 1352
EP  - 1361
PB  - Elsevier
CY  - Amsterdam
ER  - 
TY  - JOUR
A1  - Sun, Y-P
A1  - Pietzsch, Annette
A1  - Hennies, Franz
A1  - Rinkevicius, Z.
A1  - Karlsson, Hans O.
A1  - Schmitt, Thorsten
A1  - Strocov, Vladimir N.
A1  - Andersson, Joakim
A1  - Kennedy, B.
A1  - Schlappa, J.
A1  - Föhlisch, Alexander
A1  - Gel'mukhanov, F.
A1  - Rubensson, Jan-Erik
T1  - Internal symmetry and selection rules in resonant inelastic soft x-ray scattering
JF  - Journal of physics : B, Atomic, molecular and optical physics
N2  - Resonant inelastic soft x-ray scattering spectra excited at the dissociative 1 sigma(g) -> 3 sigma(u) resonance in gas-phase O(2) are presented and discussed in terms of state-of-the-art molecular theory. A new selection rule due to internal spin coupling is established, facilitating a deep analysis of the valence excited final states. Furthermore, it is found that a commonly accepted symmetry selection rule due to orbital parity breaks down, as the core hole and excited electron swap parity, thereby opening the symmetry forbidden 3 sigma(g) decay channel.
Y1  - 2011
U6  - https://doi.org/10.1088/0953-4075/44/16/161002
SN  - 0953-4075
VL  - 44
IS  - 16
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Acciari, V. A.
A1  - Aliu, E.
A1  - Arlen, T.
A1  - Aune, T.
A1  - Beilicke, M.
A1  - Benbow, W.
A1  - Bradbury, S. M.
A1  - Buckley, J. H.
A1  - Bugaev, V.
A1  - Byrum, K.
A1  - Cannon, A.
A1  - Cesarini, A.
A1  - Ciupik, L.
A1  - Collins-Hughes, E.
A1  - Connolly, M. P.
A1  - Cui, W.
A1  - Dickherber, R.
A1  - Duke, C.
A1  - Errando, M.
A1  - Falcone, A.
A1  - Finley, J. P.
A1  - Finnegan, G.
A1  - Fortson, L.
A1  - Furniss, A.
A1  - Galante, N.
A1  - Gall, D.
A1  - Gillanders, G. H.
A1  - Godambe, S.
A1  - Griffin, S.
A1  - Grube, J.
A1  - Guenette, R.
A1  - Gyuk, G.
A1  - Hanna, D.
A1  - Holder, J.
A1  - Hughes, G.
A1  - Hui, C. M.
A1  - Humensky, T. B.
A1  - Kaaret, P.
A1  - Karlsson, N.
A1  - Kertzman, M.
A1  - Kieda, D.
A1  - Krawczynski, H.
A1  - Krennrich, F.
A1  - Lang, M. J.
A1  - LeBohec, S.
A1  - Maier, G.
A1  - Majumdar, P.
A1  - McArthur, S.
A1  - McCann, A.
A1  - Moriarty, P.
A1  - Mukherjee, R.
A1  - Ong, R. A.
A1  - Orr, M.
A1  - Otte, A. N.
A1  - Park, N.
A1  - Perkins, J. S.
A1  - Pohl, Martin
A1  - Prokoph, H.
A1  - Quinn, J.
A1  - Ragan, K.
A1  - Reyes, L. C.
A1  - Reynolds, P. T.
A1  - Roache, E.
A1  - Rose, H. J.
A1  - Ruppel, J.
A1  - Saxon, D. B.
A1  - Schroedter, M.
A1  - Sembroski, G. H.
A1  - Senturk, G. D.
A1  - Smith, A. W.
A1  - Staszak, D.
A1  - Tesic, G.
A1  - Theiling, M.
A1  - Thibadeau, S.
A1  - Tsurusaki, K.
A1  - Varlotta, A.
A1  - Vassiliev, V. V.
A1  - Vincent, S.
A1  - Vivier, M.
A1  - Wakely, S. P.
A1  - Ward, J. E.
A1  - Weekes, T. C.
A1  - Weinstein, A.
A1  - Weisgarber, T.
A1  - Williams, D. A.
A1  - Zitzer, B.
T1  - VERITAS OBSERVATIONS OF THE TeV BINARY LS I+61 degrees 303 DURING 2008-2010
JF  - The astrophysical journal : an international review of spectroscopy and astronomical physics
N2  - We present the results of observations of the TeV binary LS I + 61 degrees 303 with the VERITAS telescope array between 2008 and 2010, at energies above 300 GeV. In the past, both ground-based gamma-ray telescopes VERITAS and MAGIC have reported detections of TeV emission near the apastron phases of the binary orbit. The observations presented here show no strong evidence for TeV emission during these orbital phases; however, during observations taken in late 2010, significant emission was detected from the source close to the phase of superior conjunction (much closer to periastron passage) at a 5.6 standard deviation (5.6 sigma) post-trials significance. In total, between 2008 October and 2010 December a total exposure of 64.5 hr was accumulated with VERITAS on LS I + 61 degrees 303, resulting in an excess at the 3.3 sigma significance level for constant emission over the entire integrated data set. The flux upper limits derived for emission during the previously reliably active TeV phases (i.e., close to apastron) are less than 5% of the Crab Nebula flux in the same energy range. This result stands in apparent contrast to previous observations by both MAGIC and VERITAS which detected the source during these phases at 10% of the Crab Nebula flux. During the two year span of observations, a large amount of X-ray data were also accrued on LS I + 61 degrees 303 by the Swift X-ray Telescope and the Rossi X-ray Timing Explorer Proportional Counter Array. We find no evidence for a correlation between emission in the X-ray and TeV regimes during 20 directly overlapping observations. We also comment on data obtained contemporaneously by the Fermi Large Area Telescope.
KW  - binaries: general
KW  - gamma rays: general
KW  - X-rays: binaries
Y1  - 2011
U6  - https://doi.org/10.1088/0004-637X/738/1/3
SN  - 0004-637X
VL  - 738
IS  - 1
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Stich, Michael
A1  - Beta, Carsten
T1  - Standing waves in a complex Ginzburg-Landau equation with time-delay  feedback
JF  - Discrete and continuous dynamical systems : a journal bridging mathematics and sciences
N2  - Standing waves are studied as solutions of a complex Ginsburg-Landau equation subjected to local and global time-delay feedback terms. The onset of standing waves is studied at the instability of the homogeneous periodic solution with respect to spatially periodic perturbations. The solution of this spatiotemporal wave pattern is given and is compared to the homogeneous periodic solution.
KW  - pattern formation
KW  - reaction-diffusion system
KW  - control
Y1  - 2011
SN  - 1078-0947
SN  - 1553-5231
IS  - 1
SP  - 1329
EP  - 1334
PB  - American Institute of Mathematical Sciences
CY  - Springfield
ER  - 
TY  - JOUR
A1  - Hübener, Robert
A1  - Kruszynska, Caroline
A1  - Hartmann, Lorenz
A1  - Duer, Wolfgang
A1  - Plenio, Martin B.
A1  - Eisert, Jens
T1  - Tensor network methods with graph enhancement
JF  - Physical review : B, Condensed matter and materials physics
N2  - We present applications of the renormalization algorithm with graph enhancement (RAGE). This analysis extends the algorithms and applications given for approaches based on matrix product states introduced in [Phys. Rev. A 79, 022317 (2009)] to other tensor-network states such as the tensor tree states (TTS) and projected entangled pair states. We investigate the suitability of the bare TTS to describe ground states, showing that the description of certain graph states and condensed-matter models improves. We investigate graph-enhanced tensor-network states, demonstrating that in some cases (disturbed graph states and for certain quantum circuits) the combination of weighted graph states with TTS can greatly improve the accuracy of the description of ground states and time-evolved states. We comment on delineating the boundary of the classically efficiently simulatable states of quantum many-body systems.
Y1  - 2011
U6  - https://doi.org/10.1103/PhysRevB.84.125103
SN  - 1098-0121
VL  - 84
IS  - 12
PB  - American Physical Society
CY  - College Park
ER  - 
TY  - JOUR
A1  - Schmah, Tanya
A1  - Marwan, Norbert
A1  - Thomsen, Jesper Skovhus
A1  - Saparin, Peter
T1  - Long range node-strut analysis of trabecular bone microarchitecture
JF  - Medical physics : the international journal of medical physics research and practice
N2  - Purpose: We present a new morphometric measure of trabecular bone microarchitecture, called mean node strength (NdStr), which is part of a newly developed approach called long range nodestrut analysis. Our general aim is to describe and quantify the apparent "latticelike" microarchitecture of the trabecular bone network.
 Methods: Similar in some ways to the topological node-strut analysis introduced by Garrahan et al. [J. Microsc. 142, 341-349 (1986)], our method is distinguished by an emphasis on long-range trabecular connectivity. Thus, while the topological classification of a pixel (after skeletonization) as a node, strut, or terminus, can be determined from the 3 x 3 neighborhood of that pixel, our method, which does not involve skeletonization, takes into account a much larger neighborhood. In addition, rather than giving a discrete classification of each pixel as a node, strut, or terminus, our method produces a continuous variable, node strength. The node strength is averaged over a region of interest to produce the mean node strength of the region.
 Results: We have applied our long range node-strut analysis to a set of 26 high-resolution peripheral quantitative computed tomography (pQCT) axial images of human proximal tibiae acquired 17 mm below the tibial plateau. We found that NdStr has a strong positive correlation with trabecular volumetric bone mineral density (BMD). After an exponential transformation, we obtain a Pearson's correlation coefficient of r - 0.97. Qualitative comparison of images with similar BMD but with very different NdStr values suggests that the latter measure has successfully quantified the prevalence of the "latticelike" microarchitecture apparent in the image. Moreover, we found a strong correlation (r - 0.62) between NdStr and the conventional node-terminus ratio (Nd/Tm) of Garrahan et al. The Nd/Tm ratios were computed using traditional histomorphometry performed on bone biopsies obtained at the same location as the pQCT scans.
 Conclusions: The newly introduced morphometric measure allows a quantitative assessment of the long-range connectivity of trabecular bone. One advantage of this method is that it is based on pQCT images that can be obtained noninvasively from patients, i.e., without having to obtain a bone biopsy from the patient.
KW  - trabecular bone
KW  - osteoporosis
KW  - structure analysis
KW  - histomorphometry
KW  - pQCT
Y1  - 2011
U6  - https://doi.org/10.1118/1.3622600
SN  - 0094-2405
VL  - 38
IS  - 9
SP  - 5003
EP  - 5011
PB  - American Association of Physicists in Medicine
CY  - Melville
ER  - 
TY  - JOUR
A1  - Oskinova, Lida
A1  - Todt, Helge Tobias
A1  - Ignace, Richard
A1  - Brown, John C.
A1  - Cassinelli, Joseph P.
A1  - Hamann, Wolf-Rainer
T1  - Early magnetic B-type stars X-ray emission and wind properties
JF  - Monthly notices of the Royal Astronomical Society
N2  - We present a comprehensive study of X-ray emission by, and wind properties of, massive magnetic early B-type stars. Dedicated XMM-Newton observations were obtained for three early-type B-type stars, xi(1) CMa, V2052 Oph and zeta Cas, with recently discovered magnetic fields. We report the first detection of X-ray emission from V2052 Oph and zeta Cas. The latter is one the softest X-ray sources among the early-type stars, while the former is one of the X-ray faintest. The observations show that the X-ray spectra of our programme stars are quite soft with the bulk of X-ray emitting material having a temperature of about 1 MK. We compile the complete sample of early B-type stars with detected magnetic fields to date and existing X-ray measurements, in order to study whether the X-ray emission can be used as a general proxy for stellar magnetism. We find that the X-ray properties of early massive B-type magnetic stars are diverse, and that hard and strong X-ray emission does not necessarily correlate with the presence of a magnetic field, corroborating similar conclusions reached earlier for the classical chemically peculiar magnetic Bp-Ap stars.
 We analyse the ultraviolet (UV) spectra of five non-supergiant B stars with magnetic fields (tau Sco, beta Cep, xi(1) CMa, V2052 Oph and zeta Cas) by means of non-local thermodynamic equilibrium (non-LTE) iron-blanketed model atmospheres. The latter are calculated with the Potsdam Wolf-Rayet (PoWR) code, which treats the photosphere as well as the wind, and also accounts for X-rays. With the exception of t Sco, this is the first analysis of these stars by means of stellar wind models. Our models accurately fit the stellar photospheric spectra in the optical and the UV. The parameters of X-ray emission, temperature and flux are included in the model in accordance with observations. We confirm the earlier findings that the filling factors of X-ray emitting material are very high.
 Our analysis reveals that the magnetic early-type B stars studied here have weak winds with velocities not significantly exceeding upsilon(esc). The mass-loss rates inferred from the analysis of UV lines are significantly lower than predicted by hydrodynamically consistent models. We find that, although the X-rays strongly affect the ionization structure of the wind, this effect is not sufficient in reducing the total radiative acceleration. When the X-rays are accounted for at the intensity and temperatures observed, there is still sufficient radiative acceleration to drive a stronger mass-loss than we empirically infer from the UV spectral lines.
KW  - techniques: spectroscopic
KW  - stars: magnetic field
KW  - stars: massive
KW  - stars: mass loss
KW  - X-rays: stars
Y1  - 2011
U6  - https://doi.org/10.1111/j.1365-2966.2011.19143.x
SN  - 0035-8711
VL  - 416
IS  - 2
SP  - 1456
EP  - 1474
PB  - Wiley-Blackwell
CY  - Hoboken
ER  - 
TY  - JOUR
A1  - Winkel, B.
A1  - Ben Bekhti, Nadya
A1  - Darmstaedter, V.
A1  - Floeer, L.
A1  - Kerp, J.
A1  - Richter, Philipp
T1  - The high-velocity cloud complex Galactic center negative as seen by EBHIS and GASS I. Cloud catalog and global properties
JF  - Astronomy and astrophysics : an international weekly journal
N2  - Using Milky Way data of the new Effelsberg-Bonn HI Survey (EBHIS) and the Galactic All-Sky Survey (GASS), we present a revised picture of the high-velocity cloud (HVC) complex Galactic center negative (GCN). Owing to the higher angular resolution of these surveys compared to previous studies (e.g., the Leiden Dwingeloo Survey), we resolve complex GCN into lots of individual tiny clumps, that mostly have relatively broad line widths of more than 15 km s(-1). We do not detect a diffuse extended counterpart, which is unusual for an HVC complex. In total 243 clumps were identified and parameterized which allows us to statistically analyze the data. Cold-line components (i.e.,Delta upsilon(fwhm) < 7.5 km s(-1)) are found in about 5% only of the identified cloudlets. Our analysis reveals that complex GCN is likely built up of several subpopulations that do not share a common origin. Furthermore, complex GCN might be a prime example for warm-gas accretion onto the Milky Way, where neutral HI clouds are not stable against interaction with the Milky Way gas halo and become ionized prior to accretion.
KW  - ISM: clouds
KW  - Galaxy: halo
Y1  - 2011
U6  - https://doi.org/10.1051/0004-6361/201117357
SN  - 0004-6361
VL  - 533
IS  - 18
PB  - EDP Sciences
CY  - Les Ulis
ER  - 
TY  - JOUR
A1  - Sun, Zhongkui
A1  - Yang, Xiaoli
T1  - Generating and enhancing lag synchronization of chaotic systems by white noise
JF  - Chaos : an interdisciplinary journal of nonlinear science
N2  - In this paper, we study the crucial impact of white noise on lag synchronous regime in a pair of time-delay unidirectionally coupled systems. Our result demonstrates that merely via white-noise-based coupling lag synchronization could be achieved between the coupled systems (chaotic or not). And it is also demonstrated that a conventional lag synchronous regime can be enhanced by white noise. Sufficient conditions are further proved mathematically for noise-inducing and noise-enhancing lag synchronization, respectively. Additionally, the influence of parameter mismatch on the proposed lag synchronous regime is studied, by which we announce the robustness and validity of the new strategy. Two numerical examples are provided to illustrate the validity and some possible applications of the theoretical result.
Y1  - 2011
U6  - https://doi.org/10.1063/1.3623440
SN  - 1054-1500
SN  - 1089-7682
VL  - 21
IS  - 3
PB  - American Institute of Physics
CY  - Melville
ER  - 
TY  - JOUR
A1  - Schuh, Christian
A1  - Lomadze, Nino
A1  - Rühe, Jürgen
A1  - Kopyshev, Alexey
A1  - Santer, Svetlana
T1  - Photomechanical degrafting of Azo-functionalized Poly(methacrylic acid) (PMAA) brushes
JF  - The journal of physical chemistry : B, Condensed matter, materials, surfaces, interfaces & biophysical chemistry
N2  - We report on the preparation and characterization of photosensitive polymer brushes. The brushes are synthesized through polymer analogous attachment of azobenzene groups to surface-attached poly(methacrylic acid) (PMAA) chains. The topography of the photosensitive brushes shows a strong reaction upon irradiation with UV light. While homogeneous illumination leaves the polymer topography unchanged, irradiation of the samples with interference patterns with periodically varying light intensity leads to the formation of surface relief gratings (SRG). The height of the stripes of the grating can be controlled by adjusting the irradiation time. The SRG pattern can be erased through solvent treatment when the periodicity of the stripe pattern is less than the length of the fully stretched polymer chains. In the opposite case, photomechanical scission of receding polymer chains is observed during SRG formation, and the inscribed patterns are permanent.
Y1  - 2011
U6  - https://doi.org/10.1021/jp2041229
SN  - 1520-6106
VL  - 115
IS  - 35
SP  - 10431
EP  - 10438
PB  - American Chemical Society
CY  - Washington
ER  - 
TY  - JOUR
A1  - Schuch, Norbert
A1  - Harrison, Sarah K.
A1  - Osborne, Tobias J.
A1  - Eisert, Jens
T1  - Information propagation for interacting-particle systems
JF  - Physical review : A, Atomic, molecular, and optical physics
N2  - We study the speed at which information propagates through systems of interacting quantum particles moving on a regular lattice and show that for a certain class of initial conditions there exists a maximum speed of sound at which information can propagate. Our argument applies equally to quantum spins, bosons such as in the Bose-Hubbard model, fermions, anyons, and general mixtures thereof, on arbitrary lattices of any dimension. It also pertains to dissipative dynamics on the lattice, and generalizes to the continuum for quantum fields. Our result can be seen as an analog of the Lieb-Robinson bound for strongly correlated models.
Y1  - 2011
U6  - https://doi.org/10.1103/PhysRevA.84.032309
SN  - 1050-2947
VL  - 84
IS  - 3
PB  - American Physical Society
CY  - College Park
ER  - 
TY  - JOUR
A1  - Eichler, David
A1  - Pohl, Martin
T1  - Can ultrahigh-energy cosmic rays come from Gamma-ray bursts? - cosmic rays below the ankle and galactic gamma-ray bursts
JF  - The astrophysical journal : an international review of spectroscopy and astronomical physics ; Part 2, Letters
N2  - The maximum cosmic-ray energy achievable by acceleration by a relativistic blast wave is derived. It is shown that forward shocks from long gamma-ray bursts (GRBs) in the interstellar medium accelerate protons to large enough energies, and have a sufficient energy budget, to produce the Galactic cosmic-ray component just below the ankle at 4 x 10(18) eV, as per an earlier suggestion. It is further argued that, were extragalactic long GRBs responsible for the component above the ankle as well, the occasional Galactic GRB within the solar circle would contribute more than the observational limits on the outward flux from the solar circle, unless an avoidance scenario, such as intermittency and/or beaming, allows the present-day local flux to be less than 10(-3) of the average. Difficulties with these avoidance scenarios are noted.
KW  - cosmic rays
KW  - galaxies: general
KW  - gamma-ray burst: general
Y1  - 2011
U6  - https://doi.org/10.1088/2041-8205/738/2/L21
SN  - 2041-8205
VL  - 738
IS  - 2
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Aliu, E.
A1  - Arlen, T.
A1  - Aune, T.
A1  - Beilicke, M.
A1  - Benbow, W.
A1  - Boettcher, Markus
A1  - Bouvier, A.
A1  - Bradbury, S. M.
A1  - Buckley, J. H.
A1  - Bugaev, V.
A1  - Cannon, A.
A1  - Cesarini, A.
A1  - Ciupik, L.
A1  - Collins-Hughes, E.
A1  - Connolly, M. P.
A1  - Cui, W.
A1  - Dickherber, R.
A1  - Errando, M.
A1  - Falcone, A.
A1  - Finley, J. P.
A1  - Fortson, L.
A1  - Furniss, A.
A1  - Galante, N.
A1  - Gall, D.
A1  - Gillanders, G. H.
A1  - Godambe, S.
A1  - Griffin, S.
A1  - Grube, J.
A1  - Gyuk, G.
A1  - Hanna, D.
A1  - Holder, J.
A1  - Huan, H.
A1  - Hughes, G.
A1  - Hui, C. M.
A1  - Humensky, T. B.
A1  - Kaaret, P.
A1  - Karlsson, N.
A1  - Kertzman, M.
A1  - Kieda, D.
A1  - Krawczynski, H.
A1  - Krennrich, F.
A1  - Madhavan, A. S.
A1  - Maier, G.
A1  - Majumdar, P.
A1  - McArthur, S.
A1  - McCann, A.
A1  - Moriarty, P.
A1  - Mukherjee, R.
A1  - Ong, R. A.
A1  - Orr, M.
A1  - Otte, A. N.
A1  - Park, N.
A1  - Perkins, J. S.
A1  - Pichel, A.
A1  - Pohl, Martin
A1  - Prokoph, H.
A1  - Quinn, J.
A1  - Ragan, K.
A1  - Reyes, L. C.
A1  - Reynolds, P. T.
A1  - Roache, E.
A1  - Rose, H. J.
A1  - Ruppel, J.
A1  - Saxon, D. B.
A1  - Schroedter, M.
A1  - Sembroski, G. H.
A1  - Skole, C.
A1  - Smith, A. W.
A1  - Staszak, D.
A1  - Tesic, G.
A1  - Theiling, M.
A1  - Thibadeau, S.
A1  - Tsurusaki, K.
A1  - Tyler, J.
A1  - Varlotta, A.
A1  - Vincent, S.
A1  - Vivier, M.
A1  - Wakely, S. P.
A1  - Ward, J. E.
A1  - Weinstein, A.
A1  - Weisgarber, T.
A1  - Williams, D. A.
T1  - Veritas observations of unusual extragalactic transient swift J164449.3+573451
JF  - The astrophysical journal : an international review of spectroscopy and astronomical physics ; Part 2, Letters
N2  - We report on very high energy (>100 GeV) gamma-ray observations of Swift J164449.3+573451, an unusual transient object first detected by the Swift Observatory and later detected by multiple radio, optical, and X-ray observatories. A total exposure of 28 hr was obtained on Swift J164449.3+573451 with the Very Energetic Radiation Imaging Telescope Array System ( VERITAS) during 2011 March 28-April 15. We do not detect the source and place a differential upper limit on the emission at 500 GeV during these observations of 1.4 x 10(-12) erg cm(-2) s(-1) (99% confidence level). We also present time-resolved upper limits and use a flux limit averaged over the X-ray flaring period to constrain various emission scenarios that can accommodate both the radio-through-X-ray emission detected from the source and the lack of detection by VERITAS.
KW  - accretion, accretion disks
KW  - galaxies: active
KW  - gamma rays: galaxies
KW  - radiation mechanisms: non-thermal
Y1  - 2011
U6  - https://doi.org/10.1088/2041-8205/738/2/L30
SN  - 2041-8205
VL  - 738
IS  - 2
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Kliesch, Martin
A1  - Barthel, Thomas
A1  - Gogolin, C.
A1  - Kastoryano, M.
A1  - Eisert, J.
T1  - Dissipative quantum church-turing theorem
JF  - Physical review letters
N2  - We show that the time evolution of an open quantum system, described by a possibly time dependent Liouvillian, can be simulated by a unitary quantum circuit of a size scaling polynomially in the simulation time and the size of the system. An immediate consequence is that dissipative quantum computing is no more powerful than the unitary circuit model. Our result can be seen as a dissipative Church-Turing theorem, since it implies that under natural assumptions, such as weak coupling to an environment, the dynamics of an open quantum system can be simulated efficiently on a quantum computer. Formally, we introduce a Trotter decomposition for Liouvillian dynamics and give explicit error bounds. This constitutes a practical tool for numerical simulations, e.g., using matrix-product operators. We also demonstrate that most quantum states cannot be prepared efficiently.
Y1  - 2011
U6  - https://doi.org/10.1103/PhysRevLett.107.120501
SN  - 0031-9007
VL  - 107
IS  - 12
PB  - American Physical Society
CY  - College Park
ER  - 
TY  - JOUR
A1  - Shayduk, Roman
A1  - Navirian, Hengameh
A1  - Leitenberger, Wolfram
A1  - Goldshteyn, Jevgenij
A1  - Vrejoiu, Ionela
A1  - Weinelt, Martin
A1  - Gaal, Peter
A1  - Herzog, Marc
A1  - von Korff Schmising, Clemens
A1  - Bargheer, Matias
T1  - Nanoscale heat transport studied by high-resolution time-resolved x-ray diffraction
JF  - New journal of physics : the open-access journal for physics
N2  - We report on synchrotron-based high-repetition rate ultrafast x-ray diffraction (UXRD) experiments monitoring the transport of heat from an epitaxial La(0.7)Sr(0.3)MnO(3)/SrTiO(3) superlattice (SL) into the substrate on timescales from 100 ps to 4 mu s. Transient thermal lattice expansion was determined with an accuracy of 10(-7), corresponding to a sensitivity to temperature changes down to 0.01 K. We follow the heat flow within the SL and into the substrate after the impulsive laser heating leads to a small temperature rise of Delta T = 6 K. The transient lattice temperature can be simulated very well using the bulk heat conductivities. This contradicts the interpretation of previous UXRD measurements, which predicted a long-lasting expansion of SrRuO(3) for more than 200 ps. The disagreement could be resolved by assuming that the heat conductivity changes in the first hundred picoseconds.
Y1  - 2011
U6  - https://doi.org/10.1088/1367-2630/13/9/093032
SN  - 1367-2630
VL  - 13
IS  - 11
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Lomadze, Nino
A1  - Kopyshev, Alexey
A1  - Rühe, Jürgen
A1  - Santer, Svetlana
T1  - Light-Induced chain scission in photosensitive polymer brushes
JF  - Macromolecules : a publication of the American Chemical Society
N2  - We report on a process inducing photomechanical fracture of chemical bonds in photosensitive PMAA polymer brushes. The photosensitive PMAA polymer brushes were prepared by covalent attachment of azobenzene groups to poly(methylacrylic acid) (PMAA) chains generated by surface-initiated polymerization. While homogeneous irradiation leaves the polymer topography unchanged, the azo-PMAA brushes show a strong response upon irradiation with UV interference patterns. The photoisomerization process in the surface-attached polymer films results in the irreversible formation of surface relief gratings (SRG), which are strongly enhanced upon washing with a good solvent for the polymer. The photomechanical forces during mass transport induced by the irradiation lead to the scission of covalent bounds and accordingly to a degrafting of the polymer chains in areas where the polymer is receding from. It is observed that the number of ruptured chains depends strongly on the amount of azo side chains in the polymer.
Y1  - 2011
U6  - https://doi.org/10.1021/ma201016q
SN  - 0024-9297
VL  - 44
IS  - 18
SP  - 7372
EP  - 7377
PB  - American Chemical Society
CY  - Washington
ER  - 
TY  - JOUR
A1  - Sun, Zhuanlan
A1  - Zhang, Xiaoqing
A1  - Xia, Zhongfu
A1  - Qiu, Xunlin
A1  - Wirges, Werner
A1  - Gerhard, Reimund
A1  - Zeng, Changchun
A1  - Zhang, Chuck
A1  - Wang, Ben
T1  - Polarization and piezoelectricity in polymer films with artificial void structure
JF  - Applied physics : A, Materials science & processing
N2  - Laminated polymer-film systems with well-defined void structures were prepared from fluoroethylenepropylene (FEP) and polytetrafluoroethylene (PTFE) layers. First the PTFE films were patterned and then fusion-bonded with the FEP films. The laminates were subjected to either corona or contact charging in order to obtain the desired piezoelectricity. The build-up of the "macro-dipoles" in the laminated films was studied by recording the electric hysteresis loops. The resulting electro-mechanical properties were investigated by means of dielectric resonance spectroscopy (DRS) and direct measurements of the stress-strain relationship. Moreover, the thermal stability of the piezoelectric d (33) coefficient was investigated at elevated temperatures and via thermally stimulated discharge (TSD) current measurements in short circuit. For 150 mu m thick laminated films, consisting of one 25 mu m thick PTFE layer, two 12.5 mu m thick FEP layers, and a void of 100 mu m height, the critical voltage necessary for the build-up of the "macro-dipoles" in the inner voids was approximately 1400 V, which agrees with the value calculated from the Paschen Law. A quasi-static piezoelectric d (33) coefficient up to 300 pC/N was observed after corona charging. The mechanical properties of the film systems are highly anisotropic. At room temperature, the Young's moduli of the laminated film system are around 0.37 MPa in the thickness direction and 274 MPa in the lateral direction, respectively. Using these values, the theoretical shape anisotropy ratio of the void was calculated, which agrees well with experimental observation. Compared with films that do not exhibit structural regularity, the laminates showed improved thermal stability of the d (33) coefficients. The thermal stability of d (33) can be further improved by pre-aging. E.g., the reduction of the d (33) value in the sample pre-aged at 150A degrees C for 5 h was less than 5% after annealing for 30 h at a temperature of 90A degrees C.
Y1  - 2011
U6  - https://doi.org/10.1007/s00339-011-6481-2
SN  - 0947-8396
VL  - 105
IS  - 1
SP  - 197
EP  - 205
PB  - Springer
CY  - New York
ER  - 
TY  - JOUR
A1  - Koseska, Aneta
A1  - Volkov, Evgenii
A1  - Kurths, Jürgen
T1  - Synthetic multicellular oscillatory systems controlling protein dynamics with genetic circuits
JF  - Physica scripta : an international journal for experimental and theoretical physics
N2  - Synthetic biology is a relatively new research discipline that combines standard biology approaches with the constructive nature of engineering. Thus, recent efforts in the field of synthetic biology have given a perspective to consider cells as 'programmable matter'. Here, we address the possibility of using synthetic circuits to control protein dynamics. In particular, we show how intercellular communication and stochasticity can be used to manipulate the dynamical behavior of a population of coupled synthetic units and, in this manner, finely tune the expression of specific proteins of interest, e.g. in large bioreactors.
Y1  - 2011
U6  - https://doi.org/10.1088/0031-8949/84/04/045007
SN  - 0031-8949
VL  - 84
IS  - 4
PB  - IOP Publ. Ltd.
CY  - Bristol
ER  - 
TY  - JOUR
A1  - Baushev, Anton N.
T1  - Principal properties of the velocity distribution of dark matter particles on the outskirts of the Solar system
JF  - Monthly notices of the Royal Astronomical Society
N2  - The velocity distribution of the dark matter particles on the outskirts of the Solar system remains unclear. We suggest to determine it using experimentally found properties of the oldest halo objects. Indeed, the oldest halo stars and globular clusters form a collisionless system, as well as dark matter particles do, and they evolved in the same gravitational field. If we accept this analogy, we can show that the velocity distribution of the dark matter particles should be highly anisotropic and have a sharp maximum near upsilon similar to 500 km s(-1). The distribution is totally different from the Maxwell one.
 We analyse the influence of the distribution function on the results of dark matter detection experiments. It is found that the direct detection signal should differ noticeably from the one calculated from the Maxwell distribution with <upsilon > similar or equal to 220 km s(-1), which is conventional for direct detection experiments (the ratio depends on the detector properties and typically falls within the range between 6 and 0.2). Moreover, the sharp distinction from the Maxwell distribution can be very essential to the observations of dark matter annihilation.
KW  - elementary particles
KW  - methods: analytical
KW  - dark matter
Y1  - 2011
U6  - https://doi.org/10.1111/j.1745-3933.2011.01125.x
SN  - 0035-8711
VL  - 417
IS  - 1
SP  - L83
EP  - L87
PB  - Wiley-Blackwell
CY  - Malden
ER  - 
TY  - JOUR
A1  - Döring, Sebastian
A1  - Kollosche, Matthias
A1  - Rabe, Torsten
A1  - Stumpe, Joachim
A1  - Kofod, Guggi
T1  - Electrically tunable polymer DFB laser
JF  - Advanced materials
Y1  - 2011
U6  - https://doi.org/10.1002/adma.201102465
SN  - 0935-9648
VL  - 23
IS  - 37
SP  - 4265
EP  - 4269
PB  - Wiley-VCH
CY  - Weinheim
ER  - 
TY  - JOUR
A1  - Blaha, Karen A.
A1  - Pikovskij, Arkadij
A1  - Rosenblum, Michael
A1  - Clark, Matthew T.
A1  - Rusin, Craig G.
A1  - Hudson, John L.
T1  - Reconstruction of two-dimensional phase dynamics from experiments on coupled oscillators
JF  - Physical review : E, Statistical, nonlinear and soft matter physics
N2  - Phase models are a powerful method to quantify the coupled dynamics of nonlinear oscillators from measured data. We use two phase modeling methods to quantify the dynamics of pairs of coupled electrochemical oscillators, based on the phases of the two oscillators independently and the phase difference, respectively. We discuss the benefits of the two-dimensional approach relative to the one-dimensional approach using phase difference. We quantify the dependence of the coupling functions on the coupling magnitude and coupling time delay. We show differences in synchronization predictions of the two models using a toy model. We show that the two-dimensional approach reveals behavior not detected by the one-dimensional model in a driven experimental oscillator. This approach is broadly applicable to quantify interactions between nonlinear oscillators, especially where intrinsic oscillator sensitivity and coupling evolve with time.
Y1  - 2011
U6  - https://doi.org/10.1103/PhysRevE.84.046201
SN  - 1539-3755
VL  - 84
IS  - 4
PB  - American Physical Society
CY  - College Park
ER  - 
TY  - JOUR
A1  - Tremblay, Jean Christophe
A1  - Monturet, Serge
A1  - Saalfrank, Peter
T1  - The Effects of electron-hole pair coupling on the infrared laser-controlled vibrational excitation of NO on Au(111)
JF  - The journal of physical chemistry : A, Molecules, spectroscopy, kinetics, environment & general theory
N2  - In this work, we present theoretical simulations of laser-driven vibrational control of NO adsorbed on a gold surface. Our goal is to tailor laser pulses to selectively excite specific modes and vibrational eigenstates, as well as to favor photodesorption of the adsorbed molecule. To this end, various control schemes and algorithms are applied. For adsorbates at metallic surfaces, the creation of electron hole pairs in the substrate is known to play a dominant role in the transfer of energy from the system to the surroundings. These nonadiabatic couplings are included perturbatively in our reduced density matrix simulations using a generalization of the state-resolved position-dependent anharmonic rate model we recently introduced. An extension of the reduced density matrix is also proposed to provide a sound model for photodesorption in dissipative systems.
Y1  - 2011
U6  - https://doi.org/10.1021/jp205902k
SN  - 1089-5639
VL  - 115
IS  - 39
SP  - 10698
EP  - 10707
PB  - American Chemical Society
CY  - Washington
ER  - 
TY  - JOUR
A1  - Aliu, E.
A1  - Arlen, T.
A1  - Aune, T.
A1  - Beilicke, M.
A1  - Benbow, W.
A1  - Bouvier, A.
A1  - Bradbury, S. M.
A1  - Buckley, J. H.
A1  - Bugaev, V.
A1  - Byrum, K.
A1  - Cannon, A.
A1  - Cesarini, A.
A1  - Christiansen, J. L.
A1  - Ciupik, L.
A1  - Collins-Hughes, E.
A1  - Connolly, M. P.
A1  - Cui, W.
A1  - Dickherber, R.
A1  - Duke, C.
A1  - Errando, M.
A1  - Falcone, A.
A1  - Finley, J. P.
A1  - Finnegan, G.
A1  - Fortson, L.
A1  - Furniss, A.
A1  - Galante, N.
A1  - Gall, D.
A1  - Gibbs, K.
A1  - Gillanders, G. H.
A1  - Godambe, S.
A1  - Griffin, S.
A1  - Grube, J.
A1  - Guenette, R.
A1  - Gyuk, G.
A1  - Hanna, D.
A1  - Holder, J.
A1  - Huan, H.
A1  - Hughes, G.
A1  - Hui, C. M.
A1  - Humensky, T. B.
A1  - Imran, A.
A1  - Kaaret, P.
A1  - Karlsson, N.
A1  - Kertzman, M.
A1  - Kieda, D.
A1  - Krawczynski, H.
A1  - Krennrich, F.
A1  - Lang, M. J.
A1  - Lyutikov, M.
A1  - Madhavan, A. S.
A1  - Maier, G.
A1  - Majumdar, P.
A1  - McArthur, S.
A1  - McCann, A.
A1  - McCutcheon, M.
A1  - Moriarty, P.
A1  - Mukherjee, R.
A1  - Nunez, P.
A1  - Ong, R. A.
A1  - Orr, M.
A1  - Otte, A. N.
A1  - Park, N.
A1  - Perkins, J. S.
A1  - Pizlo, F.
A1  - Pohl, Martin
A1  - Prokoph, H.
A1  - Quinn, J.
A1  - Ragan, K.
A1  - Reyes, L. C.
A1  - Reynolds, P. T.
A1  - Roache, E.
A1  - Rose, H. J.
A1  - Ruppel, J.
A1  - Saxon, D. B.
A1  - Schroedter, M.
A1  - Sembroski, G. H.
A1  - Sentuerk, G. D.
A1  - Smith, A. W.
A1  - Staszak, D.
A1  - Tesic, G.
A1  - Theiling, M.
A1  - Thibadeau, S.
A1  - Tsurusaki, K.
A1  - Tyler, J.
A1  - Varlotta, A.
A1  - Vassiliev, V. V.
A1  - Vincent, S.
A1  - Vivier, M.
A1  - Wakely, S. P.
A1  - Ward, J. E.
A1  - Weekes, T. C.
A1  - Weinstein, A.
A1  - Weisgarber, T.
A1  - Williams, D. A.
A1  - Zitzer, B.
T1  - Detection of pulsed Gamma Rays Above 100 GeV from the Crab Pulsar
JF  - Science
N2  - We report the detection of pulsed gamma rays from the Crab pulsar at energies above 100 giga-electron volts (GeV) with the Very Energetic Radiation Imaging Telescope Array System (VERITAS) array of atmospheric Cherenkov telescopes. The detection cannot be explained on the basis of current pulsar models. The photon spectrum of pulsed emission between 100 mega-electron volts and 400 GeV is described by a broken power law that is statistically preferred over a power law with an exponential cutoff. It is unlikely that the observation can be explained by invoking curvature radiation as the origin of the observed gamma rays above 100 GeV. Our findings require that these gamma rays be produced more than 10 stellar radii from the neutron star.
Y1  - 2011
U6  - https://doi.org/10.1126/science.1208192
SN  - 0036-8075
VL  - 334
IS  - 6052
SP  - 69
EP  - 72
PB  - American Assoc. for the Advancement of Science
CY  - Washington
ER  - 
TY  - JOUR
A1  - Sun, Y. -P.
A1  - Hennies, Franz
A1  - Pietzsch, Annette
A1  - Kennedy, B.
A1  - Schmitt, Thorsten
A1  - Strocov, Vladimir N.
A1  - Andersson, Joakim
A1  - Berglund, Martin
A1  - Rubensson, Jan-Erik
A1  - Aidas, K.
A1  - Gel'mukhanov, F.
A1  - Odelius, Michael
A1  - Föhlisch, Alexander
T1  - Intramolecular soft modes and intermolecular interactions in liquid acetone
JF  - Physical review : B, Condensed matter and materials physics
N2  - Resonant inelastic x-ray scattering spectra excited at the O1s(-1)pi* resonance of liquid acetone are presented. Scattering to the electronic ground state shows a resolved vibrational progression where the dominant contribution is due to the C-O stretching mode, thus demonstrating a unique sensitivity of the method to the local potential energy surface in complex molecular systems. For scattering to electronically excited states, soft vibrational modes and, to a smaller extent, intermolecular interactions give a broadening, which blurs the vibrational fine structure. It is predicted that environmental broadening is dominant in aqueous acetone.
Y1  - 2011
U6  - https://doi.org/10.1103/PhysRevB.84.132202
SN  - 1098-0121
VL  - 84
IS  - 13
PB  - American Physical Society
CY  - College Park
ER  - 
TY  - JOUR
A1  - Kiel, Mareike
A1  - Möhwald, Helmuth
A1  - Bargheer, Matias
T1  - Broadband measurements of the transient optical complex dielectric function of a nanoparticle/polymer composite upon ultrafast excitation
JF  - Physical review : B, Condensed matter and materials physics
N2  - We determined experimentally the complex transient optical dielectric function of a well-characterized polyelectrolyte/gold-nanoparticle composite system over a broad spectral range upon short pulse laser excitation by simultaneously measuring the time-dependent reflectance and transmittance of white light pulses with femtosecond pump-probe spectroscopy. We extracted directly the ultrafast changes in the real and imaginary parts of the effective dielectric function, epsilon(eff)(r) (omega,t)and epsilon(eff)(i) (omega,t), from the experiment. This complete experimental set of information on the time-dependent complex dielectric function challenges theories modeling the transient dielectric function of gold particles and the effective medium.
Y1  - 2011
U6  - https://doi.org/10.1103/PhysRevB.84.165121
SN  - 1098-0121
VL  - 84
IS  - 16
PB  - American Physical Society
CY  - College Park
ER  - 
TY  - JOUR
A1  - Berenstein, Igal
A1  - Beta, Carsten
T1  - Flow-induced control of chemical turbulence
JF  - The journal of chemical physics : bridges a gap between journals of physics and journals of chemistr
N2  - We report spatiotemporal chaos in the Oregonator model of the Belousov-Zhabotinsky reaction. Spatiotemporal chaos spontaneously develops in a regime, where the underlying local dynamics show stable limit cycle oscillations (diffusion-induced turbulence). We show that spatiotemporal chaos can be suppressed by a unidirectional flow in the system. With increasing flow velocity, we observe a transition scenario from spatiotemporal chaos via a regime of travelling waves to a stationary steady state. At large flow velocities, we recover the known regime of flow distributed oscillations.
KW  - chaos
KW  - chemical equilibrium
KW  - chemically reactive flow
KW  - reaction kinetics theory
KW  - spatiotemporal phenomena
KW  - turbulence
Y1  - 2011
U6  - https://doi.org/10.1063/1.3656248
SN  - 0021-9606
VL  - 135
IS  - 16
PB  - American Institute of Physics
CY  - Melville
ER  - 
TY  - JOUR
A1  - Blakesley, James C.
A1  - Schubert, Marcel
A1  - Steyrleuthner, Robert
A1  - Chen, Zhihua
A1  - Facchetti, Antonio
A1  - Neher, Dieter
T1  - Time-of-flight measurements and vertical transport in a high electron-mobility polymer
JF  - Applied physics letters
N2  - We investigate charge transport in a high-electron mobility polymer, poly(N, N-bis 2-octyldodecyl-naphthalene-1,4,5,8-bis dicarboximide-2,6-diyl-alt-5,5-2,2-bithiophene) [P(NDI2OD-T2), Polyera ActivInk (TM) N2200]. Time-of-flight measurements reveal electron mobilities approaching those measured in field-effect transistors, the highest ever recorded in a conjugated polymer using this technique. The modest temperature dependence and weak dispersion of the transients indicate low energetic disorder in this material. Steady-state electron-only current measurements reveal a barrier to injection of about 300 meV. We propose that this barrier is located within the P(NDI2OD-T2) film and arises from molecular orientation effects.
Y1  - 2011
U6  - https://doi.org/10.1063/1.3657827
SN  - 0003-6951
VL  - 99
IS  - 18
PB  - American Institute of Physics
CY  - Melville
ER  - 
TY  - JOUR
A1  - Huang, Tingwen
A1  - Chen, Guanrong
A1  - Kurths, Jürgen
T1  - Synchronization of chaotic of chaotic systems with time-varying coupöing delays
JF  - Discrete and continuous dynamical systems : a journal bridging mathematics and sciences ; Series B, Mathematical modelling, analysis and computations
N2  - In this paper, we study the complete synchronization of a class of time-varying delayed coupled chaotic systems using feedback control. In terms of Linear Matrix Inequalities, a sufficient condition is obtained through using a Lyapunov-Krasovskii functional and differential equation in equalities. The conditions can be easily verified and implemented. We present two simulation examples to illustrate the effectiveness of the proposed method.
KW  - Synchronization
KW  - Chaotic System
KW  - Time-varying Delay
Y1  - 2011
U6  - https://doi.org/10.3934/dcdsb.2011.16.1071
SN  - 1531-3492
VL  - 16
IS  - 4
SP  - 1071
EP  - 1082
PB  - American Institute of Mathematical Sciences
CY  - Springfield
ER  - 
TY  - JOUR
A1  - Khader, Patrick H.
A1  - Pachur, Thorsten
A1  - Meier, Stefanie
A1  - Bien, Siegfried
A1  - Jost, Kerstin
A1  - Roesler, Frank
T1  - Memory-based decision-making with heuristics evidence for a controlled activation of memory representations
JF  - Journal of cognitive neuroscience
N2  - Many of our daily decisions are memory based, that is, the attribute information about the decision alternatives has to be recalled. Behavioral studies suggest that for such decisions we often use simple strategies (heuristics) that rely on controlled and limited information search. It is assumed that these heuristics simplify decision-making by activating long-term memory representations of only those attributes that are necessary for the decision. However, from behavioral studies alone, it is unclear whether using heuristics is indeed associated with limited memory search. The present study tested this assumption by monitoring the activation of specific long-term-memory representations with fMRI while participants made memory-based decisions using the "take-the-best" heuristic. For different decision trials, different numbers and types of information had to be retrieved and processed. The attributes consisted of visual information known to be represented in different parts of the posterior cortex. We found that the amount of information required for a decision was mirrored by a parametric activation of the dorsolateral PFC. Such a parametric pattern was also observed in all posterior areas, suggesting that activation was not limited to those attributes required for a decision. However, the posterior increases were systematically modulated by the relative importance of the information for making a decision. These findings suggest that memory-based decision-making is mediated by the dorsolateral PFC, which selectively controls posterior storage areas. In addition, the systematic modulations of the posterior activations indicate a selective boosting of activation of decision-relevant attributes.
Y1  - 2011
SN  - 0898-929X
VL  - 23
IS  - 11
SP  - 3540
EP  - 3554
PB  - MIT Press
CY  - Cambridge
ER  -